Nuclear Engineering Commons^™

Development Of The University Of New Mexico Spectrometer For High-Resolution Fission Product Yield Data, Richard Emery Blakeley

Nuclear Engineering ETDs

Well-defined fission product yield data has been of increasing interest in various applications within the nuclear industry. With this need in mind, a fission fragment mass spectroscopy system was designed and developed at the University of New Mexico in collaboration with the Los Alamos National Laboratories with a stated goal of attaining a mass resolution of ≤ 1 % (FWHM/centroid) for light fragments and near 1 % for heavy fragments. The mass spectrometer utilized in this work consists of a transmission time-of-flight detection system to measure fission product velocity and an axial ionization chamber to measure the fission product energy, …

Investigating The Electrodeposition Of Plutonium And Curium For Safeguarding The Electrorefiner, Chantell L. Murphy

Nuclear Engineering ETDs

This research investigated the electrochemical deposition behavior of plutonium (Pu) and curium (Cm) for safeguarding the electrorefiner (ER) in a pyroprocessing facility. The main goal of this investigation was to evaluate the feasibility of using a safeguards concept called the neutron balance method to account for Pu in the ER. The neutron balance method relies on a known Pu/Cm ratio and measures neutrons from Cm-244 coming into and leaving a unit operation to track Pu. The application of the neutron balance approach for pyroprocessing facilities requires that Pu and Cm remain together in all extraction, product recovery, and waste streams. …

Exploration Of Radiation Damage Mechanism In Mems Devices., Pranoy Deb Shuvra

Electronic Theses and Dissertations

We explored UV, X-ray and proton radiation damage mechanisms in MEMS resonators. T-shaped MEMS resonators of different dimensions were used to investigate the effect of radiation. Radiation damage is observed in the form of resistance and resonance frequency shift of the device. The resistance change indicates a change in free carrier concentration and mobility, while the resonance frequency change indicates a change in mass and/or elastic constant. For 255nm UV radiation, we observed a persistent photoconductivity that lasts for about 60 hours after radiation is turned off. The resonance frequency also decreases 40-90 ppm during irradiation and slowly recovers at …

Investigation Of The Formation Of Γꞌꞌ Precipitates Under Ion Irradiation And Elevated Temperature Environments, James R. Pike

Nuclear Engineering ETDs

During a preventative maintenance at the Los Alamos Neutron Science Center (LANSCE) Isotope Production Facility (IPF), a beam window made of solution annealed Alloy 718 was replaced and the old beam window was analyzed. The old beam window underwent mechanical testing and microstructure analysis. During the microstructure analysis, the formation of γꞌꞌ precipitates was observed in Transmission Electron Microscopy (TEM) electron diffraction pattern. The formation of γꞌꞌ precipitates was not expected since they are not stable under irradiation. Furthermore, the formation of γꞌꞌ precipitates was observed only at a temperature of 33ºC, and a dose of 0.7 displacement per atom …

Radiation Transport In Stochastic Media, Corey Skinner

Shared Knowledge Conference

The need to investigate numerical methods for the transport of radiation (thermal photons, light, neutrons, gammas) in random mixtures of immiscible materials arises in numerous applications, including inertial confinement fusion, turbid media (e.g., skin tissue), stellar atmospheres, clouds, and pebble bed nuclear reactors. Stochastic geometry techniques enable rendering of realizations of such random media and deterministic finite difference/finite element as well as Monte Carlo techniques are used to numerically simulate radiation transport on a large ensemble of realizations. The results are then averaged to obtain statistical moments of the radiation intensity, in particular the mean and variance, to assess the …

Comparison Of Steady And Transient Flow Boiling Critical Heat Flux (Chf) For Fecral Accident Tolerant Fuel Cladding Alloy, Zircaloy, And Inconel, Soon Kyu Lee

Shared Knowledge Conference

The nuclear reactor design focuses on building a system that is robust and reliable, is efficient and economical, and do not run into undesirable transient accident scenarios. The nuclear reactor safety focuses on ensuring the system operation under the safety margins and requirements provided by the regulatory agencies. Following the Fukushima nuclear reactor accident, the US Department of Energy Office of Nuclear Energy (DOE-NE) Advanced Fuels Campaign (AFC) is working to develop fuel and cladding candidates with potentially enhanced accident tolerance: ‘Advanced Tolerant Fuel’ (ATF). As a part of the AFC, this research focuses on gaining mechanistic understanding of the …

