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- Monoclinic (3)
- Anisotropy (2)
- Augmented-Wave Method (2)
- Laalo3/Srtio3 Interface (2)
- Oxide Interfaces (2)
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- Alloys (1)
- Anharmonicity (1)
- Approximation (1)
- Atomic Layers (1)
- Band Alignment (1)
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- Gallium oxide (1)
- Half Metal (1)
- Heterostructures (1)
- Heusler Compounds (1)
- Insulator (1)
- Insulators (1)
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- Nebraska Center for Materials and Nanoscience: Faculty Publications (12)
- Evgeny Tsymbal Publications (6)
- Department of Physics and Astronomy: Dissertations, Theses, and Student Research (4)
- Alexei Gruverman Publications (3)
- Robert Streubel Papers (3)
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- Department of Electrical and Computer Engineering: Faculty Publications (2)
- Department of Physics and Astronomy: Faculty Publications (2)
- Stephen Ducharme Publications (2)
- Christian Binek Publications (1)
- Department of Electrical and Computer Engineering: Dissertations, Theses, and Student Research (1)
- Peter Dowben Publications (1)
- Shireen Adenwalla Papers (1)
Articles 1 - 30 of 38
Full-Text Articles in Physics
Magnetocrystalline Anisotropy Of "-Fe2o3, Imran Ahamed, Rohilt Pathak, Arti Kashyap
Magnetocrystalline Anisotropy Of "-Fe2o3, Imran Ahamed, Rohilt Pathak, Arti Kashyap
Nebraska Center for Materials and Nanoscience: Faculty Publications
The epsilon Fe2O3 phase of iron oxide has been studied to understand the spin structure and the magnetocrystalline anisotropy in the bulk and in thin films of "-Fe2O3 and Co-doped "-Fe2O3. The preferential magnetization direction in the nanoparticles of "-Fe2O3 is along the a-axis [M. Gich et al., Chem. Mater. 18, 3889 (2006)]. Compared to the bulk band gap of 1.9 eV, the thin-film band gap is reduced to 1.3 eV in the Co-free films and to 0.7 eV in the film with partial …
Texture Development And Coercivity Enhancement In Cast Alnico 9 Magnets, Wenyong Zhang, Shah Valloppilly, Xingzhong Li, Lanping Yue, Ralph Skomski, Iver Anderson, Matthew Kramer, Wei Tang, Jeff Shield, David J. Sellmyer
Texture Development And Coercivity Enhancement In Cast Alnico 9 Magnets, Wenyong Zhang, Shah Valloppilly, Xingzhong Li, Lanping Yue, Ralph Skomski, Iver Anderson, Matthew Kramer, Wei Tang, Jeff Shield, David J. Sellmyer
Nebraska Center for Materials and Nanoscience: Faculty Publications
The effect of Y addition and magnetic field on texture and magnetic properties of arc-melted alnico 9 magnets has been investigated. Small additions of Y (1.5 wt.%) develop a (200) texture for the arc-melted alnico 9 magnet. Such a texture is hard to form in cast samples. To achieve this goal, we set up a high-field annealing system with a maximum operation temperature of 12500 C. This system enabled annealing in a field of 45 kOe with subsequent draw annealing for the solutionized buttons; we have been able to substantially increase remanence ratio and coercivity, from 0.70 and 1200 …
Prediction Of A Mobile Two-Dimensional Electron Gas At The Lasco3/Basno3(001) Interface, Tula R. Paudel, Evgeny Y. Tsymbal
Prediction Of A Mobile Two-Dimensional Electron Gas At The Lasco3/Basno3(001) Interface, Tula R. Paudel, Evgeny Y. Tsymbal
Evgeny Tsymbal Publications
Two-dimensional electron gases (2DEG) at oxide interfaces, such as LaAlO3/SrTiO3 (001), have aroused significant interest due to their high carrier density (∼1014 cm−2) and strong lateral confinement (∼1 nm). However, these 2DEGs are normally hosted by the weakly dispersive and degenerate d bands (e.g., Ti-3d bands), which are strongly coupled to the lattice, causing mobility of such 2DEGs to be relatively low at room temperature (∼1 cm2/Vs). Here, we propose using oxide host materials with the conduction bands formed from s electrons to increase carrier mobility and soften its temperature dependence. Using …
Generalized Ellipsometry On Complex Nanostructures And Low-Symmetry Materials, Alyssa Mock
