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Faculty Publications

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Articles 511 - 540 of 685

Full-Text Articles in Astrophysics and Astronomy

Spontaneous Lorentz Violation And Nonpolynomial Interactions, Brett Altschul, V. Alan Kostelecký Nov 2005

Spontaneous Lorentz Violation And Nonpolynomial Interactions, Brett Altschul, V. Alan Kostelecký

Faculty Publications

Gauge-noninvariant vector field theories with superficially nonrenormalizable nonpolynomial interactions are studied. We show that nontrivial relevant and stable theories have spontaneous Lorentz violation, and we present a large class of asymptotically free theories. The Nambu-Goldstone modes of these theories can be identified with the photon, with potential experimental implications. © 2005 Elsevier B.V. All rights reserved.

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Using Genetic Algorithms To Map First-Principles Results To Model Hamiltonians: Application To The Generalized Ising Model For Alloys, Gus L. W. Hart, Volker Blum, Michael J. Walorski, Alex Zunger Oct 2005

Using Genetic Algorithms To Map First-Principles Results To Model Hamiltonians: Application To The Generalized Ising Model For Alloys, Gus L. W. Hart, Volker Blum, Michael J. Walorski, Alex Zunger

Faculty Publications

The cluster expansion method provides a standard framework to map first-principles generated energies for a few selected configurations of a binary alloy onto a finite set of pair and many-body interactions between the alloyed elements. These interactions describe the energetics of all possible configurations of the same alloy, which can hence be readily used to identify ground state structures and, through statistical mechanics solutions, find finite-temperature properties. In practice, the biggest challenge is to identify the types of interactions which are most important for a given alloy out of the many possibilities. We describe a genetic algorithm which automates this …

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Direct Enumeration Of Alloy Configurations For Electronic Structural Properties, Gus L. W. Hart, Peter A. Graf, Kwiseon Kim, Wesley B. Jones Oct 2005

Direct Enumeration Of Alloy Configurations For Electronic Structural Properties, Gus L. W. Hart, Peter A. Graf, Kwiseon Kim, Wesley B. Jones

Faculty Publications

We present and apply an approach to directly enumerate the band gaps and effective masses of all possible zinc blende-based alloy configurations whose unit cell contains up to a specified number of atoms. This method allows us to map the space of band gaps and effective masses versus alloy composition and atomic configuration. We demonstrate that a large number of band gaps and effective masses are available. We also discuss convergence of the method with respect to unit cell size and the combined optimization of band gap and effective mass for AlGaAs and GaInP semiconductor alloys.

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Commutation Relations For Functions Of Operators, Mark K. Transtrum, Jean-Francois S. Van Huele Jun 2005

Commutation Relations For Functions Of Operators, Mark K. Transtrum, Jean-Francois S. Van Huele

Faculty Publications

We derive an expression for the commutator of functions of operators with constant commutations relations in terms of the partial derivatives of these functions. This result extends the well-known commutation relation between one operator and a function of another operator. We discuss the range of applicability of the formula with examples in quantum mechanics

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Microgravity Studies Of Aggregation In Particulate Clouds, Todd B. Sauke, J. R. Marshall, J. N. Cuzzi Jun 2005

Microgravity Studies Of Aggregation In Particulate Clouds, Todd B. Sauke, J. R. Marshall, J. N. Cuzzi

Faculty Publications

Aggregation in clouds of submillimeter quartz and volcanic ash particles was studied in microgravity. Particle clouds generated by pulses of air immediately formed electrostatic filamentary aggregates upon cessation of air turbulence. Manual agitation of experiment chambers produced cm-size loose grain clusters which voraciously scavenged free-floating material in their vicinity. A dipole model accounts for these observations. Experimental results have ramifications for the behavior of natural cloud systems and primary accretion of solids in the early solar nebula.

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Erratum: Computing The M = 1 Diocotron Frequency Via An Equilibrium Calculation In Non-Neutral Plasmas, Ross L. Spencer May 2005

Erratum: Computing The M = 1 Diocotron Frequency Via An Equilibrium Calculation In Non-Neutral Plasmas, Ross L. Spencer

Faculty Publications

Equation 14 in this paper contains errors.

