Oceanography and Atmospheric Sciences and Meteorology Commons^™

Data Supporting “High-Resolution Lidar Observations Of Sedimentation-Induced Size Sorting Of Droplets Near A Laboratory Cloud Top”, Fan Yang, Yong Meng Sua, Zipei Zheng, Jesse Anderson, Hamed F. Sadi, Jae Min Yeom, Suryadey P. Singh, Pei Hou, Will Cantrell, Ernie R. Lewis, Alexander Kostinski, Raymond Shaw

Michigan Tech Research Data

Cloud optical properties and precipitation, which are crucial to weather and climate, are strongly influenced by cloud microphysical properties that are still poorly understood. Here, we develop a high-resolution time-correlated single-photon-counting lidar and apply it to observe cloud microphysical properties at one-centimeter range resolution in a convection chamber under well-controlled conditions. Together with concurrent in-situ measurements and theoretical analysis, our lidar observations indicate that although turbulent mixing tends to homogenize the cloud in the bulk region, entrainment and sedimentation cause inhomogeneities in droplet concentrations near the cloud top. Specifically, the topmost region is directly affected by entrainment, and lidar profiles …

Data Supporting The Paper "Enhancing Turbulent Mixing And Microphysical Uniformity In A Tall Convection-Cloud Chamber Through Idealized Heterogeneity Of Boundaries", Lois Thomas, Fan Yang, Aaron Wang, Mikhail Ovchinnikov, Kyle G. Pressel, Raymond Shaw

Michigan Tech Research Data

A large convection cloud chamber has been proposed for exploring aerosol–cloud–drizzle interactions under well-controlled turbulent conditions. Recent theoretical and numerical studies suggest that a convection cloud chamber with two heated and two cooled sidewalls can significantly enhance the liquid water content and thus benefit drizzle initiation. However, a chamber with such a sidewall configuration develops stable stratification and extremely weak turbulence therein. In this study, we conduct large-eddy simulations of a tall convection chamber with five different sidewall configurations consisting of alternating warm and cold patches. For each configuration, the total surface area of warm patches equals that of cold …

High-Resolution Temperature Profiling In The Pi Chamber: Variability Of Statistical Properties Of Temperature Fluctuations, Robert Grosz, Kamal Kant Chandrakar, Raymond A. Shaw, Jesse C. Anderson, Will Cantrell, Szymon P. Malinowski

Michigan Tech Research Data

This study delves into the small-scale temperature structure inside the turbulent convection Pi Chamber under three temperature differences (10, 15, and 20 K) at Rayleigh number Ra ~ 10^9 and Prandtl number Pr = 0.7. We performed high-frequency measurements (2 kHz) with the UltraFast Thermometer (UFT) at selected points along the vertical axis. The miniaturized design of the sensor with a resistive platinum-coated tungsten wire, 2.5 μm thick and 3 mm long, mounted on a miniature wire probe, allowed for vertically undisturbed temperature
profiling through the chamber’s depth spanning from 8 cm above the bottom to 5 cm below the …

Vertical Gradient In Atmospheric Particle Phase State: A Case Study Over The Alaskan Arctic Oil Fields, Nurun Nahar Lata, Zezhen Cheng, Darielle Dexheimer, Susan Mathai, Matthew A. Marcus, Kerri A. Pratt

Michigan Tech Publications

The phase state of atmospheric particles impacts atmospheric processes like heterogeneous reactions, cloud droplet activation, and ice nucleation, influencing Earth's climate. Factors like chemical composition, temperature, and relative humidity govern particle phase states. The Arctic atmosphere is stratified, with varying particle compositions, but vertical profiles of submicron phase states remain poorly understood due to limited aloft measurements. To address this, particle samples were collected via a tethered balloon system (TBS) at the U.S. Department of Energy Atmospheric Radiation Measurement Program's facility at Oliktok Point, Alaska, on November 19, 2020. Using an environmental scanning electron microscope with a tilted Peltier stage …

Coupled Lake-Atmosphere-Land Physics Uncertainties In A Great Lakes Regional Climate Model, William J. Pringle, Chenfu Huang, Pengfei Xue, Jiali Wang, Khachik Sargsyan, Miraj Kayastha, Et. Al.