Generalized Ellipsometry On Complex Nanostructures And Low-Symmetry Materials, Alyssa Mock
Department of Electrical and Computer Engineering: Dissertations, Theses, and Student Research
In this thesis, complex anisotropic materials are investigated and characterized by generalized ellipsometry. In recent years, anisotropic materials have gained considerable interest for novel applications in electronic and optoelectronic devices, mostly due to unique properties that originate from reduced crystal symmetry. Examples include white solid-state lighting devices which have become ubiquitous just recently, and the emergence of high-power, high-voltage electronic transistors and switches in all-electric vehicles. The incorporation of single crystalline material with low crystal symmetry into novel device structures requires reconsideration of existing optical characterization approaches. Here, the generalized ellipsometry concept is extended to include applications for materials with …
Epitaxial Thin Films Of Dirac Semimetal Antiperovskite Cu3Pdn, C. X. Quintela, N. Campbell, D. F. Shao, J. Irwin, D. T. Harris, L. Lie, T. J. Anderson, N. Reiser, X. Q. Pan, Evgeny Y. Tsymbal, M. S. Rzchowski, C B. Eom
Epitaxial Thin Films Of Dirac Semimetal Antiperovskite Cu3Pdn, C. X. Quintela, N. Campbell, D. F. Shao, J. Irwin, D. T. Harris, L. Lie, T. J. Anderson, N. Reiser, X. Q. Pan, Evgeny Y. Tsymbal, M. S. Rzchowski, C B. Eom
Evgeny Tsymbal Publications
The growth and study of materials showing novel topological states of matter is one of the frontiers in condensed matter physics. Among this class of materials, the nitride antiperovskite Cu3PdN has been proposed as a new three-dimensional Dirac semimetal. However, the experimental realization of Cu3PdN and the consequent study of its electronic properties have been hindered due to the difficulty of synthesizing this material. In this study, we report fabrication and both structural and transport characterization of epitaxial Cu3PdN thin films grown on (001)-oriented SrTiO3 substrates by reactive magnetron sputtering and post-annealed in …
Surfaces And Interfaces Of Magnetoelectric Oxide Systems, Shi Cao
Surfaces And Interfaces Of Magnetoelectric Oxide Systems, Shi Cao
Department of Physics and Astronomy: Dissertations, Theses, and Student Research
Magnetoelectric materials Cr2O3, hexagonal LuFeO3 and YbFeO3 are studied in this thesis. The surface of chromia (Cr2O3) has a surface electronic structure distinct from the bulk. Our work shows that placing a Cr2O3 single crystal into a single domain state will result in net Cr2O3 spin polarization at the boundary, even in the presence of a gold overlayer. From the Cr 2p3=2 X-ray magnetic circular dichroism signal, there is clear evidence of interface polarization with overlayers of both Pd and Pt on chromia. Cobalt thin films on Cr2O3(0001) show larger magnetic contrast in magnetic force microscopy indicating enhancement of perpendicular …
Three-Dimensional Nanomagnetism, Amalio Fernández-Pacheco, Robert Streubel, Olivier Fruchart, Riccardo Hertel, Peter Fischer, Russell P. Cowburn
Three-Dimensional Nanomagnetism, Amalio Fernández-Pacheco, Robert Streubel, Olivier Fruchart, Riccardo Hertel, Peter Fischer, Russell P. Cowburn
Robert Streubel Papers
Magnetic nanostructures are being developed for use in many aspects of our daily life, spanning areas such as data storage, sensing and biomedicine. Whereas patterned nanomagnets are traditionally two-dimensional planar structures, recent work is expanding nanomagnetism into three dimensions; a move triggered by the advance of unconventional synthesis methods and the discovery of new magnetic effects. In three-dimensional nanomagnets more complex magnetic configurations become possible, many with unprecedented properties. Here we review the creation of these structures and their implications for the emergence of new physics, the development of instrumentation and computational methods, and exploitation in numerous applications.