Use Of High Fidelity Fission Models In Criticality Calculations, Daniel H. Timmons

Shared Knowledge Conference

The use of Monte Carlo, random number sampling, for neutron transport has been used for about half a century. There are many benchmarks that have been used to validate neutronics codes, mostly for critical systems. Critical systems are systems where the neutron population from one generation to the next is the same. Subcriticality is when there are less neutrons in the next generation and supercriticality is when there are more neutrons in the next generation than there were in the previous. To calculate criticality, a set number of neutrons are started in a system. Those neutrons interact and the number …

Experimental Investigation On Heat Transfer In A Prismatic Modular Reactor Under Cosine Heat Flux, S. M. Alshehri, I. A. Said, Muthanna H. Al-Dahhan, Shoaib Usman

Chemical and Biochemical Engineering Faculty Research & Creative Works

The current study has investigated natural convection heat during pressurized conduction cooldown (PCC) accident scenario to understand the passive safety features of prismatic modular reactors (PMR) under different intensities of nonuniform center peaking step heat flux distributions (approximating cosine shape) using an advanced fast-response heat transfer technique. A scaled-down PMR module was designed and developed at Missouri S&T by the research team of the Multiphase Reactors Engineering and Applications Laboratory (mReal). The module consists of upper and lower plena connected by heated and cooled channels. Nonuniform heat flux distribution was applied to the heated channel under nonuniform heating center peaking …

Evaluation Of Eu:Licaf For Neutron Detection Utilizing Sipms And Portable Electronics, Michael A. Ford, Buckley E. O'Day Iii, John W. Mcclory, Manish K. Sharma, Areg Danagoulian

Faculty Publications

With the increasing cost and decreasing availability of ³He, there have been many efforts to find alternative neutron detection materials. Lithium calcium aluminum fluoride (LiCAF) enriched to 95% ⁶Li doped with europium was evaluated here as a replacement material for ³He. Wafers 0.5 cm thick, consisting of LiCAF crystals in a rubberized matrix, were embedded with wavelength shifting fibers (WSF) and mated to silicon photo-multipliers (SiPMs) to measure the photon response in a flux of neutrons from a DD neutron generator. Excellent discrimination was realized between neutrons and gammas, and both pulse-height discrimination and pulse-shape analysis were …

Radiation Detector Deadtime And Pile Up: A Review Of The Status Of Science, Shoaib Usman, Amol Patil

Nuclear Engineering and Radiation Science Faculty Research & Creative Works

Since the early forties, researchers from around the world have been studying the phenomenon of deadtime in radiation detectors. Many have attempted to develop models to represent this phenomenon. Two highly idealized models; paralyzable and non-paralyzable are commonly used by most individuals involved in radiation measurements. Most put little thought about the operating conditions and applicability of these ideal models for their experimental conditions. So far, there is no general agreement on the applicability of any given model for a specific detector under specific operating conditions, let alone a universal model for all detectors and all operating conditions. Further the …

Radiation Effects In Metal Oxides And Carbides, Benjamin Jackson Cowen

Nuclear Engineering ETDs

MD simulations of SiO₂, TiO₂, Cr₂O₃, Al₂O₃, MgO, and SiC, are performed to: (a) calculate TDE probability distributions and dependence on crystallographic direction, and (b) determine the number and types of defects formed with low- and high-energy PKAs and projectiles. In addition, a qualitative comparison of the MD simulation results of radiation damage in TiO₂, MgO, and crystalline and amorphous SiC thin films are compared with those of in situ TEM ion beam irradiation experiments at the Sandia National Laboratories’ I³TEM facility.

