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Articles 1 - 22 of 22
Full-Text Articles in Physics
Transient Transmission Oscillations In Doped And Undoped Lithium Niobate Induced By Near-Infrared Femtosecond Pulses, Bryan J. Crossman, Gregory J. Taft
Transient Transmission Oscillations In Doped And Undoped Lithium Niobate Induced By Near-Infrared Femtosecond Pulses, Bryan J. Crossman, Gregory J. Taft
Physics Faculty Publications
Transient transmission oscillations in X-cut and Z-cut congruent, iron-doped, and magnesium-doped lithium niobate samples were measured using 50 fs, 800 nm, 0.5 nJ pulses from a self-mode-locked Ti:sapphire laser in an optical pump–probe system. Several Raman-active oscillation modes excited by these pulses were observed as changes in the transmitted probe intensity versus time delay between the pump and probe pulses. The samples were rotated to determine how the incident polarization of the pump pulses affects the mode excitations. The observed Raman-active oscillations correspond to previously reported symmetry modes measured with traditional, continuous-wave, Raman spectroscopy using the same scattering …
Modeling Free-Carrier Absorption And Avalanching By Ultrashort Laser Pulses, Jeremy R. Gulley
Modeling Free-Carrier Absorption And Avalanching By Ultrashort Laser Pulses, Jeremy R. Gulley
Faculty and Research Publications
In the past decade it was demonstrated experimentally that negatively-chirped laser pulses can lower the surface LIDT for wide band-gap materials by decreasing the number of photons required for photoionization on the leading edge of the pulse. Similarly, simulations have shown that positively-chirped pulses resulting from selffocusing and self-phase modulation in bulk dielectrics can alter the onset of laser-induced material modifications by increasing the number of photons required for photoionization on the leading edge of the pulse. However, the role of multi-chromatic effects in free-carrier absorption and avalanching has yet to be addressed. In this work a frequency-selective model of …
Energy Scaling Of Nanosecond Gain-Switched Cr2+:Znse Lasers, Vladimir V. Fedorov, Igor S. Moskalev, M. S. Mirov, S. B. Mirov, Torrey J. Wagner, Matthew J. Bohn, Patrick A. Berry, K. L. Schepler
Energy Scaling Of Nanosecond Gain-Switched Cr2+:Znse Lasers, Vladimir V. Fedorov, Igor S. Moskalev, M. S. Mirov, S. B. Mirov, Torrey J. Wagner, Matthew J. Bohn, Patrick A. Berry, K. L. Schepler
Faculty Publications
In this paper, we report record nanosecond output energies of gain-switched CrZnSe lasers pumped by Q-switched CrTmHoYAG 100 ns at 2.096 microns and Raman shifted NdYAG lasers 7 ns at 1.906 microns. In these experiments we used Brewster cut CrZnSe gain elements with a chromium concentration of 8x1018cm-3. Under CrTmHoYAG pumping, the first CrZnSe laser demonstrated 3.1 mJ of output energy, 52 slope efficiency and 110 nm linewidth centered at a wavelength of 2.47 microns. Maximum output energy of the second CrZnSe laser reached 10.1 mJ under H2 Raman shifted NdYAG laser pumping. The slope …
Structure And Mechanism Of Copper- And Nickel-Substituted Analogues Of Metallo-Β-Lactamase L1, Zhenxin Hu, Lauren J. Spadafora, Christine E. Hajdin, Brian Bennett, Michael W. Crowder
Structure And Mechanism Of Copper- And Nickel-Substituted Analogues Of Metallo-Β-Lactamase L1, Zhenxin Hu, Lauren J. Spadafora, Christine E. Hajdin, Brian Bennett, Michael W. Crowder
Physics Faculty Research and Publications
In an effort to further probe metal binding to metallo-β-lactamase L1 (mβl L1), Cu- (Cu-L1) and Ni-substituted (Ni-L1) L1 were prepared and characterized by kinetic and spectroscopic studies. Cu-L1 bound 1.7 equiv of Cu and small amounts of Zn(II) and Fe. The EPR spectrum of Cu-L1 exhibited two overlapping, axial signals, indicative of type 2 sites with distinct affinities for Cu(II). Both signals indicated multiple nitrogen ligands. Despite the expected proximity of the Cu(II) ions, however, only indirect evidence was found for spin−spin coupling. Cu-L1 exhibited higher kcat (96 s−1) and Km (224 μM) values, as …
Effective Medium Theory, Rough Surfaces, And Moth’S Eyes, David D. Allred, Zephne Larsen, Joseph Muhlestein, R. Steven Turley, Anthony Willey
Effective Medium Theory, Rough Surfaces, And Moth’S Eyes, David D. Allred, Zephne Larsen, Joseph Muhlestein, R. Steven Turley, Anthony Willey
Faculty Publications
Optics in the extreme ultraviolet (XUV) have important applications in microelectronics, microscopy, space physics, and in imaging plasmas. Because of the short wavelengths involved in these applications, it is critical to account for interfacial roughness to accurately predict the reflection and absorption of XUV optics. This paper examines two possible effects of roughness on optical absorption, non-specular reflection and enhanced transmission and compares these to measured experimental data on a rough Y2O3 thin film.
