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Full-Text Articles in Physics

Fabrication Of Metal-Silicon Nanostructures By Reactive Laser Ablation In Liquid, Eric J. Broadhead Jan 2021

Fabrication Of Metal-Silicon Nanostructures By Reactive Laser Ablation In Liquid, Eric J. Broadhead

Theses and Dissertations

Metal-silicon nanostructures are a growing area of research due to their applications in multiple fields such as biosensing and catalysis. In addition, silicon can provide strong support effects to metal nanoparticles while being more cost effective than traditionally used supports, like titania. Traditional wet-chemical methods are capable of synthesizing metal-silicon nanostructures with a variety of composition and nanoparticle shapes, but they often require high temperatures, toxic solvents, strong reducing agents, or need capping agents added to stabilize the nanoparticles. Laser processing is an emerging technique capable of synthesizing metal-silicon composite surfaces that offers a faster, simpler, and greener synthesis route …


Two-Photon Excitation Of Cesium Alkali Metal Vapor 72D, 82D Kinetics And Spectroscopy, Ricardo C. Davila Mar 2018

Two-Photon Excitation Of Cesium Alkali Metal Vapor 72D, 82D Kinetics And Spectroscopy, Ricardo C. Davila

Theses and Dissertations

Pulsed excitation on the two-photon Cs 62S½ → 72D3/2,5/2 transition results in time-resolved fluorescence at 697 nm and 672 nm. The rates for fine structure mixing between the 72D3/2,5/2 states have been measured for helium and argon rare gas collision partners. The mixing rates are very fast, 1.26 ± 0.05 x 10-9 cm3/(atom sec) for He and 1.52 ± 0.05 x 10-10 cm3 /(atom sec) for Ar, driven by the small energy splitting and large radial distribution for the valence electron. …


Kinetics Of Higher Lying Rb States After, Pulsed Excitation Of The D2 Transition In The Presence Of Helium, Austin J. Wallerstein Mar 2016

Kinetics Of Higher Lying Rb States After, Pulsed Excitation Of The D2 Transition In The Presence Of Helium, Austin J. Wallerstein

Theses and Dissertations

The Diode Pumped Alkali Laser (DPAL) is a high power, three-level laser system that employs diode bars to optically excite an alkali metal vapor. It lases along the D1 transition, between the two lowest energy levels, 2P1/2 and 2S1/2. Higher lying energy states are produced at higher population density via energy pooling and multiphoton processes. Pulsed laser excitation of rubidium at approximately 1 MW=cm2 has been studied at helium pressure up to 900 Torr. Emissions from energy states as high as 82D suggests modest ionization, though these intensities decrease drastically at buffer gas …


Iron-Doped Zinc Selenide: Spectroscopy And Laser Development, Jonathan W. Evans Mar 2014

Iron-Doped Zinc Selenide: Spectroscopy And Laser Development, Jonathan W. Evans

Theses and Dissertations

We examine the quantum mechanics of optically active ions in crystals. Insight is developed which qualitatively explains the shape of the optical absorption and emission spectra of Fe2+ ions in II-VI materials. In addition to a discussion of the relevant theory, this work explores experimental techniques for absorption spectroscopy, laser-induced fluorescence spectroscopy, and upper-state lifetime measurements in detail. The data collected from these experiments are interpreted in the context of the theories developed herein. The theory and data are used to develop a simple model of the temperature dependence of the upper-state lifetime of Fe2+ ions in ZnSe. …


Tunable Optical Delay In Doppler-Broadened Cesium Vapor, Monte D. Anderson Dec 2010

Tunable Optical Delay In Doppler-Broadened Cesium Vapor, Monte D. Anderson

Theses and Dissertations

Variable-delay tunable optical delay line or optical buffers are critical for the development of all-optical networks components as well as interferometry and analytic instruments. Recent research on slow light may hold the key for the development of the first practical tunable optical delay device. In this research the linear dispersion delay effects in an alkali vapor. The hyperfine relaxation observations present insight into the complex bleach wave dynamics during a high-intensity pulsed pump in DPAL systems.


Rubidium Recycling In A High Intensity Short Duration Pulsed Alkali Laser, Wooddy S. Miller Mar 2010

Rubidium Recycling In A High Intensity Short Duration Pulsed Alkali Laser, Wooddy S. Miller

Theses and Dissertations

Laser induced fluorescence was used to study how pump pulse duration and alkali recycle time effects maximum power output in a Diode Pumped Alkali Laser (DPAL) system. A high intensity short pulsed pump source was used to excited rubidium atoms inside a DPAL-type laser. The maximum output power of the laser showed a strong dependence upon the temporal width of the pump pulse in addition to the input pump intensity. A linear relationship was observed between the maximum output power and the pulse width due to the effective lifetime of the excited state, defined as the time it takes for …


Q-Switched And Mode Locked Short Pulses From A Diode Pumped, Yb-Doped Fiber Laser, Seth M. Swift Mar 2009

Q-Switched And Mode Locked Short Pulses From A Diode Pumped, Yb-Doped Fiber Laser, Seth M. Swift

Theses and Dissertations

A diode-pumped, ytterbium (Yb)-doped fiber laser system was designed and demonstrated to operate in continuous wave (cw), passively Q-switched and possibly passively mode locked operation. To our knowledge, this was the first fiber laser oscillator built at the Air Force Institute of Technology. A Cr4+:YAG (Chromium: Ytterbium Aluminum Garnett) crystal was used as a saturable absorber to generate Q-switched pulses. Attempts to mode lock the laser were performed using a semiconductor saturable absorber mirror (SESAM) and through nonlinear polarization rotation (NPR). The best output power result was 5 Watts (W) while pumping at 8.3 W, yielding 60% efficiency …


