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Faculty Publications

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Full-Text Articles in Astrophysics and Astronomy

Nonequilibrium Processes In Polymers Undergoing Interchange Reactions. Part 2: Reaction-Diffusion Processes, Alejandro Garcia, J. Pojman, D. Kondepudi, C. Van De Broeck Jan 1991

Nonequilibrium Processes In Polymers Undergoing Interchange Reactions. Part 2: Reaction-Diffusion Processes, Alejandro Garcia, J. Pojman, D. Kondepudi, C. Van De Broeck

Faculty Publications

A reactiodffusion system of polymers undergoing interchange reactions is studied. The equation that describes the dynamics of the system is similar to the Boltzmann equation for a gas of hard spheres. We consider a one-dimensionsl system in which the average length and the concentrations at the boundaries are fixed. The resulting steady states are obtained analytically and with numerical integration of equations obtained by using a local equilibrium approximation. Monte Carlo simulations of experimentally realizable conditions were performed and compared. The results reveal a nonlinear distribution of molecular concentration and mass. The entropy of the polymer distributions is calculated as …

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Determination Of Rate Distributions From Kinetic Experiments, Todd B. Sauke, P. J. Steinback, K. Chu, H. Frauenfelder, J. B. Johnson, D. C. Lamb, G. U. Nienhaus, R. D. Young Jan 1991

Determination Of Rate Distributions From Kinetic Experiments, Todd B. Sauke, P. J. Steinback, K. Chu, H. Frauenfelder, J. B. Johnson, D. C. Lamb, G. U. Nienhaus, R. D. Young

Faculty Publications

Rate processes in proteins are often not adequately described by simple exponential kinetics. Instead of modeling the kinetics in the time domain, it can be advantageous to perform a numerical inversion leading to a rate distribution function f(lambda). The features observed in f(lambda) (number, positions, and shapes of peaks) can then be interpreted. We discuss different numerical techniques for obtaining rate distribution functions, with special emphasis on the maximum entropy method. Examples are given for the application of these techniques to flash photolysis data of heme proteins.

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The Transmittances Of Thin Polymer Films And Their Suitability As A Supportive Substrate For A Soft X-Ray Solar Filter, Memorie Williams, Evan Hansen, A. Reyes-Mena, David D. Allred Jan 1991

The Transmittances Of Thin Polymer Films And Their Suitability As A Supportive Substrate For A Soft X-Ray Solar Filter, Memorie Williams, Evan Hansen, A. Reyes-Mena, David D. Allred

Faculty Publications

This paper discusses soft x-ray filter designs for the Brigham Young University "Goldhelox Project". Three polymers intended for use as a supportive substrate for a soft x-ray solar filter, having a passband centered at 171 angstroms are examined. The use of polymer substrates is examined because of vibrational and mechanical stresses associated with the shuttle launch, preventing the use of a free standing filter, and because of Goldhelox's special need to locate the filter near the imaging plane. The uniform consistency of a polymer support will prevent any imaging of the filter support structure, as would occur if a traditional …

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Structure And Optical Characterization Of Znxcd1-Xte Thin Films Prepared By The Close Spaced Vapor Transport Method, David D. Allred, Jesus González-Hernández, O. Zelaya, J. G. Mendoza-Alverez, E. López-Cruz, D. A. Pawlik Jan 1991

Structure And Optical Characterization Of Znxcd1-Xte Thin Films Prepared By The Close Spaced Vapor Transport Method, David D. Allred, Jesus González-Hernández, O. Zelaya, J. G. Mendoza-Alverez, E. López-Cruz, D. A. Pawlik

Faculty Publications

Zinc cadmium telluride (ZnxCd1-xTe) solid solution films with 0≤x≤0.12 were deposited by the close spaced vapor transport method and characterized using photoluminescence, x-ray diffraction, and scanning electron microscopy. The two former techniques indicate that films with high crystalline quality can be prepared with moderate substrate temperatures and low argon pressures. Under these conditions deposition rates of up to 1000 Å/s are achieved and Zn concentration in the film is the same as that of the source. The electron micrographs show grain sizes comparable to the film thickness.

