Nuclear Engineering Commons^™

A Comparison Of Fixed Versus Moving Eulerian Meshes For 1-D Radiative Shock Problems, Dylan Weatherred

Nuclear Engineering ETDs

Testing codes used to solve the radiation-hydrodynamics equations requires the use of radiative shock problems. These problems contain stiff shocks and test the coupling of the material motion and the energy exchange between the radiation and material. However, these problems are difficult to solve due to large differences in time scale between radiation and material equations, resolving shocks, and modeling radiation and material interactions. This thesis will look to solve radiative shock problems in 1-D using the Eulerian formulation on fixed and moving meshes. The moving mesh method proposed takes advantage of the more simple Eulerian formulation of the radiation …

Preparation Of High Entropy Titanite Pyrochlore And Radiation Stability Study, Adam Gootgeld

All Theses

Pyrochlore has been studied as a host phase for safe storage of radionuclides and exists naturally with long-term stability with good long-range order [1]. High entropy oxides show promising tunable properties that could demonstrate favorable bulk deposit of radioactive materials such as spent nuclear fuel (Uranium and other actinides). It is proposed that using high entropy oxides (HEOs) as the cation in this framework will shift the gibbs free energy so that radioactive nuclear waste will be stabilized for safe, long-term, eco-friendly storage. We have established a consistent method to fabricate high entropy titanite pyrochlores. In this study, ion beam …

Miniature, Submersible Electromagnetic Pumps Of Molten Lead And Sodium For Gen-Iv Nuclear Reactors Development, Ragai M. Altamimi

Nuclear Engineering ETDs

Heavy metals and alkali Liquid Metals are suitable coolants for Generation IV terrestrial nuclear reactors for operating at elevated temperatures for achieving plant thermal efficiency more than 40% and the thermochemical generation of hydrogen fuel. In addition, the low vapor pressure of these liquids eliminates the need for a pressure vessel and instead operates slightly below ambient pressure. A primary issue with the uses of these coolants is their compatibility with nuclear fuel, cladding and core structure materials at elevated temperatures more than 500oC. Therefore, in pile and out-of-pile test loops have been constructed or being considered for quantifying the …

Electrochemical Approaches To Life-Support Resources In Space Missions And Nuclear Technologies: Hydrogen Peroxide And Uranium Films, Armando Manuel Pena-Duarte

Open Access Theses & Dissertations

Space race has developed several technological advances that have achieved and continue to achieve the success of space missions in the aerospace timeline. Currently, the number of space technical and scientific innovations is still growing––demanding new materials and developments for extreme performing applications of fuel cells, batteries, supercapacitors, and systems of nuclear energy. Space missions require life-support solutions, auto-sustainable closed-loop living environments, cleaning and sanitizing solutions against pathogens, and safe nuclear-based resources of energy––with fissile materials with well-controlled dimensions within the core fuel elements. Likewise, to guarantee safety conditions, reduce costs, and facilitate operational logistics, space missions must reduce their …

Sensitivity And Uncertainty Analysis Of Inertial Confinement Fusion Experiments, Colin A. Weaver

Nuclear Engineering ETDs

Sandia National Laboratories conducts Magnetized Liner Inertial Fusion (MagLIF) experiments at the Z Pulsed Power Facility. Their objective is to study the burning plasma formed under magnetic direct drive Inertial Confinement Fusion (ICF) conditions and use the inferred information to reduce uncertainty in computational models and improve experimental designs. The Z machine has five neutron time-of-flight (nToF) detectors that measure the fusion neutron time spectrum from three lines-of-sight. Together, these signals are used to infer the ion temperature, target liner mass density, and the burn history of the MagLIF experiment from measured data. These parameters are a few used by …

Measurements Of Scintillation Light Quenching For Protons In Rare-Earth Inorganic Scintillators, Tatiana Nathaly Espinoza

Nuclear Engineering ETDs

Scintillator detectors have become a leading choice of radiation detectors for a variety of applications, including space science. Due to their intrinsic characteristics, rare-earth inorganic scintillators provide the capability to detect both gamma and charged particles in a small detector. The response of these detectors is typically characterized using isotropic gamma sources. However, the light output produced in the scintillator from an incident gamma of a particular energy differs from the light output produced from an incident charged particle of the same energy; a phenomenon known as quenching. Using two types of rare-earth inorganic scintillators, Y2SiO5(YSO:Ce), and Gd₃Al₂Ga₃O₁₂(GAGG:Ce), we measured …

Conceptual Design And Preliminary Safety Analysis Of A Proposed Nuclear Microreactor For Mobile Application, A. S. M. Fakhrul Islam

