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Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

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Full-Text Articles in Oceanography and Atmospheric Sciences and Meteorology

Atlantic Ocean Variability And European Alps Winter Precipitation, Giuseppe Formetta, Jonghun Kam, Sahar Sadeghi, Glenn Tootle, Thomas Piechota Nov 2021

Atlantic Ocean Variability And European Alps Winter Precipitation, Giuseppe Formetta, Jonghun Kam, Sahar Sadeghi, Glenn Tootle, Thomas Piechota

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Winter precipitation (snowpack) in the European Alps provides a critical source of freshwater to major river basins such as the Danube, Rhine, and Po. Previous research identified Atlantic Ocean variability and hydrologic responses in the European Alps. The research presented here evaluates Atlantic Sea Surface Temperatures (SSTs) and European Alps winter precipitation variability using Singular Value Decomposition. Regions in the north and mid-Atlantic from the SSTs were identified as being tele-connected with winter precipitation in the European Alps. Indices were generated for these Atlantic SST regions to use in prediction of precipitation. Regression and non-parametric models were developed using the …


Spatial Distribution Of Pm2.5-Related Premature Mortality In China, Sheng Zheng, Uwe Schlink, Kin-Fai Ho, Ramesh P. Singh, Andrea Pozzer Nov 2021

Spatial Distribution Of Pm2.5-Related Premature Mortality In China, Sheng Zheng, Uwe Schlink, Kin-Fai Ho, Ramesh P. Singh, Andrea Pozzer

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

PM2.5 is a major component of air pollution in China and has a serious threat to public health. It is very important to quantify spatial characteristics of the health effects caused by outdoor PM2.5 exposure. This study analyzed the spatial distribution of PM2.5 concentration (45.9 μg/m3 national average in 2016) and premature mortality attributed to PM2.5 in cities at the prefectural level and above in China in 2016. Using the Global Exposure Mortality Model (GEMM), the total premature mortality in China was estimated to be 1.55 million persons, and the per capita mortality was 11.2 …


Spatial Distribution Of Pm2.5-Related Premature Mortality In China, Sheng Zheng, Uwe Schlink, Kin-Fai Ho, Ramesh P. Singh, Andrea Pozzer Nov 2021

Spatial Distribution Of Pm2.5-Related Premature Mortality In China, Sheng Zheng, Uwe Schlink, Kin-Fai Ho, Ramesh P. Singh, Andrea Pozzer

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

PM2.5 is a major component of air pollution in China and has a serious threat to public health. It is very important to quantify spatial characteristics of the health effects caused by outdoor PM2.5 exposure. This study analyzed the spatial distribution of PM2.5 concentration (45.9 μg/m3 national average in 2016) and premature mortality attributed to PM2.5 in cities at the prefectural level and above in China in 2016. Using the Global Exposure Mortality Model (GEMM), the total premature mortality in China was estimated to be 1.55 million persons, and the per capita mortality was 11.2 …


California Drought Outlooks Based On Climate Change Models’ Effects On Water Availability, Lauren Lynam, Thomas Piechota Nov 2021

California Drought Outlooks Based On Climate Change Models’ Effects On Water Availability, Lauren Lynam, Thomas Piechota

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Future streamflow in California is evaluated based on eight climate projections models and the effects on water availability. The unimpaired projected streamflow for eleven California rivers, collected from Cal-Adapt, are compared with unimpaired historical flows (1950–2015) using eight climate model projections (2020–2099) identified as representative as possible future scenarios; Warm Dry RCP 4.5, Average RCP 4.5, Cool Wet RCP 4.5, Other RCP 4.5, Warm Dry RCP 8.5, Average RCP 8.5, Cool Wet RCP 8.5, and Other RCP 8.5. Projected drought deficits (or magnitudes), durations, and intensities are statistically tested against historical values to determine significance of differences between past streamflow …


Hydrological Feedbacks On Peatland Ch4 Emission Under Warming And Elevated Co2: A Modeling Study, Fenghui Yuan, Yihui Wang, Daniel M. Ricciuto, Xiaoying Shi, Fengming Yuan, Thomas Brehme, Scott Bridgham, Jason Keller, Jeffrey M. Warren, Natalie A. Griffiths, Stephen D. Sebestyen, Paul J. Hanson, Peter E. Thornton, Xiaofeng Xu Nov 2021

Hydrological Feedbacks On Peatland Ch4 Emission Under Warming And Elevated Co2: A Modeling Study, Fenghui Yuan, Yihui Wang, Daniel M. Ricciuto, Xiaoying Shi, Fengming Yuan, Thomas Brehme, Scott Bridgham, Jason Keller, Jeffrey M. Warren, Natalie A. Griffiths, Stephen D. Sebestyen, Paul J. Hanson, Peter E. Thornton, Xiaofeng Xu