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The Effect Of Externally Applied Oscillating Electric Fields On The L=1 And L=2 Diocotron Modes In Non-Neutral Plasmas, Ross L. Spencer Oct 1990

The Effect Of Externally Applied Oscillating Electric Fields On The L=1 And L=2 Diocotron Modes In Non-Neutral Plasmas, Ross L. Spencer

Faculty Publications

A high-frequency oscillating electric field can change the properties of diocotron modes in non-neutral plasmas. The effect depends crucially on the azimuthal mode number, m, of the applied field. For m=0, plus or minus 1 there is no effect, and for applied standing waves there is also no effect. But if the applied field has the form of a traveling wave with the norm of m greater than or equal to 2, the frequency of stable diocotron modes can be modified and for the norm of m greater than or equal to 3, the l=2 instability of hollow density profiles …

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Photoluminescence Studies In Znxcd1-Xte Single Crystals, David D. Allred, Jesus González-Hernández, Elías López-Cruz, Worth P. Allred Mar 1990

Photoluminescence Studies In Znxcd1-Xte Single Crystals, David D. Allred, Jesus González-Hernández, Elías López-Cruz, Worth P. Allred

Faculty Publications

The crystalline quality of ZnxCd1-xTe single crystals prepared by a modified Bridgman method with 0≤x≤0.05 has been analyzed using photoluminescence. The spectrum of a typical sample is dominated by lines originating from the recombination of free and bound excitons. Lines due to free excitons in their ground and first excited states are observed in both the pure CdTe and the mixed crystals. Excitons bound to Dc vacancies are observed in the pure CdTe crystal but not in the mixed crystal. Weaker and broader features appearing at energies below the exciton emission range were associated with transitions involving free-to-bound and bound-to-bound …

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Inhomogeneous Broadening In Spectral Bands Of Carbonmonoxymyoglobin: The Connection Between Spectral And Functional Heterogeneity, Todd B. Sauke, P. Ormos, A. Ansari, D. Braunstein, B. R. Cowen, H. Fraunfelder, M. K. Hong, I. E. T. Iben, P. J. Steinbach, R. D. Young Jan 1990

Inhomogeneous Broadening In Spectral Bands Of Carbonmonoxymyoglobin: The Connection Between Spectral And Functional Heterogeneity, Todd B. Sauke, P. Ormos, A. Ansari, D. Braunstein, B. R. Cowen, H. Fraunfelder, M. K. Hong, I. E. T. Iben, P. J. Steinbach, R. D. Young

Faculty Publications

The rebinding kinetics of CO to myoglobin after flash photolysis is nonexponential in time below approximately 180 K; the kinetics is governed by a distribution of enthalpic barriers. This distribution results from inhomogeneities in the protein conformation, referred to as conformational substates. Hole-burning experiments on the Soret and IR CO-stretch bands test the assumption that an inhomogeneous distribution of conformational substates results in inhomogeneously broadened spectra. CO was slowly photolyzed at different wavelengths in the Soret band at 10 K. Both the Soret band and the CO-stretch band A1, centered at 1,945 cm-1, shift during photolysis, demonstrating that different wavelengths …

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Design Of High Performance Soft X-Ray Windows, Raymond T. Perkins, David D. Allred, Larry V. Knight, James M. Thorne Jan 1990

Design Of High Performance Soft X-Ray Windows, Raymond T. Perkins, David D. Allred, Larry V. Knight, James M. Thorne

Faculty Publications

X-ray windows are used in sources and detectors to separate the neighborhood of the x-ray generation or detection from the use environment. While each use has its own requirements, there are some principles that should be used in designing an optimal x-ray window. Because x-rays are absorbed to some extent by all materials, minimizing absorption is one criterion in preparing windows. Also, for most uses there is a pressure difference across the window so that ensuring pinhole-free structure and sufficient mechanical strength to support the differential is another criterion for window design. Traditionally, absorption is minimized by fabricating the window …

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Photoconductive Characterization Of Znxcd1-Xte (0≤X≤0.25) Single Crystal Alloys, David D. Allred, Elías López-Cruz, Jesus González-Hernández, Worth P. Allred Jan 1990

