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Articles 1 - 29 of 29
Full-Text Articles in Physics
Physical, Optical, And Chemical Properties Of Light Absorbing Aerosols And Their Climatic Impacts, Susan Mathai
Physical, Optical, And Chemical Properties Of Light Absorbing Aerosols And Their Climatic Impacts, Susan Mathai
Dissertations, Master's Theses and Master's Reports
Aerosols are particles suspended in the atmosphere; they are emitted during natural phenomena such as dust storms, wildfires, and volcanic eruptions, and during anthropogenic activities like household wood burning, vehicles operations, and industrial productions, or they can form in the atmosphere from gas to particle partition. Aerosols impact earth’s weather and climate by absorbing and scattering the incoming solar and the outgoing earth thermal radiation and interacting with clouds. The optical properties of aerosols evolve as the chemical and physical properties vary during their residence in the atmosphere. In addition, the aerosols’ properties strongly depend on the vertical distribution in …
Optical And Single Particle Properties Of North Atlantic Free Tropospheric Aerosols And Implications For Aerosol Direct Radiative Forcing, Megan Morgenstern
Optical And Single Particle Properties Of North Atlantic Free Tropospheric Aerosols And Implications For Aerosol Direct Radiative Forcing, Megan Morgenstern
Dissertations, Master's Theses and Master's Reports
Human-induced climate change has steadily become a reality rather than a possibility. One factor that plays into climate change is radiative forcing due to aerosol-radiation interactions (ARI). As such, it is important to understand how aerosols (atmospheric particles) interact with solar radiation. This work looks at seven samples of well-aged aerosols (aerosols traveling in the atmosphere for at least a few days) collected at Pico Mountain Observatory in the summer of 2015. Pico Mountain Observatory is located in a remote, high elevation site in the Azores, in the Eastern-North Atlantic Ocean. The goals of the study were to analyze the …
The Hitran2020 Molecular Spectroscopic Database, I. E. Gordon, L. S. Rothman, R. J. Hargreaves, R. Hashemi, E. V. Karlovets, F. M. Skinner, E. K. Conway, C. Hill, R. V. Kochanov, Y. Tan, P. Wcisło, A.A. Finenko, K. Nelson, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, A. Coustenis, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, E. J. Mlawer, A. V. Nikitin, V.I. Perevalov, M. Rotger, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, E. M. Adkins, A. Baker, A. Barbe, E. Canè, A. G. Császár, A. Dudaryonok, O. Egorov, A. J. Fleisher, H. Fleurbaey, A. Foltynowicz, T. Furtenbacher, J. J. Harrison, J.M. Hartmann, V.- M. Horneman, X. Huang, T. Karman, J. Karns, S. Kassi, I. Kleiner, V. Kofman, F. Kwabia-Tchana, N.N. Lavrentieva, T. J. Lee, D. A. Long, A. A. Lukashevskaya, O. M. Lyulin, V. Yu Makhnev, W. Matt, S. T. Massie, M. Melosso, S. N. Mikhailenko, D. Mondelain, H.S.P. Müller, O. V. Naumenko, A. Perrin, O. L. Polyansky, E. Raddaoui, P. L. Raston, Z. D. Reed, M. Rey, C. Richard, R. Tóbiás, I. Sadiek, D. W. Schwenke, E. Starikova, K. Sung, F. Tamassia, S. A. Tashkun, J. Vander Auwera, I.A. Vasilenko, A.A. Vigasin, G.L. Villanueva, B. Vispoel, G. Wagner, A. Yachmenev, S. N. Yurchenko