Nanosecond X-Ray Photon Correlation Spectroscopy On Magnetic Skyrmions, M. H. Seaberg, B. Holladay, J. C.T. Lee, M. Sikorski, A. H. Reid, S. A. Montoya, G. L. Dakovski, J. D. Koralek, G. Coslovich, S. Moeller, W. F. Schlotter, R. Streubel, S. D. Kevan, P. Fischer, E. E. Fullerton, J. L. Turner, F. J. Decker, S. K. Sinha, S. Roy, J. J. Turner
Nanosecond X-Ray Photon Correlation Spectroscopy On Magnetic Skyrmions, M. H. Seaberg, B. Holladay, J. C.T. Lee, M. Sikorski, A. H. Reid, S. A. Montoya, G. L. Dakovski, J. D. Koralek, G. Coslovich, S. Moeller, W. F. Schlotter, R. Streubel, S. D. Kevan, P. Fischer, E. E. Fullerton, J. L. Turner, F. J. Decker, S. K. Sinha, S. Roy, J. J. Turner
Robert Streubel Papers
We report an x-ray photon correlation spectroscopy method that exploits the recent development of the two-pulse mode at the Linac Coherent Light Source. By using coherent resonant x-ray magnetic scattering, we studied spontaneous fluctuations on nanosecond time scales in thin films of multilayered Fe/Gd that exhibit ordered stripe and Skyrmion lattice phases. The correlation time of the fluctuations was found to differ between the Skyrmion phase and near the stripe-Skyrmion boundary. This technique will enable a significant new area of research on the study of equilibrium fluctuations in condensed matter.
Novel Half-Metallic And Spin-Gapless Heusler Compounds, Yunlong Jin
Novel Half-Metallic And Spin-Gapless Heusler Compounds, Yunlong Jin
Department of Physics and Astronomy: Dissertations, Theses, and Student Research
This thesis is devoted to experimental studies of Heusler compounds CoFeCrAl, CoFeCrX (X = Si, Ge) and Mn2PtSn. These Heusler alloys present an interesting class of ferromagnetic materials for spintronic applications since they are predicted to be spin gapless semiconductors and have half-metallic properties with 100 % spin polarization at the Fermi level. In this thesis, the structural, magnetic, spin-polarization and electron- transport properties of the fabricated alloys were studied. CoFeCrAl thin films deposited on MgO exhibit nearly perfect epitaxy and a high degree of L21 Heusler order. All considered types of chemical disorder destroy the spin-gapless …
Model Of Orbital Populations For Voltage-Controlled Magnetic Anisotropy In Transition-Metal Thin Films, Jia Zhang, Pavel V. Lukashev, Sitaram Jaswal, Evgeny Y. Tsymbal
Model Of Orbital Populations For Voltage-Controlled Magnetic Anisotropy In Transition-Metal Thin Films, Jia Zhang, Pavel V. Lukashev, Sitaram Jaswal, Evgeny Y. Tsymbal
Evgeny Tsymbal Publications
Voltage-controlled magnetic anisotropy (VCMA) is an efficient way to manipulate the magnetization states in nanomagnets and is promising for low-power spintronic applications. The underlying physical mechanism for VCMA is known to involve a change in the d orbital occupation on the transition-metal interface atoms with an applied electric field. However, a simple qualitative picture of how this occupation controls the magnetocrystalline anisotropy (MCA) and even why in certain cases the MCA has the opposite sign remains elusive. In this paper, we exploit a simple model of orbital populations to elucidate a number of features typical for the interface MCA, and …
Spin-Polarized Two-Dimensional Electron Gas At Gdtio3/Srtio3 Interfaces: Insight From First-Principles Calculations, J. Betancourt, Tula R. Paudel, Evgeny Y. Tsymbal, J. P. Velev
Spin-Polarized Two-Dimensional Electron Gas At Gdtio3/Srtio3 Interfaces: Insight From First-Principles Calculations, J. Betancourt, Tula R. Paudel, Evgeny Y. Tsymbal, J. P. Velev
Evgeny Tsymbal Publications
