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Full-Text Articles in Physics

Aspects Of Postcollision Interactions (Pci) Near The Ar L-Shell, James A.R. Samson, Y. Lu, Wayne C. Stolte Oct 1997

Aspects Of Postcollision Interactions (Pci) Near The Ar L-Shell, James A.R. Samson, Y. Lu, Wayne C. Stolte

Chemistry and Biochemistry Faculty Research

In the present work we are interested in near-threshold photoionization experiments involving postcollision effects related to the Auger decay of a vacancy in the Ar L shell. In particular, we have measured the photoelectron energy spectrum resulting from the above postcollision interaction effects and have observed electrons produced by the process of electron capture and reemission.


Neutron Resonance Spectroscopy Of 107ag, And 109ag, L Y. Lowie, J D. Bowman, Bret E. Crawford, P P J. Delheij, T Haseyama, J N. Knudsen, A Masaike, Y Matsuda, G E. Mitchell, S I. Penttila, H Postma, N R. Roberson, S J. Seestrom, E I. Sharapov, Sharon L. Stephenson, Y-F Yen, V W. Yuan Jul 1997

Neutron Resonance Spectroscopy Of 107ag, And 109ag, L Y. Lowie, J D. Bowman, Bret E. Crawford, P P J. Delheij, T Haseyama, J N. Knudsen, A Masaike, Y Matsuda, G E. Mitchell, S I. Penttila, H Postma, N R. Roberson, S J. Seestrom, E I. Sharapov, Sharon L. Stephenson, Y-F Yen, V W. Yuan

Physics and Astronomy Faculty Publications

Parity violation has been observed in a number of previously unreported neutron resonances in silver. Analysis of these parity violation data requires improved neutron resonance spectroscopy. The neutron total cross section for natural silver was measured for En=10–800 eV with the time-of-flight method at the Los Alamos Neutron Scattering Center. The neutron capture reaction was studied with both a natural silver target and a highly enriched sample (98.29%) of 107Ag. A total of 38 previously unreported resonances were observed. The combination of the two measurements allowed assignment of the newly observed resonances to 107Ag or to …


Nondipole Resonant X-Ray-Raman Spectroscopy: Polarized Inelastic Scattering At The K Edge Of Cl2, J. D. Mills, J. A. Sheehy, T. A. Ferrett, S. H. Southworth, R. Mayer, Dennis W. Lindle, P. W. Langhoff Jul 1997

Nondipole Resonant X-Ray-Raman Spectroscopy: Polarized Inelastic Scattering At The K Edge Of Cl2, J. D. Mills, J. A. Sheehy, T. A. Ferrett, S. H. Southworth, R. Mayer, Dennis W. Lindle, P. W. Langhoff

Chemistry and Biochemistry Faculty Research

Experimental and theoretical studies are reported on the inelastic (Raman) scattering of wavelength-selected polarized x rays from the K edge of gas-phase chlorine molecules. The polarized emission spectra exhibit prominent nondipole features consequent of phase variations of the incident and emitted radiation over molecular dimensions, as predicted by the Kramers-Heisenberg scattering formalism. Issues pursuant to the detection of core-hole localization by resonant Raman scattering from homonuclear diatomic molecules are critically examined. [S0031-9007(97)03486-8]


Core Scattering Of Stark Wave Packets, M. L. Naudeau, C. I. Sukenik, P. H. Bucksbaum Jul 1997

Core Scattering Of Stark Wave Packets, M. L. Naudeau, C. I. Sukenik, P. H. Bucksbaum

Physics Faculty Publications

We investigate the wave packet dynamics of electrons bound in the nonseparable potential of cesium in a static electric field using time-domain Ramsey interferometry. Specially shaped wave packets with low radial dispersion enable us to view the interaction between the wave packet and the atomic core. Experiments in cesium, together with quantum defect calculations of cesium and hydrogen, demonstrate changes in the motion and shape of these wave packets due to core scattering.


On The Stark Broadening Parameters Of The Two Nii Spectral Lines Of The 3d-4f Transition, Vladimir Milosavljevic, Stevan Djenize Jun 1997

On The Stark Broadening Parameters Of The Two Nii Spectral Lines Of The 3d-4f Transition, Vladimir Milosavljevic, Stevan Djenize

Articles

Stark parameters (width and shift) of two singly ionized nitrogen spectral lines, that belong to 3d-4f transition have been measured in a linear pulsed, low pressure, arc discharge in the nitrogen-oxygen plasma at a 54000 K electron temperature and at a 2.8×10 23 m−3 electron density. The measured values have been compared to the existing experimental and calculated data


Breakdown Of The Independent Particle Approximation In High-Energy Photoionization, E. W. B. Dias, H. S. Chakraborty, P. C. Deshmukh, S. T. Manson, Oliver Hemmers, P. Glans, D. Hansen, H. Wang, S. B. Whitfield, Dennis W. Lindle, R. Wehlitz, Jon C. Levin, I. A. Sellin Jun 1997

Breakdown Of The Independent Particle Approximation In High-Energy Photoionization, E. W. B. Dias, H. S. Chakraborty, P. C. Deshmukh, S. T. Manson, Oliver Hemmers, P. Glans, D. Hansen, H. Wang, S. B. Whitfield, Dennis W. Lindle, R. Wehlitz, Jon C. Levin, I. A. Sellin

Environmental Studies Faculty Publications

The independent particle approximation is shown to break down for the photoionization of both inner and outer nℓ (ℓ>0) electrons of all atoms, at high enough energy, owing to interchannel interactions with the nearby ns photoionization channels. The effect is illustrated for Ne 2p in the 1 keV photon energy range through a comparison of theory and experiment. The implications for x-ray photoelectron spectroscopy of molecules and condensed matter are discussed.


Roughening And Preroughening Of Diamond-Cubic {111} Surfaces, Donald L. Woodraska, John A. Jaszczak Jan 1997

Roughening And Preroughening Of Diamond-Cubic {111} Surfaces, Donald L. Woodraska, John A. Jaszczak

Department of Physics Publications

A solid-on-solid model for {111} surfaces of diamond-cubic materials that correctly takes into account the diamond-cubic crystal structure has been developed for Monte Carlo simulation. In addition to a roughening transition at temperature TR, a distinct preroughening transition at TPR≈0.43TR is indicated by divergences in the surface specific heat and order-parameter susceptibility. Preroughening appears to arise naturally in our nearest-neighbor bond model from the entropic freedom available in the nontrivial crystal structure. Preroughening is shown to dramatically lower the nucleation barrier for growth and etching at low driving forces.


Quantum Coherence In Small Antiferromagnets, S. E. Barnes, R. Ballou, B. Barbara, J. Strelen Jan 1997

Quantum Coherence In Small Antiferromagnets, S. E. Barnes, R. Ballou, B. Barbara, J. Strelen

Physics Articles and Papers

An antiferromagnetic particle with an excess spin j⃗ has 2 degrees of freedom. The one associated with j⃗ is ferromagnetic, while the antiferromagnetic behavior involves Néel vector n⃗. It is shown that the spin-parity effect described by Loss et al. has to do with the ferromagnetic degree of freedom and does not imply the localization of n⃗ for small enough particles for half-integer spin. It is also shown that the tunnel splitting associated with n⃗ is insensitive to applied fields.