The Hitran2020 Molecular Spectroscopic Database, I. E. Gordon, L. S. Rothman, R. J. Hargreaves, R. Hashemi, E. V. Karlovets, F. M. Skinner, E. K. Conway, C. Hill, R. V. Kochanov, Y. Tan, P. Wcisło, A.A. Finenko, K. Nelson, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance, A. Coustenis, B. J. Drouin, J.-M. Flaud, R. R. Gamache, J. T. Hodges, D. Jacquemart, E. J. Mlawer, A. V. Nikitin, V.I. Perevalov, M. Rotger, J. Tennyson, G. C. Toon, H. Tran, V. G. Tyuterev, E. M. Adkins, A. Baker, A. Barbe, E. Canè, A. G. Császár, A. Dudaryonok, O. Egorov, A. J. Fleisher, H. Fleurbaey, A. Foltynowicz, T. Furtenbacher, J. J. Harrison, J.M. Hartmann, V.- M. Horneman, X. Huang, T. Karman, J. Karns, S. Kassi, I. Kleiner, V. Kofman, F. Kwabia-Tchana, N.N. Lavrentieva, T. J. Lee, D. A. Long, A. A. Lukashevskaya, O. M. Lyulin, V. Yu Makhnev, W. Matt, S. T. Massie, M. Melosso, S. N. Mikhailenko, D. Mondelain, H.S.P. Müller, O. V. Naumenko, A. Perrin, O. L. Polyansky, E. Raddaoui, P. L. Raston, Z. D. Reed, M. Rey, C. Richard, R. Tóbiás, I. Sadiek, D. W. Schwenke, E. Starikova, K. Sung, F. Tamassia, S. A. Tashkun, J. Vander Auwera, I.A. Vasilenko, A.A. Vigasin, G.L. Villanueva, B. Vispoel, G. Wagner, A. Yachmenev, S. N. Yurchenko
Chemistry & Biochemistry Faculty Publications
The HITRAN database is a compilation of molecular spectroscopic parameters. It was established in the early 1970s and is used by various computer codes to predict and simulate the transmission and emission of light in gaseous media (with an emphasis on terrestrial and planetary atmospheres). The HITRAN compilation is composed of five major components: the line-by-line spectroscopic parameters required for high-resolution radiative-transfer codes, experimental infrared absorption cross-sections (for molecules where it is not yet feasible for representation in a line-by-line form), collision-induced absorption data, aerosol indices of refraction, and general tables (including partition sums) that apply globally to the data. …
Calibration Of Gas Flow Meters Using Choked Flow And An Evacuated Vessel, Max B. Trueblood, Otmar Schmid, Nicholas Altese, Christian J. Hurst, Wenyan Liu, Teresa Gelles, Steven C. Achterberg, Philip D. Whitefield, Donald E. Hagen
Calibration Of Gas Flow Meters Using Choked Flow And An Evacuated Vessel, Max B. Trueblood, Otmar Schmid, Nicholas Altese, Christian J. Hurst, Wenyan Liu, Teresa Gelles, Steven C. Achterberg, Philip D. Whitefield, Donald E. Hagen
Chemistry Faculty Research & Creative Works
The measurement of gas flow rates is of great importance in a wide range of modern technologies. This paper introduces a simple, yet accurate technique for in-house calibration of gas FMs (mass and volumetric) even under harsh environmental conditions such as encountered during field measurement campaigns. The method requires only readily available, low cost components: a vessel of known volume, an air pump, a pressure sensor and a metal plate orifice or a needle valve to act as a CO. The unique property of choked flow in the CO is used here for flow calibration. In the method presented here …
Observation Of New Particle Formation In The Northern Hemisphere At Altitude From 4 To 20 Km, Mohamed Saad
Observation Of New Particle Formation In The Northern Hemisphere At Altitude From 4 To 20 Km, Mohamed Saad
Electronic Theses and Dissertations
New particle formation (NPF) is investigated using measurements of aerosol size distributions and meteorological variables made in two continents, including USA and Europe. Despite the considerably different aerosol particle abundances among the sites, a common relationship was found between the characteristics of NPF events and the air mass convective and/or advective transport. CO and O3 act as tracers of tropospheric and stratospheric air, respectively, their statistical relationship can be used to quantify air mass characteristics and origins. The mixing ratio values of CO increased within the upper troposphere layer before/during NPF events, which may serve as an indicator of occurring …
The Aging And Impacts Of Atmospheric Soot: Closing The Gap Between Experiments And Models, Ogochukwu Yvonne Enekwizu
The Aging And Impacts Of Atmospheric Soot: Closing The Gap Between Experiments And Models, Ogochukwu Yvonne Enekwizu