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Peatland carbon cycling is critical for the land–atmosphere exchange of greenhouse gases, particularly under changing environments. Warming and elevated atmospheric carbon dioxide (eCO2) concentrations directly enhance peatland methane (CH4) emission, and indirectly affect CH4 processes by altering hydrological conditions. An ecosystem model ELM-SPRUCE, the land model of the E3SM model, was used to understand the hydrological feedback mechanisms on CH4 emission in a temperate peatland under a warming gradient and eCO2 treatments. We found that the water table level was a critical regulator of hydrological feedbacks that affect peatland CH4 dynamics; the …


Radiocarbon Analyses Quantify Peat Carbon Losses With Increasing Temperature In A Whole Ecosystem Warming Experiment, Rachel M. Wilson, Natalie A. Griffiths, Ate Visser, Karis J. Mcfarlane, Stephen D. Sebestyen, Keith C. Oleheiser, Samantha Bosman, Anya M. Hopple, Malak M. Tfaily, Randall K. Kolka, Paul J. Hanson, Joel E. Kostka, Scott D. Bridgham, Jason K. Keller, Jeffrey P. Chanton Oct 2021

Radiocarbon Analyses Quantify Peat Carbon Losses With Increasing Temperature In A Whole Ecosystem Warming Experiment, Rachel M. Wilson, Natalie A. Griffiths, Ate Visser, Karis J. Mcfarlane, Stephen D. Sebestyen, Keith C. Oleheiser, Samantha Bosman, Anya M. Hopple, Malak M. Tfaily, Randall K. Kolka, Paul J. Hanson, Joel E. Kostka, Scott D. Bridgham, Jason K. Keller, Jeffrey P. Chanton

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Climate warming is expected to accelerate peatland degradation and release rates of carbon dioxide (CO2) and methane (CH4). Spruce and Peatlands Responses Under Changing Environments is an ecosystem-scale climate manipulation experiment, designed to examine peatland ecosystem response to climate forcings. We examined whether heating up to +9 °C to 3 m-deep in a peat bog over a 7-year period led to higher C turnover and CO2 and CH4 emissions, by measuring 14C of solid peat, dissolved organic carbon (DOC), CH4, and dissolved CO2 (DIC). DOC, a major substrate for heterotrophic respiration, increased significantly with warming. There was no 7-year trend …


Changes In The Flood Plains And Water Quality Along The Himalayan Rivers After The Chamoli Disaster Of 7 February 2021, Sansar Raj Meena, Kushanav Bhuyan, Akshansa Chauhan, Ramesh P. Singh Aug 2021

Changes In The Flood Plains And Water Quality Along The Himalayan Rivers After The Chamoli Disaster Of 7 February 2021, Sansar Raj Meena, Kushanav Bhuyan, Akshansa Chauhan, Ramesh P. Singh

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

The Himalayan regions are vulnerable to all kinds of natural hazards. On 7 February 2021, a deadly disaster occurred near the Tapovan, in Uttarakhand, Himalayas. During the event, large volume of debris along with broken glacial fragments flooded the Rishi Ganga River and washed away the nearby hydropower plants (Rishi Ganga and Tapovan), which was revealed from detailed analysis of multi spectral and bi-temporal satellite data. We present the impact of the Chamoli disaster on the flood plains and water quality of Himalayan rivers, Rishi Ganga near Tapovan, Alaknanda near Srinagar and Ganga near Haridwar and Bijnor. We used four …


An Integrative Model For Soil Biogeochemistry And Methane Processes: I. Model Structure And Sensitivity Analysis, Daniel M. Ricciuto, Xiaofeng Xu, Xiaoying Shi, Yihui Wang, Xia Song, Christopher W. Schadt, Natalie A. Griffiths, Jiafu Mao, Jeffrey M. Warren, Peter E. Thornton, Jeff Chanton, Jason K. Keller, Scott D. Bridgham, Jessica Gutknecht, Stephen D. Sebestyen, Adrien Finzi, Randall Kolka, Paul J. Hanson Jul 2021

An Integrative Model For Soil Biogeochemistry And Methane Processes: I. Model Structure And Sensitivity Analysis, Daniel M. Ricciuto, Xiaofeng Xu, Xiaoying Shi, Yihui Wang, Xia Song, Christopher W. Schadt, Natalie A. Griffiths, Jiafu Mao, Jeffrey M. Warren, Peter E. Thornton, Jeff Chanton, Jason K. Keller, Scott D. Bridgham, Jessica Gutknecht, Stephen D. Sebestyen, Adrien Finzi, Randall Kolka, Paul J. Hanson

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Environmental changes are anticipated to generate substantial impacts on carbon cycling in peatlands, affecting terrestrial-climate feedbacks. Understanding how peatland methane (CH4) fluxes respond to these changing environments is critical for predicting the magnitude of feedbacks from peatlands to global climate change. To improve predictions of CH4 fluxes in response to changes such as elevated atmospheric CO2 concentrations and warming, it is essential for Earth system models to include increased realism to simulate CH4 processes in a more mechanistic way. To address this need, we incorporated a new microbial-functional group-based CH4 module into the Energy …