Photoconductive Characterization Of Znxcd1-Xte (0≤X≤0.25) Single Crystal Alloys, David D. Allred, Elías López-Cruz, Jesus González-Hernández, Worth P. Allred

Faculty Publications

Large grain polycrystalline and single crystals of ZnxCd1-xTe grown by a modified Bridgman method were studied using the photoluminescence and photoconductivity techniques. The temperature dependence of the band gap, as determined by photoluminescence, follows the Varshni equation for measuring temperature in the range of 15-290 K. One of the fitted parameters, the Debye temperature, monotonically decreases with the increase of the atomic zinc concentration. A close correlation between the photoluminescence and photoconductivity measurements is also found. Samples in which the photoluminescence spectra exhibit emission bands associated to cadmium vacancies and other structural defects, show a photoresponse curve which includes, in …

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Advanced Infrared Optically Black Baffle Materials, David D. Allred, Ronald D. Seals, C. M. Egert Jan 1990

Advanced Infrared Optically Black Baffle Materials, David D. Allred, Ronald D. Seals, C. M. Egert

Faculty Publications

Infrared optically black baffle surfaces are an essential component of many advanced optical systems. All internal surfaces in advanced infrared optical sensors that require stray light management to achieve resolution are of primary concern in baffle design. Current industrial materials need improvements to meet advanced optical sensor systems requirements for optical, survivability, and endurability. Baffles are required to survive and operate in potentially severe environments. Robust diffuse-absorptive black surfaces, which are (1) thermally and mechanically stable to threats of x-ray, launch, and in-flight maneuver conditions, with specific densities to allow an acceptable weight load, (2) handleable during assembly, (3) cleanable, …

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Annealing Behavior Of The Photoluminescence Lines In Cdte And Znx Cd1-X Te Single Crystals, David D. Allred, A. Reyes-Mena, Jesus González-Hernández, Elías López-Cruz, Worth P. Allred Jan 1990

Annealing Behavior Of The Photoluminescence Lines In Cdte And Znx Cd1-X Te Single Crystals, David D. Allred, A. Reyes-Mena, Jesus González-Hernández, Elías López-Cruz, Worth P. Allred

Faculty Publications

The main lines in the photoluminescence spectra of Zn1Cd1-xTe single crystals grown by a modified Bridgman method in the compositional range of 0≤X≤0.25 have been identified. All crystals show only near-band-edge emission. To assist in the identification, various samples with different compositions were annealed under a Cd atmosphere. In the pure crystals, the prominent (A°, X) bound exciton line, as well as the doublet at longer wavelengths, disappear after the annealing. In contrast, the treatments do not change significantly the PL spectra of the mixed crystals.

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Characterization Of Metal/Carbon Multilayers By Raman Spectroscopy, David D. Allred, Qi Wang, Jesus González-Hernández Jan 1990

Characterization Of Metal/Carbon Multilayers By Raman Spectroscopy, David D. Allred, Qi Wang, Jesus González-Hernández

Faculty Publications

Laser Raman spectroscopy has been found to be useful for characterizing amorphous semiconductor multilayers, especially the interfaces of multilayers. Recently, we have extended this technique to the characterization of magnetron sputtered multilayers commonly used as reflectors in soft x-ray optics. Unlike the multilayers previously studied which contained only semiconductors and dielectrics, these are generally semiconductor/metal multilayers. We report here on the Raman characterization of the most common class of multilayers used in soft x-ray optics, those that contain a high density metal like tungsten interspersed with layers of carbon. In all of the metal/carbon multilayers the dominate feature in the …

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Deposition Of Zinc Selenide By Atomic Layer Epitaxy For Multilayer X-Ray Optics, J.K. Shurtleff, David D. Allred, R. T. Perkins, J. M. Thorne Jan 1990

Deposition Of Zinc Selenide By Atomic Layer Epitaxy For Multilayer X-Ray Optics, J.K. Shurtleff, David D. Allred, R. T. Perkins, J. M. Thorne