Dissertations
The main goal of this dissertation is to generate data and parameterizations to accurately represent soot aerosols in atmospheric models. Soot from incomplete combustion of fossil fuels and biomass burning is a major air pollutant and a significant contributor to climate warming. The environmental impacts of soot are strongly dependent on the particle morphology and mixing state, which evolve continuously during atmospheric transport via a process known as aging. To make predictions of soot impacts on the environment, most atmospheric models adopt simplifications of particle structure and mixing state, which lead to substantial uncertainties. Using an experimentally constrained modeling approach, …
Growth Of Small Particles In Nonequilibrium Plasmas, Necip Berker Üner
Growth Of Small Particles In Nonequilibrium Plasmas, Necip Berker Üner
McKelvey School of Engineering Theses & Dissertations
Nonequilibrium plasma (NEP) is an extraordinary environment for material synthesis. NEP is comprised of hot electrons with temperatures greater than 10000 K and of cold ions and neutrals that are usually at few hundred kelvins above room temperature. Due to this large difference in species’ temperatures, the assumption of local thermal equilibrium does not hold in NEP. Therefore, NEP can act as a unique processor of mass, and it can transform materials along pathways that are not accessible by methods wherein local thermal equilibrium is valid. For decades, NEPs have been employed in the semiconductor industry to manufacture many thin …
Long-Range Aerosol Transport And Impacts On Size-Resolved Aerosol Composition In Metro Manila, Philippines, Rachel A. Braun, Mojtaba Azadi Aghdam, Paola Angela Bañaga, Grace Betito, Maria Obiminda L. Cambaliza, Melliza Templonuevo Cruz, Genevieve Rose Lorenzo, Alexander B. Macdonald, James Bernard Simpas, Connor Stahl, Armin Sorooshian
Long-Range Aerosol Transport And Impacts On Size-Resolved Aerosol Composition In Metro Manila, Philippines, Rachel A. Braun, Mojtaba Azadi Aghdam, Paola Angela Bañaga, Grace Betito, Maria Obiminda L. Cambaliza, Melliza Templonuevo Cruz, Genevieve Rose Lorenzo, Alexander B. Macdonald, James Bernard Simpas, Connor Stahl, Armin Sorooshian
Physics Faculty Publications
This study analyzes long-range transport of aerosol and aerosol chemical characteristics based on instances of high- and low-aerosol-loading events determined via ground-based size-resolved aerosol measurements collected at the Manila Observatory in Metro Manila, Philippines, from July to October 2018. Multiple data sources, including models, remote sensing, and in situ measurements, are used to analyze the impacts of long-range aerosol transport on Metro Manila and the conditions at the local and synoptic scales facilitating this transport. Through the use of case studies, evidence of long-range transport of biomass burning aerosol and continental emissions is identified in Metro Manila. Long-range transport of …
Investigation Of An Unusual Thin Layer Descending Through The Upper Stratosphere, Houston D. Bentley
Investigation Of An Unusual Thin Layer Descending Through The Upper Stratosphere, Houston D. Bentley
Physics Capstone Projects
Lidar observations on the night of 19-20 February 2004 at Logan, Utah (41.74 N, 111.81 W) revealed a strange thin layer which descended from roughly 55 km to 30 km over seven hours. Approximations are made for the dimensions and descent rate of the layer. Although the particle radius and density are unknown, a range can be determined from the descent rate and reference to the sizes of known particles. Several possible sources for the layer are explored, concluding that an object entering the Earth’s atmosphere was the most probable cause.