Michigan Tech Publications

This study develops a surrogate-based method to assess the uncertainty within a convective permitting integrated modeling system of the Great Lakes region, arising from interacting physics parameterizations across the lake, atmosphere, and land surface. Perturbed physics ensembles of the model during the 2018 summer are used to train a neural network surrogate model to predict lake surface temperature (LST) and near-surface air temperature (T2m). Average physics uncertainties are determined to be 1.5°C for LST and T2m over land, and 1.9°C for T2m over lake, but these have significant spatiotemporal variations. We find that atmospheric physics parameterizations alone are the dominant …

Light Absorbing Aerosol Interactions With Warm Clouds, Shreya Joshi

Dissertations, Master's Theses and Master's Reports

Atmospheric particles such as biomass-burning aerosols, including black carbon - are critical in altering the Earth's energy balance through interactions with light and clouds. Biomass-burning aerosols also contain organic carbon, a diverse mix of organic compounds. As these aerosols age, they evolve by interacting with other atmospheric species, including cloud water, leading to changes in particle morphology and the development of coatings that impact their lifetime and ability to interact with clouds and light.

Some biomass-burning aerosols serve as cloud condensation nuclei. When cloud water droplets form, the properties of the nucleating particles can change. Many clouds evaporate before precipitating, …

Great Lakes And Its Regional Climate In The Future, Miraj Bhakta Kayastha

Dissertations, Master's Theses and Master's Reports

The overarching objective of this dissertation is to enhance our predictive understanding of the Great Lakes regional climate by utilizing advanced modeling techniques and provide comprehensive insights into the future of the Great Lakes. This dissertation focuses on four areas pertinent to the future of the Great Lakes hydroclimate and extreme events, beginning with the derivation of robust water level projections for the Great Lakes in Chapter 2. Using a regional climate modeling system with a two-way coupled three-dimensional (3D) hydrodynamic lake and ice model for the Great lakes, we analyze long-term future changes in the over-lake precipitation, lake evaporation, …

Dam It All: A Multi-Scalar Investigation Into The Ecological Role And Function Of Beaver Dams, Kenneth Larsen

Dissertations, Master's Theses and Master's Reports

The central theme of this dissertation is ecological scaling, which examines how small, localized features, such as beaver ponds, contribute to large-scale watershed processes and how different modeling approaches at various scales reveal distinct insights. Through a combination of probabilistic modeling and high-resolution empirical research, this work demonstrates that small ponded systems, particularly those created by beavers (Castor canadensis), serve as critical biogeochemical control points, whose contributions to sediment and nutrient dynamics have been historically underestimated.

In Chapter 1, I contextualize this research within the broader fields of freshwater ecology, watershed modeling, and ecological restoration. I introduce the …

Investigating Microphysical Variability And Entrainment In Clouds Using Airborne Digital Holography, Machine Learning, And Large Eddy Simulations, Nithin Allwayin

Dissertations, Master's Theses and Master's Reports

Advancing our understanding of cloud microphysics—the processes governing cloud particles' formation, growth, and interactions—is essential for accurate weather and climate modeling. In this work, we investigate how droplet size distributions vary in a cloud and explore how microphysical properties such as droplet size and number concentration respond to entrainment and mixing.

In the first part of the work, a novel algorithm is developed combining hypothesis testing with density-based clustering to identify characteristic cloud droplet size distribution types in marine stratocumulus clouds. Applied to data from the airborne Holographic Detector for Clouds (HOLODEC), the algorithm successfully identifies a relatively small set …

The Effect Of Seasonal Ice Cover Duration On Shoreline Erosion In Lake Michigan, Ryan S. Navarre