Two-dimensional electron gases (2DEGs) at oxide interfaces have been a topic of intensive research due to their high carrier mobility and strong confinement. Additionally, strong correlations in the oxide materials can give rise to new and interesting physics, such as magnetism and metal-insulator transitions at the interface. Using first-principles calculations based on density functional theory, we demonstrate the presence of a highly spin-polarized 2DEG at the interface between the Mott insulator GdTiO3 and a band insulator SrTiO3. The strong correlations in the dopant cause ferromagnetic alignment of the interface Ti atoms and result in a fully spin-polarized …
Simulation Of Alnico Coercivity, Liqin Ke, Ralph Skomski, Todd D. Hoffman, Lin Zhoue, Wei Tang, Duane D. Johnson, Matthew J. Kramer, Iver E. Anderson, C.Z. Wang
Simulation Of Alnico Coercivity, Liqin Ke, Ralph Skomski, Todd D. Hoffman, Lin Zhoue, Wei Tang, Duane D. Johnson, Matthew J. Kramer, Iver E. Anderson, C.Z. Wang
Nebraska Center for Materials and Nanoscience: Faculty Publications
Micromagnetic simulations of alnico show substantial deviations from Stoner-Wohlfarth behavior due to the unique size and spatial distribution of the rod-like Fe-Co phase formed during spinodal decomposition in an external magnetic field. The maximum coercivity is limited by single-rod effects, especially deviations from ellipsoidal shape, and by interactions between the rods. Both the exchange interaction between connected rods and magnetostatic interaction between rods are considered, and the results of our calculations show good agreement with recent experiments. Unlike systems dominated by magnetocrystalline anisotropy, coercivity in alnico is highly dependent on size, shape, and geometric distribution of the Fe-Co phase, all …
Reversible Spin Texture In Ferroelectric Hfo2, L. L. Tao, Tula R. Paudel, Alexey Kovalev, Evgeny Tsymbal
Reversible Spin Texture In Ferroelectric Hfo2, L. L. Tao, Tula R. Paudel, Alexey Kovalev, Evgeny Tsymbal
Evgeny Tsymbal Publications
Spin-orbit coupling effects occurring in noncentrosymmetric materials are known to be responsible for nontrivial spin configurations and a number of emergent physical phenomena. Ferroelectric materials may be especially interesting in this regard due to reversible spontaneous polarization making possible a nonvolatile electrical control of the spin degrees of freedom. Here, we explore a technologically relevant oxide material, HfO2, which has been shown to exhibit robust ferroelectricity in a noncentrosymmetric orthorhombic phase. Using theoretical modelling based on density-functional theory, we investigate the spin-dependent electronic structure of the ferroelectric HfO2 and demonstrate the appearance of chiral spin textures driven …
Electronic Structure And Direct Observation Of Ferrimagnetism In Multiferroic Hexagonal Ybfeo3, Shi Cao, Kishan Sinha, Xin Zhang, Xiaozhe Zhang, Xiao Wang, Yuewei Yin, Alpha T. N’Diaye, Jian Wang, David J. Keavney, Tula R. Paudel, Yaohua Liu, Xuemei Cheng, Evgeny Y. Tsymbal, Peter A. Dowben, Xiaoshan Xu
Electronic Structure And Direct Observation Of Ferrimagnetism In Multiferroic Hexagonal Ybfeo3, Shi Cao, Kishan Sinha, Xin Zhang, Xiaozhe Zhang, Xiao Wang, Yuewei Yin, Alpha T. N’Diaye, Jian Wang, David J. Keavney, Tula R. Paudel, Yaohua Liu, Xuemei Cheng, Evgeny Y. Tsymbal, Peter A. Dowben, Xiaoshan Xu
Evgeny Tsymbal Publications