The TDE …

Neutron Spectroscopy Using Rubberized Eu:Licaf Wafers, Michael A. Ford

Theses and Dissertations

With the increasing cost and decreasing availability of ³He, there have been many efforts to find alternative neutron detection materials. Lithium calcium aluminum fluoride (LiCAF) enriched to 95% ⁶Li doped with europium was evaluated here as a replacement material for ³He, based on the absorption of thermalized neutrons by the ⁶Li and subsequent energy release of the ⁶Li(n,t)⁴He reaction. Wafers 0.5 cm thick, consisting of LiCAF crystals in a rubberized matrix, were embedded with wavelength shifting fibers (WSF) and mated to silicon photo-multipliers (SiPMs) to measure the photon response in a flux of …

Direct Synthesis Of Radioactive Nanoparticles Involving Neutrons, Carlos Henry Castano Giraldo, Maria Camila Garcia Toro, Brian Michael Mills

Nuclear Engineering and Radiation Science Faculty Research & Creative Works

A method to synthesize radioactive nanoparticles includes the production of metallic and multimetallic nanoparticles in a single step by providing an aqueous solution of the metal precursor, and irradiating the aqueous solution thereby producing nanoparticles. The obtained nanoparticles include one or more radioactive isotopes of gold, such as 198Au and 199Au as well as radioisotopes of silver when the obtained nanoparticles are bimetallic. The aqueous solution is irradiated in a radiation field that includes neutrons and gamma rays. The radiation field may be provided by a nuclear reactor. The aqueous solution may include silver, and bimetallic nanoparticles may be produced. …

A Security Approach For The Example Sodium Fast Reactor, Christian X. Young, Robert S. Bean

The Summer Undergraduate Research Fellowship (SURF) Symposium

Increases in the spread of nuclear technology and the rise of non-state terrorism in the modern era has proved the need for effective security approaches to new nuclear facilities. Many documents about security approaches for nuclear plants are non-public material, however, making it difficult to teach others about the basics of security design. To alleviate this issue, we used available texts in the security realm to design a security approach for the Generation IV International Forum’s Example Sodium Fast Reactor. Our approach utilized infrared, microwave, fiber optic, and other advanced technologies to provide security for the special nuclear material present. …

Incorporating Collisions And Resistance Into The Transition From Field Emission To The Space Charge Regime, Samuel D. Dynako, Adam M. Darr, Allen L. Garner

The Summer Undergraduate Research Fellowship (SURF) Symposium

Advancements in microelectromechanical systems (MEMS) and microplasmas, particularly with respect to applications in combustion and biotechnology, motivate studies into microscale gas breakdown to enable safe system design and implementation. Breakdown at microscale deviates from that predicted by Paschen’s law due to field emission—the stripping of electrons from the cathode in the presence of strong surface field—and follows the Fowler-Nordheim (FN) law. As injected current increases at this length scale, electrons accumulate in the gap and FN electron emission becomes space charge limited, leading to the Child-Langmuir (CL) law at vacuum and the Mott-Gurney (MG) law at high pressure. While theoretical …

Pnnl Dark Matter Bubble Chamber, Ryan Robinson

STAR Program Research Presentations

The Pacific Northwest National Laboratory (PNNL) prototype bubble chamber is intended to address issues encountered with the current PICO dark matter search detectors and improve the functionality of future experimental designs. The PNNL bubble chamber accomplishes this with a simplified interface between the hydraulic pressure controls and the target vessel and altering the standard chamber design such that it can be easily exchanged and replaced with vessels of various sizes and materials for testing purposes. The chamber itself is a glass vessel which houses perfluorobutane and holds the target fluid above room temperature and atmospheric pressure. The target fluid becomes …

Sonomechanical Enhanced Sparging Techniques For Advanced Reactor Applications, Floren V. Rubio

Nuclear Engineering ETDs

The fluoride salt cooled high temperature reactor (FHR) is a Generation IV advanced reactor design that has potential to produce efficient, low carbon, and safe energy. But, there are significant engineering challenges that need to be addressed before the deployment of this reactor. One of the key challenges is tritium release mitigation and sequestration. Because the FHR utilizes a eutectic LiF-BeF2 (flibe) salt as a coolant, the coolant is a significant source of tritium.

High-power ultrasonics have been used in many industrial process streams such as food processing, metal production, chemical production, and pharmaceutical manufacturing. Techniques and concepts from these …

Recommended Corrective Security Measures To Address The Weaknesses Identified Within The Shapash Nuclear Research Institute, Khadija Moussaid, Oum Keltoum Hakam

International Journal of Nuclear Security

The Shapash Nuclear Research Institute (SNRI) data book was issued by the International Atomic Energy Agency (IAEA) in 2013. The hypothetical facility data book describes the hypothetical site, which is divided into two areas: the low-security area, known as the administrative area, and the very high-security area, known as the protected area. The book contains detailed descriptions of each area’s safety and security measures, along with figures of multiple buildings in both areas, and also includes information about the site’s computer networks.