Dissertations, Master's Theses and Master's Reports

Shoreline erosion in Lake Michigan has been a significant concern for coastal management. Promoting coastal stability and resilience is paramount to protecting these environments, especially amid climate change. While several factors are key in understanding shoreline erosion, seasonal ice cover duration is a prominent yet understudied factor in the Great Lakes region. Here, the relationship between ice cover duration and shoreline erosion rates is assessed across 7 regions of Lake Michigan. An ice cover duration dataset was created for Lake Michigan for 2011 – 2020 and its shorelines were digitized for years with available high-resolution aerial imagery. The statistical relationship …

Data Supporting The Paper "Droplet Growth Or Evaporation Does Not Buffer The Variability In Supersaturation In Clean Clouds", Jesse Anderson, Ian Helman, Raymond Shaw, Will Cantrell

Michigan Tech Research Data

Water vapor supersaturation in clouds is a random variable that drives activation and growth of cloud droplets. The Pi Convection-Cloud Chamber generates a turbulent cloud with a microphysical steady-state that can be varied from clean to polluted by adjusting the aerosol injection rate. The supersaturation distribution and its moments, e.g., mean and variance, are investigated for varying cloud microphysical conditions. High-speed and co-located Eulerian measurements of temperature and water vapor concentration are combined to obtain the temporally resolved supersaturation distribution. This allows quantification of the contributions of variances and covariances between water vapor and temperature. Results are consistent with expectations …

Cloud Microphysical Response To Entrainment And Mixing Is Locally Inhomogeneous And Globally Homogeneous: Evidence From The Lab, Jaemin Yeom, Ian Helman, Prasanth Prabhakaran, Jesse Anderson, Fan Yang, Raymond Shaw, Will Cantrell

Michigan Tech Research Data

The effects of entrainment-mixing on the cloud droplet size distribution are examined in the Pi cloud chamber that creates a turbulent supersaturated environment for cloud formation. The experiments are conducted with a temperature-controlled flange to mimic the entrainment-mixing process. The entrainment zone is created at the center of the top surface of the chamber, allowing dry air of controlled temperature (T_e) and flow rate (Q_e) to flow into the mixing cloud region. Due to the large-scale circulation, the downwind region is directly affected by entrained dry air from the flange, whereas the upwind region is representative …

Molecular Dynamics Simulation Data: Mw And Mlmw Water Model Ice Nucleation On A Hydrophilic Substrate With Negative Pressure, Will Cantrell, Tianshu Li, Issei Nakamura, Elise Rosky, Raymond Shaw

Michigan Tech Research Data

This dataset contains the data supporting Figures in the study by Rosky et al., "Molecular simulations reveal that heterogeneous ice nucleation occurs at higher temperatures in water under capillary tension", submitted for publication in Atmospheric Chemistry and Physics in February 2023. Input files for reproducing the molecular dynamics simulations are included.

The abstract from the paper reads: Using a molecular model of water freezing on a hydrophilic substrate, it is found that heterogeneous ice nucleation rates occur at higher temperatures in water that is under tension, in other words under negative pressure. For pressures ranging from from 1 atm to …

Joint Probability Analysis Of Extreme Precipitation And Water Level For Chicago, Illinois, Anna Li Holey

Dissertations, Master's Theses and Master's Reports

A compound flooding event occurs when there is a combination of two or more extreme factors that happen simultaneously or in quick succession and can lead to flooding. In the Great Lakes region, it is common for a compound flooding event to occur with a high lake water level and heavy rainfall. With the potential of increasing water levels and an increase in precipitation under climate change, the Great Lakes coastal regions could be at risk for more frequent and severe flooding. The City of Chicago which is located on Lake Michigan has a high population and dense infrastructure and …

An Exploration Of Cloud Droplet Growth By Condensation And Collision-Coalescence In A Convection-Cloud Chamber, Jacob T. Kuntzleman

Dissertations, Master's Theses and Master's Reports

Atmospheric clouds are crucial to weather and climate, and the rate at which droplets collide and coalesce to form precipitation is one of the fundamental controlling processes. The convection-cloud chamber allows the interactions between aerosols and cloud droplets produced by condensation to be investigated within a turbulent environment. Studying the full range of microphysical conditions in atmospheric clouds is not possible, however, unless conditions for droplet growth by collision and coalescence are also achieved. In this study, we explore the conditions favorable to collision-coalescence growth in convection-cloud chambers, extending previous work on steady-state droplet size distributions due to condensation alone. …