The magnetic interactions between rare-earth and Fe ions in hexagonal rare-earth ferrites (h-RFeO3), may amplify the weak ferromagnetic moment on Fe, making these materials more appealing as multiferroics. To elucidate the interaction strength between the rare-earth and Fe ions as well as the magnetic moment of the rare-earth ions, element-specific magnetic characterization is needed. Using x-ray magnetic circular dichroism, we have studied the ferrimagnetism in h-YbFeO3 by measuring the magnetization of Fe and Yb separately. The results directly show antialignment of magnetization of Yb and Fe ions in h-YbFeO3 at low temperature, …
Vortex Circulation Patterns In Planar Microdisk Arrays, Sven Velten, Robert Streubel, Alan Farhan, Noah Kent, Mi Young Im, Andreas Scholl, Scott Dhuey, Carolin Behncke, Guido Meier, Peter Fischer
Vortex Circulation Patterns In Planar Microdisk Arrays, Sven Velten, Robert Streubel, Alan Farhan, Noah Kent, Mi Young Im, Andreas Scholl, Scott Dhuey, Carolin Behncke, Guido Meier, Peter Fischer
Robert Streubel Papers
We report a magnetic X-ray microscopy study of the pattern formation of circulation in arrays of magnetic vortices ordered in a hexagonal and a honeycomb lattice. In the honeycomb lattice, we observe at remanence an ordered phase of alternating circulations, whereas in the hexagonal lattice, small regions of alternating lines form. A variation in the edge-to-edge distance shows that the size of those regions scales with the magnetostatic interaction. Micromagnetic simulations reveal that the patterns result from the formation of flux closure states during the nucleation process.
Ferroelectric-Domain-Patterning-Controlled Schottky Junction State In Monolayer Mos2, Zhiyong Xiao, Jingfeng Song, David K. Ferry, Stephen Ducharme, Xia Hong
Ferroelectric-Domain-Patterning-Controlled Schottky Junction State In Monolayer Mos2, Zhiyong Xiao, Jingfeng Song, David K. Ferry, Stephen Ducharme, Xia Hong
Stephen Ducharme Publications
We exploit scanning-probe-controlled domain patterning in a ferroelectric top layer to induce nonvolatile modulation of the conduction characteristic of monolayer MoS2 between a transistor and a junction state. In the presence of a domain wall, MoS2 exhibits rectified I-V characteristics that are well described by the thermionic emission model. The induced Schottky barrier height ΦeffB varies from 0.38 to 0.57 eV and is tunable by a SiO2 global back gate, while the tuning range of ΦeffB depends sensitively on the conduction-band-tail trapping states. Our work points to a new route to achieving programmable …
Reversible Spin Texture In Ferroelectric Hfo2, L. L. Tao, Tula R. Paudel, Alexey Kovalev, Evgeny Tsymbal
Reversible Spin Texture In Ferroelectric Hfo2, L. L. Tao, Tula R. Paudel, Alexey Kovalev, Evgeny Tsymbal
Department of Physics and Astronomy: Faculty Publications
Spin-orbit coupling effects occurring in noncentrosymmetric materials are known to be responsible for nontrivial spin configurations and a number of emergent physical phenomena. Ferroelectric materials may be especially interesting in this regard due to reversible spontaneous polarization making possible a nonvolatile electrical control of the spin degrees of freedom. Here, we explore a technologically relevant oxide material, HfO2, which has been shown to exhibit robust ferroelectricity in a noncentrosymmetric orthorhombic phase. Using theoretical modelling based on density-functional theory, we investigate the spin-dependent electronic structure of the ferroelectric HfO2 and demonstrate the appearance of chiral spin textures driven by spin-orbit coupling. …
Fabrication And Study Of The Structure And Magnetism Of Rare-Earth Free Nanoclusters, Bhaskar Das
Fabrication And Study Of The Structure And Magnetism Of Rare-Earth Free Nanoclusters, Bhaskar Das
Department of Physics and Astronomy: Dissertations, Theses, and Student Research
No abstract provided.
