Nuclear Engineering Commons^™

Validation Of Electromagnetic Shower Development In A Reduced Alice Focal-E Detector Model Using Geant4, Isaac Lara Romo

Physics

This project focuses on the preliminary simulation of a reduced FoCal-E detector model for the ALICE experiment at CERN. Beamline tests were simulated using an electron gun at various incident energies, and the results were compared with those of the FoCal group. The longitudinal charge deposition per sensor layer was compared between the two setups to verify that the reduced model exhibited expected calorimeter behavior. Additionally, the transverse signal across the high-granularity sensor layers was examined to determine whether the reduced model reproduced the expected lateral development of electromagnetic showers. The results obtained from these measurements show that the reduced …

Radiation Protection Factor Research: The Keystone For Conventional-Nuclear Integration (Cni), Andrew W. Decker

Faculty Publications

This article briefly describes Defense Threat Reduction Agency (DTRA) vehicle Radiation Protection Factor (RPF) research and explains its critical role in enabling future Operations in a Nuclear Environment (ONE) and Conventional-Nuclear Integration (CNI) on behalf of the US Department of War (DoW).1 As such, the background and practical utility of RPF values is discussed, as well as the justification for renewed Army and DoW investment into RPF research to enhance Joint military planning, survivability, and lethality on tomorrow’s nuclear battlefields. Advances in DTRA RPF research directly strengthen US strategic and extended deterrence efforts and support all Agencies and Departments responsible …

Improving Modeling Of Corrosion Products In The Primary Circuit Of Light Water Reactors Through The Experimental Determination Of Crud Characteristics, Sri Saravana Konganapuram Narasimma Bharathi

Electronic Theses & Dissertations (2024 - present)

High-temperature water flowing through the coolant circuits in pressurized water reactors (PWRs) creates a harsh environment, deteriorating these materials. This corrosion results in the formation of oxide layer(s) primarily composed of nickel ferrites, iron oxides, nickel oxides, and other nickel-iron-chrome spinel oxides. Being exposed to fluid with high flow rates and pressure, these oxide layers can be eroded, resulting in particulate fouling due to the release of corrosion products (Chalk River Unidentified Deposits, CRUD) into the coolant circuit. When CRUD subsequently deposits on fuel surfaces, it negatively affects the fuel performance (heat transfer and fuel failure); in addition, the particles …

Constraining Nuclear Data Uncertainty Requirements For The 19F(A, N)22Na Reaction For Non-Proliferation Applications, Tyler R. M. Smith

Theses and Dissertations

This thesis explores the requirements on nuclear data uncertainties needed for the use of the ¹⁹F(α, n)²²Na reaction for nuclear non-proliferation applications. An overview of how neutrons are produced from alpha decays in a UF₆ medium is discussed. Calculation demonstrate the role nuclear data uncertainties effect the neutron yield and energy spectra as a function of enrichment.

The Effects Of Snow Cover On The Dynamic Pressure Of Nuclear Detonation Blast Waves, Adam Card, Andrew W. Decker

Faculty Publications

Blast pressure is the primary military targeting metric for nuclear weapons. Any local conditions that affect blast pressure have the potential for altering nuclear plans, both from defensive and offensive standpoints. Understanding the impact of snow to the blast wave, therefore, provides a benefit both to military planners and to warfighters on the ground, for any operation occurring in arctic environments. No existing data provides a quantitative description of how snow on the ground affects a nuclear detonation blast wave passing over it. Similar blast waves passing over dust have experimentally proven to enhance blast pressure in a localized region.1 …

Multiphysics Modeling Of Material Response To High-Intensity X-Ray And Laser Pulses: Heating, Ablation, And Plasma Expansion, Youssef Abouhussien

Theses and Dissertations

This dissertation presents a computational framework to investigate material response under high-intensity X-ray fluxes produced by an exo-atmospheric nuclear detonation and laser-material irradiations, with a focus on heating, ablation, and plasma expansion phenomena relevant to satellite vulnerability and high-energy-density environments. A hybrid Monte Carlo and Two-Temperature Model (MC-TTM) was developed to simulate X-ray and laser energy deposition and thermal relaxation in metals and semiconductors across a range of X-ray and laser pulse durations from femtoseconds to nanoseconds. Results demonstrate distinct thermal behavior between materials, with ablation thresholds and phase transitions captured in good agreement with experimental data.

