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Removal Of Trace Organic Contaminants By An Mbr Comprising A Mixed Culture Of Bacteria And White-Rot Fungi, Luong Nguyen, Faisal Hai, Shufan Yang, Jinguo Kang, Frederic Leusch, Felicity Roddick, William Price, Long Nghiem
Removal Of Trace Organic Contaminants By An Mbr Comprising A Mixed Culture Of Bacteria And White-Rot Fungi, Luong Nguyen, Faisal Hai, Shufan Yang, Jinguo Kang, Frederic Leusch, Felicity Roddick, William Price, Long Nghiem
Faisal I Hai
The degradation of 30 trace organic contaminants (TrOC) by a white-rot fungus-augmented membrane bioreactor (MBR) was investigated. The results show that white-rot fungal enzyme (laccase), coupled with a redox mediator (1-hydroxy benzotriazole, HBT), could degrade TrOC that are resistant to bacterial degradation (e.g. diclofenac, triclosan, naproxen and atrazine) but achieved low removal of compounds (e.g. ibuprofen, gemfibrozil and amitriptyline) that are well removed by conventional activated sludge treatment. Overall, the fungus-augmented MBR showed better TrOC removal compared to a system containing conventional activated sludge. The major role of biodegradation in removal by the MBR was noted. Continuous mediator dosing to …
Enhancement Of Removal Of Trace Organic Contaminants By Powdered Activated Carbon Dosing Into Membrane Bioreactors, Ngoc Luong Nguyen, Faisal Ibney Hai, Long Nghiem, Jinguo Kang, William Price, Chul Park, Kazuo Yamamoto
Enhancement Of Removal Of Trace Organic Contaminants By Powdered Activated Carbon Dosing Into Membrane Bioreactors, Ngoc Luong Nguyen, Faisal Ibney Hai, Long Nghiem, Jinguo Kang, William Price, Chul Park, Kazuo Yamamoto
Faisal I Hai
This study compared the removal efficiency of 22 widespread trace organic contaminants by a laboratory-scale membrane bioreactor (MBR) with and without direct addition of powdered activated carbon (PAC) into the activated sludge reactor over a period of 312 days. The removal of hydrophilic and biologically persistent trace organic contaminants was immediately improved to above 95% after the addition of PAC into MBR. However, a compound-specific gradual decrease in removal underscored the requirement for the addition of fresh PAC. Adsorption onto PAC-added sludge appeared to play a significant role in the relatively more effective aqueous phase removal of a few resistant …
Removal Of Pharmaceuticals, Steroid Hormones, Phytoestrogens, Uv-Filters, Industrial Chemicals And Pesticides By Trametes Versicolor: Role Of Biosorption And Biodegradation, Luong Nguyen, Faisal Ibney Hai, Shufan Yang, Jinguo Kang, Frederic Leusch, Felicity Roddick, William E. Price, Long D. Nghiem
Removal Of Pharmaceuticals, Steroid Hormones, Phytoestrogens, Uv-Filters, Industrial Chemicals And Pesticides By Trametes Versicolor: Role Of Biosorption And Biodegradation, Luong Nguyen, Faisal Ibney Hai, Shufan Yang, Jinguo Kang, Frederic Leusch, Felicity Roddick, William E. Price, Long D. Nghiem
Faisal I Hai
This study reports the removal of 30 diverse trace organic contaminants (TrOC) by live (biosorption þ biodegradation), intracellular enzyme-inhibited and chemically inactivated (biosorption only) whole-cell preparations and the fungal extracellular enzyme extract (predominantly laccase) from Trametes versicolor (ATCC 7731). Because phenolic substrates are amenable to degradation by laccase, all 14 phenolic TrOC were readily biodegraded. On the other hand, only eight of the 16 non-phenolic TrOC were readily biodegraded while the removal of hydrophilic TrOC (log D < 3) was negligible. With the exception of diclofenac, no non-phenolic TrOC were degraded by the extracellular enzyme extract. The whole-cell culture showed considerably …
Wastewater Reuse: Removal Of Emerging Trace Organic Contaminants (Troc), Faisal Hai, Long Nghiem, Stuart Khan, William Price, Kazuo Yamamoto
Wastewater Reuse: Removal Of Emerging Trace Organic Contaminants (Troc), Faisal Hai, Long Nghiem, Stuart Khan, William Price, Kazuo Yamamoto
Faisal I Hai
This chapter reviews current and new technologies for the removal of emerging TrOC from wastewater for reuse purposes. In particular, it compares the relative performance of Membrane bioreactors (MBR) with other conventional biological processes. It is shown that MBR has many intrinsic advantages over other methods leading to superior performance. Fundamental to this is the presence of a membrane barrier which provides a range of other adsorption mechanisms for TrOC. However, in practice there are many factors affecting TrOC removal by MBR, leading to sometimes conflicting reports in the literature from both lab scale studies as well as full scale …
Removal Of Emerging Trace Organic Contaminants By Mbr-Based Hybrid Treatment Processes, Luong Nguyen, Faisal Ibney Hai, Jinguo Kang, William E. Price, Long D. Nghiem
Removal Of Emerging Trace Organic Contaminants By Mbr-Based Hybrid Treatment Processes, Luong Nguyen, Faisal Ibney Hai, Jinguo Kang, William E. Price, Long D. Nghiem