Physical, Optical, And Chemical Properties Of Light Absorbing Aerosols And Their Climatic Impacts, Susan Mathai

Dissertations, Master's Theses and Master's Reports

Aerosols are particles suspended in the atmosphere; they are emitted during natural phenomena such as dust storms, wildfires, and volcanic eruptions, and during anthropogenic activities like household wood burning, vehicles operations, and industrial productions, or they can form in the atmosphere from gas to particle partition. Aerosols impact earth’s weather and climate by absorbing and scattering the incoming solar and the outgoing earth thermal radiation and interacting with clouds. The optical properties of aerosols evolve as the chemical and physical properties vary during their residence in the atmosphere. In addition, the aerosols’ properties strongly depend on the vertical distribution in …

Large Cloud Droplets And The Initiation Of Ice By Pressure Fluctuations: Molecular Simulations And Airborne In-Situ Observations, Elise Rosky

Dissertations, Master's Theses and Master's Reports

From the molecular dynamics of water molecules to the global processes that control atmospheric circulation: describing the evolution of atmospheric clouds necessitates physics that spans vast spatial scales. In this work, steps are taken towards connecting the molecular physics of ice-nucleation to the growth and subsequent freezing of cloud droplets in convective cumulus clouds. Motivated by experimental evidence of ice nucleation triggered by agitation and distortion of a water droplet surface, the first study in this dissertation uses molecular dynamics simulations to demonstrate that negative Laplace pressure from a curved water surface leads to heterogeneous ice nucleation at higher temperatures. …

An Intercomparison Of Large-Eddy Simulations Of A Convection Cloud Chamber Using Haze-Capable Bin And Lagrangian Cloud Microphysics Schemes, Fan Yang, Fabian Hoffmann, Raymond Shaw, Mikhail Ovchinnikov, Andrew Vogelmann

Michigan Tech Research Data

Recent in-situ observations show that haze particles exist in a convection cloud chamber. The microphysics schemes previously used for large-eddy simulations of the cloud chamber could not fully resolve haze particles and the associated processes, including their activation and deactivation. Specifically, cloud droplet activation is modeled based on Twomey-type parameterizations, wherein cloud droplets are formed when a critical supersaturation for the available cloud condensation nuclei (CCN) is exceeded and haze particles are not explicitly resolved. Here, we develop and adapt haze-capable bin and Lagrangian microphysics schemes to properly resolve the activation and deactivation processes. Results are compared with the Twomey-type …

Data Supporting: Scaling Of Turbulence And Microphysics In A Convection-Cloud Chamber Of Varying Height, Subin Thomas, Fan Yang, Mikhail Ovchinnikov, Will Cantrell, Raymond Shaw

Michigan Tech Research Data

The file contains the data corresponding to the figures in the paper. Abstract for the paper: The convection-cloud chamber enables measurement of aerosol and cloud microphysics, as well as their interactions, within a turbulent environment under steady-state conditions. Increasing the size of a convection-cloud chamber, while holding the imposed temperature difference constant, leads to increased Rayleigh, Reynolds and Nusselt numbers. Large-eddy simulation coupled with a bin microphysics model allows the influence of increased velocity, time, and spatial scales on cloud microphysical properties to be explored. Simulations of a convection--cloud chamber, with fixed aspect ratio and increasing heights of H=1, 2, …

Emissions, Shawn Urbanski, Susan O'Neill, Amara L. Holder, Sarah Green, Rick L. Graw

Michigan Tech Publications, Part 1

This chapter assesses the current state of the science regarding the composition, intensity, and drivers of wildland fire emissions in the USA and Canada. Globally and in the USA wildland fires are a major source of gases and aerosols which have significant air quality impacts and climate interactions. Wildland fire smoke can trigger severe pollution episodes with substantial effects on public health. Fire emissions can degrade air quality at considerable distances downwind, hampering efforts by air regulators to meet air standards. Fires are a major global source of aerosols which affect the climate system by absorbing and scattering radiation and …