In parallel, a …

Development Of Group Iii-V Quantum Confinement-Enabled Detectors: Bias-Tunable Quantum Well Infrared Photodetector (Qwip) And Quantum Dot Scintillation Detector (Qdsd), Gyana R. Biswal

Electronic Theses & Dissertations (2024 - present)

This dissertation discloses the physics, fabrication, characterization, and analysis of two novel types of group III-V semiconductor detectors relying on quantum confinement of carriers, namely voltage-tunable quantum well infrared photodetectors (QWIP) and a high-yield ultrafast quantum dot scintillation detector (QDSD). Both QWIP and QDSD heterostructures presented here were grown on 3” GaAs (001) substrates using molecular beam epitaxy (MBE).

A major part of the dissertation focuses on development of the voltage-tunable QWIPs targeting detection in the mid-wave infrared region (MWIR) (3μm -5μm) and long-wave infrared region (LWIR) (8μm -12μm) with control of sensitivity by the applied bias. The QWIPs utilize …

Generation And Implementation Of Mixed Radiation From Laser Interactions On A Liquid Target, Benjamin M. Knight

Theses and Dissertations

The simultaneous generation of different forms of radiation from the same source is highly desirable but technically challenging. We present the generation of D-D fusion neutrons and >MeV-energy x-rays from extreme intensity (∼ 10¹⁹ W/cm² ), high repetition-rate (1 kHz) laser pulses on a thin liquid target. Total neutron fluxes of ∼ 105 neutrons/s and x-ray exposure rates up to ∼ 200 R/hr at 74 cm are measured. Evidence of D-D fusion is verified with a measurement suite including three independent neutron detection systems: an EJ-309 organic scintillator, a ³He proportional counter, and a set of 36 …

Thermal Hydraulic Analysis For Different Subchannels Of Generic Vver-1200, Mosaddak Ahamed Zahid, Md. Imam Mehedi, Shamsul Arefin Shibly, A. S. Mollah

International Journal of Nuclear Security

The demand for nuclear energy is steadily increasing all over the world. Most nuclear power is used for peaceful applications such as power generation, healthcare, agriculture, food security, industry, and research. One of the primary applications of nuclear energy is the generation of electricity through nuclear power plants based on nuclear reactors. Many developing countries around the world (such as Bangladesh) are moving toward nuclear power plants because they have huge advantages, including low-cost energy, reliable energy sources, zero carbon emissions, and high energy concentration. As a result, the demand for nuclear reactor protection and operational protection of nuclear power …

Pulsed-Power Neutron Production With Deuterated Polymer Accelerator Targets, Anthony O. Hagey, Juan J. Manfredi, Whitman T. Dailey, S. L. Jackson, E. R. Kaiser, J, W. Schumer

Faculty Publications

This document presents an investigation of the effect of deuterated accelerator targets on the neutron fluence from a local mass injection dense plasma focus (LMIDPF) driven by the United States Naval Research Laboratory's (NRL) Hawk pulsed-power generator. Deuterated targets were made using two methods: a well-established thin-film casting technique for flat targets and a more novel additive manufacturing technique that allowed targets to be three-dimensional (3D) printed in both flat and conical geometries. These targets were then tested during neutron-producing experiments conducted using Hawk, and theneutron fluences measured for the various target types were compared. Additive manufacturing was used as …

Neutron Spectrum Unfolding From Activation Foils Irradiated In Gamble Ii Using Deuterated Polyethylene Anodes, Christopher J. Smith

Theses and Dissertations

Neutrons can cause irreparable harm to electronics, and experiments are needed to understand their effects fully. This work explores using pulsed power, which is low-cost compared to other sources, to create a useful neutron-rich environment. Deuterated polyethylene was used as anode and catcher material to generate the neutrons from the Deuterium-Deuterium (DD) fusion reaction. A simple, effective, and repeatable method was employed to directly cast deuterated polyethylene onto polyethylene sheets to fabricate the anode and catcher. The DD reactions were made by an ion beam-driven pulsed power generator, Gamble II, with the catcher located in the cathode. Zinc, copper, aluminum, …

Radiation Exposure Calibration Of The Al2o3:C With Radium-226 And Cesium-137 Using The Osl Method, Selma Tepeli Aydin

All Theses

Optically stimulated luminescence (OSL) dosimetry was utilized to calibrate Al₂O₃:C powder dosimeters, available commercially as the nanoDot® from Landauer Inc., and compare the dosimeter response to radium-226 (²²⁶Ra) and cesium-137 (¹³⁷Cs). The signal from the OSL was quantified using a microSTARii^® OSL reader also produced by Landauer Inc. Dose-response curves were developed for ²²⁶Ra and ¹³⁷Cs experiments (5 dosimeters each) at thirteen absorbed doses. Individual dosimeter response was tracked by serial number. Linear regression analysis was performed to determine if there were significant differences between the intercepts of the …

