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The Role Of Diffusive Transport On Low And Intermediate Temperature Hydrocarbon Oxidation: Numerical Simulations Using The Wang-Mou Mechanism, Howard Pearlman, Michael R. Foster
The Role Of Diffusive Transport On Low And Intermediate Temperature Hydrocarbon Oxidation: Numerical Simulations Using The Wang-Mou Mechanism, Howard Pearlman, Michael R. Foster
Faculty Publications - Biomedical, Mechanical, and Civil Engineering
The spatio-temporal temperature and species concentration distributions associated with low and intermediate temperature hydrocarbon oxidation are computed using a global thermo kinetic scheme augmented with diffusive transport. The scheme used for the computations was proposed by Wang and Mou and is extended to include diffusion of species and heat. The conservation equations for species and energy are then derived and solved for a one-dimensional and an axisymmetric, spherical domain for temperatures ranging from 540 to 660 Kat subatmospheric pressures. The predictions are then used to develop ignition diagrams for different Lewis ( Le) numbers. Increasing Le is found to promote …
The Role Of Diffusive Transport On Low And Intermediate Temperature Hydrocarbon Oxidation: Closed Reactor Experiments Using Equimolar N-Butane + Oxygen Premixtures At Reduced-Gravity, Howard Pearlman, Michael R. Foster
The Role Of Diffusive Transport On Low And Intermediate Temperature Hydrocarbon Oxidation: Closed Reactor Experiments Using Equimolar N-Butane + Oxygen Premixtures At Reduced-Gravity, Howard Pearlman, Michael R. Foster
Faculty Publications - Biomedical, Mechanical, and Civil Engineering
Experiments were conducted in a closed, spherical reactor aboard NASA's KC-135 reduced-gravity aircraft using an equimolar n-C4H10 + 0 2 premixture ( Le = 1.3) at subatmospheric · pressures to compliment model predictions and further explore the reactive-diffusive structure of cool flames and ignitions. The pressure and radial temperature histories were recorded and analyzed for different initial conditions. In addition, the visible light emission from excited formaldehyde was recorded using an intensified video camera and was observed to be radially symmetric in all cases. Unexpectedly, however, the measured temperature distributions during (and after the passage of) the cool flames and …
Cool Flames At Terrestrial, Partial, And Near-Zero Gravity, Michael R. Foster, Howard Pearlman
Cool Flames At Terrestrial, Partial, And Near-Zero Gravity, Michael R. Foster, Howard Pearlman
Faculty Publications - Biomedical, Mechanical, and Civil Engineering
Natural convection plays an important role in all terrestrial, Lunar, and Martian-based, unstirred, static reactor cool flame and low-temperature autoignitions, since the Rayleigh number (Ra) associated with the self-heating of the reaction exceeds the critical Ra (approximately 600) for onset of convection. At near-zero gravity, Ra < 600 can be achieved and the effects of convection suppressed. To systematically vary the Ra without varying the mixture stoichiometry, reactor pressure, or vessel size, cool flames are studied experimentally in a closed, unstirred, static reactor subject to different gravitational accelerations (terrestrial, 1g; Martian, 0.38g; Lunar, 0.16g; a n dr e - duced gravity, ∼10−2g). Representative results show the evolution of the visible light emission using an equimolar n-butane:oxygen premixture at temperatures ranging from 320 to 350 ◦C (593–623 K) at subatmospheric pressures. For representative reduced-gravity, spherically propagating cool flames, the flame radius based on the peak light intensity is plotted as a function of time and the flame radius (and speed) is calculated from a polynomial fit to data. A skeletal chemical kinetic Gray-Yang model developed previously for a one-dimensional, reactive– diffusive system by Fairlie and co-workers is extended to a two-dimensional axisymmetric, spherical geometry. The coupled species, energy, and momentum equations are solved numerically and the spatio-temporal variations in the temperature profiles are presented. A qualitative comparison is made with the experimental results.
An Existing Global Heptane Mechanism Augmented With Diffusive Transport, Michael R. Foster, Howard Pearlman
An Existing Global Heptane Mechanism Augmented With Diffusive Transport, Michael R. Foster, Howard Pearlman
Faculty Publications - Biomedical, Mechanical, and Civil Engineering
The couplings between diffusive transport and the temperature and species concentration distributions associated with low and intermediate temperature heptane oxidation are explored using an existing four-step heptane mechanism, tuned for elevated pressures. The energy and species concentration equations are augmented with diffusive fluxes for heat and species and solved numerically in a one-dimensional domain. The ignition delay times are also tabulated and compared with the zero-dimensional data reported in the literature.