Faculty Publications

Thin film deposition techniques currently being used to produce multilayer x-ray optics (MXOs) have difficulty producing smooth, uniform multilayers with d-spacings less than about twelve angstroms. We are investigating atomic layer epitaxy (ALE) as an alternative to these techniques. ALE is a chemical vapor deposition technique which deposits an atomic layer of material during each cycle of the deposition process. The thickness of a film deposited by ALE depends only on the number of cycles. Multilayers deposited by ALE should be smooth and uniform with precise d-spacings which makes ALE an excellent technique for producing multilayer x-ray optics. We have …

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Diffuse Absorbing Beryllium Coatings Produced By Magnetron Sputtering, David D. Allred, C. M. Egert Jan 1990

Diffuse Absorbing Beryllium Coatings Produced By Magnetron Sputtering, David D. Allred, C. M. Egert

Faculty Publications

Beryllium coatings with varying thicknesses and columnar grain sizes were deposited by low temperature magnetron sputtering and wet chemically etched to enhance diffuse absorption of light. After etching these coatings exhibited a matte black surface finish and low specular reflectance (below 2%) in the IR up to a critical wavelength dependent upon the original grain size of the coating. Extremely thick coatings (350 µm) with original grain sizes of 10 to 12 µm were produced which exhibited specular reflectances below 0.5% up to 50 µm wavelength and a Lambertian BRDF at 10.6 µm averaging 4.3x10-3 ster-1. Scanning electron micrographs are …

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Nonlocal Symmetries And Backlund Transformations For The Self-Dual Yang-Mills System, C. J. Papachristou, Kent B. Harrison Jan 1988

Nonlocal Symmetries And Backlund Transformations For The Self-Dual Yang-Mills System, C. J. Papachristou, Kent B. Harrison

Faculty Publications

The observation is made that generalized evolutionary isovectors of the self-dual Yang–Mills equation, obtained by "verticalization'' of the geometrical isovectors derived in a previous paper [J. Math. Phys. 28, 1261 (1987)], generate Bäcklund transformations for the self-dual system. In particular, new Bäcklund transformations are obtained by "verticalizing'' the generators of point transformations on the solution manifold. A geometric ansatz for the derivation of such (generally nonlocal) symmetries is proposed.

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Comparison Of Effective Medium Procedures For Optical Modeling Of Laminar Structures, David D. Allred, Robert F. Edgerton Jan 1988

Comparison Of Effective Medium Procedures For Optical Modeling Of Laminar Structures, David D. Allred, Robert F. Edgerton

Faculty Publications

This study addresses the question, "How can the optical properties of matter in ultrathin amorphous nonmetallic films in multilayers best be determined from reflectance (R) and transmission (T) measurements?" A blue shift in the band gap of plasma CVD a-Si:H/a-SiNx:H multilayers was reported several years ago. It was suggested that the shift in the band gap, Eg, Relative to bulk a-Si:H as given by the Tauç plot was due to quantum confinement effects. The purpose of this study is to evaluate the usefulness of various effective media theories (EMT) for determining the optical constants of materials in a multilayer and …

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Surface Conductance Of A Copper Wire In A Fluid At High Pressure, Daniel L. Decker Jul 1987

Surface Conductance Of A Copper Wire In A Fluid At High Pressure, Daniel L. Decker

Faculty Publications

The three-dimensional flow of heat in a wire carrying a current and immersed in a liquid is solved in detail. Using this exact result the surface conductance of copper in petroleum ether has been measured as a function of pressure to 40 kbars. The measured surface conductance for copper in a fluid is very small, justifying approximations which yield results that are in agreement with a simplified one-dimensional heat-flow problem. Surprisingly, even at 40 kbars pressure a very large fraction of the joule heating within a wire with a length-to-diameter ratio of ~100 is dissipated through the ends of the …

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Superconductivity At 155 K, David D. Allred, S. R. Ovshinsky, R. T. Young, G. Demaggio, G. A. Van Der Leeden Jun 1987

Superconductivity At 155 K, David D. Allred, S. R. Ovshinsky, R. T. Young, G. Demaggio, G. A. Van Der Leeden

Faculty Publications

Transition to a superconducting zero-resistance state at 155 K is observed for the first time in bulk material. A new five-element compound has been synthesized with nominal composition Y1Ba2Cu3F2Oy. Fluorine plays a critical role in achieving this effect. X-ray diffraction and electron microprobe analysis indicate that the samples are multiphasic. Evidence is presented that the samples contain superconducting phases with onset temperatures considerably above 155 K. Magnetic measurements suggest a flux-trapping effect below 260 K, and diamagnetic deviations from Curie-Weiss behavior in the range from 250 K≤T≤100 K indicate that Meissner effect in a small superconducting volume fraction.