This paper aims to identify security weaknesses related to the institute’s location, the Administrative Area (AA), the Protected …

Radiation Effects In Apatite And High Entropy Alloy Under Energetic Ions And Electrons, Jianren Zhou

LSU Doctoral Dissertations

Radiation effects in apatite and high entropy alloy under energetic ions and electrons are studied in this doctoral dissertation to develop advanced crystalline ceramic waste forms and nuclear structural materials. Apatite is proposed as a ceramic waste form for the immobilization of radionuclides, but its performance is strongly affected by the irradiation of the incorporated radionuclides. It is thus important to understand the radiation effects in apatite structure and the underlying physics. Effects of chemical composition, grain size, interfacial structure, as well as radiation conditions on the microstructural evolution, phase transformation and damage mechanisms of apatite under alpha-decay and beta-decay …

The Continuing Quest For Missile Defense: When Lofty Goals Confront Reality, Peter J. Pella

Gettysburg College Faculty Books

For almost three quarters of a century, the United States has spent billions of dollars and countless person-hours in the pursuit of a national missile defense system that would protect the country from intercontinental ballistic missiles (ICBM) carrying nuclear warheads. The system currently in place consists of 44 long-range antiballistic missiles stationed in Alaska and California to protect the United States from a possible nuclear weapon carrying ICBM attack from North Korea. After all this effort, this system is still imperfect, being successful only 10 out of 18 tests.

This book will provide an historical description of past efforts in …

Detector Arrays For Nuclear Security And Safeguards Applications, Jessica Hartman

UNLV Theses, Dissertations, Professional Papers, and Capstones

Over the last two decades it has become increasingly apparent that there is a need for new technologies capable of reliable and efficient fast neutron detection. As national and international stockpiles of 3He continue to dwindle, the need to find a new gold standard of neutron detection becomes more critical. Moreover, neutrons are generated typically in the MeV energy range. The use of 3He detectors for fast neutron measurements requires the use of moderators. Detector arrays capable of fast neutron detection are one solution to this problem. To this end, the focus of this work was the study of detector …

Analysis Of Double-Wall And Twisted-Tube Heat Exchanger Concepts For Use In Fluoride Salt-Cooled High-Temperature Reactors, Bryan M. Wallace

Nuclear Engineering ETDs

Fluoride Salt-cooled High-temperature Reactors (FHRs) are an attractive fourth generation reactor concept. Like other fourth generation concept designs, FHRs offer characteristics such as a high-temperature low-pressure molten salt coolant allowing the reactor to be combined with a high-temperature high-efficiency power generation cycle such as an air-Brayton or supercritical carbon dioxide (SCO2). \par

Like most Gen IV reactor concepts, there are a few problems which need to be addressed with the design before it can be licensed. One particular design is the Mark 1 pebble bed FHR, a design put out by the University of California Berkeley. Two problems that need …

Irradiation Experiment For Living Insect-Based Radiological Dispersal Device, Braden Goddard, Walid Metwally, Ahmad Ababneh

International Journal of Nuclear Security

People generally associate fear with “nuclear”, “radioactive” and “insects”. It is speculated that a release of radioactive living insects would instill more fear into the general public than a “traditional” style radiological dispersion device (RDD). This paper evaluates the potential threat of an insect-based RDD using experimental data. The results of this project found that insect-based RDDs are an insignificant threat due to the challenges in making insects radioactive enough to pose any danger to humans without killing the insects.

Design And Characterization Of Systems For Direct Spatial Imaging Of Low-Energy Gamma-Radiation Sources, Phoenix Baldez

Nuclear Engineering ETDs

This work describes the development of radiation detection systems to identify and image special nuclear material (SNM) using low energy gamma rays. The imaging of these materials is crucial for timely, in the field responses to potential threats to national security. Using a spectroscopy system, the sources can be identified while images can be produced concurrently for the sources which are present. Two systems were designed and characterized in this study, a collimated imager which used collimation in front of a small CdTe detector, and a pixelated pinhole imager, using a pinhole mask in front of a pixelated CZT detector. …

Developing Kenya’S Educational Capacity In Nuclear Security Through Nuclear Forensics Research, Hudson Kalambuka Angeyo