Faisal I Hai
The aim of this study was to demonstrate the complementarity of combining membrane bioreactor (MBR) treatment with UV oxidation or high pressure membrane filtration processes such as nanofiltration (NF) or reverse osmosis (RO) for the removal of trace organic contaminants (TrOC). The results suggest that the removal mechanisms of TrOC by either UV oxidation or NF/RO membrane filtration differ significantly from those of an MBR system. Thus, they can complement MBR treatment very well to significantly improve the removal of TrOC. MBR treatment can effectively remove hydrophobic and readily biodegradable hydrophilic TrOC. The remaining hydrophilic and biologically persistent TrOC were …
Removal And Fate Of Micropollutants In A Sponge-Based Moving Bed Bioreactor, Yunlong Luo, Wenshan Guo, Huu H. Ngo, Long Nghiem, Faisal Ibney Hai, Jinguo Kang, Siqing Xia, Zhiqiang Zhang, William Price
Removal And Fate Of Micropollutants In A Sponge-Based Moving Bed Bioreactor, Yunlong Luo, Wenshan Guo, Huu H. Ngo, Long Nghiem, Faisal Ibney Hai, Jinguo Kang, Siqing Xia, Zhiqiang Zhang, William Price
Faisal I Hai
This study investigated the removal of micropollutants using polyurethane sponge as attached-growth carrier. Batch experiments demonstrated that micropollutants could adsorb to non-acclimatized sponge cubes to varying extents. Acclimatized sponge showed significantly enhanced removal of some less hydrophobic compounds (logD < 2.5), such as ibuprofen, acetaminophen, naproxen, and estriol, as compared with non-acclimatized sponge. The results for bench-scale sponge-based moving bed bioreactor (MBBR) system elucidated compound-specific variation in removal, ranging from 25.9% (carbamazepine) to 96.8% (b-Estradiol 17-acetate) on average. In the MBBR system, biodegradation served as a major removal pathway for most compounds. However, sorption to sludge phase was also a notable …
Comparison Between Sequential And Simultaneous Application Of Activated Carbon With Membrane Bioreactor For Trace Organic Contaminant Removal, Luong N. Nguyen, Faisal I. Hai, Jinguo Kang, Long D. Nghiem, William E. Price, Wenshan Guo, Huu H. Ngo, Kuo-Lun Tung
Comparison Between Sequential And Simultaneous Application Of Activated Carbon With Membrane Bioreactor For Trace Organic Contaminant Removal, Luong N. Nguyen, Faisal I. Hai, Jinguo Kang, Long D. Nghiem, William E. Price, Wenshan Guo, Huu H. Ngo, Kuo-Lun Tung
Faisal I Hai
The removal efficiency of 22 selected trace organic contaminants by sequential application of granular activated carbon (GAC) and simultaneous application of powdered activated carbon (PAC) with membrane bioreactor (MBR) was compared in this study. Both sequential application of GAC following MBR treatment (MBR–GAC) and simultaneous application of PAC within MBR (PAC–MBR) achieved improved removal (over 95%) of seven hydrophilic and biologically persistent compounds, which were less efficiently removed by MBR-only treatment (negligible to 70%). However, gradual breakthrough of these compounds occurred over an extended operation period. Charged compounds, particularly, fenoprop and diclofenac, demonstrated the fastest breakthrough (complete and 50–70%, in …
Coupling Granular Activated Carbon Adsorption With Membrane Bioreactor Treatment For Trace Organic Contaminant Removal: Breakthrough Behaviour Of Persistent And Hydrophilic Compounds, Luong N. Nguyen, Faisal I. Hai, William E. Price, Jinguo Kang, Long D. Nghiem
Coupling Granular Activated Carbon Adsorption With Membrane Bioreactor Treatment For Trace Organic Contaminant Removal: Breakthrough Behaviour Of Persistent And Hydrophilic Compounds, Luong N. Nguyen, Faisal I. Hai, William E. Price, Jinguo Kang, Long D. Nghiem
Faisal I Hai
This study investigated the removal of trace organic contaminants by a combined membrane bioreactor - granular activated carbon (MBR-GAC) system over a period of 196 days. Of the 22 compounds investigated here, all six hydrophilic compounds with electron-withdrawing functional groups (i.e., metronidazole, carbamazepine, ketoprofen, naproxen, fenoprop and diclofenac) exhibited very low removal efficiency by MBR-only treatment. GAC post-treatment initially complemented MBR treatment very well; however, a compound-specific gradual deterioration of the removal of the above-mentioned problematic compounds was noted. While a 20% breakthrough of all four negatively charged compounds namely ketoprofen, naproxen, fenoprop and diclofenac occurred within 1000-3000 bed volumes …
Coupling Powdered Activated Carbon (Pac) Adsorption With Membrane Bioreactor (Mbr) Treatment For Enhanced Removal Of Trace Organics, Luong Nguyen, Faisal Ibney Hai, Long Nghiem, Jinguo Kang, William Price
Coupling Powdered Activated Carbon (Pac) Adsorption With Membrane Bioreactor (Mbr) Treatment For Enhanced Removal Of Trace Organics, Luong Nguyen, Faisal Ibney Hai, Long Nghiem, Jinguo Kang, William Price