Theses and Dissertations

Conceptual design and preliminary safety analysis of a proposed helium-cooled Micro Nuclear reactor In ONe megawatt (MINION) thermal output is done through three-dimensional computational analysis. Compared with the conventional high temperature gas-cooled reactors (HTGR) that use tri-structural or bi-structural isotropic (TRISO or BISO) fuel particles, MINION uses traditional clad fuel pellets. This greatly simplifies the core design and allows for a substantially more compact design thanks to the fuel’s signif-icantly higher U-235 atom density. Uranium carbide (UC) enriched up to 19.75% in U-235 is used as fuel. In the power-flattened design, U-235 enrichment varies radially between 19.75% and 10.5% in …

Vi Energy-Efficient Memristor-Based Neuromorphic Computing Circuits And Systems For Radiation Detection Applications, Jorge Iván Canales Verdial

Electrical and Computer Engineering ETDs

Radionuclide spectroscopic sensor data is analyzed with minimal power consumption through the use of neuromorphic computing architectures. Memristor crossbars are harnessed as the computational substrate in this non-conventional computing platform and integrated with CMOS-based neurons to mimic the computational dynamics observed in the mammalian brain’s visual cortex. Functional prototypes using spiking sparse locally competitive approximations are presented. The architectures are evaluated for classification accuracy and energy efficiency. The proposed systems achieve a 90% true positive accuracy with a high-resolution detector and 86% with a low-resolution detector.

Material Reliability For A Molten Chloride Salt System, Aaron A.H. Overacker

Nuclear Engineering ETDs

Energy efficiency and cost reduction can both be improved upon using overall higher temperatures for the working fluid. This interest is shared in both nuclear energy as well as concentrated solar power. To achieve higher temperatures would require industry to change working fluids. The United States Department of Energy set out a goal of operating concentrated solar to above 700℃. This would help reduce the cost by having more efficiency in the thermal energy storage, while not a concern for nuclear, these high temperatures can reduce the safety risk and pressure use with the implementation of molten salts. The National …

Molecular Dynamics Study For Tritium Adsorption On Novel Materials, Jason Viscardi, Benjamin Robinson, Asher Flanagan

Symposium of Student Scholars

In this study, novel materials will be researched, and their potential uses for tritium control. 12 studies have been collected on various materials that give a solid foundation for future research that will be conducted regarding tritium control. All these studies used molecular dynamics simulation (MDS) to generate results. The first paper found from a university in Crete, Greece discussed pillared graphene to store hydrogen in a novel 3D carbon nanostructure in which pore size and surface area can be adjusted to suit the need. This was the first of several studies that aim to arrange the graphene in such …

Understanding The Behavior Of Upper Subcritical Limit Calculations, Bobbi Riedel

Nuclear Engineering ETDs

This research consists of two comparison studies: the first study employed standard practices to characterize Upper Subcritical Limit (USL) estimation methods. A series of 33 neutronic systems that used standardized nuclear data and benchmark libraries were studied to compare the Whisper, TSURFER, and USLSTATS methods relative to a stochastic USL. USLs were also estimated for these 20 systems using the Whisper 1.1 code. Sensitivity data files were produced using MCNP6.2 and then used with the ORNL TSURFER and USLSTATS methods to estimate USLs for a cross-method USL comparison. The results show that USLs for each of the loosely coupled system …

Application Of An Empirical Density Law Via Python For Aqueous Plutonium Nitrate Systems, Tara L. Robertson

Nuclear Engineering ETDs

A predictive density tool has been developed to reduce bias and uncertainty in nuclear criticality safety calculations for aqueous plutonium nitrate systems. Multiple methods to calculate the density were reviewed and an empirical method was selected for use. The selected method was then implemented into a Python tool to calculate the solution density and the atom densities for an MCNP6.2 input file.

The Python tool has been validated and verified against the International Handbook of Evaluated Criticality Safety Benchmark Experiments to predict densities within ± 2.6%. The capability to calculate and utilize densities from this tool is a large improvement …

Numerical Study Of Turbulent Flow And Heat Transfer In A Novel Design Of Serpentine Channel Coupled With D-Shaped Jaggedness Using Hybrid Nanofluid, Raditun E. Ratul, Farid Ahmed, Syed B. Alam, Md Rezwanul Karim, Arafat A. Bhuiyan

