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Articles 31 - 60 of 179
Full-Text Articles in Nuclear Engineering
Aerial Radiation Detection Identification And Measurement System Detector Material Comparison Study, Benjamin C. Troxell, Kacey D. Mcgee, Christina L. Dugan
Aerial Radiation Detection Identification And Measurement System Detector Material Comparison Study, Benjamin C. Troxell, Kacey D. Mcgee, Christina L. Dugan
Faculty Publications
The 20th Chemical Biological Radiological Nuclear and Explosives Command (CBRNE) currently utilizes an airborne sodium iodide gamma and beta detection system to map radiation fields over large areas of interest. The 20th CBRNE explored emergent detector technologies utilizing two detection materials; thallium-activated cesium iodide and high purity germanium (HPGe). These detectors were simulated at various altitudes and compared to background measurements. The sodium iodide detector failed to provide isotopic discrimination at distance. The thallium-activated cesium iodide CsI(Tl) detector provided sufficient absolute efficiency and energy resolution to identify isotopics at distance. The HPGe detector provided the best energy resolution. However, current …
Capability Development For Advanced (N,X) Nuclear Data Measurements, Brian G. Frandsen
Capability Development For Advanced (N,X) Nuclear Data Measurements, Brian G. Frandsen
Theses and Dissertations
Nuclear reaction data are the heart of radiation transport calculations, models, and simulations. Unique approaches are required to improve the measurement capability for many reactions where data are inaccurate or do not exist. First, the newly developed Gamma Energy Neutron Energy Spectrometer for Inelastic Scattering (GENESIS) provides the ability to measure neutron inelastic scattering cross sections on different targets. An initial experiment measuring the 16O(n,n’��) reaction calculated the count rate from the second excited state using the full energy and escape peaks. Second, a set of photocurable scintillator resin formulations capable of neutron-gamma discrimination were developed to support light-based …
Verficiation And Validation Of Unstructured Meshing Capabilities In Mcnp6, Micah C. Jeroutek
Verficiation And Validation Of Unstructured Meshing Capabilities In Mcnp6, Micah C. Jeroutek
Theses and Dissertations
Discrepancies were found between the legacy CSGs and the new UMs with the latter's introduction in MCNP6. As such, V&V of UMs in MCNP must be conducted to assist in their further development and increase user confidence in them. Currently, the MCNP test suite is lacking in UM benchmarks, and of the few that are present, their range in problem type is limited. To address these issues, two preliminary test cases covering new applications of UMs were developed for future inclusion in the test suite. The first was for the Athena-I experiment which involved the study of electronic devices' responses …
Modeling Gadolinium Self Powered Neutron Detectors In A Transient Reactor, Alexander L. Q. Spring
Modeling Gadolinium Self Powered Neutron Detectors In A Transient Reactor, Alexander L. Q. Spring
Theses and Dissertations
Contributions to the electron current from the three components of a gadolinium SPND, emitter, insulator, and sheath, are identified, characterized, and quantified to provide information on how the SPND interacts within the transient neutron and photon flux of the TREAT to create a measurable current. These contributions are measured by defining the SPND interactions as a dose response function used within a Monte Carlo simulation of a TREAT experiment. The data obtained from the Monte Carlo simulations are then used to compare against two analytic models, developed by Jaschik and Warren, as well as the experimental results. It was found …
Deep Learning Approach To Multi-Phenomenological Nuclear Fuel Cycle Signals For Nonproliferation Applications, Preston J. Dicks
Deep Learning Approach To Multi-Phenomenological Nuclear Fuel Cycle Signals For Nonproliferation Applications, Preston J. Dicks
Theses and Dissertations
In order to reduce the time required for data analysis and decision-making relevant to nuclear proliferation detection, Artificial Intelligence (AI) techniques are applied to multi-phenomenological signals emitted from nuclear fuel cycle facilities to identify non-human readable characteristic signatures of operations for use in detecting proliferation activities. Seismic and magnetic emanations were collected in the vicinity of the High Flux Isotope Reactor (HFIR) and the McClellan Nuclear Research Center (MNRC). A novel bi-phenomenology DL network is designed to test the viability of transfer learning between nuclear reactor facilities. It is found that the network produces an 84.1% accuracy (99.4% without transient …