Black Hole Particle Emission In Higher-Dimensional Spacetimes, Vitor Cardoso, Marco Cavaglia, Leonardo Gualtieri
Black Hole Particle Emission In Higher-Dimensional Spacetimes, Vitor Cardoso, Marco Cavaglia, Leonardo Gualtieri
Physics Faculty Research & Creative Works
In models with extra dimensions, a black hole evaporates both in the bulk and on the visible brane, where standard model fields live. The exact emissivities of each particle species are needed to determine how the black hole decay proceeds. We compute and discuss the absorption cross sections, the relative emissivities, and the total power output of all known fields in the evaporation phase. Graviton emissivity is highly enhanced as the spacetime dimensionality increases. Therefore, a black hole loses a significant fraction of its mass in the bulk. This result has important consequences for the phenomenology of black holes in …
Variational Approach To The Volume Viscosity Of Fluids, Allan J. Zuckerwar, Robert L. Ash
Variational Approach To The Volume Viscosity Of Fluids, Allan J. Zuckerwar, Robert L. Ash
Mechanical & Aerospace Engineering Faculty Publications
The variational principle of Hamilton is applied to develop an analytical formulation to describe the volume viscosity in fluids. The procedure described here differs from those used in the past in that a dissipative process is represented by the chemical affinity and progress variable (sometimes called "order parameter") of a reacting species. These state variables appear in the variational integral in two places: first, in the expression for the internal energy, and second, in a subsidiary condition accounting for the conservation of the reacting species. As a result of the variational procedure, two dissipative terms appear in the Navier-Stokes equation. …
Progress Towards Terahertz Acoustic Phonon Generation In Doping Superlattices, Thomas E. Wilson
Progress Towards Terahertz Acoustic Phonon Generation In Doping Superlattices, Thomas E. Wilson
Physics Faculty Research
Progress is described in experiments to generate coherent terahertz acoustic phonons in silicon doping superlattices by the resonant absorption of nanosecond-pulsed far-infrared laser radiation. Future experiments are proposed that would use the superlattice as a transducer in a terahertz cryogenic acoustic reflection microscope with sub-nanometer resolution.
Progress Towards Terahertz Acoustic Phonon Generation In Doping Superlattices, Thomas E. Wilson
Progress Towards Terahertz Acoustic Phonon Generation In Doping Superlattices, Thomas E. Wilson
Physics Faculty Research
Progress is described in experiments to generate coherent terahertz acoustic phonons in silicon doping superlattices by the resonant absorption of nanosecond-pulsed far-infrared laser radiation. Future experiments are proposed that would use the superlattice as a transducer in a terahertz cryogenic acoustic reflection microscope with sub-nanometer resolution.