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Some Aspects Of The Isogroup Of The Self-Dual Yang-Mills System, C. J. Papachristou, B. Kent Harrison Jun 1987

Some Aspects Of The Isogroup Of The Self-Dual Yang-Mills System, C. J. Papachristou, B. Kent Harrison

Faculty Publications

A generalized isovector formalism is used to derive the isovectors and isogroup of the self-dual Yang-Mills (SDYM) equation in the so-called J formulation. In particular, the infinitesimal "hidden symmetry'' transformation, a linear system, and a well-known Backlund transformation of the SDYM equation are derived in the process. Thus symmetry and integrability aspects of the SDYM system appear in natural relationship to each other within the framework of the isovector approach.

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Hydrodynamic Fluctuations In A Fluid Under Constant Shear, Alejandro Garcia, M. Malek Mansour, G. Lie, E. Clementi, M. Mareschal Jan 1987

Hydrodynamic Fluctuations In A Fluid Under Constant Shear, Alejandro Garcia, M. Malek Mansour, G. Lie, E. Clementi, M. Mareschal

Faculty Publications

No abstract provided.

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Fluctuating Hydrodynamics In A Dilute Gas, Alejandro Garcia, G. Lie, E. Clementi Jan 1987

Fluctuating Hydrodynamics In A Dilute Gas, Alejandro Garcia, G. Lie, E. Clementi

Faculty Publications

Hydrodynamic fluctuations in a dilute gas subjected to a constant heat flux are studied by both a computer simulation and the Landau-Lifshitz formalism. The latter explicitly incorporates the boundary conditions of the finite system, thus permitting quantitative comparison with the former. Good agreement is demonstrated.

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Anneal Induced Changes In Amorphous Semiconductor Multilayers, David D. Allred, Jesus González-Hernández, O. V. Nguyen Jan 1987

Anneal Induced Changes In Amorphous Semiconductor Multilayers, David D. Allred, Jesus González-Hernández, O. V. Nguyen

Faculty Publications

We have prepared, heat treated and characterized various amorphous semiconductor periodic multilayers and ultrathin films. These were prepared by several vapor deposition techniques at substrate temperatures ranging from 25°C to 300°C and possessed periodicities from 22 to 400Å. Films were subjected to isochronal thermal treatments at progressively higher temperatures. Two effects were observed: enhanced diffusion and retarded crystallization. Interdiffusion, at rates which are many orders of magnitude higher than those anticipated from crystalline data, was observed in a-Si/a-Ge multilayers. Crystallization of germanium, the more readily crystallized member of the couple, is retarded; the extent depends on the thickness of the …

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Equilibrium Properties Of Short Field-Reversed Configurations, Ross L. Spencer, M. Tuszewski Nov 1986

Equilibrium Properties Of Short Field-Reversed Configurations, Ross L. Spencer, M. Tuszewski

Faculty Publications

Some features of short field-reversed configuration (FRC) equilibria relevant to transport and stability are studied numerically and analytically. It is shown that magnetic field curvature effects significantly increase the FRC magnetization for plasma elongations epsilon is less than or equal to 4.

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Considerations Of Temperature Stability In A Cylindrical Plasma, S. Neil Rasband, Yao-Hui Xu Aug 1986

Considerations Of Temperature Stability In A Cylindrical Plasma, S. Neil Rasband, Yao-Hui Xu

Faculty Publications

A variational formulation is used to consider thermal equilibrium and stability for a cylindrical plasma modeled by dissipative magnetohydrodynamics. The parameter dependence of equilibrium solutions and their stability is followed using homotopy techniques. Solution branches and their connections are studied in relation to the applied fields.