Effect Of Aerosol Distributions On Precipitation Patterns Needed For A Rapid Ice Age, Steven M. Gollmer
Effect Of Aerosol Distributions On Precipitation Patterns Needed For A Rapid Ice Age, Steven M. Gollmer
Proceedings of the International Conference on Creationism
Introduced in the Genesis Flood by Whitcomb and Morris (1961) and fleshed out by Oard (1979) a model for an ice age in the wake of the Genesis flood was used to explain the evidence of glaciation in Canada and the United States without resorting to eons of time. It was proposed that this rapid ice age was the consequence of post flood warm oceans, barren land and volcanic aerosols. The impact of warm oceans was simulated by Vardiman (1998) and Gollmer (2013) using climate models. Although warm oceans increase precipitation in the Arctic, global surface temperatures become unbearably hot …
Comparison Of Various Mean Field Formulations For Retrieving Refractive Indices Of Aerosol Particles Containing Inclusions, Kristin S. Dooley, Jessica Deyoung
Comparison Of Various Mean Field Formulations For Retrieving Refractive Indices Of Aerosol Particles Containing Inclusions, Kristin S. Dooley, Jessica Deyoung
Journal of the Arkansas Academy of Science
Application of effective medium approximation (EMA) methods to two-component systems are presented. Systems studied are composed of water, sulfate, soot, and dust as these are commonly encountered atmospheric aerosol components. Atmospheric models often employ EMAs to include internally mixed aerosols without the computational burden of exact theory. In the current work, several types of mixing rules (Maxwell-Garnet, Bruggeman, and coherent potential approximation) have been applied to various two-component internally mixed particles at 550 nm using volume fractions of the minor component below 0.1. As expected, results show that the formulations tested produce very similar effective refractive indices indicating that electric …
The Hitran2016 Molecular Spectroscopic Database, I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance
The Hitran2016 Molecular Spectroscopic Database, I. E. Gordon, L. S. Rothman, C. Hill, R. V. Kochanov, Y. Tan, P. F. Bernath, M. Birk, V. Boudon, A. Campargue, K. V. Chance
Chemistry & Biochemistry Faculty Publications
This paper describes the contents of the 2016 edition of the HITRAN molecular spectroscopic compilation. The new edition replaces the previous HITRAN edition of 2012 and its updates during the intervening years. The HITRAN molecular absorption compilation is composed of five major components: the traditional line-by-line spectroscopic parameters required for high-resolution radiative-transfer codes, infrared absorption cross-sections for molecules not yet amenable to representation in a line-by-line form, collision-induced absorption data, aerosol indices of refraction, and general tables such as partition sums that apply globally to the data. The new HITRAN is greatly extended in terms of accuracy, spectral coverage, additional …
Retrival Of Atmospheric Aerosol Size Distributions Using Stochastic Particle Swarm Optimization, Benjamin D. Nault-Maurer
Retrival Of Atmospheric Aerosol Size Distributions Using Stochastic Particle Swarm Optimization, Benjamin D. Nault-Maurer
All College Thesis Program, 2016-2019
A stochastic particle swarm optimization (SPSO) technique’s robustness is studied in regards to atmospheric aerosol size distribution estimations for a bimodal distribution that focuses on Aitken and accumulation mode aerosols. The SPSO method is used to calculate a set of 11 aerosol optical depth (AOD) values based on a size distribution and match them to an inputted set of AOD values. This method is tested using computer generated AOD values with fixed distribution parameters, generated AOD values with varying distribution parameters, two sets of AOD measurements in clear conditions, and one set of AOD values in hazy conditions. The SPSO …
Importance And Reliability Of Small Basis Set Ccsd(T) Corrections To Mp2 Binding And Relative Energies Of Water Clusters, Berhane Temelso, Carla Renner, George Shields
Importance And Reliability Of Small Basis Set Ccsd(T) Corrections To Mp2 Binding And Relative Energies Of Water Clusters, Berhane Temelso, Carla Renner, George Shields
Berhane Temelso
MP2 describes hydrogen-bonded systems well, yet a higher-order electron correlation correction in the form of a CCSD(T) calculation is usually necessary to achieve benchmark quality energies. We evaluated the importance and reliability of small basis set CCSD(T) corrections to MP2(δCCSD(T)) both on the binding (ΔE) and relative (ΔΔE) MP2 energies for a large number of systems including four water dimer stationary points and 57 other clusters up to undecamers, (H2O)11. By comparing the MP2 energies with CCSD(T) and the explicitly correlated MP2-F12 energies with variants of CCSD(T)-F12 using different basis sets, we were able to establish that the correction to …
Laboratory Measurements Of Contact Freezing By Dust And Bacteria At Temperatures Of Mixed-Phase Clouds, Joseph Niehaus, John Becker, Alexander Kostinski, Will Cantrell
Laboratory Measurements Of Contact Freezing By Dust And Bacteria At Temperatures Of Mixed-Phase Clouds, Joseph Niehaus, John Becker, Alexander Kostinski, Will Cantrell
Department of Physics Publications