Thorium-Based Thin Films As Highly Reflective Mirrors In The Euv, David D. Allred, William R. Evans, Jed E. Johnson, Richard L. Sandberg, R. Steven Turley
Thorium-Based Thin Films As Highly Reflective Mirrors In The Euv, David D. Allred, William R. Evans, Jed E. Johnson, Richard L. Sandberg, R. Steven Turley
Faculty Publications
As applications for extreme ultraviolet (EUV) radiation have been identified, the demand for better optics has also increased. Thorium and thorium oxide thin films (19 to 61 nm thick) were RF-sputtered and characterized using atomic force microscopy (AFM), spectroscopic ellipsometry, low-angle x-ray diffraction (LAXRD), x-ray photoelectron spectroscopy (XPS), and x-ray absorption near edge structure (XANES) in order to assess their capability as EUV reflectors. Their reflectance and absorption at different energies were also measured and analyzed at the Advanced Light Source in Berkeley. The reflectance of oxidized thorium is reported between 2 and 32 nm at 5, 10, and 15 …
Complete Measurement Of Three-Body Photodisintegration Of 3He For Photon Energies Between 0.35 And 1.55 Gev, H. Bagdasaryan, M. Bektasoglu, K. V. Dharmawardane, G. E. Dodge, T. A. Forest, G. Gavalian, N. Guler, C. E. Hyde-Wright, A. Klein, S. E. Kuhn, L. M. Qin, S. Stepanyan, L. B. Weinstein, J. Yun, Et Al., The Clas Collaboration
Complete Measurement Of Three-Body Photodisintegration Of 3He For Photon Energies Between 0.35 And 1.55 Gev, H. Bagdasaryan, M. Bektasoglu, K. V. Dharmawardane, G. E. Dodge, T. A. Forest, G. Gavalian, N. Guler, C. E. Hyde-Wright, A. Klein, S. E. Kuhn, L. M. Qin, S. Stepanyan, L. B. Weinstein, J. Yun, Et Al., The Clas Collaboration
Physics Faculty Publications
The three-body photodisintegration of 3He has been measured with the CLAS detector at Jefferson Lab, using tagged photons of energies between 0.35 GeV and 1.55 GeV. The large acceptance of the spectrometer allowed us for the first time to cover a wide momentum and angular range for the two outgoing protons. Three kinematic regions dominated by either two- or three-body contributions have been distinguished and analyzed. The measured cross sections have been compared with results of a theoretical model, which, in certain kinematic ranges, have been found to be in reasonable agreement with the data.
Substrate Specificity, Metal Binding Properties, And Spectroscopic Characterization Of The Dape-Encoded N-Succinyl-L,L-Diaminopimelic Acid Desuccinylase From Haemophilus Influenzae, David L. Bienvenue, Danuta M. Gilner, Ryan S. Davis, Brian Bennett, Richard C. Holz
Substrate Specificity, Metal Binding Properties, And Spectroscopic Characterization Of The Dape-Encoded N-Succinyl-L,L-Diaminopimelic Acid Desuccinylase From Haemophilus Influenzae, David L. Bienvenue, Danuta M. Gilner, Ryan S. Davis, Brian Bennett, Richard C. Holz
Physics Faculty Research and Publications
The catalytic and structural properties of divalent metal ion cofactor binding sites in the dapE-encoded N-succinyl-l,l-diaminopimelic acid desuccinylase (DapE) from Haemophilus influenzae were investigated. Co(II)-substituted DapE enzyme was 25% more active than the Zn(II)-loaded form of the enzyme. Interestingly, Mn(II) can activate DapE, but only to ∼20% of the Zn(II)-loaded enzyme. The order of the observed kcat values are Co(II) > Zn(II) > Cd(II) > Mn(II) >Ni(II) ∼ Cu(II) ∼ Mg(II). DapE was shown to only hydrolyze l,l-N-succinyl-diaminopimelic acid (l,l-SDAP) and was inactive toward d,l-, l,d-, and d,d-SDAP. DapE was also inactive toward several acetylated amino acids as …
Density Of Resonant States And A Manifestation Of Photonic Band Structure In Small Clusters Of Spherical Particles, Alexey Yamilov, Hui Cao
Density Of Resonant States And A Manifestation Of Photonic Band Structure In Small Clusters Of Spherical Particles, Alexey Yamilov, Hui Cao
Physics Faculty Research & Creative Works