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Nonequilibrium Fluctuations Studied By A Rarefied Gas Simulation, Alejandro Garcia Jan 1986

Nonequilibrium Fluctuations Studied By A Rarefied Gas Simulation, Alejandro Garcia

Faculty Publications

A dilute gas under a constant heat flux is studied with use of a Monte Carlo simulation based on the Boltzmann equation. Results for several spatial correlation functions of equal-time fluctuations are reported and compared qualitatively with previous fluctuating hydrodynamics calculations for liquids.

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A Generalized Molien Function For Field Theoretical Hamiltonians, Jeffrey W. Felix, Dorian M. Hatch Jul 1985

A Generalized Molien Function For Field Theoretical Hamiltonians, Jeffrey W. Felix, Dorian M. Hatch

Faculty Publications

A generating function, or Molien function, the coefficients of which give the number of independent polynomial invariants in G, has been useful in the Landau and renormalization group theories of phase transitions. Here a generalized Molien function for a field theoretical Hamiltonian (with short-range interactions) of the most general form invariant in a group G is derived. This form is useful for more general renormalization group calculations. Its Taylor series is calculated to low order for the FGamma-2 representation of the space group R[3 bar]c and also for the l=1 (faithful) representation of SO(3).

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Example Of A Group Action Determined Phase Transition, Jeffrey W. Felix, Dorian M. Hatch Feb 1985

Example Of A Group Action Determined Phase Transition, Jeffrey W. Felix, Dorian M. Hatch

Faculty Publications

The principles of the group action approach to structural phase transitions are outlined. It is assumed that all properties of the transition are determined by the action of a single physically irreducible represention of the space group of the more symmetric phase. We determine the isotropy groups using the image space of the representation. The free energy minima are determined to fourth order and to all orders using the results of Gufan and then compared. This theory is applied to Calcite (Roverline3c) to determine all possible continuous commensurate phase transitions.

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Isee/Ice Data Reduction And Analysis: Magnetic Fields, Edward J. Smith, Douglas E. Jones, George L. Siscoe, Bruce T. Tsurutani Jul 1984

Isee/Ice Data Reduction And Analysis: Magnetic Fields, Edward J. Smith, Douglas E. Jones, George L. Siscoe, Bruce T. Tsurutani

Faculty Publications

In accordance with the instructions provided by GSFC, the work has been divided into a number of individual study tasks. For each task, a brief narrative description and a budget are provided. Task I, the Core Task, is treated as a single task. Task II, concerning the comet, is a single task. Task III is subdivided into three major categories: (A) on-going interplanetary studies begun in prior years (B) on-going magnetotail studies begun in FY'84 and (C) new studies proposed for FY'85 and '86.

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Isotropy Group Description Of A Phase Transition In Nano3, W. Scott Stornetta, Dorian M. Hatch Jun 1984

Isotropy Group Description Of A Phase Transition In Nano3, W. Scott Stornetta, Dorian M. Hatch

Faculty Publications

Predictions of the possible post-transition symmetries of an R 3c zone center continuous phase transition are made using recent extensions of the Landau theory. The Landau theory is summarized and direct group theoretical methods are applied to the R 3c phase. General techniques for solving systems of nonlinear polynomial equations are reviewed and these techniques are applied to the minimization of the free energy F for the aforementioned possible symmetries. The results of the direct methods and the minimization procedures are shown to be compatible. It is shown that the transition to R 3c in NaNO3 is consistent with the …

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Unification Of Ernst-Equation Backlund Transformations Using A Modified Wahlquist-Estabrook Technique; Wahlquist-Estabrook, B. Kent Harrison Aug 1983

Unification Of Ernst-Equation Backlund Transformations Using A Modified Wahlquist-Estabrook Technique; Wahlquist-Estabrook, B. Kent Harrison

Faculty Publications

The three known Backlund transformations for the Ernst equation are derived using a modification of the Wahlquist-Estabrook prolongation procedure. The modification requires that the equation to be studied be cast into a set of differential forms and their exterior derivatives, such that all coefficients are constant (a "CC ideal''). Analysis of the resulting equations produces 16 solutions composed of the three basic transformations combined with identity and other essentially trivial transformations. The group structure of the transformations is discussed. A Backlund transformation (already known) for the Ernst-Maxwell equations can be found by the same method. Promising generalizations are mentioned.

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