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The Effect Of Inharmonic Partials On Pitch Of Piano Tones, Brian E. Anderson, William J. Strong Apr 2005

The Effect Of Inharmonic Partials On Pitch Of Piano Tones, Brian E. Anderson, William J. Strong

Faculty Publications

Piano tones have partials whose frequencies are sharp relative to harmonic values. A listening test was conducted to determine the effect of inharmonicity on pitch for piano tones in the lowest three octaves of a piano. Nine real tones from the lowest three octaves of a piano were analyzed to obtain frequencies, relative amplitudes, and decay rates of their partials. Synthetic inharmonic tones were produced from these results. Synthetic harmonic tones, each with a twelfth of a semitone increase in the fundamental, were also produced. A jury of 21 listeners matched the pitch of each synthetic inharmonic tone to one …

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Two-Photon Photoionization Of The Ca 4s3d^1d2 Level In An Optical Dipole Trap, E. A. Cummings, J. E. Daily, Dallin S. Durfee, Scott D. Bergeson, R. Gommers Apr 2005

Two-Photon Photoionization Of The Ca 4s3d^1d2 Level In An Optical Dipole Trap, E. A. Cummings, J. E. Daily, Dallin S. Durfee, Scott D. Bergeson, R. Gommers

Faculty Publications

We report an optical dipole trap for calcium. The trap is created by focusing a 488-nm argon-ion laser beam into a calcium magneto-optical trap. The argon-ion laser photoionizes atoms in the trap because of a near-resonance with the 4s4f 1^F3 level. By measuring the dipole-trap decay rate as a function of argon-ion laser intensity, we determine the 1^F3 photoionization cross section at our wavelength to be approximately 230 Mb.

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Sound-Quality Analysis Of Sewing Machines (A), James Chatterley, Andrew Boone, Jonathan T. Blotter, Scott D. Sommerfeldt Apr 2005

Sound-Quality Analysis Of Sewing Machines (A), James Chatterley, Andrew Boone, Jonathan T. Blotter, Scott D. Sommerfeldt

Faculty Publications

Sound quality analysis procedure and results for six sewing machines ranging from entry level to professional grade will be presented. The procedure consisted of jury-based listening tests and quantification of sound quality using standard metrics. The procedures and analysis of the jury testing will be presented and discussed. The correlation between the quantitative metrics and the qualitative jury results will be presented. Sound localization scans, using near field acoustic holography techniques with accompanying results, performed in order to determine machine sound hot spots and possible sources for undesired sounds, will also be presented. Proposed modifications to machine structure in order …

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Mass-To-Light Ratio Gradients In Early-Type Galaxy Haloes, N. R. Napolitano, M. Capaccioli, Aaron J. Romanowsky, N. G. Douglas, M. R. Merrifield, K. Kuijken, M. Arnaboldi, O. Gerhard, K. C. Freeman Jan 2005

Mass-To-Light Ratio Gradients In Early-Type Galaxy Haloes, N. R. Napolitano, M. Capaccioli, Aaron J. Romanowsky, N. G. Douglas, M. R. Merrifield, K. Kuijken, M. Arnaboldi, O. Gerhard, K. C. Freeman

Faculty Publications

Owing to the fact that the near future should see a rapidly expanding set of probes of the halo masses of individual early-type galaxies, we introduce a convenient parameter for characterizing the halo masses from both observational and theoretical results: ∇ℓϒ, the logarithmic radial gradient of the mass-to-light ratio. Using halo density profiles from Λ-cold dark matter (CDM) simulations, we derive predictions for this gradient for various galaxy luminosities and star formation efficiencies εSF. As a pilot study, we assemble the available ∇ℓϒ data from kinematics in early-type galaxies – representing the first unbiased study of halo masses in a …

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Thorium-Based Thin Films As Highly Reflective Mirrors In The Euv, David D. Allred, William R. Evans, Jed E. Johnson, Richard L. Sandberg, R. Steven Turley Jan 2005

Thorium-Based Thin Films As Highly Reflective Mirrors In The Euv, David D. Allred, William R. Evans, Jed E. Johnson, Richard L. Sandberg, R. Steven Turley

Faculty Publications

As applications for extreme ultraviolet (EUV) radiation have been identified, the demand for better optics has also increased. Thorium and thorium oxide thin films (19 to 61 nm thick) were RF-sputtered and characterized using atomic force microscopy (AFM), spectroscopic ellipsometry, low-angle x-ray diffraction (LAXRD), x-ray photoelectron spectroscopy (XPS), and x-ray absorption near edge structure (XANES) in order to assess their capability as EUV reflectors. Their reflectance and absorption at different energies were also measured and analyzed at the Advanced Light Source in Berkeley. The reflectance of oxidized thorium is reported between 2 and 32 nm at 5, 10, and 15 …