Pumping Of Magnons In A Dzyaloshinskii-Moriya Ferromagnet, Alexey Kovalev, Vladimir Zyuzin, Bo Li
Pumping Of Magnons In A Dzyaloshinskii-Moriya Ferromagnet, Alexey Kovalev, Vladimir Zyuzin, Bo Li
Department of Physics and Astronomy: Faculty Publications
We formulate a microscopic linear response theory of magnon pumping applicable to multiple-magnonic-band uniform ferromagnets with Dzyaloshinskii-Moriya interactions. From the linear response theory, we identify the extrinsic and intrinsic contributions where the latter is expressed via the Berry curvature of magnonic bands. We observe that in the presence of a time-dependent magnetization Dzyaloshinskii-Moriya interactions can act as fictitious electric fields acting on magnons. We study various current responses to this fictitious field and analyze the role of Berry curvature. In particular, we obtain an analog of the Hall-like response in systems with nontrivial Berry curvature of magnon bands. After identifying …
Tuning The Effective Anisotropy In A Voltage-Susceptible Exchange-Bias Heterosystem, Will Echtenkamp, Mike Street, Ather Mahmood, Christian Binek
Tuning The Effective Anisotropy In A Voltage-Susceptible Exchange-Bias Heterosystem, Will Echtenkamp, Mike Street, Ather Mahmood, Christian Binek
Christian Binek Publications
Voltage- and temperature-tuned ferromagnetic hysteresis is investigated by a superconducting quantum-interference device and Kerr magnetometry in a thin-film heterostructure of a perpendicular anisotropic Co/Pd ferromagnet exchange coupled to the magnetoelectric antiferromagnet Cr2O3. An abrupt disappearance of exchange bias with a simultaneous more than twofold increase in coercivity is observed and interpreted as a competition between the effective anisotropy of Cr2O3 and the exchange-coupling energy between boundary magnetization and the adjacent ferromagnet. The effective anisotropy energy is given by the intrinsic anisotropy energy density multiplied by the effective volume separated from the bulk through …
Effect Of Disorder On The Resistivity Of Cofecral Films, Y. Jin, R. Skomski, P. Kharel, S.R. Valloppilly, D. J. Sellmyer
Effect Of Disorder On The Resistivity Of Cofecral Films, Y. Jin, R. Skomski, P. Kharel, S.R. Valloppilly, D. J. Sellmyer
Nebraska Center for Materials and Nanoscience: Faculty Publications
Structural and electron-transport properties of thin films of the ferrimagnetic Heusler compound CoFeCrAl have been investigated to elucidate structure-property relationships. The alloy is, ideally, a spin-gapless semiconductor, but structural disorder destroys the spin-gapless character and drastically alters the transport behavior. Two types of CoFeCrAl films were grown by magnetron sputtering deposition at 973 K, namely polycrystalline films on Si substrates and epitaxial films on MgO (001) substrates. The resistivity decreases with increasing temperature, with relatively small temperature coefficients of –0.19 cm=K for the polycrystalline films and –0.12 cm=K for the epitaxial films. The residual resistivity of the polycrystalline films deposited …
Half-Metallic Magnetism In Ti3co5-Xfexb2, Rohit Pathak, Imran Ahamed, W. Y. Zhang, Shah Vallopilly, D. J. Sellmyer, Ralph Skomski, Arti Kashyap
Half-Metallic Magnetism In Ti3co5-Xfexb2, Rohit Pathak, Imran Ahamed, W. Y. Zhang, Shah Vallopilly, D. J. Sellmyer, Ralph Skomski, Arti Kashyap
Nebraska Center for Materials and Nanoscience: Faculty Publications
Bulk alloys and thin films of Fe-substituted Ti3Co5B2 have been investigated by first-principle density-functional calculations. The series, which is of interest in the context of alnico magnetism and spin electronics, has been experimentally realized in nanostructures but not in the bulk. Our bulk calculations predict paramagnetism for Ti3Co5B2, Ti3Co4FeB2 and Ti3CoFe4B2, whereas Ti3Fe5B2 is predicted to be ferromagnetic. The thin films are all ferromagnetic, indicating that moment formation may be facilitated at nanostructural …