Changes In Tropospheric Ozone Associated With Strong Earthquakes And Possible Mechanism, Feng Jing, Ramesh P. Singh May 2021

Changes In Tropospheric Ozone Associated With Strong Earthquakes And Possible Mechanism, Feng Jing, Ramesh P. Singh

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

The index of ozone anomaly (IOA) has been proposed to detect changes in tropospheric ozone associated with strong earthquakes. The tropospheric ozone prior and after the 2008 Wenchuan earthquake has been analyzed using IOA. Atmospheric infrared sounder ozone volume mixing ratio (O3 VMR) at different pressure levels (600, 500, 400, 300, 200 hPa) for an 18-year period 2003–2020 has been considered to identify the unique behavior associated with the strong earthquakes. Our results show distinct enhancement in tropospheric ozone occurred 5 d (7 May 2008) prior to the main event and distributed along the Longmenshan fault zone. An enhancement in …


Representing Methane Emissions From Wet Tropical Forest Soils Using Microbial Functional Groups Constrained By Soil Diffusivity, Debjani Sihi, Xiaofeng Xu, Mónica Salazar Ortiz, Christine S. O'Connell, Whendee L. Silver, Carla López-Lloreda, Julia M. Brenner, Ryan K. Quinn, Jana R. Phillips, Brent D. Newman, Melanie A. Mayes Mar 2021

Representing Methane Emissions From Wet Tropical Forest Soils Using Microbial Functional Groups Constrained By Soil Diffusivity, Debjani Sihi, Xiaofeng Xu, Mónica Salazar Ortiz, Christine S. O'Connell, Whendee L. Silver, Carla López-Lloreda, Julia M. Brenner, Ryan K. Quinn, Jana R. Phillips, Brent D. Newman, Melanie A. Mayes

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Tropical ecosystems contribute significantly to global emissions of methane (CH4), and landscape topography influences the rate of CH4 emissions from wet tropical forest soils. However, extreme events such as drought can alter normal topographic patterns of emissions. Here we explain the dynamics of CH4 emissions during normal and drought conditions across a catena in the Luquillo Experimental Forest, Puerto Rico. Valley soils served as the major source of CH4 emissions in a normal precipitation year (2016), but drought recovery in 2015 resulted in dramatic pulses in CH4 emissions from all topographic positions. Geochemical parameters …


Air Quality Over Major Cities Of Saudi Arabia During Hajj Periods Of 2019 And 2020, Ashraf Farahat, Akshansha Chauhan, Mohammed Al Otaibi, Ramesh P. Singh Feb 2021

Air Quality Over Major Cities Of Saudi Arabia During Hajj Periods Of 2019 And 2020, Ashraf Farahat, Akshansha Chauhan, Mohammed Al Otaibi, Ramesh P. Singh

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Mecca and Madinah are two holy cities where millions of people in general, visit throughout the years, during Hajj (Muslim's pilgrimage) time number of people visit these holy cities from different parts of the world is very high. However, the Government of Saudi Arabia only allowed 1000 pilgrims during the 2020 Hajj especially when the world is suffering from COVID-19. In the present paper, a detailed analysis of air quality parameters available from ground measurements have been carried over major cities of Saudi Arabia, Mecca, Madinah, and Jeddah from June to September 2019 and 2020. At Mecca and Jeddah, PM …


Effect Of Lockdown On Hcho And Trace Gases Over India During March 2020, Akshansha Chauhan, Ramesh P. Singh Nov 2020

Effect Of Lockdown On Hcho And Trace Gases Over India During March 2020, Akshansha Chauhan, Ramesh P. Singh

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

COVID-19 is one of the deadly Epidemics that has impacted people living in more than 200 countries. In order to mitigate the impact of COVID-19, India observed total lockdown in the first phase for a period of 21 days (24 March–13 May 2020), so that social distancing is maintained. However, this sudden decision severely affected the normal life of people. The air quality improved due to lockdown, some relaxation was given in different cities and within some areas in the city where the people were not affected by COVID-19. In this paper, we discuss results of detailed analysis of trace …