International Journal of Nuclear Security

Nuclear energy’s distinctive characteristics give rise to special educational requirements. These requirements are necessary to not only address the danger of nuclear proliferation, but also to build capacity for a secure nuclear fuel circle. In this paper, I assess the status of educational capacity in nuclear security both in response to, and in support of, Kenya’s nuclear power program. I highlight the nuclear security educational infrastructure’s key features in the context of nuclear power, noting the low capacity at Kenyan universities. I identify the steps required to ensure that the country’s dynamic nuclear regulatory infrastructural framework is used effectively to …

Patient Specific Radiation Doses From Projection Radiography Images: Improving The Accuracy Of Low Dose Radiation Calculations, Daniel J. Sandoval

Nuclear Engineering ETDs

Due to an increase in regulatory scrutiny and medical facility accreditation requirements to monitor patient radiation dose from diagnostic imaging procedures, there is a growing necessity to determine and record accurate patient radiation dose from diagnostic medical imaging procedures. Current methods of patient dosimetry in diagnostic imaging are both extremely difficult and time consuming, require large computing resources (such as Monte Carlo computations), or lack accuracy due to using data based on homogeneous materials and “standard-man sized” anthropomorphic models.

This dissertation provides an algorithm that calculates a more accurate dose using patient-specific projection radiographic images. The algorithm includes measurements acquired …

An Exploration Of The Optical Detection Of Ionizing Radiation Utilizing Modern Optics Technology, Sean D. Fournier, Adam Hecht, Cassiano De Oliveira, Jeffrey B. Martin, Richard K. Harrison, Charles Potter

Nuclear Engineering ETDs

Modern ultraviolet (UV) cameras, when combined with UV-transmitting lenses/filter arrangements, can be used to detect radiation dose in air. Ionizing radiation excites nitrogen molecules in ambient air, the resulting decay includes weak emission of ultraviolet photons. Previous work has proven this phenomenon is detectable using highly-sensitive electronically cooled cameras traditionally used in astronomy for low-background imaging. While the ability to detect the presence of radiation (i.e. qualitative measurement) has been demonstrated at Sandia National Laboratories, there are several challenges in correlating images to known dose-fields (quantitative measurement). These challenges include: a low signal to background ratio, interferences due to electronic …

Case Study On The Development Of Engineering Design Modification Projects For U.S. Nuclear Power Plants: A Knowledge Retention Tool In Support Of The Longevity And Resilience Of The Nuclear Power Industry, Pamela M. Torres-Jiménez

Engineering Management & Systems Engineering Theses & Dissertations

The nuclear power industry in the United States (U.S.) has gone through various changes throughout its history. Most recently, plans to grow the industry through the construction of new power plants have ceased. Because of this, the industry is at a period where the longevity and resilience of existing nuclear power plants are vital to its subsistence.

One of the ways existing nuclear power plants can assure longevity and resilience is by performing engineering design modifications efficiently and at a lower cost. Strategic plans, such as the Delivering the Nuclear Promise, can support nuclear utilities to achieve this. Another strategy …

Development Of A Novel Framework For The Application Of Signature Based Safeguards (Sbs) To Pyroprocessing, Philip Leo Lafreniere

Nuclear Engineering ETDs

Traditional nuclear material accountancy (NMA) faces several challenges when applied to pyroprocessing facilities. To address these challenges, alternative methods of safeguarding nuclear material are being developed. One method is process monitoring (PM). PM involves taking operational process data and applying it to safeguards using an advanced framework. Signature Based Safeguards (SBS), a proposed PM framework, involves the identification of anomalous scenarios and the subsequent identification and detection of their respective PM signatures from a system of measurements. SBS has previously focused on failure modes that result in transfer of mass to unexpected places in the mass flowsheet. This work developed …

The "Double Standard" Of Nonproliferation: Regime Type And The U.S. Response To Nuclear Weapons Program, Alina Shymanska

International Journal of Nuclear Security

There is no doubt that the NPT regime is far from being equal for all states involved. As the predominant hegemonic power since WWII, the United States plays a major role in deciding the fates of non-great power proliferators. This article tries to find the logical explanation of the phenomenon whereby some nuclear proliferators are absolved regardless of their active accumulation of nuclear arsenals while others are labeled as “rogue states” and ordered to disarm. The article suggests that a particular proliferator’s political regime could affect the way in which its state is approached by the U.S., known for its …