Direct Measurement Of The 114cd(N, Gamma)115cd Cross Section In The 1 Ev To 300 Kev Energy Range, Kofi Tutu Addo Assumin-Gyimah

Theses and Dissertations

The large thermal cross section of cadmium makes it ideal for many practical applications where screening of thermal neutrons is desired. For example, in non-destructive assay techniques, or for astrophysical studies of the s-process. All such applications require precise knowledge of the neutron-capture cross section on cadmium. Although there are some data on neutron-capture cross sections particularly at thermal energies and at energies relevant for astrophysics, there is very little data at most other energies. Further, the evaluated cross sections from the ENDF and JENDL databases disagree at high energies. Therefore, there is a critical need for precise knowledge of …

Measuring Radiation Protection: Partners From Across The Nuclear Enterprise Evaluate The Radiation Protection Of Us Army Vehicles, Andrew W. Decker, Robert Prins

Faculty Publications

Recent mounting nuclear threats and postures from adversary nation-states, such as Russia, China, North Korea, and Iran, represent a clear danger to the interests and security of the United States of America and its Allies. To meet these threats, the 2022 Nuclear Posture Review requires the Department of Defense (DoD) to design, develop, and manage a combat-credible U.S. military which, among other prioritizations, is survivable. A survivable force can generate combat power despite adversary attacks. As such, the US Army must prepare today to set the conditions for successful conventional warfare on the nuclear battlefields of tomorrow. Our Army cannot …

Automated Additive Layering Of Vat Polymerized Plastic Organic Scintillators, Chandler J. Moore

Theses and Dissertations

The current technology for fast neutron detection imaging is limited in achieving the required high spatial resolution, strong neutron discrimination, and practical time of manufacturing. Traditional fabrication methods require days of thermal polymerization and hundreds of man-hours to produce average resolution pixelated scintillator arrays. The present work helps to eliminate this limitation by developing an additive manufacturing technique to construct such detectors for use in in dual particle imaging applications. In this work, fast-, light-curing resins are used in a prototype automated assembly machine, capable of layering of individual light-cured resin layers and optical segmentation with a self-bonded specular reflector, …

Simulation Of Neutron Generation From Laser-Driven Fusion In A Liquid D2o Sheet Using Novel Warpx Module, Colton R. Stoner

Theses and Dissertations

Using WarpX’s new nuclear fusion module, this work attempts to model an experimental system at the ELL at the AFIT with WarpX and draw conclusions about fusion products from resulting simulations. Recently, a table-top, high repetition rate, mixed radiation source was demonstrated at the ELL employing a HIL to fuse the deuterium nuclei present in a unique liquid target of heavy water. Analysis of the simulations predicted an isotropic output of neutrons from deuterium-deuterium fusion. These simulated neutrons were created in tens of femtoseconds from dense bodies of deuterons that were perturbed by the laser. However, it was found that …

Pulsed Power Neutron Production With Deuterated Polymer Accelerator Targets, Anthony O. Hagey

Theses and Dissertations

This document presents an investigation of the effect of deuterated polyethylene accelerator targets on the neutron fluence from a local mass injection dense plasma focus driven by the United States Naval Research Laboratory’s Hawk pulsed-power generator. After successful production of thin targets, the acquisition of thicker targets, and testing inside Hawk, it was found that the presence of a deuterated polyethylene target increased the neutron fluence. Results suggested that fluence can significantly increase with the presence of a deuterated target vs a nondeuterated target. Additive manufacturing printing was used as a production method in order to determine if deuterated accelerator …

Enabling Rapid Chemical Analysis Of Plutonium Alloys Via Machine Learning-Enhanced Atomic Spectroscopy Techniques, Ashwin P. Rao

Theses and Dissertations

Analytical atomic spectroscopy methods have the potential to provide solutions for rapid, high fidelity chemical analysis of plutonium alloys. Implementing these methods with advanced analytical techniques can help reduce the chemical analysis time needed for plutonium pit production, directly enabling the 80 pit-per-year by 2030 manufacturing goal outlined in the 2018 Nuclear Posture Review. Two commercial, handheld elemental analyzers were validated for potential in situ analysis of Pu. A handheld XRF device was able to detect gallium in a Pu surrogate matrix with a detection limit of 0.002 wt% and a mean error of 8%. A handheld LIBS device was …