Cooperative And Noncooperative Magnetization Reversal In Alnicos, Raplh Skomski, Liqin Ke, Matthew J. Kramer, Iver E. Anderson, C.Z. Wang, W.Y. Zhang, Jeff E. Shield, D. J. Sellmyer
Cooperative And Noncooperative Magnetization Reversal In Alnicos, Raplh Skomski, Liqin Ke, Matthew J. Kramer, Iver E. Anderson, C.Z. Wang, W.Y. Zhang, Jeff E. Shield, D. J. Sellmyer
Nebraska Center for Materials and Nanoscience: Faculty Publications
It is investigated how magnetostatic interactions affect the coercivity of alnicotype magnets. Starting from exact micromagnetic relations, we analyze two limits, namely cooperative reversal processes operative on short lengths scales and noncooperative reversal processes on long length scales. In alnicos, intrawire interactions are predominantly cooperative, whereas interwire effects are typically noncooperative. However, the transition between the regimes depends on feature size and hysteresis-loop shape, and interwire cooperative effects are largest for nearly rectangular loops. Our analysis revises the common shape-anisotropy interpretation of alnicos.
Epitaxial Strain Controlled Magnetocrystalline Anisotropy In Ultrathin Ferh/Mgo Bilayers, Guohul Zheng, San-Huang Ke, Maosheng Miao, Jinwoong Kim, R, Ramesh, Nicholas Kioussis
Epitaxial Strain Controlled Magnetocrystalline Anisotropy In Ultrathin Ferh/Mgo Bilayers, Guohul Zheng, San-Huang Ke, Maosheng Miao, Jinwoong Kim, R, Ramesh, Nicholas Kioussis
Nebraska Center for Materials and Nanoscience: Faculty Publications
Using ab initio electronic structure calculations we have investigated the effect of epitazial strain on the magnetocrystalline anisotropy (MCA) of ultrathin FeRh/MgO heterostructures. Analysis of the energy- and k-resolved distribution of the orbital character of the band structure reveals that MCA largely arises from the spin-orbit coupling (SOC) between dx2-y2 and dxz/dyz orbitlas of Fe atoms at the FeRh/MhO interface. We demonstrate that the strain has significant effects on the MCA: It not only affects the value of the MCA but also induces a switching of the magnetic easy axis from perpendicular on in-plane direction. The …
Band-To-Band Transitions, Selection Rules, Effective Mass, And Excitonic Contributions In Monoclinic Β-Ga2o3, Alyssa Mock, Rafal Korlacki, Chad Briley, Vanya Darakchieva, Bo Monemar, Yoshinao Kumagai, Ken Goto, Masataka Higashiwaki, Mathias Schubert
Band-To-Band Transitions, Selection Rules, Effective Mass, And Excitonic Contributions In Monoclinic Β-Ga2o3, Alyssa Mock, Rafal Korlacki, Chad Briley, Vanya Darakchieva, Bo Monemar, Yoshinao Kumagai, Ken Goto, Masataka Higashiwaki, Mathias Schubert
Department of Electrical and Computer Engineering: Faculty Publications
We employ an eigenpolarization model including the description of direction dependent excitonic effects for rendering critical point structures within the dielectric function tensor of monoclinic β-Ga2O3 yielding a comprehensive analysis of generalized ellipsometry data obtained from 0.75–9 eV. The eigenpolarization model permits complete description of the dielectric response. We obtain, for single-electron and excitonic band-to-band transitions, anisotropic critical point model parameters including their polarization vectors within the monoclinic lattice. We compare our experimental analysis with results from density functional theory calculations performed using the Gaussian-attenuation-Perdew-Burke-Ernzerhof hybrid density functional. We present and discuss the order of the …
Anisotropy, Phonon Modes, And Lattice Anharmonicity From Dielectric Function Tensor Analysis Of Monoclinic Cadmium Tungstate, Alyssa Mock, Rafal Korlacki, Sean Knight, Mathias Schubert