Cosore: A Community Database For Continuous Soil Respiration And Other Soil-Atmosphere Greenhouse Gas Flux Data, Ben Bond-Lamberty, Danielle S. Christianson, Avni Malhotra, Stephanie C. Pennington, Debjani Sihi, Amir Aghakouchak, Hassan Anjileli, M. Altaf Arain, Juan J. Armesto, Samaneh Ashraf, Mioko Ataka, Dennis Baldocchi, Thomas Andrew Black, Nina Buchmann, Mariah S. Carbone, Shih-Chieh Chang, Patrick Crill, Peter S. Curtis, Eric A. Davidson, Ankur R. Desai, John E. Drake, Tarek S. El-Madany, Michael Gavazzi, Carolyn-Monika Görres, Christopher M. Gough, Michael Goulden, Jillian Gregg, Omar Gutiérrez Del Arroyo, Jin-Sheng He, Takashi Hirano, Anya Hopple, Holly Hughes, Järvi Järveoja, Rachhpal Jassal, Jinshi Jian, Haiming Kan, Jason Kaye, Yuji Kominami, Naishen Liang, David Lipson, Catriona A. Macdonald, Kadmiel Maseyk, Kayla Mathes, Marguerite Mauritz, Melanie A. Mayes, Steve Mcnulty, Guofang Miao, Mirco Migliavacca, Scott Miller, Chelcy F. Miniat, Jennifer G. Nietz, Mats B. Nilsson, Asko Noormets, Hamidreza Norouzi, Christine S. O'Connell, Bruce Osborne, Cecilio Oyonarte, Zhuo Pang, Matthias Peichl, Elise Pendall, Jorge F. Perez-Quezada, Claire L. Phillips, Richard P. Phillips, James W. Raich, Alexandre A. Renchon, Nadine K. Ruehr, Enrique P. Sánchez-Cañete, Matthew Saunders, Kathleen E. Savage, Marion Schrumpf, Russell L. Scott, Ulli Seibt, Whendee L. Silver, Wu Sun, Daphne Szutu, Kentaro Takagi, Masahiro Takagi, Munemasa Teramoto, Mark G. Tjoelker, Susan Trumbore, Masahito Ueyama, Rodrigo Vargas, Ruth K. Varner, Joseph Verfaillie, Christoph Vogel, Jinsong Wang, Greg Winston, Tana E. Wood, Juying Wu, Thomas Wutzler, Jiye Zeng, Tianshan Zha, Quan Zhang, Junliang Zou Oct 2020

Cosore: A Community Database For Continuous Soil Respiration And Other Soil-Atmosphere Greenhouse Gas Flux Data, Ben Bond-Lamberty, Danielle S. Christianson, Avni Malhotra, Stephanie C. Pennington, Debjani Sihi, Amir Aghakouchak, Hassan Anjileli, M. Altaf Arain, Juan J. Armesto, Samaneh Ashraf, Mioko Ataka, Dennis Baldocchi, Thomas Andrew Black, Nina Buchmann, Mariah S. Carbone, Shih-Chieh Chang, Patrick Crill, Peter S. Curtis, Eric A. Davidson, Ankur R. Desai, John E. Drake, Tarek S. El-Madany, Michael Gavazzi, Carolyn-Monika Görres, Christopher M. Gough, Michael Goulden, Jillian Gregg, Omar Gutiérrez Del Arroyo, Jin-Sheng He, Takashi Hirano, Anya Hopple, Holly Hughes, Järvi Järveoja, Rachhpal Jassal, Jinshi Jian, Haiming Kan, Jason Kaye, Yuji Kominami, Naishen Liang, David Lipson, Catriona A. Macdonald, Kadmiel Maseyk, Kayla Mathes, Marguerite Mauritz, Melanie A. Mayes, Steve Mcnulty, Guofang Miao, Mirco Migliavacca, Scott Miller, Chelcy F. Miniat, Jennifer G. Nietz, Mats B. Nilsson, Asko Noormets, Hamidreza Norouzi, Christine S. O'Connell, Bruce Osborne, Cecilio Oyonarte, Zhuo Pang, Matthias Peichl, Elise Pendall, Jorge F. Perez-Quezada, Claire L. Phillips, Richard P. Phillips, James W. Raich, Alexandre A. Renchon, Nadine K. Ruehr, Enrique P. Sánchez-Cañete, Matthew Saunders, Kathleen E. Savage, Marion Schrumpf, Russell L. Scott, Ulli Seibt, Whendee L. Silver, Wu Sun, Daphne Szutu, Kentaro Takagi, Masahiro Takagi, Munemasa Teramoto, Mark G. Tjoelker, Susan Trumbore, Masahito Ueyama, Rodrigo Vargas, Ruth K. Varner, Joseph Verfaillie, Christoph Vogel, Jinsong Wang, Greg Winston, Tana E. Wood, Juying Wu, Thomas Wutzler, Jiye Zeng, Tianshan Zha, Quan Zhang, Junliang Zou

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Globally, soils store two to three times as much carbon as currently resides in the atmosphere, and it is critical to understand how soil greenhouse gas (GHG) emissions and uptake will respond to ongoing climate change. In particular, the soil-to-atmosphere CO2 flux, commonly though imprecisely termed soil respiration (RS), is one of the largest carbon fluxes in the Earth system. An increasing number of high-frequency RS measurements (typically, from an automated system with hourly sampling) have been made over the last two decades; an increasing number of methane measurements are being made with such systems …


Long Term Air Quality Analysis In Reference To Thermal Power Plants Using Satellite Data In Singrauli Region, India, H. K. Romana, Ramesh P. Singh, D. P. Shukla Aug 2020

Long Term Air Quality Analysis In Reference To Thermal Power Plants Using Satellite Data In Singrauli Region, India, H. K. Romana, Ramesh P. Singh, D. P. Shukla