Computational Models To Detect Radiation In Urban Environments: An Application Of Signal Processing Techniques And Neural Networks To Radiation Data Analysis, Jose Nicolas Gachancipa

Beyond: Undergraduate Research Journal

Radioactive sources, such as uranium-235, are nuclides that emit ionizing radiation, and which can be used to build nuclear weapons. In public areas, the presence of a radioactive nuclide can present a risk to the population, and therefore, it is imperative that threats are identified by radiological search and response teams in a timely and effective manner. In urban environments, such as densely populated cities, radioactive sources may be more difficult to detect, since background radiation produced by surrounding objects and structures (e.g., buildings, cars) can hinder the effective detection of unnatural radioactive material. This article presents a computational model …

Nuclear Fuel Cycle: Safe Management Of Spent Nuclear Fuel, Robert L. Sindelar

Journal of the South Carolina Academy of Science

The aim for storage of spent nuclear fuel (SNF) either in wet or in dry storage systems is to ensure general safety objectives are met throughout a desired storage period. Staff at the Savannah River National Laboratory (SRNL), in collaborations with partners at other national laboratories, industry research organizations, and the University of South Carolina (UofSC), have performed materials aging testing and analyses, and have established nuclear materials aging management programs to support extended periods of safe storage of research reactor (RR) SNF and of commercial power reactor (PR) SNF pending ultimate disposal. Several example challenges include susceptibility of aluminum …

Aerial Radiation Detection Identification And Measurement System Detector Material Comparison Study, Benjamin C. Troxell, Kacey D. Mcgee, Christina L. Dugan

Faculty Publications

The 20th Chemical Biological Radiological Nuclear and Explosives Command (CBRNE) currently utilizes an airborne sodium iodide gamma and beta detection system to map radiation fields over large areas of interest. The 20th CBRNE explored emergent detector technologies utilizing two detection materials; thallium-activated cesium iodide and high purity germanium (HPGe). These detectors were simulated at various altitudes and compared to background measurements. The sodium iodide detector failed to provide isotopic discrimination at distance. The thallium-activated cesium iodide CsI(Tl) detector provided sufficient absolute efficiency and energy resolution to identify isotopics at distance. The HPGe detector provided the best energy resolution. However, current …

There From The Beginning: The Women Of Los Alamos National Laboratory Supporting National And International Nuclear Security, Olga Martin, Laura Mcclellan, Octavio Ramos, Heather Quinn

International Journal of Nuclear Security

From the beginning of the Manhattan Project in the early 1940s, the women of what would become Los Alamos National Laboratory (LANL) worked in technical positions alongside their male counterparts, played a key role as computers, and worked in administrative jobs as secretaries, phone operators, bookkeepers, and on behalf of the U.S. Army in the Women’s Army Corps.

Throughout the history of the Laboratory, women experts at LANL helped establish and lead important national and international security programs, with careers in science, technology, engineering, and mathematics. Over time, the women of Los Alamos have come together under various Employee Resource …

Particle Swarm Optimization For Critical Experiment Design, Cole Michael Kostelac

Masters Theses

“Critical experiments are used by nuclear data evaluators and criticality safety engineers to validate nuclear data and computational methods. Many of these experiments are designed to maximize the sensitivity to a certain nuclide-reaction pair in an energy range of interest. Traditionally, a parameter sweep is conducted over a set of experimental variables to find a configuration that is critical and maximally sensitive. As additional variables are added, the total number of configurations increases exponentially and quickly becomes prohibitively computationally expensive to calculate, especially using Monte Carlo methods.

This work presents the development of a particle swarm optimization algorithm to design …

Effects Of Vacancies And Electron Temperature On The Electron Phonon Coupling In Cubic Silicon Carbide And Their Connection To The Inelastic Thermal Spike, Salah Al-Smairat

Doctoral Dissertations

“The electron-phonon interaction is an important interaction in many solids as it influences transport phenomena and related quantities such as the electrical and thermal conductivities, especially in nuclear and space applications. The importance of the electron-phonon interaction in primary damage production in 3C-SiC is the subject of this research.