Optimization Of A Multi-Layered Target For A Pulsed Power Neutron Source, Zachary D. Bretz
Optimization Of A Multi-Layered Target For A Pulsed Power Neutron Source, Zachary D. Bretz
Theses and Dissertations
The ability to create neutron environments is critical fora wide variety of applications including national security, materials science, and medical research. It is also helpful in medical, material, and other research. The U.S. Naval Research Laboratory (NRL), Washington, DC, is interested in leveraging their pulsed-power facilities to produce an in-house, relatively inexpensive neutron source. NRL’s facilities produce 2 MeV (from Gamble II) and 5 MeV (from Mercury) protons and deuterons. This research explored combinations of target materials to produce the most neutrons in the forward direction. Models of the reactions involved were first validated against literature experiments, then target designs …
Feasibility Of Fireball Trail Detection Using Ground-Based Gps Receivers, Ian R. Moffett
Feasibility Of Fireball Trail Detection Using Ground-Based Gps Receivers, Ian R. Moffett
Theses and Dissertations
The feasibility of using GPS data to detect fireballs is analyzed by first modeling the fireball’s trail diffusion and plasma chemistry to get a resulting ion density profile of the trail over time. The signal perturbation caused by the fireball trail is simulated for a ground receiver using an analytic solution for diffraction from a Gaussian lens. Five cases were modeled with varying initial peak ion densities and altitudes taken from fireball and reentry vehicle data. This paper shows that it is feasible to detect a fireball trail using GPS if the fireball has a sufficiently high initial ion density, …
Neutron Spectral Effect On Microelectronic Performance Response, Wade Kloppenburg
Neutron Spectral Effect On Microelectronic Performance Response, Wade Kloppenburg
Theses and Dissertations
Response of 2N2222 bipolar junction transistors to neutrons from a pulsed thermonuclear or pulsed fission source are researched. Measurements used for comparing performance included the base-collector junction current-voltage and capacitance-voltage characteristics and device gain degradation. Little change was detected in steady-state operation of the base-collector junction, but evidence in the dynamic and capacitance measurements establish effects based on environment. Experimental results are compared to literature results and parameters are explored using a device model simulation code.
Analysis Of Microscopic Carbon Fiber Fragments, Zachary R. Scott
Analysis Of Microscopic Carbon Fiber Fragments, Zachary R. Scott
Theses and Dissertations
Carbon Fiber (CF) has different tensile strengths and transverse moduli depending on how they are fabricated. Some CF is export controlled as it can be used for weapons, spacecraft, or gas centrifuges for enriching nuclear fuel. This research project explored a new way to prepare micron sized single CF threads to measure their transverse modulus and compare the moduli of non-export controlled CF to that of an export controlled CF. Five total polyacrylonitrile (PAN) fibers were used in this project, one of which was an export controlled fiber.
Athena: A Unique Radiation Environment Platform At The National Ignition Facility, Nicholas J. Quartemont, George Peterson, Colton Moran, Adib J. Samin, Buguo Wang, Charles Yeamans, Brandon Woodworth, Darren Holland, James C. Petrosky, James E. Bevins
Athena: A Unique Radiation Environment Platform At The National Ignition Facility, Nicholas J. Quartemont, George Peterson, Colton Moran, Adib J. Samin, Buguo Wang, Charles Yeamans, Brandon Woodworth, Darren Holland, James C. Petrosky, James E. Bevins
Faculty Publications
This paper describes the ATHENA platform, an energy tuning assembly, which was developed to spectrally shape the National Ignition Facility (NIF) deuterium–tritium fusion neutron source to a thermonuclear (fusion) plus prompt fission neutron spectrum with a capability to act as a short-pulse neutron source. This unique, otherwise inaccessible radiation environment complements existing experimental facilities and capabilities. The flexible ATHENA irradiation positions were modeled using an ensemble of Monte Carlo simulations with stochastic sampling of the nuclear cross-sections to characterize the radiation environments and uncertainty for the platform. Validation of the internal neutron spectrum produced from fielding ATHENA at NIF occurred …