Demonstration Of A Strategy To Perform Two-Dimensional Diode Laser Tomography, Ryan N. Givens Mar 2008

Demonstration Of A Strategy To Perform Two-Dimensional Diode Laser Tomography, Ryan N. Givens

Theses and Dissertations

Demonstration of a strategy to perform two-dimensional diode laser tomography using a priori knowledge from symmetry arguments and computational fluid dynamic (CFD) calculations is presented for a flat flame burner. The strategy uses an optimization technique to determine flame diameter and location using a vector quantization approach. Next, the variance in a training set, produced from CFD calculations, is captured using principal components analysis. The information in the training set allows interpolation between beam paths resulting in temperature and density maps. Finally, the TDLAS temperature and density maps are shown to agree with traditional thermocouple measurements of the flat flame …


Time Resolution Of Collapse Events During The Progation Of Ultraviolet Filaaments, Teresa J. Fondren Oct 2007

Time Resolution Of Collapse Events During The Progation Of Ultraviolet Filaaments, Teresa J. Fondren

Theses and Dissertations

Long distance propagation, or filamentation, of short, intense laser pulses is suggested to be possible through the balance of two effects: self-focusing, when a nonlinear index of refraction of air is induced by high intensities, and de-focusing, due to the plasma created by the pulse. Applications for filamentation include areas such as remote sensing and directed energy. A split-step spectral propagation simulation is used to model the behavior of a high intensity ultraviolet laser pulse propagating through air. Convergence of femtosecond duration collapses that form on the leading edge of the pulse in the time domain is achieved with an …


Direct Diode Pumped Raman Amplifier Based On A Multimode Graded Index Fiberr, Charles James Baird Mar 2007

Direct Diode Pumped Raman Amplifier Based On A Multimode Graded Index Fiberr, Charles James Baird

Theses and Dissertations

The direct pumping of a Raman fiber amplifier (RFA) was attempted using an array of four 25W, fiber pigtailed diodes at 936nm, combined via a 7 channel fiber beam combiner. The initial attempt was conducted using a 1.8 km, 100 micron core, GRIN fiber with an NA of .29 and attenuation 3.6 dB/km at 936nm. While amplification was not achieved, over 200mW of conversion was shown, with 10.4W of pump power and 3.5W of seed. This corresponds to an average conversion efficiency of 2.2%. The subsequent effort utilized a 2km long, 200 micron core, GRIN fiber, with NA of .27 …


Direct Observation Of Laser Filamentation In High-Order Harmonic Generation, John Charles Painter May 2006

Direct Observation Of Laser Filamentation In High-Order Harmonic Generation, John Charles Painter

Theses and Dissertations

We investigate the spatial evolution of an intense laser pulse as it generates high-order harmonics in a long gas cell, filled with 80 torr of helium. A thin foil separates the gas-filled region of the cell from a subsequent evacuated region. The exit plane of the gas cell can be scanned along the laser axis so that the evolution of the laser throughout the focus can be observed (full scanning range of 9 cm). We constructed an apparatus that images the laser radial energy profile as it exits the cell. The high harmonics, odd orders ranging from 45 to 91, …


Comparison Of Climatological Optical Turbulence Profiles To Standard, Statistical And Numerical Models Using Heleeos, Liesebet E. Gravley Mar 2006

Comparison Of Climatological Optical Turbulence Profiles To Standard, Statistical And Numerical Models Using Heleeos, Liesebet E. Gravley

Theses and Dissertations

Optical turbulence within earth’s atmosphere plays a significant role in electromagnetic radiation propagation from a high energy laser. The index of refraction structure constant, Cn2, characterizes turbulent spatial fluctuations due to temperature gradients. These changes in the index of refraction affect the intensity of the laser wave front on its intended target. It is important to characterize this parameter throughout the atmosphere, the boundary layer and above, for its applications regarding the Airborne Laser (ABL) and the Advanced Tactical Laser (ATL). There are several ways to obtain values of optical turbulence, including standard and statistical models, physically-based numerical models, and …


Phasing A Dual Optical Path System Using An Optical Fiber As A Phase Conjugate Mirror, Shawn M. Willis Mar 2003

Phasing A Dual Optical Path System Using An Optical Fiber As A Phase Conjugate Mirror, Shawn M. Willis

Theses and Dissertations

Phase conjugation properties of stimulated Brillouin scattering (SBS) in a short multimode fiber have been investigated with an eye towards its application for a multi-channel double pass master oscillator power amplifier (MOPA) system. In particular, properties of the SBS beam to compensate for the axial and transverse phase distortion between individual channels in a multi-channel amplifier system were studied. Two optical paths were created by covering half of the laser beam with a microscope slide, and also by spatially splitting the wavefronts with a 4 prism set-up. The Stokes beams that traversed the same optical paths as the pump beams …


Algorithm Development For On-Line Control Of The Airborne Laser, Michael W. Oppenheimer Sep 2000

Algorithm Development For On-Line Control Of The Airborne Laser, Michael W. Oppenheimer

Theses and Dissertations

The use of adaptive optics entails the design of a controller. This requires the development of a model of the plant to be controlled, which, in this case, Consists of the atmosphere through which light is traveling. In optics, Zemike polynornials are used as a basis set for the expansion of wavefront phase distortions. Due to the turbulence induced stochastic nature of the underlying process involved, the spatial-temporal correlation functions of the Zemike polynomial phase expansion coefficients must be evaluated if a proper stochastic model of the plant is to be developed and adaptive optics is to be employed. In …