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Full-Text Articles in Physics

Anomalous Nonlinear X-Ray Compton Scattering, Matthias Fuchs, Mariano Trigo, Jian Chen, Shambhu Ghimire, Sharon Shwartz, Michael Kozina, Mason Jiang, Thomas Henighan, Crystal Bray, Georges Ndabashimiye, Philip H. Bucksbaum, Yiping Feng, Sven Herrmann, Gabriella A. Carini, Jack Pines, Philip Hart, Christopher Kenney, Serge Guillet, Sébastien Boutet, Garth J. Williams, Marc Messerschmidt, M. Marvin Seibert, Stefan Moeller, Jerome B. Hastings, David A. Reis Jan 2015

Anomalous Nonlinear X-Ray Compton Scattering, Matthias Fuchs, Mariano Trigo, Jian Chen, Shambhu Ghimire, Sharon Shwartz, Michael Kozina, Mason Jiang, Thomas Henighan, Crystal Bray, Georges Ndabashimiye, Philip H. Bucksbaum, Yiping Feng, Sven Herrmann, Gabriella A. Carini, Jack Pines, Philip Hart, Christopher Kenney, Serge Guillet, Sébastien Boutet, Garth J. Williams, Marc Messerschmidt, M. Marvin Seibert, Stefan Moeller, Jerome B. Hastings, David A. Reis

Matthias Fuchs Publications

X-ray scattering is typically used as a weak linear atomic-scale probe of matter. At high intensities, such as produced at free-electron lasers, nonlinearities can become important, and the probe may no longer be considered weak. Here we report the observation of one of the most fundamental nonlinear X-ray–matter interactions: the concerted nonlinear Compton scattering of two identical hard X-ray photons producing a single higher-energy photon. The X-ray intensity reached 4 × 1020 W cm−2, corresponding to an electric field well above the atomic unit of strength and within almost four orders of magnitude of the quantum-electrodynamic critical …


Below Gap Optical Absorption In Gaas Driven By Intense, Single-Cycle Coherent Transition Radiation, J. Goodfellow, Matthias Fuchs, D. Daranciang, S. Ghimire, F. Chen, H. Loos, D. A. Reis, A. S. Fisher, A. M. Lindenberg Jul 2014

Below Gap Optical Absorption In Gaas Driven By Intense, Single-Cycle Coherent Transition Radiation, J. Goodfellow, Matthias Fuchs, D. Daranciang, S. Ghimire, F. Chen, H. Loos, D. A. Reis, A. S. Fisher, A. M. Lindenberg

Matthias Fuchs Publications

Single-cycle terahertz fields generated by coherent transition radiation from a relativistic electron beam are used to study the high field optical response of single crystal GaAs. Large amplitude changes in the sub-band-gap optical absorption are induced and probed dynamically by measuring the absorption of a broad-band optical beam generated by transition radiation from the same electron bunch, providing an absolutely synchronized pump and probe geometry. This modification of the optical properties is consistent with strong-field-induced electroabsorption. These processes are pertinent to a wide range of nonlinear terahertz-driven lightmatter interactions anticipated at accelerator-based sources.


X-Ray Second Harmonic Generation, S. Shwartz, Matthias Fuchs, J. B. Hastings, Y. Inubushi, T. Ishikawa, T. Katayama, D. A. Reis, T. Sato, K. Tono, M. Yabashi, S. Yudovich, S. E. Harris Apr 2014

X-Ray Second Harmonic Generation, S. Shwartz, Matthias Fuchs, J. B. Hastings, Y. Inubushi, T. Ishikawa, T. Katayama, D. A. Reis, T. Sato, K. Tono, M. Yabashi, S. Yudovich, S. E. Harris

Matthias Fuchs Publications

We report clear experimental evidence for second harmonic generation at hard x-ray wavelengths. Using a 1.7 Å pumping beam generated by a free electron laser, we observe second harmonic generation in diamond. The generated second harmonic is of order 10 times the background radiation, scales quadratically with pump pulse energy, and is generated over a narrow phase-matching condition. Of importance for future experiments, our results indicate that it is possible to observe nonlinear x-ray processes in crystals at pump intensities exceeding 1016 W/cm2.