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Computing The M = 1 Diocotron Frequency Via An Equilibrium Calculation In Non-Neutral Plasmas, Ross L. Spencer Oct 2004

Computing The M = 1 Diocotron Frequency Via An Equilibrium Calculation In Non-Neutral Plasmas, Ross L. Spencer

Faculty Publications

The m = 1 diocotron mode in non-neutral plasmas has long been thought of as a shifted equilibrium, and its frequency has been approximately calculated in this way by Fine and Driscoll [Phys. Plasmas 5, 601 (1998)]. This article shows that this idea can be coupled with a standard axisymmetric equilibrium calculation on a grid to calculate the frequency of this mode to very high precision including both finite-length and thermal effects, provided that the Debye length is small enough. As the Debye length begins to approach the plasma size not only does the shifted equilibrium calculation fail to predict …

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Optical Properties And Application Of Uranium-Based Thin Films For The Extreme Ultraviolet And Soft X-Ray Region, Richard L. Sandberg, David D. Allred, Shannon Lunt, Marie K. Urry, R. Steven Turley Oct 2004

Optical Properties And Application Of Uranium-Based Thin Films For The Extreme Ultraviolet And Soft X-Ray Region, Richard L. Sandberg, David D. Allred, Shannon Lunt, Marie K. Urry, R. Steven Turley

Faculty Publications

Uranium oxide and uranium nitride thin films reflect significantly more than all previously known/standard reflectors (e.g., nickel, gold, and iridium) for most of the 4-10 nm range at low angles of incidence. This work includes measurements of the EUV/soft x-ray (2-20 nm) reflectance of uranium-based thin films (~20 nm thick) and extraction of their optical constants (d and ?). We report the reflectances at 5, 10, and 15 degrees grazing incidence of air-oxidized sputtered uranium, reactively sputtered (O2) uranium oxide, and reactively sputtered (N2) uranium nitride thin films measured at Beamline 6.3.2 at the Advanced Light Source (ALS) at Lawrence …

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Removing Surface Contaminants From Silicon Wafers To Facilitate Euv Optical Characterization, Richard L. Sandberg, David D. Allred, A. L. Jackson, J. E. Johnson, W. Evans, T. Doughty, A. E. Baker, K. Adamson, A. Jacquier, R. E. Robinson Apr 2004

Removing Surface Contaminants From Silicon Wafers To Facilitate Euv Optical Characterization, Richard L. Sandberg, David D. Allred, A. L. Jackson, J. E. Johnson, W. Evans, T. Doughty, A. E. Baker, K. Adamson, A. Jacquier, R. E. Robinson

Faculty Publications

The extreme ultraviolet (EUV) is becoming increasingly important. Principal applications include orbital space-based astronomy and lithography for integrated circuit computer chips. A main impediment to further development of efficient mirrors is the lack of reliable optical constants for various materials in this region of the electromagnetic spectrum. One reason for the unreliability of the optical constants is that the sample surfaces are often contaminated with foreign material, especially organic compounds, when exposed to laboratory air. Several cleaning techniques were evaluated, namely: 1) strippable solid optical cleaner (Opticlean®); 2) oxygen plasma etch; 3) high energy UV light/ozone; 4) strippable coating followed …

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Microsecond Spin-Flip Times In N-Gaas Measured By Time-Resolved Polarization Of Photoluminescence, John S. Colton, T. A. Kennedy, A. S. Bracker, D. Gammon Mar 2004

Microsecond Spin-Flip Times In N-Gaas Measured By Time-Resolved Polarization Of Photoluminescence, John S. Colton, T. A. Kennedy, A. S. Bracker, D. Gammon

Faculty Publications

We have observed microsecond spin-flip times in lightly doped n-GaAs, by measuring the photoluminescence polarization in the time domain with pump and probe pulses. Times up to 1.4 μs have been measured. Our results as a function of magnetic field indicated three regions governing the spin relaxation: a low field region, where spin-flip times increase due to suppression of the nuclear hyperfine interaction for localized electrons, a medium field region where spin-flip times increase due to narrowing of the hyperfine relaxation for interacting electrons, and a high field region where spin-flip times begin to level off due to the increasing …

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Boron Alloying In Gan, Gus L. W. Hart, Laurian Escalanti Feb 2004

Boron Alloying In Gan, Gus L. W. Hart, Laurian Escalanti

Faculty Publications

Using first-principles calculations in the local density approximation, we studied effects of adding up to 6% boron to zinc-blende GaN. We found that the band gap increases monotonically with boron incorporation, in agreement with experiment. A composition-independent band-gap bowing parameter of 4.30 eV was determined, and proved to be large compared to bowing for other mixed cation systems. The formation enthalpy of mixing, ΔH, was determined for BxGa1-xN, BxGa1-xAs, and GaAs1-xNx. A comparison of enthalpies indicates that the production of BxGa1-xN films with boron concentrations of at least 5% may be possible.