Nuclear Engineering and Radiation Science Faculty Research & Creative Works

This Study Aimed to Examine Numerically the Effects of a Dimpled Surface over a Mini-Channel Heat Exchanger on the Flow Characteristics and Heat Transfer Across a Serpentine Channel with a Uniform Rectangular Cross-Section. the Dimples Were Arranged in Parallel with a Spanwise (Y/d) Distance of 3.125 and Streamwise (X/d) Distance of 11.25 Along Just One Side of the Serpentine Channel's Surface. Turbulent Flow Regime with Reynolds Number Ranging from 5 X 103 to 20 X 103 in the Channel with the Surface Modification Was Studied using Water and Various Volume Concentrations (Φ = 0.1%, 0.33%, 0.75%, 1%) of Al2O3-Cu/water Hybrid …

Measuring Radiation Protection: Partners From Across The Nuclear Enterprise Evaluate The Radiation Protection Of Us Army Vehicles, Andrew W. Decker, Robert Prins

Faculty Publications

Recent mounting nuclear threats and postures from adversary nation-states, such as Russia, China, North Korea, and Iran, represent a clear danger to the interests and security of the United States of America and its Allies. To meet these threats, the 2022 Nuclear Posture Review requires the Department of Defense (DoD) to design, develop, and manage a combat-credible U.S. military which, among other prioritizations, is survivable. A survivable force can generate combat power despite adversary attacks. As such, the US Army must prepare today to set the conditions for successful conventional warfare on the nuclear battlefields of tomorrow. Our Army cannot …

Oh, My Darling Clementine: A Detailed History And Data Repository Of The Los Alamos Plutonium Fast Reactor, Hannah K. Patenaude, Franz J. Freibert

College of Sciences Graduate Student Research

The Los Alamos Plutonium Fast Reactor, Clementine, provided the first fast neutron spectrum using a metallic plutonium fuel system and liquid mercury coolant. Clementine is often mentioned in the history of fast, metal-fueled, or metal-cooled designs, with little public information regarding the specifications or timeline. This paper contains a synopsis of each report regarding the development, operation, experimental results, failures, and subsequent disassembly of Clementine to explore this unique reactor within the context of modern advanced reactor development.

Fast-, Light-Cured Scintillating Plastic For 3d-Printing Applications, Brian G. Frandsen, Michael Febbraro, Thomas Ruland, Theodore W. Stephens, Paul A. Hausladen, Juan J. Manfredi, James E. Bevins

Faculty Publications

Additive manufacturing techniques enable a wide range of possibilities for novel radiation detectors spanning simple to highly complex geometries, multi-material composites, and metamaterials that are either impossible or cost prohibitive to produce using conventional methods. The present work identifies a set of promising formulations of photocurable scintillator resins capable of neutron-gamma pulse shape discrimination (PSD) to support the additive manufacturing of fast neutron detectors. The development of these resins utilizes a step-by-step, trial-and-error approach to identify different monomer and cross-linker combinations that meet the requirements for 3D printing followed by a 2-level factorial parameter study to optimize the radiation detection …

Studies On The Enrichment Feasibility Of Rare Earth-Bearing Minerals In Mine Tailings, Jose L. Corchado-Albelo, Lana Z. Alagha

Mining Engineering Faculty Research & Creative Works

This Study Aimed to Investigate the Potential of Enrichment of Rare-Earth-Bearing Minerals in Historic Mine Tailing using the Froth Flotation Process. Characterization Studies Indicated that Tailings Contained 11,000 Ppm of Rare Earth Elements (REEs). the Major Mineral in the Tailings Was Apatite at ~84%, Which Was Associated with Iron Oxides (~16%). TESCAN's Integrated Mineral Analysis (TIMA) Showed that Monazite Was the Main REE Mineral, and 69% of Monazite Was Locked in Apatite Grains. Characterization Studies Suggested that the Separation of REEs-Bearing Apatite from Iron Oxides is Possible using Froth Flotation, Wherein Apatite Was Floated and Iron Oxides Were Depressed. Zeta …

Automated Additive Layering Of Vat Polymerized Plastic Organic Scintillators, Chandler J. Moore

Theses and Dissertations

The current technology for fast neutron detection imaging is limited in achieving the required high spatial resolution, strong neutron discrimination, and practical time of manufacturing. Traditional fabrication methods require days of thermal polymerization and hundreds of man-hours to produce average resolution pixelated scintillator arrays. The present work helps to eliminate this limitation by developing an additive manufacturing technique to construct such detectors for use in in dual particle imaging applications. In this work, fast-, light-curing resins are used in a prototype automated assembly machine, capable of layering of individual light-cured resin layers and optical segmentation with a self-bonded specular reflector, …

Angle Resolved Photoelectron Spectroscopy Study Of Germanium Tin: Experimentally Determined Electronic Band Gap And Surface Analysis, Jeremy M. Hunter