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

The exponentially growing population and related anthropogenic activities have led to modifications in local environment. The change in local environment, evolving pattern of land use, concentrations of greenhouse gases and aerosols alter the energy balance of our climate system. This alteration in climate is leading to pre-mature deaths worldwide. This study analyses the air quality of Singrauli region, Madhya Pradesh, India for the past 15 years. Otherwise known as Urjanchal “the energy capital” of India has been declared as critically polluted by CPCB. The study provides an updated list of thermal power plants in the study area and their emission …


Global Atmospheric Budget Of Acetone: Air-Sea Exchange And The Contribution To Hydroxyl Radicals, Siyuan Wang, Eric C. Apel, Rebecca H. Schwantes, Kelvin H. Bates, Daniel J. Jacob, Emily V. Fischer, Rebecca S. Hornbrook, Alan J. Hills, Louisa K. Emmons, Laura L. Pan, Shawn Honomichl, Simone Tilmes, Jean‐François Lamarque, Mingxi Yang, Christa A. Marandino, E. S. Saltzman, Warren J. De Bruyn, Sohiko Kameyama, Hiroshi Tanimoto, Yuko Omori, Samuel R. Hall, Kirk Ullmann, Thomas B. Ryerson, Chelsea R. Thompson, Jeff Peischl, Bruce C. Daube, Róisín Commane, Kathryn Mckain, Colm Sweeney, Alexander B. Thames, David O. Miller, William H. Brune, Glenn S. Diskin, Joshua P. Digangi, Steven C. Wofsy Jul 2020

Global Atmospheric Budget Of Acetone: Air-Sea Exchange And The Contribution To Hydroxyl Radicals, Siyuan Wang, Eric C. Apel, Rebecca H. Schwantes, Kelvin H. Bates, Daniel J. Jacob, Emily V. Fischer, Rebecca S. Hornbrook, Alan J. Hills, Louisa K. Emmons, Laura L. Pan, Shawn Honomichl, Simone Tilmes, Jean‐François Lamarque, Mingxi Yang, Christa A. Marandino, E. S. Saltzman, Warren J. De Bruyn, Sohiko Kameyama, Hiroshi Tanimoto, Yuko Omori, Samuel R. Hall, Kirk Ullmann, Thomas B. Ryerson, Chelsea R. Thompson, Jeff Peischl, Bruce C. Daube, Róisín Commane, Kathryn Mckain, Colm Sweeney, Alexander B. Thames, David O. Miller, William H. Brune, Glenn S. Diskin, Joshua P. Digangi, Steven C. Wofsy

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Acetone is one of the most abundant oxygenated volatile organic compounds (VOCs) in the atmosphere. The oceans impose a strong control on atmospheric acetone, yet the oceanic fluxes of acetone remain poorly constrained. In this work, the global budget of acetone is evaluated using two global models: CAM‐chem and GEOS‐Chem. CAM‐chem uses an online air‐sea exchange framework to calculate the bidirectional oceanic acetone fluxes, which is coupled to a data‐oriented machine‐learning approach. The machine‐learning algorithm is trained using a global suite of seawater acetone measurements. GEOS‐Chem uses a fixed surface seawater concentration of acetone to calculate the oceanic fluxes. Both …


Massive Peatland Carbon Banks Vulnerable To Rising Temperatures, A. M. Hopple, R. M. Wilson, M. Kolton, Cassandra A. Zalman, J. P. Chanton, J. Kostka, P. J. Hanson, Jason K. Keller, S. D. Bridgham May 2020

Massive Peatland Carbon Banks Vulnerable To Rising Temperatures, A. M. Hopple, R. M. Wilson, M. Kolton, Cassandra A. Zalman, J. P. Chanton, J. Kostka, P. J. Hanson, Jason K. Keller, S. D. Bridgham

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Peatlands contain one-third of the world’s soil carbon (C). If destabilized, decomposition of this vast C bank could accelerate climate warming; however, the likelihood of this outcome remains unknown. Here, we examine peatland C stability through five years of whole-ecosystem warming and two years of elevated atmospheric carbon dioxide concentrations (eCO2). Warming exponentially increased methane (CH4) emissions and enhanced CH4 production rates throughout the entire soil profile; although surface CH4 production rates remain much greater than those at depth. Additionally, older deeper C sources played a larger role in decomposition following prolonged warming. Most …


Changes In Atmospheric, Meteorological, And Ocean Parameters Associated With The 12 January 2020 Taal Volcanic Eruption, Feng Jing, Akshansa Chauhan, Ramesh P. Singh, Prasanjit Dash Mar 2020

Changes In Atmospheric, Meteorological, And Ocean Parameters Associated With The 12 January 2020 Taal Volcanic Eruption, Feng Jing, Akshansa Chauhan, Ramesh P. Singh, Prasanjit Dash