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Rectification Of Thermal Fluctuations In Ideal Gases, Alejandro Garcia, P. Meurs, C. Van De Broeck Jan 2004

Rectification Of Thermal Fluctuations In Ideal Gases, Alejandro Garcia, P. Meurs, C. Van De Broeck

Faculty Publications

We calculate the systematic average speed of the adiabatic piston and a thermal Brownian motor, introduced by C. Van den Broeck, R. Kawai and P. Meurs [Phys. Rev. Lett. 93, 090601 (2004)], by an expansion of the Boltzmann equation and compare with the exact numerical solution.

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Uranium Oxide As A Highly Reflective Coating From 100-400 Ev, Richard L. Sandberg, David D. Allred, Luke J. Bissell, Jed E. Johnson, R. Steven Turley Jan 2004

Uranium Oxide As A Highly Reflective Coating From 100-400 Ev, Richard L. Sandberg, David D. Allred, Luke J. Bissell, Jed E. Johnson, R. Steven Turley

Faculty Publications

We present the measured reflectances (Beamline 6.3.2, ALS and LBNL) of naturally oxidized uranium and naturally oxidized nickel thin films from 100-460 eV (2.7 to 11.6 nm) at 5 and 15 degrees grazing incidence. These show that uranium as UO2, can fulfill its promise as the highest known single surface reflector for this portion of the soft x-ray region, being nearly twice as reflective as nickel in the 124-250 eV (5-10 nm) region. This is due to its large index of refraction coupled with low absorption. Nickel is commonly used in soft x-ray applications in astronomy and synchrotrons. (Its reflectance …

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Long Coherence Times At 300 K For Nitrogen-Vacancy Center Spins In Diamond Grown By Chemical Vapor Deposition, John S. Colton, T. A. Kennedy, J. E. Butler, R. C. Linares, P.J. Doering Nov 2003

Long Coherence Times At 300 K For Nitrogen-Vacancy Center Spins In Diamond Grown By Chemical Vapor Deposition, John S. Colton, T. A. Kennedy, J. E. Butler, R. C. Linares, P.J. Doering

Faculty Publications

Electron-spin-echo experiments reveal phase-memory times as long as 58 μs at 300 K for nitrogen-vacancy centers in chemical vapor deposition (CVD) single crystals. The spins were optically polarized and optically detected. Two high-quality CVD samples were studied. From the current results, it is not clear whether these phase-memory times represent a fundamental limit or are limited by an external source of decoherence.

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Ordering Tendencies In Octahedral Mgo-Zno Alloys, Gus L. W. Hart, Mahdi Sanati, Alex Zunger Oct 2003

Ordering Tendencies In Octahedral Mgo-Zno Alloys, Gus L. W. Hart, Mahdi Sanati, Alex Zunger

Faculty Publications

Isostrutural II-VI alloys whose components are either rocksalt stable (e.g., CaO-MgO) or zincblende stable (e.g., ZnS-ZnSe) are known to be thermodynamically unstable at low temperatures, showing a miscibility gap and no bulk ordering. In contrast, we show that heterostructural MgO-ZnO is stable, under certain conditions, in the sixfold-coordinated structure for Zn concentrations below 67%, giving rise to spontaneously ordered alloys. Using first-principles calculations, we explain the origin of this stability, the structures of their low-temperature ordered phases, short-range-order patterns, and their optical band-gap properties.

