Condensed Matter Physics Commons^™

A Systematic Study Of The Effect Of Spin-Orbit Interaction On Properties Of Tetravalent And Pentavalent Iridate Compounds, Jasminka Terzic

Theses and Dissertations--Physics and Astronomy

Previous studies of iridates have shown that an interplay of strong SOI, Coulomb interaction U, Hund’s rule coupling and crystalline electric fields result in unexpected insulating states with complex magnetic states. The novel J_eff =1/2 insulating state first observed in Sr₂IrO₄ is a direct consequence of such an intriguing interplay and is one of the central foci of this dissertation study.

The work presented here consists of three projects: (1) Effects of Tb doping on Sr₂IrO₄ having tetravalent Ir⁴⁺(5d⁵) ions; (2) Emergence of unexpected magnetic states in double-perovskite (Ba …

A Systematic Study Of Transport, Magnetic And Thermal Properties Of Layered Iridates, Oleksandr B. Korneta

Theses and Dissertations--Physics and Astronomy

A unique feature of the 5d-iridates is that the spin-orbit interaction (SOI) and Coulomb interactions U are of comparable strength and therefore compete vigorously. The relative strength of these interactions stabilizes new exotic ground states that provide a fertile ground for studying new physics. SOI is proportional to Z^4 (Z is the atomic number), and it is now recognized that strong SOI can drive novel narrow-gap insulating states in heavy transition metal oxides such as iridates. Indeed, strong SOI necessarily introduces strong lattice degrees of freedom that become critical to new physics in the iridates. This dissertation thoroughly examines a …

The Development And Implementation Of Electromechanical Devices To Study The Physical Properties Of Sr2iro4 And Tas3, John A. Nichols

Theses and Dissertations--Physics and Astronomy

Transition metal oxides (TMO) have proven to exhibit novel properties such as high temperature superconductivity, magnetic ordering, charge and spin density waves, metal to insulator transitions and colossal magnetoresistance. Among these are a spin-orbit coupling (SOC) induced Mott insulator Sr₂IrO₄. The electric transport properties of this material remain finite even at cryogenic temperatures enabling its complex electronic structure to be investigated by a scanning tunneling microscope. At T = 77 K, we observed two features which represent the Mott gap with a value of 2D ~ 615 meV. Additionally an inelastic loss feature was observed inside …