Regularized Heuristic Method For Activation Monitor Neutron Spectrum Unfolding, Nicholas J. Quartemont, James E. Bevins
Regularized Heuristic Method For Activation Monitor Neutron Spectrum Unfolding, Nicholas J. Quartemont, James E. Bevins
Faculty Publications
his paper describes an activation foil measurement based neutron flux unfolding method utilizing a heuristic optimization approach. A regularization parameter based on the differential neutron flux was introduced into the optimization cost function to remove large nonphysical oscillations in the unfolded neutron energy spectrum. The procedure was completed for two example case studies ranging from thermal energies up to 20 MeV demonstrating recovery of neutron flux energy information on radiation environments where a model was partially missing or there was a discrepancy in a reaction channel. The unfolded results provided a distribution of unfolded spectra that conformed to the activation …
Verification And Validation Of Radiation Protection Factors From Monte Carlo Simulations, William J. Erwin
Verification And Validation Of Radiation Protection Factors From Monte Carlo Simulations, William J. Erwin
Theses and Dissertations
This dissertation describes the verification and validation of methods for producing radiation protection factors (RPFs) using experiments and Monte Carlo N-Particle 6 (MCNP6) simulations. RPF validation of a steel enclosure using a plutonium-beryllium source produced a validated RPF with statistically significant agreement between neutron MCNP6 models and experiments and a gamma protection factor (GPF) with statistically significant agreement to the measured GPF. Efforts to validate more complex enclosures using the Fast Burst Reactor (FBR) yielded the first-ever direct measurements of this reactor’s prompt gamma emission spectrum and revealed irreconcilable differences between the FBR facility-provided source spectrum and spectrometer measurements, resulting …
Neutron Energy Tuning Assemblies For Nuclear Weapon Environment Applications At The National Ignition Facility, Nicholas J. Quartemont
Neutron Energy Tuning Assemblies For Nuclear Weapon Environment Applications At The National Ignition Facility, Nicholas J. Quartemont
Theses and Dissertations
An energy tuning assembly was developed to spectrally shape the National Ignition Facility deuterium-tritium fusion neutron source to a notional thermonuclear and prompt fission neutron spectrum to fulfill neutron source capability gaps. The experimental neutron environment was characterized with activation dosimetry, neutronics and covariance models, and unfolded to determine the as-fielded neutron spectrum. The first energy tuning assembly was demonstrated to create synthetic spectrally accurate post-detonation fission products, enhancing U.S. technical nuclear forensics capabilities. ATHENA, a second-generation energy tuning assembly, was also optimized to meet similar objectives, but the new platform neutron fluence efficiency was increased by a factor of …
Uranium Integral Fission Product Yields For A Spectrally-Shaped 14.1 Mev Neutron Source At The National Ignition Facility, Nicholas J. Quartemont, N. Gharibyan, K. Moody, James E. Bevins
Uranium Integral Fission Product Yields For A Spectrally-Shaped 14.1 Mev Neutron Source At The National Ignition Facility, Nicholas J. Quartemont, N. Gharibyan, K. Moody, James E. Bevins
Faculty Publications
This paper describes the experimental results for an energy tuning assembly created to modify the National Ignition Facility deuterium–tritium fusion neutron source into a notional thermonuclear and prompt fission neutron spectrum, which has applications in integral measurements, nuclear data benchmarks, and radiation effects on microelectronics. The Monte Carlo neutron transport utilized MCNP5 to estimate the ETA-modified fluence using the ENDF-B/VIII.0 and IRDFF-II continuous energy nuclear data libraries, and SCALE Sampler was used to estimate the systematic nuclear data covariance using ENDF-B/VII.1 and IRDFF-II in a 252-group structure. The experiment fielded eight activation foils and a highly enriched uranium sample. This …
Acquiring And Modeling Of Si Solar Cell Transient Response To Pulsed X-Ray, Lei Pan, Praneeth Kandlakunta, Matthew Van Zile, Xuezeng Dai, Jinsong Huang, John W. Mcclory, Lei R. Cao
Acquiring And Modeling Of Si Solar Cell Transient Response To Pulsed X-Ray, Lei Pan, Praneeth Kandlakunta, Matthew Van Zile, Xuezeng Dai, Jinsong Huang, John W. Mcclory, Lei R. Cao