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

The Taal volcano erupted on 12 January 2020, the first time since 1977. About 35 mild earthquakes (magnitude greater than 4.0) were observed on 12 January 2020 induced from the eruption. In the present paper, we analyzed optical properties of volcanic aerosols, volcanic gas emission, ocean parameters using multi-satellite sensors, namely, MODIS (Moderate Resolution Imaging Spectroradiometer), AIRS (Atmospheric Infrared Sounder), OMI (Ozone Monitoring Instrument), TROPOMI (TROPOspheric Monitoring Instrument) and ground observations, namely, Argo, and AERONET (AErosol RObotic NETwork) data. Our detailed analysis shows pronounced changes in all the parameters, which mainly occurred in the western and south-western regions because the …


Methanethiol, Dimethyl Sulfide And Acetone Over Biologically Productive Waters In The Southwest Pacific Ocean, Sarah J. Lawson, Cliff S. Law, Mike J. Harvey, Thomas G. Bell, Carolyn F. Walker, Warren J. De Bruyn, Eric S. Saltzman Mar 2020

Methanethiol, Dimethyl Sulfide And Acetone Over Biologically Productive Waters In The Southwest Pacific Ocean, Sarah J. Lawson, Cliff S. Law, Mike J. Harvey, Thomas G. Bell, Carolyn F. Walker, Warren J. De Bruyn, Eric S. Saltzman

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Atmospheric methanethiol (MeSHa), dimethyl sulfide (DMSa) and acetone (acetonea) were measured over biologically productive frontal waters in the remote southwest Pacific Ocean in summertime 2012 during the Surface Ocean Aerosol Production (SOAP) voyage. MeSHa mixing ratios varied from below the detection limit (< 10 ppt) up to 65 ppt and were 3 %–36 % of parallel DMSa mixing ratios. MeSHa and DMSa were correlated over the voyage (R2=0.3, slope = 0.07) with a stronger correlation over a coccolithophore-dominated phytoplankton bloom (R2=0.5, slope 0.13). The diurnal cycle for MeSHa shows similar behaviour to DMSa with mixing ratios …


Air/Sea Transfer Of Highly Soluble Gases Over Coastal Waters, J. G. Porter, Warren J. De Bruyn, S. D. Miller, E. S. Saltzman Jan 2020

Air/Sea Transfer Of Highly Soluble Gases Over Coastal Waters, J. G. Porter, Warren J. De Bruyn, S. D. Miller, E. S. Saltzman

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

The deposition of soluble trace gases to the sea surface is not well studied due to a lack of flux measurements over the ocean. Here we report simultaneous air/sea eddy covariance flux measurements of water vapor, sulfur dioxide (SO2), and momentum from a coastal North Atlantic pier. Gas transfer velocities were on average about 20% lower for SO2 than for H2O. This difference is attributed to the difference in molecular diffusivity between the two molecules (D SO 2/D H 2O = 0.5), in reasonable agreement with bulk parameterizations in air/sea gas …


Global Sinusoidal Seasonality In Precipitation Isotopes, Scott T. Allen, Scott Jasechko, Wouter R. Berghuijs, Jeffrey M. Welker, Gregory R. Goldsmith, James W. Kirchner Aug 2019

Global Sinusoidal Seasonality In Precipitation Isotopes, Scott T. Allen, Scott Jasechko, Wouter R. Berghuijs, Jeffrey M. Welker, Gregory R. Goldsmith, James W. Kirchner

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Quantifying seasonal variations in precipitation δ2H and δ18O is important for many stable isotope applications, including inferring plant water sources and streamflow ages. Our objective is to develop a data product that concisely quantifies the seasonality of stable isotope ratios in precipitation. We fit sine curves defined by amplitude, phase, and offset parameters to quantify annual precipitation isotope cycles at 653 meteorological stations on all seven continents. At most of these stations, including in tropical and subtropical regions, sine curves can represent the seasonal cycles in precipitation isotopes. Additionally, the amplitude, phase, and offset parameters of …


Seasonal Origins Of Soil Water Used By Trees, Scott T. Allen, James W. Kirchner, Sabine Braun, Rolf T. W. Siegwolf, Gregory R. Goldsmith Mar 2019

Seasonal Origins Of Soil Water Used By Trees, Scott T. Allen, James W. Kirchner, Sabine Braun, Rolf T. W. Siegwolf, Gregory R. Goldsmith

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Rain recharges soil water storages and either percolates downward into aquifers and streams or is returned to the atmosphere through evapotranspiration. Although it is commonly assumed that summer rainfall recharges plant-available water during the growing season, the seasonal origins of water used by plants have not been systematically explored. We characterize the seasonal origins of waters in soils and trees by comparing their midsummer isotopic signatures (δ2H) to seasonal isotopic cycles in precipitation, using a new seasonal origin index. Across 182 Swiss forest sites, xylem water isotopic signatures show that summer rain was not the predominant water source …


Spatial Variation In Throughfall, Soil, And Plant Water Isotopes In A Temperate Forest, Gregory R. Goldsmith, Scott T. Allen, Sabine Braun, Nadine Engbersen, Clara Romero González-Quijano, James W. Kirchner, Rolf T. W. Siegwolf Nov 2018