Laboratory measurements of freezing by aerosol particles in contact mode are presented. The fraction of particles catalyzing freezing is quantified for three mineral dusts and three strains of bacteria. This is the most comprehensive such dataset to date for temperatures greater than −20°C, relevant for warm, mixed-phase clouds. For Arizona Test Dust, feldspar, or rhyolitic ash, more than 103 particles are required to initiate a freezing event at −20°C in the contact mode. At −15°C, more than 105 particles are required. An ice-negative strain of Pseudomonas fluorescens is an order of magnitude more effective than the mineral dusts …
Analysis Of Atmospheric Aerosols Collected In An Urban Area In Upstate Ny Using Proton Induced X-Ray Emission (Pixe) Spectroscopy, Jeremy Smith
Honors Theses
We have performed a PIXE analysis of atmospheric aerosol samples collected in Schenectady, NY, to study airborne pollution in an urban environment. The samples were collected using a PIXE International, 9-stage, cascade impactor that separates the airborne particles according to aerodynamic diameter and deposits them on thin Kapton foils. The impacted foils were bombarded with 2.2-MeV proton beams from the Union College 1.1-MV Pelletron accelerator and the emitted X-rays were detected with an Amptek silicon drift detector. The X-ray energy spectra were analyzed using GUPIX software to determine the elemental concentrations in the samples. A broad range of elements from …
Electron Loss And Meteoric Dust In The Mesosphere, M. Friedrich, M. Rapp, T. Blix, U. P. Hoppe, K. Torkar, S. Robertson, S. Dickson, Kristina Lynch
Electron Loss And Meteoric Dust In The Mesosphere, M. Friedrich, M. Rapp, T. Blix, U. P. Hoppe, K. Torkar, S. Robertson, S. Dickson, Kristina Lynch
Dartmouth Scholarship
No abstract provided.
Comparative Study Of Aerosols Using Particle Induced X-Ray Emission, Colin L. Gleason
Comparative Study Of Aerosols Using Particle Induced X-Ray Emission, Colin L. Gleason
Honors Theses
A comparative study of atmospheric aerosols was performed on samples collected in Schenectady, NY using Particle Induced X-ray Emission (PIXE) spectroscopy. PIXE is an elemental analysis technique used to measure the elemental concentration of a sample. This is part of a systematic study to identify the sources and understand the transport, transformation, and e˙ects of airborne pollutants and the connection between aerosols, the deposition of pollution, and the uptake of pollutants by wildlife and vegetation. The atmo-spheric aerosols were collected with a nine-stage cascade impactor that allows for the analysis of the particulate matter as a function of particle size. …
Integration Of A Worldwide Atmospheric Based Model With A Live Virtual Constructive Simulation Environment, David B. Simmons
Integration Of A Worldwide Atmospheric Based Model With A Live Virtual Constructive Simulation Environment, David B. Simmons
Theses and Dissertations
Yearly DoD spends millions of dollars on Modeling and Simulation tools in order to accomplish two fundamental tasks: make better decisions and develop better skills. Simulators that are based on realistic models enable the USAF to properly train, educate, and employ military forces. LEEDR is an atmospheric model based on worldwide historic weather data that is able to predict the extinction, absorption, and scattering of radiation across a broad range of the electromagnetic spectrum. Through this study LEEDR models the propagation of 1.0642 micron laser radiation at worldwide locations and through various environmental conditions. This modeled laser transmission output, based …
Evidence Of The Harmonic Faraday Instability In Ultrasonic Atomization Experiments With A Deep, Inviscid Fluid, Andrew P. Higginbotham '09, Aaron Guillen '11, Nathan C. Jones '10, Thomas D. Donnelly, Andrew J. Bernoff
Evidence Of The Harmonic Faraday Instability In Ultrasonic Atomization Experiments With A Deep, Inviscid Fluid, Andrew P. Higginbotham '09, Aaron Guillen '11, Nathan C. Jones '10, Thomas D. Donnelly, Andrew J. Bernoff
All HMC Faculty Publications and Research
A popular method for generating micron-sized aerosols is to submerge ultrasonic (ω~MHz) piezoelectric oscillators in a water bath. The submerged oscillator atomizes the fluid, creating droplets with radii proportional to the wavelength of the standing wave at the fluid surface. Classical theory for the Faraday instability predicts a parametric instability driving a capillary wave at the subharmonic (ω/2) frequency. For many applications it is desirable to reduce the size of the droplets; however, using higher frequency oscillators becomes impractical beyond a few MHz. Observations are presented that demonstrate that smaller droplets may also be created by …
Monitoring Automotive Particulate Matter Emissions With Lidar: A Review, Claudio Mazzoleni, Hampden D. Kuhns, Hans Moosmüller
Monitoring Automotive Particulate Matter Emissions With Lidar: A Review, Claudio Mazzoleni, Hampden D. Kuhns, Hans Moosmüller
Michigan Tech Publications
Automotive particulate matter (PM) causes deleterious effects on health and visibility. Physical and chemical properties of PM also influence climate change. Roadside remote sensing of automotive emissions is a valuable option for assessing the contribution of individual vehicles to the total PM burden. LiDAR represents a unique approach that allows measuring PM emissions from in-use vehicles with high sensitivity. This publication reviews vehicle emission remote sensing measurements using ultraviolet LiDAR and transmissometer systems. The paper discusses the measurement theory and documents examples of how these techniques provide a unique perspective for exhaust emissions of individual and groups of vehicles.