Faculty Publications
We report on the acquisition and modeling of the transient response of a commercial silicon (Si) solar cell using a benchtop pulsed X-ray source. The solar-cell transient output to the X-ray pulses was acquired under the dark and steady-state light illumination to mimic the practical operation of a solar cell under different light illumination levels. A solar-cell circuit model was created to develop a fundamental understanding of the transient current/voltage response of solar cell at read-out circuit level. The model was validated by a good agreement between the simulation and experimental results. It was found that the solar-cell resistance ( …
Characterization Of A Boron-Loaded Deuterated Liquid Scintillator For Fast And Thermal Neutron Detection, Bryan V. Egner, Michael Febbraro, James E. Bevins
Characterization Of A Boron-Loaded Deuterated Liquid Scintillator For Fast And Thermal Neutron Detection, Bryan V. Egner, Michael Febbraro, James E. Bevins
Faculty Publications
The preparation and characterization of novel boron-loaded deuterated liquid scintillators (BLDLS) are presented for the first time to investigate the performance of a detector sensitive to both fast and thermal neutrons intended for future neutron spectroscopy measurements. Three deuterated toluene-based scintillation cocktails were produced, one without boron, one loaded with ortho-carborane (natural boron isotopic abundance), and one with 96 wt% 10B enriched ortho-carborane. General optical and material properties were analyzed to include the composition, density, index of refraction, photoluminescence emission spectra, and absorbance spectra in addition to the relative light yield, resolution, relative efficiency, and pulse-shape-discrimination performance for all three …
Application Of Artificial Neural Networks To Elemental Assay Data For Nuclear Forensics Analysis, Jason G. Seik
Application Of Artificial Neural Networks To Elemental Assay Data For Nuclear Forensics Analysis, Jason G. Seik
Theses and Dissertations
There is a need to quickly and accurately determine the likely physical origins of a collected sample for nuclear treaty verification purposes. The objective of this research is to prove there is a means to relate different samples (Q-values) to one another using a 'same versus not-same' artificial neural network called a Siamese network. This would provide the capability of comparing an unknown sample to a database of samples with known physical origins. Using moment transformations on current data has shown to increase the prediction capabilities of a Siamese network, and using a triplet loss function in connection with the …
Lithium Compound Characterization Via Laser Induced Breakdown Spectroscopy And Raman Spectroscopy, James T. Stofel
Lithium Compound Characterization Via Laser Induced Breakdown Spectroscopy And Raman Spectroscopy, James T. Stofel
Theses and Dissertations
Industries such as lithium-ion battery producers and the nuclear industry community seek to produce and store lithium in pure chemical forms. However, these lithium compounds are reactive with the atmosphere and quickly degrade into less desirable forms. Therefore, industry desires a fast and effective quality control approach to quantify the ingrowth of these secondary lithium chemical forms. This research presents a novel approach using Laser-Induced Breakdown Spectroscopy (LIBS) and Raman spectroscopy in tandem to enhance lithium compound characterization beyond what is achieved by either technique alone. The resulting spectral data are aggregated using data fusion and analyzed using chemometrics for …
Characterization And Analysis Of Bomarc Accident Debris, Aaron J. Heffelfinger
Characterization And Analysis Of Bomarc Accident Debris, Aaron J. Heffelfinger
Theses and Dissertations
Accidents involving nuclear weapons, such as the Boeing Michigan Aeronautical Research Center (BOMARC) accident in 1960, always pose a significant risk of allowing particles composed of nuclear materials to enter the environment. These particles often differ in characteristics and can be of greatly varying sizes. Gamma ray analysis was conducted on the soil sample and radioisotopes within the sample were identified. Two non-destructive methods for locating actinide bearing particles within the sample were testing, resulting in 70 actinide bearing particles ranging from 1-34 microns being identified. These 70 particles underwent both morphological and elemental characterization, indicating uranium and other elements.