Spatial Variation In Throughfall, Soil, And Plant Water Isotopes In A Temperate Forest, Gregory R. Goldsmith, Scott T. Allen, Sabine Braun, Nadine Engbersen, Clara Romero González-Quijano, James W. Kirchner, Rolf T. W. Siegwolf

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Studies of stable isotopes of water in the environment have been fundamental to advancing our understanding of how water moves through the soil‐plant‐atmosphere continuum; however, much of this research focuses on how water isotopes vary in time, rather than in space. We examined the spatial variation in the δ18O and δ2H of throughfall and bulk soil water, as well as branch xylem and bulk leaf water of Picea abies (Norway Spruce) and Fagus sylvatica (Beech), in a 1 ha forest plot in the northern Alps of Switzerland. Means and ranges of water isotope ratios varied considerably …


Eddy Flux Measurements Of Sulfur Dioxide Deposition To The Sea Surface, Jack G. Porter, Warren J. De Bruyn, Eric S. Saltzman Oct 2018

Eddy Flux Measurements Of Sulfur Dioxide Deposition To The Sea Surface, Jack G. Porter, Warren J. De Bruyn, Eric S. Saltzman

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Deposition to the sea surface is a major atmospheric loss pathway for many important trace gases, such as sulfur dioxide (SO2). The air–sea transfer of SO2 is controlled entirely on the atmospheric side of the air–sea interface due to high effective solubility and other physical– chemical properties. There have been few direct field measurements of such fluxes due to the challenges associated with making fast-response measurements of highly soluble trace gases at very low ambient levels. In this study, we report direct eddy covariance air–sea flux measurements of SO2, sensible heat, water vapor, and momentum. The measurements were made over …


Balancing Tradeoffs: Reconciling Multiple Environmental Goals When Ecosystem Services Vary Regionally, Christine S. O'Connell, Kimberly M. Carlson, Santiago Cuadra, Kenneth J. Feeley, James Gerber, Paul C. West, Stephen Polasky May 2018

Balancing Tradeoffs: Reconciling Multiple Environmental Goals When Ecosystem Services Vary Regionally, Christine S. O'Connell, Kimberly M. Carlson, Santiago Cuadra, Kenneth J. Feeley, James Gerber, Paul C. West, Stephen Polasky

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

As the planet’s dominant land use, agriculture often competes with the preservation of natural systems that provide globally and regionally important ecosystem services. How agriculture impacts ecosystem service delivery varies regionally, among services being considered, and across spatial scales. Here, we assess the tradeoffs between four ecosystem services—agricultural production, carbon storage, biophysical climate regulation, and biodiversity—using as a case study the Amazon, an active frontier of agricultural expansion. We find that the highest values for each of the ecosystem services are concentrated in different regions. Agricultural production potential and carbon storage are highest in the north and west, biodiversity greatest …


Predicting Spatial Patterns In Precipitation Isotope (Δ2h And Δ18o) Seasonality Using Sinusoidal Isoscapes, Scott T. Allen, James W. Kirchner, Gregory R. Goldsmith May 2018

Predicting Spatial Patterns In Precipitation Isotope (Δ2h And Δ18o) Seasonality Using Sinusoidal Isoscapes, Scott T. Allen, James W. Kirchner, Gregory R. Goldsmith

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Understanding how precipitation isotopes vary spatially and temporally is important for tracer applications. We tested how well month‐to‐month variations in precipitation δ18O and δ2H were captured by sinusoidal cycles, and how well spatial variations in these seasonal cycles could be predicted, across Switzerland. Sine functions representing seasonal cycles in precipitation isotopes explained between 47% and 94% of the variance in monthly δ18O and δ2H values at each monitoring site. A significant sinusoidal cycle was also observed in line‐conditioned excess. We interpolated the amplitudes, phases, and offsets of these sine functions across the landscape, using multiple linear …


Drought Drives Rapid Shifts In Tropical Rainforest Soil Biogeochemistry And Greenhouse Gas Emissions, Christine S. O'Connell, Leilei Ruan, Whendee L. Silver Apr 2018

Drought Drives Rapid Shifts In Tropical Rainforest Soil Biogeochemistry And Greenhouse Gas Emissions, Christine S. O'Connell, Leilei Ruan, Whendee L. Silver

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Climate change models predict more frequent and severe droughts in the humid tropics. How drought will impact tropical forest carbon and greenhouse gas dynamics is poorly understood. Here we report the effects of the severe 2015 Caribbean drought on soil moisture, oxygen, phosphorus (P), and greenhouse gas emissions in a humid tropical forest in Puerto Rico. Drought significantly decreases inorganic P concentrations, an element commonly limiting to net primary productivity in tropical forests, and significantly increases organic P. High-frequency greenhouse gas measurements show varied impacts across topography. Soil carbon dioxide emissions increase by 60% on slopes and 163% in valleys. …


No Evidence For Trace Metal Limitation On Anaerobic Carbon Mineralization In Three Peatland Soils, Jason K. Keller, Jillian Wade Nov 2017