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Allowed Mesoscopic Point Group Symmetries In Domain Average Engineering Of Perovskite Ferroelectric Crystals, Dorian M. Hatch, H. T. Stokes, W. Cao Oct 2003

Allowed Mesoscopic Point Group Symmetries In Domain Average Engineering Of Perovskite Ferroelectric Crystals, Dorian M. Hatch, H. T. Stokes, W. Cao

Faculty Publications

In multivariant systems, several energetically degenerate low temperature domain states can be produced at the structural phase transition. Coexistence of these domain states can produce mesoscopic structures that possess symmetries distinct from the microscopic single domain crystal symmetry. Such engineered domain structures in certain ferroelectric materials have been proven to give superior piezoelectric properties and extremely soft shear moduli. The objective of this article is to consider the variety of symmetries that can be produced through domain average engineering in proper ferroelectric systems arising from the cubic Pm[overline 3]m symmetry perovskite structure.

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Search For ΝΜ→ΝE Oscillations In The Nomad Experiment, Nomad Collaboration, P. Astier, D. Autiero, A. Baldisseri, M. Baldo-Ceolin, M. Banner, G. Bassompierre, K. Benslama, N. Besson, I. Bird, B. Blumenfeld, F. Bobisut, J. Bouchez, S. Boyd, A. Bueno, S. Buyatov, L. Camilleri, A. Cardini, P. W. Cattaneo, V. Cavasinni, Roberto Petti, Et. Al. Sep 2003

Search For ΝΜ→ΝE Oscillations In The Nomad Experiment, Nomad Collaboration, P. Astier, D. Autiero, A. Baldisseri, M. Baldo-Ceolin, M. Banner, G. Bassompierre, K. Benslama, N. Besson, I. Bird, B. Blumenfeld, F. Bobisut, J. Bouchez, S. Boyd, A. Bueno, S. Buyatov, L. Camilleri, A. Cardini, P. W. Cattaneo, V. Cavasinni, Roberto Petti, Et. Al.

Faculty Publications

We present the results of a search for νµ → νe oscillations in the NOMAD experiment at CERN. The experiment looked for the appearance of νe in a predominantly νµ wide-band neutrino beam at the CERN SPS. No evidence for oscillations was found. The 90% confidence limits obtained are ∆m2 < 0.4 eV2 for maximal mixing and sin2(2θ)−3 for large ∆m2. This result excludes the LSND allowed region of oscillation parameters with ∆m2 ≳∆10 eV2.

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First-Principles Calculations For Nitrogen-Containing Single-Walled Carbon Nanotubes, James P. Lewis, Mingwen Zhao, Yueyugan Xia, Ruiqin Zhang Aug 2003

First-Principles Calculations For Nitrogen-Containing Single-Walled Carbon Nanotubes, James P. Lewis, Mingwen Zhao, Yueyugan Xia, Ruiqin Zhang

Faculty Publications

We present calculations for possible configurations of nitrogen-containing single-walled carbon nanotubes and their electronic properties obtained with the ab initio tight-binding FIREBALL method. It is found that nitrogen atoms can be energetically incorporated into the carbon network in three forms: Substitution, substitution with formation of a vacancy structure, and chemical adsorption. The different forms exhibit different local densities of states near the Fermi levels, which might suggest a potential method to control the electronic properties of nitrogen-doped carbon nanotubes

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Observation Of And Model For Nonlinear Mode Conversion In A Non-Neutral Plasma, Grant W. Hart, Bryan G. Peterson, Ross L. Spencer Jul 2003

Observation Of And Model For Nonlinear Mode Conversion In A Non-Neutral Plasma, Grant W. Hart, Bryan G. Peterson, Ross L. Spencer

Faculty Publications

The nonlinear interaction of the two lowest Trivelpiece-Gould modes in a non-neutral plasma has been observed. Because of coupling in the nonlinear terms of the continuity and momentum equations, the two modes can exchange energy and convert one to the other. This can be modeled using the cold fluid equations and the averaging method. Experimentally, this process always stops with the lower frequency mode dominating the final state. Numerical integration of the model suggests that this occurs because the higher frequency mode is more strongly damped than the lower frequency mode.