Theses and Dissertations

The germanium tin band gap is responsive to wavelengths in the mid to near infrared spectrum; this shows promise in meeting the detection demands of the next generation infrared detectors. Recent developments in germanium tin (GeSn) alloy growth techniques have peaked the scientific community’s interest in GeSn based optoelectrical and detection devices. Detection materials made entirely of group IV elements are compatible with complementary metal-oxide semiconductor manufacturing techniques. Understanding the surface chemistry of this alloy is fundamental for solid state device design and must be analyzed to optimize device performance. Studies have shown that with the addition of tin, the …

Fast Engineering Model For Defect Production In Magnesium Oxide, Henry R. Little

Theses and Dissertations

Defect production from irradiation of materials with thicknesses much less than the mean free path for neutron interaction is explored. A model is developed using the Monte Carlo N-Particle transport code from Los Alamos National Laboratory, experimental data from irradiations at the Oak Ridge High Flux Isotope Reactor, defect production theory, and atomistic simulation results to predict the total number of F-centers resulting from neutron irradiation of a MgO rod. This model accurately predicts the concentration of atomic defects under conditions closely matching experiments at long timescales, for large geometries, and requiring only 6.9 minutes on a single CPU. Results …

Fabrication And Testing Of A Novel Layered Metascintillator For Neutron And Gamma Discrimination, Evan W. Threlkeld

Theses and Dissertations

By leveraging new developments in fast-curing of plastic scintillators, it is possible to fabricate multi-material plastic scintillators, or metascintillators, which offer improved and/or novel capabilities for radiation detection. This document proposes one geometry of metascintillator that uses layers of green and blue scintillating material to discriminate neutron/gamma radiation, details the devices necessary to fabricate it, and analyzes the metascintillator’s response to radiation. A model of the metascintillator using Geant4 and Python suggested that spectral-based neutron/gamma event discrimination is possible with 63% of gamma events and only 1% of neutron events being multi-color. Fabrication of a 500 µm per layer metascintillator …

Thermal Analysis Of Si-Igbt Based Power Electronic Modules In 50kw Traction Inverter Application, Mohammad Shahjalal, Tamanna Shams, Sadat Bin Hossain, Md Rishad Ahmed, Mominul Ahsan, Julfikar Haider, Rajib Goswami, Syed B. Alam, Atif Iqbal

Nuclear Engineering and Radiation Science Faculty Research & Creative Works

Estimation of Accurate IGBT Junction Temperature is Crucial for Reliability Assessment. the Well-Known RC Lumped Approach Can Help Predict Junction Temperature. However, This Method Suffers from Inaccuracy While Characterizing the Thermal Behavior of Several IGBT Modules Mounted to the Liquid-Cooled Heatsink. Specifically, the Thermal Challenge Originates from the Thermal Cross-Coupling and Module-To-Module Heat Spreading and the Converter Cooling Condition. This Article Demonstrates a Methodology to Study the Impact of Heat Spreading, Thermal Interface Material, and Massive Size Liquid Cold-Plate on the overall Thermal Behavior. a Case Study of 50 KW Traction Inverter is Chosen to Demonstrate the Benefit of Early …

Exploring Variations In Fast Curing Plastic Scintillator Formulations: Optimizing Tpo And Evaluating The Effects Of High-Z Loading And Novel Waveshifters, Andrew K. Nesbitt

Theses and Dissertations

Organic plastic scintillators are widely used due to their relative low cost, physical robustness, and fast timing properties, but typically provide lower light yields and photon sensitivity compared to other alternatives. Photocuring novel plastics offers a viable method for producing fast curing plastic scintillators. The current formulations include an acrylic polymer base and utilize diphenyl (2,4,6-trimethylbenzoyl) phosphine oxide (TPO) as the photo-initiator for polymerization; however at higher concentrations of TPO may adversely affect scintillator light output. The present research refined the optimal TPO concentrations that fully cure these acrylic-base scintillators and maximize light production to 0.4-0.5% by weight. Additionally, this …

Simulation Of Neutron Generation From Laser-Driven Fusion In A Liquid D2o Sheet Using Novel Warpx Module, Colton R. Stoner

Theses and Dissertations

Using WarpX’s new nuclear fusion module, this work attempts to model an experimental system at the ELL at the AFIT with WarpX and draw conclusions about fusion products from resulting simulations. Recently, a table-top, high repetition rate, mixed radiation source was demonstrated at the ELL employing a HIL to fuse the deuterium nuclei present in a unique liquid target of heavy water. Analysis of the simulations predicted an isotropic output of neutrons from deuterium-deuterium fusion. These simulated neutrons were created in tens of femtoseconds from dense bodies of deuterons that were perturbed by the laser. However, it was found that …