Ultrahigh Resolution Ote-Ms Data For Ambient Daytime And Nighttime Aerosol And Ambient Fog Water From San Pietro Capofiume, Matthew Brege, Lynn Mazzoleni

Michigan Tech Research Data

This dataset and the methods used to obtain it are described in Chapter 3 of "EXTREME MOLECULAR DIVERSITY IN BIOMASS BURNING ATMOSPHERIC ORGANIC AEROSOL OBSERVED THROUGH ULTRAHIGH RESOLUTION MASS SPECTROMETRY" a Dissertation prepared by Matthew Brege and submitted as a Doctoral Thesis. This work can be accessed here: https://doi.org/10.37099/mtu.dc.etdr/927

Briefly, four days worth of concurrent daytime/nighttime aerosol and fog water samples were collected at San Pietro Capofiume in the Emilia Romagna region of Italy from 1-Dec to 4-Dec, 2015. The water soluble extracts of the aerosol filters and aliquots of the fog water were analyzed using ultrahigh resolution Orbitrap mass …

Ultrahigh Resolution Ote-Ms Data For Wildfire-Influenced Tar Ball Aerosol From The Pacific Northwest, Matthew Brege, Simeon Schum, Lynn Mazzoleni

Michigan Tech Research Data

This dataset and the methods used to obtain it are described in Chapter 4 of "EXTREME MOLECULAR DIVERSITY IN BIOMASS BURNING ATMOSPHERIC ORGANIC AEROSOL OBSERVED THROUGH ULTRAHIGH RESOLUTION MASS SPECTROMETRY" a Dissertation prepared by Matthew Brege and submitted as a Doctoral Thesis. Access this associated work here: https://doi.org/10.37099/mtu.dc.etdr/927

Briefly, two samples of ambient aerosol were collected in the Pacific Northwest of the United States in 2017 which were heavily influenced by atmospheric tar balls. The acetonitrile soluble extracts of the aerosol filters were analyzed using ultrahigh resolution Orbitrap mass spectrometry (OTE-MS) using positive and negative modes of electrospray ionization as …

Using Uncrewed Aerial Vehicles For Identifying The Extent Of Invasive Phragmites Australis In Treatment Areas Enrolled In An Adaptive Management Program, Colin Brooks, Charlotte Weinstein, Andrew Poley, Amanda Grimm, Nicholas Marion, Laura Bourgeau-Chavez, Dana Hansen, Kurt Kowalski

Michigan Tech Publications, Part 1

Higher spatial and temporal resolutions of remote sensing data are likely to be useful for ecological monitoring efforts. There are many different treatment approaches for the introduced European genotype of Phragmites australis, and adaptive management principles are being integrated in at least some long-term monitoring efforts. In this paper, we investigated how natural color and a smaller set of near-infrared (NIR) images collected with low-cost uncrewed aerial vehicles (UAVs) could help quantify the aboveground effects of management efforts at 20 sites enrolled in the Phragmites Adaptive Management Framework (PAMF) spanning the coastal Laurentian Great Lakes region. We used object-based image …

Data Supporting The Paper "Is The Water Vapor Supersaturation Distribution Gaussian?", Subin Thomas, Prasanth Prabhakaran, W. Cantrell, Raymond Shaw

Michigan Tech Research Data

The data in this file are from the MTU Pi Cloud Chamber and large eddy simulations. This work was supported by NSF grant AGS-1754244. Data are made available in support of the above publication by Thomas et al.. For any further use, e.g., for publication elsewhere, the authors should be contacted to ensure the appropriate use of the data and proper acknowledgment.