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Decay Of Trapped-Particle Asymmetry Modes In Non-Neutral Plasmas In A Malmberg-Penning Trap, Grant W. Mason May 2003

Decay Of Trapped-Particle Asymmetry Modes In Non-Neutral Plasmas In A Malmberg-Penning Trap, Grant W. Mason

Faculty Publications

The mechanism for the strong damping of diocotron-like azimuthal trapped-particle asymmetry modes in a Malmberg-Penning trap is investigated with a detailed three-dimensional particle-in-cell computer simulation. The m = 1,kzis not equal to 0 modes are created by a voltage squeeze from a mid-detector ring followed by a displacement of trapped particles in opposite directions on either side of the ring. The voltage squeeze creates a population of particles confined to half the trap length (trapped) and a population of particles that move longitudinally along the full length of the cylinder (untrapped). The damping of the modes is found to be …

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Optically Oriented And Detected Electron Spin Resonance In A Lightly Doped N-Gaas Layer, John S. Colton, T. A. Kennedy, A. S. Bracker, D. Gammon, J. B. Miller Apr 2003

Optically Oriented And Detected Electron Spin Resonance In A Lightly Doped N-Gaas Layer, John S. Colton, T. A. Kennedy, A. S. Bracker, D. Gammon, J. B. Miller

Faculty Publications

Spin resonance of localized electrons bound to donors in a specially designed n-GaAs layer has been performed at 236 MHz and 41 mT, using circular polarized light to polarize the electrons and photoluminescence to detect the electronic polarization. The polarization was diminished under the resonance condition. The electronic g factor obtained by this measurement is - 0.41 ± 0.01. The resonance linewidth of 2 mT corresponds to a spin lifetime of 28 ns. In order to observe the electronic spin resonance, nuclear effects were eliminated by application of rf fields to simultaneously resonate the nuclear spins.

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Modes In A Non-Neutral Plasma Of Finite Length, M = 0,1, S. Neil Rasband, Ross L. Spencer Apr 2003

Modes In A Non-Neutral Plasma Of Finite Length, M = 0,1, S. Neil Rasband, Ross L. Spencer

Faculty Publications

For realistic, cold equilibria of finite length representing a pure electron plasma confined in a cylindrical Malmberg–Penning trap, the mode spectrum for Trivelpiece–Gould, m=0, and for diocotron, m=1, modes is calculated numerically. A novel method involving finite elements is used to successfully compute eigenfrequencies and eigenfunctions for plasma equilibria shaped like pancakes, cigars, long cylinders, and all things in between. Mostly sharp-boundary density configurations are considered but also included in this study are diffuse density profiles including ones with peaks off axis leading to instabilities. In all cases the focus has been on elucidating the role of finite length in …

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What The Universe Means To People Like Me, David D. Allred Mar 2003

What The Universe Means To People Like Me, David D. Allred

Faculty Publications

When I picked up David's paper to read it, I had a pencil in my hand. Years of reading my students' and my own papers made it natural to edit as I read. However, I heard in my mind the voice of my mother advising me to put the pencil down. This wasn't time to edit but to hear and understand. Still, I kept the pencil in my hand for the first few pages and made a few notes before I put it down and just read. I could hear David's voice speaking the words I read. It was good …

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Neutral-Plasma Oscillations At Zero Temperature, Scott D. Bergeson, Ross L. Spencer Feb 2003

Neutral-Plasma Oscillations At Zero Temperature, Scott D. Bergeson, Ross L. Spencer

Faculty Publications

Cold plasma theory is used to calculate the response of an ultracold neutral plasma to an applied rf field. The free oscillation of the system has a continuous spectrum and an associated damped quasimode. This quasimode dominates the driven response and is resonant in the tail of the density distribution. Recent experiments used the plasma response to an applied rf field to determine the plasma density in an expanding ultracold plasma. The comparison between experiment and theory indicates that this method accurately determines the expansion velocity and underestimates the initial plasma density by a factor of 3 in weakly collisional …

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Chemomechanical Surface Patterning And Functionalization Of Silicon Surfaces Using An Atomic Force Microscope, Brent A. Wascaser, Michael J. Maughan, Travis L. Niederhauser, Matthew R. Linford, Robert C. Davis, Ian A. Mowat Feb 2003

Chemomechanical Surface Patterning And Functionalization Of Silicon Surfaces Using An Atomic Force Microscope, Brent A. Wascaser, Michael J. Maughan, Travis L. Niederhauser, Matthew R. Linford, Robert C. Davis, Ian A. Mowat

Faculty Publications

Surface modification and patterning at the nanoscale is a frontier in science with significant possible applications in biomedical technology and nanoelectronics. Here we show that an atomic force microscope (AFM) can be employed to simultaneously pattern and functionalize hydrogen-terminated silicon (111) surfaces. The AFM probe was used to break Si-H and Si-Si bonds in the presence of reactive molecules, which covalently bonded to the scribed Si surface. Functionalized patches and patterned lines of molecules were produced. Linewidths down to 30 nm were made by varying the force at the tip

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