No Evidence For Trace Metal Limitation On Anaerobic Carbon Mineralization In Three Peatland Soils, Jason K. Keller, Jillian Wade

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Peatlands store roughly one-third of the terrestrial soil carbon and release the potent greenhouse gas methane (CH4) to the atmosphere, making these wetlands among the most important ecosystems in the global carbon cycle. Despite their importance, the controls of anaerobic decomposition of organic matter to carbon dioxide (CO2) and CH4 within peatlands are not well understood. It is known, however, that the enzymes responsible for CH4 production require cobalt, iron and nickel, and there is a growing appreciation for the potential role of trace metal limitation in anaerobic decomposition. To explore the possibility of …


Estimation Of Bubble-Mediated Air–Sea Gas Exchange From Concurrent Dms And Co2 Transfer Velocities At Intermediate–High Wind Speeds, Thomas G. Bell, Sebastian Landwehr, Scott D. Miller, Warren J. De Bruyn, Adrian H. Callaghan, Brian Scanlon, Brian Ward, Mingxi Yang, Eric S. Saltzman Jul 2017

Estimation Of Bubble-Mediated Air–Sea Gas Exchange From Concurrent Dms And Co2 Transfer Velocities At Intermediate–High Wind Speeds, Thomas G. Bell, Sebastian Landwehr, Scott D. Miller, Warren J. De Bruyn, Adrian H. Callaghan, Brian Scanlon, Brian Ward, Mingxi Yang, Eric S. Saltzman

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Simultaneous air–sea fluxes and concentration differences of dimethylsulfide (DMS) and carbon dioxide (CO2/ were measured during a summertime North Atlantic cruise in 2011. This data set reveals significant differences between the gas transfer velocities of these two gases (1kw/ over a range of wind speeds up to 21ms􀀀1. These differences occur at and above the approximate wind speed threshold when waves begin breaking. Whitecap fraction (a proxy for bubbles) was also measured and has a positive relationship with 1kw, consistent with enhanced bubble-mediated transfer of the less soluble CO2 relative to that of the more soluble DMS. However, the correlation …


Temporal Variation In Optical Properties Of Chromophoric Dissolved Organic Matter (Cdom) In Southern California Coastal Waters With Nearshore Kelp And Seagrass, Catherine D. Clark, Warren J. De Bruyn, Paige Aiona Oct 2015

Temporal Variation In Optical Properties Of Chromophoric Dissolved Organic Matter (Cdom) In Southern California Coastal Waters With Nearshore Kelp And Seagrass, Catherine D. Clark, Warren J. De Bruyn, Paige Aiona

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Optical properties of chromophoric dissolved organic matter (CDOM) were measured in surf zone waters in diurnal field studies at a Southern California beach with nearshore kelp and seagrass beds and intertidal plant wrack. Absorption coefficients (aCDOM(300 nm)) ranged from 0.35 m21 to 3.7 m21 with short-term variability<1 h, increases at ebb and flood tides and higher values (6 m21) during an offshore storm event. Spectral slopes (S) ranged from 0.0028 nm21 to 0.017 nm21, with higher values after the storm; S was generally inversely correlated with aCDOM(300 nm). 3-D excitation–emission matrix spectra (EEMs) for samples with lower S values had humic-type peaks associated with terrestrial material (A, C), marine microbial material (M) and protein peaks, characteristic of freshly produced organic material. Samples with high S values had no or reduced protein peaks, consistent with aged material. Fluorescent indexes (f450/f500 >2.5, BIX>1.1) were consistent with microbial aquatic sources. Leachates of senescent kelp and seagrass had protein and humic-type EEM peaks. After solar simulator irradiation (4 h), protein peaks rapidly photochemically degraded, humic-type peak C increased in intensity and peak M disappeared. Optical characteristics of kelp leachates were most similar to field samples, …


Dimethylsulfide Gas Transfer Coefficients From Algal Blooms In The Southern Ocean, T. G. Bell, Warren J. De Bruyn, Christa A. Marandino, S. D. Miller, C. S. Law, Eric S. Saltzman Jan 2015

Dimethylsulfide Gas Transfer Coefficients From Algal Blooms In The Southern Ocean, T. G. Bell, Warren J. De Bruyn, Christa A. Marandino, S. D. Miller, C. S. Law, Eric S. Saltzman

Biology, Chemistry, and Environmental Sciences Faculty Articles and Research

Air-sea dimethylsulfide (DMS) fluxes and bulk air-sea gradients were measured over the Southern Ocean in February-March 2012 during the Surface Ocean Aerosol Production (SOAP) study. The cruise encountered three distinct phytoplankton bloom regions, consisting of two blooms with moderate DMS levels, and a high biomass, dinoflagellate-dominated bloom with high seawater DMS levels (> 15 nM). Gas transfer coefficients were considerably scattered at wind speeds above 5 m s(-1). Bin averaging the data resulted in a linear relationship between wind speed and mean gas transfer velocity consistent with that previously observed. However, the wind-speed-binned gas transfer data distribution at all wind …