We introduce a numerical recipe for calculating the density of the resonant states of the clusters of dielectric spheres. Using truncated multipole expansions (generalized multisphere Mie solution) we obtain the scattering matrix of the problem. By introducing an infinitesimal absorption in the spheres we express the dwell time of the electromagnetic wave in terms of the elements of the scattering matrix. Using the parameters in recent light localization experiments [Phys. Rev. Lett. 87, 153901 (2001)], we demonstrate that the density of the resonant states, related to the dwell time, shows the formation of the photonic band structure in small clusters …
In-Situ X-Ray-Absorption Spectroscopy Study Of Hydrogen Absorption By Nickel-Magnesium Thin Films, B. Farangis, Ponnusamy Nachimuthu, T. J. Richardson, J. L. Slack, Rupert C. Perera, Eric M. Gullikson, Dennis W. Lindle, M. Rubin
In-Situ X-Ray-Absorption Spectroscopy Study Of Hydrogen Absorption By Nickel-Magnesium Thin Films, B. Farangis, Ponnusamy Nachimuthu, T. J. Richardson, J. L. Slack, Rupert C. Perera, Eric M. Gullikson, Dennis W. Lindle, M. Rubin
Chemistry and Biochemistry Faculty Research
Structural and electronic properties of co-sputtered Ni-Mg thin films with varying Ni to Mg ratio were studied by in-situ x-ray absorption spectroscopy in the Ni L-edge and Mg K-edge regions. Co-deposition of the metals led to increased disorder and decreased coordination around Ni and Mg compared to pure metal films. Exposure of the metallic films to hydrogen resulted in formation of hydrides and increased disorder. The presence of hydrogen as a near neighbor around Mg caused a drastic reduction in the intensities of multiple scattering resonances at higher energies. The optical switching behavior and changes in the x-ray spectra varied …
Scaling In One-Dimensional Localized Absorbing Systems, Lev I. Deych, Alexey Yamilov, Alexander A. Lisyansky
Scaling In One-Dimensional Localized Absorbing Systems, Lev I. Deych, Alexey Yamilov, Alexander A. Lisyansky
Physics Faculty Research & Creative Works
Numerical study of the scaling of transmission fluctuations in the one-dimensional localization problem in the presence of absorption is carried out. Violations of single-parameter scaling for lossy systems are found and explained on the basis of a new criterion for different types of scaling behavior derived by Deych et al.
Femtosecond Laser-Produced Plasma X-Rays From Periodically Modulated Surface Targets, J. C. Gautheir, S. Bastiani, P. Audebert, J. P. Geindre, K. Neuman, Thomas D. Donnelly, M. Hoffer, R. W. Falcone, R. Shepherd, D. Price, B. White
Femtosecond Laser-Produced Plasma X-Rays From Periodically Modulated Surface Targets, J. C. Gautheir, S. Bastiani, P. Audebert, J. P. Geindre, K. Neuman, Thomas D. Donnelly, M. Hoffer, R. W. Falcone, R. Shepherd, D. Price, B. White
All HMC Faculty Publications and Research
We have studied theoretically and experimentally the x-ray production above 1 keV from femtosecond laser plasmas generated on periodically modulated surface targets. Laser energy coupling to plasma surface waves has been modeled using a numerical differential method. Almost total absorption of incident laser radiation is predicted for optimized interaction conditions. Silicon gratings have been irradiated by a 120fs Ti:sapphire laser at irradiances in excess of 1016 W/cm2. X-ray intensities above 1.5 keV (K-shell lines) have been measured as a function of the incidence angle. Results show a distinct x-ray emission maximum for the first order diffraction …
Xenon 147-Nm Resonance Ƒ Value And Trapped Decay Rates, H. M. Anderson, Scott D. Bergeson, D. A. Doughty, J. E. Lawler
Xenon 147-Nm Resonance Ƒ Value And Trapped Decay Rates, H. M. Anderson, Scott D. Bergeson, D. A. Doughty, J. E. Lawler
Faculty Publications
The absorption oscillator strength of the xenon 147-nm resonance transition is measured to be 0.264±0.016. This value is from direct absorption measurements with equivalent widths from ≈ 1 to ≈ 10 cm-1. This ƒ-value measurement is compared to others in the literature and is used in Monte Carlo simulations of trapped decay rates. The simulations include an angle-dependent partial frequency redistribution. The simulation results are compared to trapped decay rates in the literature.
