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Condensed Matter Physics Commons

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Full-Text Articles in Condensed Matter Physics

Pyseg: A Python Package For 2d Material Flake Localization, Segmentation, And Thickness Prediction, Diana B. Horangic Dec 2022

Pyseg: A Python Package For 2d Material Flake Localization, Segmentation, And Thickness Prediction, Diana B. Horangic

Student Research Projects

Thin materials are of interest for their extraordinary physical, mechanical, thermal, electrical, and optical properties. Monolayers and bilayers of 2D materials can be manufactured through a variety of exfoliation methods. To determine layer thickness, Raman spectroscopy or other methods like Rayleigh scattering are used. These methods are, however, slow, and they require equipment beyond an optical microscope. A Python package that automates flake identification processes was built, with access solely to RGB data from an optical microscope assumed. My package, pyseg, localizes flakes on a substrate and then makes a rough estimate of their thickness from first principles. It can …


Resonant Plasmonic–Biomolecular Chiral Interactions In The Far-Ultraviolet: Enantiomeric Discrimination Of Sub-10 Nm Amino Acid Films, Tiago Ramos Leite, Lin Zschiedrich, Orhan Kizilkaya, Kevin M. Mcpeak Sep 2022

Resonant Plasmonic–Biomolecular Chiral Interactions In The Far-Ultraviolet: Enantiomeric Discrimination Of Sub-10 Nm Amino Acid Films, Tiago Ramos Leite, Lin Zschiedrich, Orhan Kizilkaya, Kevin M. Mcpeak

Faculty Publications

Resonant plasmonic–molecular chiral interactions are a promising route to enhanced biosensing. However, biomolecular optical activity primarily exists in the far-ultraviolet regime, posing significant challenges for spectral overlap with current nano-optical platforms. We demonstrate experimentally and computationally the enhanced chiral sensing of a resonant plasmonic–biomolecular system operating in the far-UV. We develop a full-wave model of biomolecular films on Al gammadion arrays using experimentally derived chirality parameters. Our calculations show that detectable enhancements in the chiroptical signals from small amounts of biomolecules are possible only when tight spectral overlap exists between the plasmonic and biomolecular chiral responses. We support this conclusion …


Control Of Nonlinear Properties Of Van Der Waals Materials, Rezlind Bushati Sep 2022

Control Of Nonlinear Properties Of Van Der Waals Materials, Rezlind Bushati

Dissertations, Theses, and Capstone Projects

Van der Waals materials are a broad class of materials that exhibit unique optoelectronic properties. They provide a rich playground for which they can be integrated into current on-chip devices due to their nanometer-scale size, and be utilized for studying fundamental physics. Strong coupling of emitters to microcavities provides many opportunities for new exotic physics through the formation of hybrid quasi-particles exciton-polaritons. This thesis
focuses on exploring and enhancing nonlinearity of van der Waals materials through strongly coupling to microcavities. By taking advantage of the stacking order of TMDs, we show intense second-harmonic generation from bulk, centrosymmetric TMD systems. In …


Exploring Magneto-Excitons In Bulk And Mono-Layer Semiconductors Using Non-Linear Spectroscopy Techniques, Varun Mapara Mar 2022

Exploring Magneto-Excitons In Bulk And Mono-Layer Semiconductors Using Non-Linear Spectroscopy Techniques, Varun Mapara

USF Tampa Graduate Theses and Dissertations

The research in two-dimensional (2D) materials has evolved from ``traditional" quantum wells based on group III-V and II-VI semiconductors to atomically thin sheets of van der Waals materials such as 2D semiconducting Transition Metal Dichalcogenides (TMDs). These 2D materials remain a stimulating field that continues to introduce new challenges. From both a fundamental physics and technological perspective, magneto-optical spectroscopy has been an essential tool in this research field. TMDs, for example, pose the challenge of characterizing their spin-valley-resolved physics and deriving implications in quantum computation and information research. With the discovery of valley Zeeman effects, the spin-valley physics of TMDs …


Charge Transport And Spin Dynamics Of Color Centers In Diamond, Damon Daw Feb 2022

Charge Transport And Spin Dynamics Of Color Centers In Diamond, Damon Daw

Dissertations, Theses, and Capstone Projects

Solid state defects in diamond are promising candidates for room temperature quantum information processors (1, 3, 5). Chief among these defects is the nitrogen vacancy center (‘NV center’ or ‘NV’). The NV has long coherence times (at 300K) and its state is easily initialized, manipulated and read out (5). However, the outstanding issue of entangling NV centers in a scalable fashion, at room temperature remains a challenge. This thesis presents experimental and theoretical work aimed at achieving this goal by developing the ‘flying qubit’ framework in (1). This method for remote entanglement utilizes a charge carrier (initialized into a definite …


Hot-Carrier Dynamics And Transport Mechanisms In Inas/Alassb Multiple Quantum Wells, Herath Pathiranage Janaka Chathuranga Piyathilaka Jan 2022

Hot-Carrier Dynamics And Transport Mechanisms In Inas/Alassb Multiple Quantum Wells, Herath Pathiranage Janaka Chathuranga Piyathilaka

Graduate Theses, Dissertations, and Problem Reports

Semiconductor photovoltaics convert light into electricity through the extraction of photo-excited charge carriers. Among the most important parameters for a photovoltaic cell are good optical absorption in the desired region of the electromagnetic spectrum, and sufficient excited-state lifetimes and mobilities of the photocarriers to allow for charge separation and extraction before recombination. For solar cell applications there are significant challenges to overcome to improve the efficiency of the light-to-electricity conversion. The cells are most commonly made of silicon, which has a nearly perfect bandgap for absorbing the most solar radiation, an indirect bandgap to give a long photocarrier lifetime and …


Characterization And Coherent Spin Selective Manipulation Of Quantum Dot Energy Levels, Tristan Anthony Wilkinson Jan 2022

Characterization And Coherent Spin Selective Manipulation Of Quantum Dot Energy Levels, Tristan Anthony Wilkinson

Graduate Theses, Dissertations, and Problem Reports

Semiconductor quantum dots (QDs) are promising candidates to fulfill a wide range of applications in real-world quantum computing, communication, and networks. Their excellent optical properties such as high brightness, single-photon purity, and narrow linewidths show potential utility in many areas. In order to realize long term goals of integration into complex and scalable quantum information systems, many current challenges must be overcome. One of these challenges is accomplishment of all necessary computing operations within a QD, which might be enabled by coherent manipulation of single QD energy level structures. In the realm of scalability for quantum devices, a way to …


Charge Dynamics Of Inas Quantum Dots Under Resonant And Above-Band Excitation, Gary R. Lander Jr Jan 2022

Charge Dynamics Of Inas Quantum Dots Under Resonant And Above-Band Excitation, Gary R. Lander Jr

Graduate Theses, Dissertations, and Problem Reports

Research involving light-matter interactions in semiconductor nanostructures has been an interesting topic of investigation for decades. Many systems have been studied for not only probing fundamental physics of the solid state, but also for direct development of technological advancements. Research regarding self-assembled, epitaxially grown quantum dots (QDs) has proven to be prominent in both regards. The development of a reliable, robust source for the production of quantum bits to be utilized in quantum information protocols is a leading venture in the world of condensed matter and solid-state physics. Fluorescence from resonantly driven QDs is a promising candidate for the production …