Analysis Of Expedient Field Decontamination Methods For The Xmx/2l-Mil High-Volume Aerosol Sampler, Brandon C. Laroche
Analysis Of Expedient Field Decontamination Methods For The Xmx/2l-Mil High-Volume Aerosol Sampler, Brandon C. Laroche
Theses and Dissertations
The XMX/2L-MIL is a high volume air sampler used by the Air Force Bioenvironmental Engineering community to collect biological aerosols. Without a verified decontamination technique, however, the XMX cannot be used effectively. The objective of this study was to evaluate several proposed methods for expedient field decontamination of the XMX. This study centered on the inactivation of Bacillus atrophaeus spores and vegetative Erwinia herbicola organisms from the XMX inner canister. The goals in this investigation were twofold: 1) to verify the antimicrobial efficacy of a 10% bleach solution and 2) to determine if wiping the components with a bleach-soaked paper …
Generation Of Mie Size Microdroplet Aerosols With Applications In Laser-Driven Fusion Experiments, Andrew P. Higginbotham '09, O. Semonin '06, S. Bruce '08, C. Chan '08, M. Maindi '07, Thomas D. Donnelly, M. Maurer, W. Bang, I. Churina, J. Osterholz, I. Kim, A. C. Bernstein, T. Ditmire
Generation Of Mie Size Microdroplet Aerosols With Applications In Laser-Driven Fusion Experiments, Andrew P. Higginbotham '09, O. Semonin '06, S. Bruce '08, C. Chan '08, M. Maindi '07, Thomas D. Donnelly, M. Maurer, W. Bang, I. Churina, J. Osterholz, I. Kim, A. C. Bernstein, T. Ditmire
All HMC Faculty Publications and Research
We have developed a tunable source of Mie scale microdroplet aerosols that can be used for the generation of energetic ions. To demonstrate this potential, a terawatt Ti:Al2O3 laser focused to 2×1019 W/cm2 was used to irradiate heavy water (D2O) aerosols composed of micron-scale droplets. Energetic deuterium ions, which were generated in the laser-droplet interaction, produced deuterium-deuterium fusion with approximately 2×103 fusion neutrons measured per joule of incident laser energy.
Using Ultrasonic Atomization To Produce An Aerosol Of Micron-Scale Particles, Thomas D. Donnelly, J. Hogan '03, A. Mugler '04, M. Schubmehl '02, N. Schommer '04, Andrew J. Bernoff, S. Dasnurkar, T. Ditmire
Using Ultrasonic Atomization To Produce An Aerosol Of Micron-Scale Particles, Thomas D. Donnelly, J. Hogan '03, A. Mugler '04, M. Schubmehl '02, N. Schommer '04, Andrew J. Bernoff, S. Dasnurkar, T. Ditmire
All HMC Faculty Publications and Research
A device that uses ultrasonic atomization of a liquid to produce an aerosol of micron-scale droplets is described. This device represents a new approach to producing targets relevant to laser-driven fusion studies, and to rare studies of nonlinear optics in which wavelength-scale targets are irradiated. The device has also made possible tests of fluid dynamics models in a novel phase space. The distribution of droplet sizes produced by the device and the threshold power required for droplet production are shown to follow scaling laws predicted by fluid dynamics.