Multi-Source Eo For Dynamic Wetland Mapping And Monitoring In The Great Lakes Basin, Michael Battaglia, Sarah Banks, Amir Behnamian, Laura Bourgeau-Chavez

Michigan Tech Publications, Part 1

Wetland managers, citizens and government leaders are observing rapid changes in coastal wetlands and associated habitats around the Great Lakes Basin due to human activity and climate variability. SAR and optical satellite sensors offer cost effective management tools that can be used to monitor wetlands over time, covering large areas like the Great Lakes and providing information to those making management and policy decisions. In this paper we describe ongoing efforts to monitor dynamic changes in wetland vegetation, surface water extent, and water level change. Included are assessments of simulated Radarsat Constellation Mission data to determine feasibility of continued monitoring …

Mapping Michigan's Historic Coastlines, Ryan A. Williams

Dissertations, Master's Theses and Master's Reports

This five-year project, sponsored by the Michigan Department of Environment, Great Lakes, and Energy, is working to map how Michigan’s Great Lakes shorelines have changed over the past 80+ years. Products of this project include publicly available digital, georeferenced, historic aerial photography datasets, as well as map layers depicting the locations of historic shorelines and bluff lines from 1938, 1980, 2009, 2016, 2018, and 2020. Additional products include bluff retreat risk areas, shoreline rate of change map layers, and tools to assist in the development of future Coastal Vulnerability Index projects for the Great Lakes. All products are available as …

Predicting The Impacts Of Climate Change On The Great Lakes Water Levels Using A Fully Coupled 3d Regional Modeling System, Miraj Kayastha

Dissertations, Master's Theses and Master's Reports

The Great Lakes of North America are the largest surface freshwater system in the world and many ecosystems, industries, and coastal processes are sensitive to the changes in their water levels. The recent changes in the Great Lakes climate and water levels have particularly highlighted the importance of water level prediction. The water levels of the Great Lakes are primarily governed by the net basin supplies (NBS) of each lake which are the sum of over-lake precipitation and basin runoff minus lake evaporation. Recent studies have utilized Regional Climate Models (RCMs) with a fully coupled one-dimensional (1D) lake model to …

Understanding The Effects Of Water Vapor And Temperature On Aerosol Using Novel Measurement Methods, Tyler Jacob Capek

Dissertations, Master's Theses and Master's Reports

Aerosol and water are inexorably linked, and both are ubiquitous within our atmosphere and required components for cloud formation. Relative humidity (RH), a temperature dependent quantity, can have a significant influence on the size, shape, and ultimately, the optical properties of the aerosol. RH can vary substantially on small spatial and short temporal scales in turbulent conditions due to rapid fluctuations in temperature and water vapor mixing ratio. Accurate assessment of optical enhancements due to an increase in RH is key for determining the particles’ impact on the climate and visibility.

A humidity-controlled cavity attenuated phase-shift albedometer (H-CAPS-PM_SSA) …

Investigating Ice Nucleation At Negative Pressures Using Molecular Dynamics: A First Order Approximation Of The Dependence Of Ice Nucleation Rate On Pressure, Elise Rosky

Dissertations, Master's Theses and Master's Reports

Atmospheric scientists and climate modelers are faced with uncertainty around the process of ice production in clouds. While significant progress has been made in predicting homogeneous and heterogeneous ice nucleation rates as a function of temperature, recent experiments have shown that ice nucleation rates can be enhanced without decreasing temperature, through various mechanical agitations. One hypothesis for these findings is that mechanisms of stretching water and thereby inducing negative pressure in the liquid could lead to an increase in freezing rate. To better understand the viability of this concept, the effect of negative pressure on ice nucleation rates needs to …

Physicochemical Properties Of Atmospheric Aerosols And Their Effect On Ice Cloud Formation, Nurun Nahar Lata

Dissertations, Master's Theses and Master's Reports

Atmospheric aerosols play a vital role in the Earth's energy budget-directly by scattering and absorbing solar radiation and indirectly by acting as cloud condensation nuclei and ice-nucleating particles [1, 2]. The cloud formation potential of aerosol is driven by multiple factors, including surface properties, size distribution, composition, mixing state, phase state, and morphology [3]. The interaction of aerosols with clouds alters the aerosol's physicochemical properties. Those properties can also evolve during transport due to atmospheric processing, in turn, affect the aerosol's ice nucleation and cloud formation activities. This thesis presents experimental studies to understand the role of physicochemical properties of …