Space To High-Altitude Region Adjoint Neutron Transport, Zachary W. Lamere
Space To High-Altitude Region Adjoint Neutron Transport, Zachary W. Lamere
Theses and Dissertations
The goal of this work was to use the adjoint transport equation to characterize the energy spectrum of a point neutron source using the time-energy fluence at the satellite. The adjoint transport was solved via Monte Carlo methods in the new program called Space to Air High-Altitude Region Adjoint (SAHARA). A new adjoint source event estimator was developed to improve the computational efficiency. This work explores SAHARA’s performance using mono-energetic and continuous sources. In general, the identified source spectra were noticeably shifted towards lower energies, but were able to capture the source spectrum shapes. Lastly, SAHARA was applied to the …
Characterization Of The Spatial Distribution And Evolution Of Cerium And Calcium In Laser Produced Plasma, Michael G. Rynders
Characterization Of The Spatial Distribution And Evolution Of Cerium And Calcium In Laser Produced Plasma, Michael G. Rynders
Theses and Dissertations
Understanding plasma plumes and the distribution of plasma species microseconds after their formation has a variety of applications in fields such as hypersonics, explosion and combustion dynamics, and nuclear fireball chemistry. In this work, Laser Induced Breakdown Spectroscopy (LIBS) using double pulses of 532 nm light were used to analyze samples of cerium in atmospheres of air, vacuum, and argon. Cerium was used in this experiment to serve as a plutonium surrogate. CeO2 powder was pressed with CaO at 90-10 ratio to produce calcium doped pellets for use as sputtering targets. Inclusion of calcium impurities allowed the identification of …
An Assessment Of The Spatial Variation Of Isotopic Ratios In A Candu Reactor For Nuclear Treaty Monitoring, Aaron W. Burkhardt, James E. Bevins, Stephen H. Baxter
An Assessment Of The Spatial Variation Of Isotopic Ratios In A Candu Reactor For Nuclear Treaty Monitoring, Aaron W. Burkhardt, James E. Bevins, Stephen H. Baxter
Faculty Publications
A 3-D Quarter-Core CANDU-6 is modeled using Serpent 2 for nuclear treaty monitoring. The spatial variation of flux spectra and isotopic concentrations is analyzed to determine the potential isotopic distribution of key radionuclides from standard reactor operations relevant to non-proliferation. The initial results of the model show a 46% difference in overall flux magnitude throughout the core as well as a 2-30% difference in discrete energy flux. The coupled production rate (magnitude) and spectral differences can contribute to significant spatial variations in isotope ratios throughout the core. Initial results indicate 239 Pu/ 240 Pu ratios vary by as much as …
Development Of A Modular Mixed-Radiation Directional Rotating Scatter Mask Detection System, Bryan V. Egner, Darren E. Holland, Larry W. Burggraf, James E. Bevins
Development Of A Modular Mixed-Radiation Directional Rotating Scatter Mask Detection System, Bryan V. Egner, Darren E. Holland, Larry W. Burggraf, James E. Bevins
Faculty Publications
The ability to simultaneously identify the direction of both fast neutrons, above 1 MeV, and gamma rays using a light-weight system consisting of a single 1” EJ-309 organic liquid scintillator and a plastic Spartan rotating scatter mask (RSM) is demonstrated computationally through Monte Carlo simulations and validated with experimental measurements. Two sets of directional measurements were performed with an americium–beryllium source, emitting both neutrons and gamma rays. The RSM identified the direction of the source within one 10° rotational increment in the azimuthal and polar directions based on both the neutron and gamma-ray induced signals discriminated by charge integration pulse-shape …
Impact Of Neutron Energy On Asteroid Deflection Performance, Lansing S. Horan Iv, Darren E. Holland, Megan Bruck Syal, James E. Bevins, Joseph W. Wasem
Impact Of Neutron Energy On Asteroid Deflection Performance, Lansing S. Horan Iv, Darren E. Holland, Megan Bruck Syal, James E. Bevins, Joseph W. Wasem
Faculty Publications
In the future, a hazardous asteroid will find itself on a collision course with Earth. For asteroids of moderate size or larger, a nuclear device is one of humanity's only technologies capable of mitigating this threat via deflection on a timescale of less than a decade. This work examined how the output neutron energy from a nuclear device standoff detonation affects the deflection of a notional asteroid that is 300 meters in diameter and composed of silicon dioxide at a bulk density of 1.855 g/cm3. 14.1 MeV and 1 MeV neutron energy sources were modeled in MCNP to …
Applications Of Portable Libs For Actinide Analysis, Ashwin P. Rao, John D. Auxier Ii, Dung Vu, Michael B. Shattan
Applications Of Portable Libs For Actinide Analysis, Ashwin P. Rao, John D. Auxier Ii, Dung Vu, Michael B. Shattan
Faculty Publications
A portable LIBS device was used for rapid elemental impurity analysis of plutonium alloys. This device demonstrates the potential for fast, accurate in-situ chemical analysis and could significantly reduce the fabrication time of plutonium alloys.