Small Angle Neutron Scattering From D2o–H2o Nanodroplets And Binary Nucleation Rates In A Supersonic Nozzle, Christopher H. Heath, Kiril A. Streletzky, Barbara E. Wyslouzil, Judith Woelk, Reinhard Strey
Small Angle Neutron Scattering From D2o–H2o Nanodroplets And Binary Nucleation Rates In A Supersonic Nozzle, Christopher H. Heath, Kiril A. Streletzky, Barbara E. Wyslouzil, Judith Woelk, Reinhard Strey
Physics Faculty Publications
Small angle neutron scattering (SANS) experiments were used to characterize binary nanodroplets composed of D2O and H2O. The droplets were formed by expanding dilute mixtures of condensible vapor in a N2 carrier gas through a supersonic nozzle, while maintaining the onset of condensation at a fixed position in the nozzle. It is remarkable, given the small coherent scattering length density of light water, that even the pure H2O aerosol gave a scattering signal above background. The scattering spectra were analyzed assuming a log-normal distribution of droplets. On average, the geometric radius of the nanodroplets rg was rg=13 (±1) nm, the …
Controlling Nucleation And Growth Of Nanodroplets In Supersonic Nozzles, Kiril A. Streletzky, Yury Zvinevich, Barbara E. Wyslouzil, Reinhard Strey
Controlling Nucleation And Growth Of Nanodroplets In Supersonic Nozzles, Kiril A. Streletzky, Yury Zvinevich, Barbara E. Wyslouzil, Reinhard Strey
Physics Faculty Publications
We present the first results for a new supersonic nozzle that decouples nucleation and droplet growth, and closely controls the supersaturation and temperature during nucleation. We characterize the expansions using pressure trace measurements, and the aerosol properties using light scattering and small angle neutron scattering. We show that when nucleation and droplet growth are separated, the aerosol number density decreases, the average particle size increases, and the aerosol can be more monodisperse than that formed in a conventional nozzle. Under these conditions, we can estimate the nucleation rate J as a function of supersaturation S and temperature T directly from …
Neutron Scattering From Aerosols: Intraparticle Structure Factor, Guinier Analysis Of Particle Speed, And Crossed Beam Kinematics, Gerald Wilemski
Neutron Scattering From Aerosols: Intraparticle Structure Factor, Guinier Analysis Of Particle Speed, And Crossed Beam Kinematics, Gerald Wilemski
Physics Faculty Research & Creative Works
A theoretical formalism for neutron scattering from systems of particles is applied to liquid nanodroplet aerosols. A term arising from intraparticle, intermolecular correlations is identified. The kinematical theory of two body scattering is recast into a form convenient for interpreting the results of experiments with crossed beams of neutrons and aerosol particles. Based on a theoretical analysis of the scattered intensity in the Guinier region, a method for determining the particle velocity directly from the experimental data is outlined. The method is not restricted by assumptions about particle shape, composition, uniformity, or size distribution.
In Situ Measurement Of The Aerosol Size Distribution In Stratospheric Solid Rocket Motor Exhaust Plumes, Martin N. Ross, Philip D. Whitefield, Donald E. Hagen, Alfred R. Hopkins
In Situ Measurement Of The Aerosol Size Distribution In Stratospheric Solid Rocket Motor Exhaust Plumes, Martin N. Ross, Philip D. Whitefield, Donald E. Hagen, Alfred R. Hopkins
Chemistry Faculty Research & Creative Works
The concentration and size distribution of aerosol in the stratospheric exhaust plumes of two Space Shuttle rockets and one Titan IV rocket were measured using a two component aerosol sampling system carried aboard a WB‐57F aircraft. Aerosol size distribution in the 0.01 µm to 4 µm diameter size range was measured using a two component sampling system. The measured distributions display a trimodal form with modes near 0.005 µm, 0.09 µm, and 2.03 µm and are used to infer the relative mass fractionation among the three modes. While the smallest mode has been estimated to contain as much as 10% …
An Assessment Of The Transmission Electron Microscope For The Study Of Aerosol-Gas Interactions: Direct Observations Of Sodium Chloride Hydration Phenomena, Antony David Clarke
An Assessment Of The Transmission Electron Microscope For The Study Of Aerosol-Gas Interactions: Direct Observations Of Sodium Chloride Hydration Phenomena, Antony David Clarke
Dissertations and Theses
An experimental study of solid-gas interactions was made for sodium chloride particles, using a specially fabricated environmental chamber in a transmission electron microscope. It was found that under suitable conditions the hydration and dehydration of these particles could be directly observed and quantitatively measured. Measurements of growth were obtained with a time resolution of one-thirtieth of a second for particles having diameters ranging from 0.02 μm to 1.0 μm.