The electron-phonon coupling factor was calculated using a hybrid Density Functional Perturbation Theory - Classical Electron Gas model. The coupling factor was calculated as a function of electron temperature in pristine and defective 3C-SiC, and relaxed defective cells. The electron-phonon coupling is found to depend strongly on the electronic temperature and …

Athena: A Unique Radiation Environment Platform At The National Ignition Facility, Nicholas J. Quartemont, George Peterson, Colton Moran, Adib J. Samin, Buguo Wang, Charles Yeamans, Brandon Woodworth, Darren Holland, James C. Petrosky, James E. Bevins

Faculty Publications

This paper describes the ATHENA platform, an energy tuning assembly, which was developed to spectrally shape the National Ignition Facility (NIF) deuterium–tritium fusion neutron source to a thermonuclear (fusion) plus prompt fission neutron spectrum with a capability to act as a short-pulse neutron source. This unique, otherwise inaccessible radiation environment complements existing experimental facilities and capabilities. The flexible ATHENA irradiation positions were modeled using an ensemble of Monte Carlo simulations with stochastic sampling of the nuclear cross-sections to characterize the radiation environments and uncertainty for the platform. Validation of the internal neutron spectrum produced from fielding ATHENA at NIF occurred …

Regularized Heuristic Method For Activation Monitor Neutron Spectrum Unfolding, Nicholas J. Quartemont, James E. Bevins

Faculty Publications

his paper describes an activation foil measurement based neutron flux unfolding method utilizing a heuristic optimization approach. A regularization parameter based on the differential neutron flux was introduced into the optimization cost function to remove large nonphysical oscillations in the unfolded neutron energy spectrum. The procedure was completed for two example case studies ranging from thermal energies up to 20 MeV demonstrating recovery of neutron flux energy information on radiation environments where a model was partially missing or there was a discrepancy in a reaction channel. The unfolded results provided a distribution of unfolded spectra that conformed to the activation …

Neutron Energy Tuning Assemblies For Nuclear Weapon Environment Applications At The National Ignition Facility, Nicholas J. Quartemont

Theses and Dissertations

An energy tuning assembly was developed to spectrally shape the National Ignition Facility deuterium-tritium fusion neutron source to a notional thermonuclear and prompt fission neutron spectrum to fulfill neutron source capability gaps. The experimental neutron environment was characterized with activation dosimetry, neutronics and covariance models, and unfolded to determine the as-fielded neutron spectrum. The first energy tuning assembly was demonstrated to create synthetic spectrally accurate post-detonation fission products, enhancing U.S. technical nuclear forensics capabilities. ATHENA, a second-generation energy tuning assembly, was also optimized to meet similar objectives, but the new platform neutron fluence efficiency was increased by a factor of …

Characterization Of A Boron-Loaded Deuterated Liquid Scintillator For Fast And Thermal Neutron Detection, Bryan V. Egner, Michael Febbraro, James E. Bevins

Faculty Publications

The preparation and characterization of novel boron-loaded deuterated liquid scintillators (BLDLS) are presented for the first time to investigate the performance of a detector sensitive to both fast and thermal neutrons intended for future neutron spectroscopy measurements. Three deuterated toluene-based scintillation cocktails were produced, one without boron, one loaded with ortho-carborane (natural boron isotopic abundance), and one with 96 wt% 10B enriched ortho-carborane. General optical and material properties were analyzed to include the composition, density, index of refraction, photoluminescence emission spectra, and absorbance spectra in addition to the relative light yield, resolution, relative efficiency, and pulse-shape-discrimination performance for all three …

Spectator Proton Detection And Reconstruction In Deep Inelastic D(E,EpS) Scattering, David Payette

Physics Theses & Dissertations

A Radial Time Projection Chamber (RTPC) was designed and installed in Jefferson Lab's Hall B as part of the BONuS12 (Barely Off-shell Nucleon Structure) experiment. The goal of BONuS12 is to accurately measure the structure function of the neutron by scattering 11 GeV electrons and detecting them with the CLAS12 spectrometer. Deuterium gas was used as an effective neutron target, and the new RTPC was used to detect low- momentum spectator protons. Protons follow a curved path in the 5 Tesla solenoid that is part of CLAS12, ionizing the He-CO2 gas in an annular drift region surrounding the target. These …

Lithium Compound Characterization Via Laser Induced Breakdown Spectroscopy And Raman Spectroscopy, James T. Stofel

Theses and Dissertations

Industries such as lithium-ion battery producers and the nuclear industry community seek to produce and store lithium in pure chemical forms. However, these lithium compounds are reactive with the atmosphere and quickly degrade into less desirable forms. Therefore, industry desires a fast and effective quality control approach to quantify the ingrowth of these secondary lithium chemical forms. This research presents a novel approach using Laser-Induced Breakdown Spectroscopy (LIBS) and Raman spectroscopy in tandem to enhance lithium compound characterization beyond what is achieved by either technique alone. The resulting spectral data are aggregated using data fusion and analyzed using chemometrics for …