Faisal I Hai
the occurrence of trace organics such as pesticides, pharmaceutically active compounds, natural and synthetic hormones as well as varous industrial compounds in the aquatic environment is of great concern due to their potential adverse effects on human health and those of other biota. Therefore, the removal of these compounds from wastewater is an important consideration to ensure safe drinking water and better protection of the environment. In the literature, several techniques have been explored for trace organics removal, namely, conventional activated sludge, membrane bioreactors (MBRs), and absorptioin. However it has been found that neither MBR nor activated carbon on its …
A Novel Membrane Distillation-Thermophilic Bioreactor System: Biological Stability And Trace Organic Compound Removal, Kaushalya Wijekoon, Faisal Hai, Jinguo Kang, William Price, Wenshan Guo, Hao Ngo, Tzahi Cath, Long Nghiem
A Novel Membrane Distillation-Thermophilic Bioreactor System: Biological Stability And Trace Organic Compound Removal, Kaushalya Wijekoon, Faisal Hai, Jinguo Kang, William Price, Wenshan Guo, Hao Ngo, Tzahi Cath, Long Nghiem
Faisal I Hai
The removal of trace organic compounds (TrOCs) by a novel membrane distillation-thermophilic bioreactor (MDBR) system was examined. Salinity build-up and the thermophilic conditions to some extent adversely impacted the performance of the bioreactor, particularly the removal of total nitrogen and recalcitrant TrOCs. While most TrOCs were well removed by the thermophilic bioreactor, compounds containing electron withdrawing functional groups in their molecular structure were recalcitrant to biological treatment and their removal efficiency by the thermophilic bioreactor was low (0-53%). However, the overall performance of the novel MDBR system with respect to the removal of total organic carbon, total nitrogen, and TrOCs …
Biocatalytic Membrane Reactors For The Removal Of Recalcitrant And Emerging Pollutants From Wastewater, F Hai, L Nghiem, O Modin
Biocatalytic Membrane Reactors For The Removal Of Recalcitrant And Emerging Pollutants From Wastewater, F Hai, L Nghiem, O Modin
Faisal I Hai
The potential fields of application of biocatalytic membrane reactors have widened considerably in recent years. Although biocatalytic membrane reactors, in general, are yet to achieve broad industrial application, in the not too far future they are expected to play a major role, not only for the production, transformation and valorization of raw materials but also for environmental remediations. This chapter comprehensively reviews the laboratory scale studies which demonstrate the potential of biocatalytic membrane reactors in wastewater treatment applications. Studies reponed in the literature, however, serve as proof of concept only. Issues that need to be addressed in order to achieve …
Removal Of Bisphenol A And Diclofenac By A Novel Fungal Membrane Bioreactor Operated Under Non-Sterile Conditions, Shufan Yang, Faisal I. Hai, Long D. Nghiem, Luong N. Nguyen, Felicity Roddick, William E. Price
Removal Of Bisphenol A And Diclofenac By A Novel Fungal Membrane Bioreactor Operated Under Non-Sterile Conditions, Shufan Yang, Faisal I. Hai, Long D. Nghiem, Luong N. Nguyen, Felicity Roddick, William E. Price
Faisal I Hai
Previous studies have confirmed significant removal of various trace organic contaminants (TrOCs) by white-rot fungal cultures under sterile batch test conditions. However, little is known about TrOC removal in continuous flow fungal reactors in a non-sterile environment. This study reports the removal of two TrOCs, namely, bisphenol A and diclofenac, by a fungal membrane bioreactor (MBR).
A Review On The Occurrence Of Micropollutants In The Aquatic Environment And Their Fate And Removal During Wastewater Treatment, Yunlong Luo, Wenshan Guo, Huu Hao Ngo, Long Duc Nghiem, Faisal Ibney Hai, Jian Zhang, Shuang Liang, Xiaochang C. Wang
A Review On The Occurrence Of Micropollutants In The Aquatic Environment And Their Fate And Removal During Wastewater Treatment, Yunlong Luo, Wenshan Guo, Huu Hao Ngo, Long Duc Nghiem, Faisal Ibney Hai, Jian Zhang, Shuang Liang, Xiaochang C. Wang
Faisal I Hai
Micropollutants are emerging as a new challenge to the scientific community. This review provides a summary of the recent occurrence of micropollutants in the aquatic environment including sewage, surface water, groundwater and drinking water. The discharge of treated effluent from WWTPs is a major pathway for the introduction of micropollutants to surface water. WWTPs act as primary barriers against the spread of micropollutants. WWTP removal efficiency of the selected micropollutants in 14 countries/regions depicts compound-specific variation in removal, ranging from 12.5 to 100%. Advanced treatment processes, such as activated carbon adsorption, advanced oxidation processes, nanofiltration, reverse osmosis, and membrane bioreactors …