A Physics-Based Machine Learning Study Of The Behavior Of Interstitial Helium In Single Crystal W–Mo Binary Alloys, Adib J. Samin
A Physics-Based Machine Learning Study Of The Behavior Of Interstitial Helium In Single Crystal W–Mo Binary Alloys, Adib J. Samin
Faculty Publications
In this work, the behavior of dilute interstitial helium in W–Mo binary alloys was explored through the application of a first principles-informed neural network (NN) in order to study the early stages of helium-induced damage and inform the design of next generation materials for fusion reactors. The neural network (NN) was trained using a database of 120 density functional theory (DFT) calculations on the alloy. The DFT database of computed solution energies showed a linear dependence on the composition of the first nearest neighbor metallic shell. This NN was then employed in a kinetic Monte Carlo simulation, which took into …
Measurement Of The 160Gd(P,N)160Tb Excitation Function From 4 18 Mev, Using A Stacked Foil Technique, Ryan K. Chapman
Measurement Of The 160Gd(P,N)160Tb Excitation Function From 4 18 Mev, Using A Stacked Foil Technique, Ryan K. Chapman
Theses and Dissertations
A stack of thin Gd, Ti, and Cu foils were irradiated with an 18 MeV proton beam at Lawrence-Berkeley National Laboratory's 88-Inch Cyclotron to investigate the 160Gd(p,n)160Tb nuclear reaction for nuclear forensics applications. This experiment will improve knowledge of 160Tb production rates, allowing 160Tb to be efficiently created in a foil stack consisting of other proton induced isotopes for forensics applications. A set of 15 measured cross sections between 4-18 MeV for 160Gd(p,n)160Tb were obtained using a stacked foil technique. The foil stack consisted of one stainless steel, one iron, fifteen gadolinium, …
Analysis Of The Correlation Between Re Filament Surface Features And Tims Performance, Christopher J. Mihal
Analysis Of The Correlation Between Re Filament Surface Features And Tims Performance, Christopher J. Mihal
Theses and Dissertations
Thermal Ionization Mass Spectrometry (TIMS) is an invaluable tool in nuclear forensics as it enables isotopic assays of actinides to be measured, permitting analysis to include special nuclear material isotopic assays, nuclear reactor monitoring, and treaty verification. In one method of measurement for the TIMS system, samples are deposited in solution form on high-purity rhenium filaments. The filaments are heated to evaporate the solvent, and then further heated to cause sample ionization, permitting the sample to be transmitted through a magnetic field which separates ions based on mass to charge ratio into detectors for counting. Heavier ions will be deflected …
The Effect Of Aeration Rate And Free-Floating Carrier Media On The Emission Of Bacillus Globigii In Bioaerosols, Andrew J. Owens
The Effect Of Aeration Rate And Free-Floating Carrier Media On The Emission Of Bacillus Globigii In Bioaerosols, Andrew J. Owens
Theses and Dissertations
Aerosols produced by turbulent mechanical mixing and bubble aeration at Waste Water Treatment Plants (WWTPs) become bioaerosols with the entrainment of biological materials. Bioaerosols become a public health risk when human pathogens are present. This study evaluated bioaerosols containing Bacillus globigii (BG) spores, and the effects that aeration rate and the addition of Free-Floating Carrier Media (FFCM) had on the amount of BG spores collected following aerosolization. A series of laboratory-scale experiments investigated two different sizes of floating polystyrene spheres as FFCM and four different aeration rates. When the differences in compared aeration rates were sufficiently large, a positive correlation …
An Assessment Of The Spatial Variation Of Isotopic Ratios In A Candu-6 Reactor For Nuclear Treaty Monitoring, Aaron W. Burkhardt
An Assessment Of The Spatial Variation Of Isotopic Ratios In A Candu-6 Reactor For Nuclear Treaty Monitoring, Aaron W. Burkhardt
Theses and Dissertations
The Preparatory Commission for the Comprehensive Nuclear Test Ban Treaty Organization developed the International Monitoring System for monitoring for nuclear explosive testing and compliance with nuclear treaties. Many of the International Monitoring System stations are capable of detecting radionuclides that can be used to determine their origin and creation environment. However, there is not a single unique signature associated with each creation environment. Nuclear reactors, for example, can have a wide range of isotopic concentrations caused by spatial variations in neutron flux intensity and energy. As a single sample only provides a single isotopic measurement, this can make disambiguation difficult …