Pulsed Power Neutron Production With Deuterated Polymer Accelerator Targets, Anthony O. Hagey

Theses and Dissertations

This document presents an investigation of the effect of deuterated polyethylene accelerator targets on the neutron fluence from a local mass injection dense plasma focus driven by the United States Naval Research Laboratory’s Hawk pulsed-power generator. After successful production of thin targets, the acquisition of thicker targets, and testing inside Hawk, it was found that the presence of a deuterated polyethylene target increased the neutron fluence. Results suggested that fluence can significantly increase with the presence of a deuterated target vs a nondeuterated target. Additive manufacturing printing was used as a production method in order to determine if deuterated accelerator …

Assessment Of Emergency Cooling Requirement For Nuclear Reactor Loss-Of-Coolant Accidents, Michael T. Lindsay

Theses and Dissertations

The 2022 Russia-Ukraine War marks the first time in modern history of conventional military forces targeting and seizing control of an operational nuclear power plant. Power supply and operational cooling systems are critical to avert reactor loss-of-coolant accidents (LOCA) in the event of emergency shutdown, or SCRAM. A wartime non-design based reactor accident causing loss of reactor power and coolant supply would require an emergency heat exchange via coolant to mitigate reactor core heat. At present, the military does not have a well-defined model which characterizes this requirement for operational planning should such an event occur. SCALE 6.2.4 is used …

Data Augmentation For Neutron Spectrum Unfolding With Neural Networks, James Mcgreivy, Juan J. Manfredi, Daniel Siefman

Faculty Publications

Neural networks require a large quantity of training spectra and detector responses in order to learn to solve the inverse problem of neutron spectrum unfolding. In addition, due to the under-determined nature of unfolding, non-physical spectra which would not be encountered in usage should not be included in the training set. While physically realistic training spectra are commonly determined experimentally or generated through Monte Carlo simulation, this can become prohibitively expensive when considering the quantity of spectra needed to effectively train an unfolding network. In this paper, we present three algorithms for the generation of large quantities of realistic and …

Incorporation Of Poly(Tfema) In Perovskite Thin Films Using A Supercritical Fluid, Kasey Handy, Gary C. Tepper

Mechanical and Nuclear Engineering Publications

A new process is reported for the incorporation of a fluoropolymer into a solid perovskite film. Poly(trifluoroethyl methacrylate) [CH₂C(CH₃)(CO₂CH₂CF₃)]_n was delivered to methylammonium lead iodide (CH₃NH₃PbI₃) perovskite films by crystallizing the film in supercritical carbon dioxide/ethanol containing the dissolved fluoropolymer. The surface was characterized before and after fluoropolymer exposure using scanning electron microscopy, Raman spectroscopy, and contact angle measurements. The results indicate that the fluoropolymer was incorporated into the perovskite film during the supercritical fluid crystallization process. The incorporation of a hydrophobic fluoropolymer …

Radiation Shielding Effectiveness Of Hafnium Diboride (Hfb2) Reinforced Epoxy Composites For Enhanced Radiation Protection And Safety, Furkan Erdogan

Theses and Dissertations

This thesis investigates the radiation shielding effectiveness of hafnium diboride (HfB2) reinforced epoxy composites, with the aim of enhancing radiation protection and safety in various applications. The study focuses on the development and characterization of HfB2-epoxy composites with varying weight percentages of HfB2 nanoparticles, as well as on the evaluation of their shielding effectiveness against gamma rays and thermal neutrons. The radiation shielding performance of the composites is assessed using gamma-ray spectroscopy and neutron counting, and the neutron attenuation efficacy is compared with that of 5% borated high-dense polyethylene. The results indicate that the HfB2-epoxy composites exhibit promising radiation shielding …

A Study On The Effects Of Historical Meteorological Data Set On Simulated Radioactive Dispersion From A Nuclear Power Plant Accident By Nacac Code, Narakhan Khunsrimek

Chulalongkorn University Theses and Dissertations (Chula ETD)

Quantifying the variability in the prediction of atmospheric dispersion code from the Influences of variations in meteorological data is investigated in this study. Historical meteorological data from 2016 to 2020 by the National Centers for Environmental Prediction (NCEP) and the overlap hypothetical accident Loss Of Offsite Power (LOOP) and Large-Break Loss Of Coolant Accident (LBLOCA) are used as initial and boundary conditions. The Fangchenggang nuclear power plant in China, close to Thailand, is considered a study location. The Nuclear Accident Consequence Assessment Code (NACAC) is used as a simulation tool for the investigation process. The NACAC prediction performance is verified …