Multinucleon Effects In Muon Capture On ³He At High Energy Transfer, S. E. Kuhn, W. J. Cummings, G. E. Dodge, S. S. Hanna, B. H. King, Y. M. Shin, J. G. Congleton, R. Helmer, R. B. Schubank, N. R. Stevenson, U. Wienands, Y. K. Lee, G. R. Mason, B. E. King, K. S. Chung, J. M. Lee, D. P. Rosenzweig
Multinucleon Effects In Muon Capture On ³He At High Energy Transfer, S. E. Kuhn, W. J. Cummings, G. E. Dodge, S. S. Hanna, B. H. King, Y. M. Shin, J. G. Congleton, R. Helmer, R. B. Schubank, N. R. Stevenson, U. Wienands, Y. K. Lee, G. R. Mason, B. E. King, K. S. Chung, J. M. Lee, D. P. Rosenzweig
Physics Faculty Publications
Energy spectra of both protons and deuterons emitted following the capture of negative muons by 3He nuclei have been measured for energies above 15 MeV. A limited number of proton-neutron pairs emitted in coincidence were also observed. A simple plane wave impulse approximation (PWIA) model calculation yields fair agreement with the measured proton energy spectra, but underpredicts the measured rate of deuteron production above our energy threshold by a large factor. A more sophisticated PWIA calculation for the two-body breakup channel, based on a realistic three-body wave function for the initial state, is closer to the deuteron data at …
Photoluminescence And Absorption Studies Of Defects In Cdte And Znxcd1-Xte Crystals, Cheryl Barnett Davis, David D. Allred, A. Reyes-Mena, Jesus González-Hernández, Ovidio González, Bret C. Hess, Worth P. Allred
Photoluminescence And Absorption Studies Of Defects In Cdte And Znxcd1-Xte Crystals, Cheryl Barnett Davis, David D. Allred, A. Reyes-Mena, Jesus González-Hernández, Ovidio González, Bret C. Hess, Worth P. Allred
Faculty Publications
We have studied at cryogenic temperatures photoluminescence features which lie more than 0.15 eV below the band edge in ZnxCd1-xTe (0≤x≤0.09) crystals. The same features, namely a defect band which lies at about 0.13-0.20 eV below the band-gap energy and a peak at 1.1 eV, that are observed in pure CdTe samples are observed in these alloy materials. In annealed samples we observe that the 1.1 eV feature, which has been attributed to tellurium vacancies, increases with fast cooling. Increased concentrations of tellurium vacancies can be understood in terms of the phase diagram of CdTe which indicates that higher concentrations …
Alkali Metal Adsorbates On W(110): Ionic, Covalent, Or Metallic?, D. Mark Riffe, G. K. Wertheim, P. H. Citrin
Alkali Metal Adsorbates On W(110): Ionic, Covalent, Or Metallic?, D. Mark Riffe, G. K. Wertheim, P. H. Citrin
All Physics Faculty Publications
The photoemission signal from the first atomic layer of W(110) is used to assess the nature of the interaction between the surface atoms of the metal substrate and the adsorbates Na, K, and Cs for coverages up to 1 atomic layer. Our results indicate that there is little or no charge transfer from the alkali metal to the W surface, even in the limit of low coverage. The satellite structure of the photoemission lines of the outermost p shell of the alkali metals confirms this conclusion. While contrary to the conventional picture of alkali-metal-charge donation, these findings fully support recent …
Design Of High Performance Soft X-Ray Windows, Raymond T. Perkins, David D. Allred, Larry V. Knight, James M. Thorne
Design Of High Performance Soft X-Ray Windows, Raymond T. Perkins, David D. Allred, Larry V. Knight, James M. Thorne
Faculty Publications
X-ray windows are used in sources and detectors to separate the neighborhood of the x-ray generation or detection from the use environment. While each use has its own requirements, there are some principles that should be used in designing an optimal x-ray window. Because x-rays are absorbed to some extent by all materials, minimizing absorption is one criterion in preparing windows. Also, for most uses there is a pressure difference across the window so that ensuring pinhole-free structure and sufficient mechanical strength to support the differential is another criterion for window design. Traditionally, absorption is minimized by fabricating the window …
Chemical Vapor Deposited Amorphous Silicon For Use In Photothermal Conversion, David D. Allred, D. C. Booth, M. Janai, G. Weiser, B. O. Seraphin
Chemical Vapor Deposited Amorphous Silicon For Use In Photothermal Conversion, David D. Allred, D. C. Booth, M. Janai, G. Weiser, B. O. Seraphin
Faculty Publications
Efficient photothermal conversion requires surfaces of high solar absorptance and low thermal emittance. This can be accomplished by the tandem action of a good infrared reflector overlaid by a film of sufficient solar absorptance that is transparent in the infrared. Crystalline silicon is a suitable candidate for the absorber layer. Its indirect band gap, however, results in a shallow absorption edge that extends to far into the visible. In contrast, the absorption edge of amorphous silicon is steeper and located farther into the infrared, resulting in a larger solar absorptance. We report on the fabrication of amorphous silicon absorbers by …