Anisotropy, Phonon Modes, And Lattice Anharmonicity From Dielectric Function Tensor Analysis Of Monoclinic Cadmium Tungstate, Alyssa Mock, Rafal Korlacki, Sean Knight, Mathias Schubert
Department of Electrical and Computer Engineering: Faculty Publications
We determine the frequency dependence of four independent Cartesian tensor elements of the dielectric function for CdWO4 using generalized spectroscopic ellipsometry within mid-infrared and far-infrared spectral regions. Different single crystal cuts, (010) and (001), are investigated. From the spectral dependencies of the dielectric function tensor and its inverse we determine all long-wavelength active transverse and longitudinal optic phonon modes with Au and Bu symmetry as well as their eigenvectors within the monoclinic lattice. We thereby demonstrate that such information can be obtained completely without physical model line-shape analysis in materials with monoclinic symmetry. We then augment the …
First-Principle Investigation Of Structural, Electronic And Magnetic Properties Of Co2vin And Covin Heusler Compounds, Zipporah Muthui, Rohit Pathak, Robinson Musembi, Julius Mwabora, Ralph Skomski, Arti Kashyap
First-Principle Investigation Of Structural, Electronic And Magnetic Properties Of Co2vin And Covin Heusler Compounds, Zipporah Muthui, Rohit Pathak, Robinson Musembi, Julius Mwabora, Ralph Skomski, Arti Kashyap
Nebraska Center for Materials and Nanoscience: Faculty Publications
Investigation of the structural, electronic and magnetic properties of full-Heusler Co2VIn as well as half-Heusler CoVIn Cobalt based Heusler compounds using density functional theory (DFT) leads to the general conclusion that Co2VIn and CoVIn are half-metallic materials with a gap at the Fermi level in the minority states and majority states respectively. A Hubbard-like Coulomb correlation term U has been included in the DFT (DFT+U) for the computation of the electronic and magnetic properties of the compounds. The structural properties have been calculated for the paramagnetic and ferromagnetic phases, and both Co2VIn …
Effect Of Disorder On The Magnetic And Electronic Structure Of A Prospective Spin-Gapless Semiconductor Mncrval, P. Kharel, J. Herran, P. Lukashev, Y. Jin, J. Waybright, S. Gilbert, B. Staten, P. Gray, S. Valloppilly, Y. Huh, D. J. Sellmyer
Effect Of Disorder On The Magnetic And Electronic Structure Of A Prospective Spin-Gapless Semiconductor Mncrval, P. Kharel, J. Herran, P. Lukashev, Y. Jin, J. Waybright, S. Gilbert, B. Staten, P. Gray, S. Valloppilly, Y. Huh, D. J. Sellmyer
Nebraska Center for Materials and Nanoscience: Faculty Publications
Recent discovery of a new class of materials, spin-gapless semiconductors (SGS), has attracted considerable attention in the last few years, primarily due to potential applications in the emerging field of spin-based electronics (spintronics). Here, we investigate structural, electronic, and magnetic properties of one potential SGS compound, MnCr-VAl, using various experimental and theoretical techniques. Our calculations show that this material exhibits ≈ 0.5 eV band gap for the majority-spin states, while for the minority-spin it is nearly gapless. The calculated magnetic moment for the com- pletely ordered structure is 2.9 μB/f.u., which is different from our experimentally measured value …
Controlling The Microstructure And Associated Magnetic Properties Of Ni0.2mn3.2ga0.6 Melt-Spun Ribbons By Annealing, Mahmud Khan, Ohud Alshammari, Balamurugan Balamurugan, Bhaskar Das, David J. Sellmyer, Ahmad Us Saleheen, Shane Stadler
Controlling The Microstructure And Associated Magnetic Properties Of Ni0.2mn3.2ga0.6 Melt-Spun Ribbons By Annealing, Mahmud Khan, Ohud Alshammari, Balamurugan Balamurugan, Bhaskar Das, David J. Sellmyer, Ahmad Us Saleheen, Shane Stadler
Nebraska Center for Materials and Nanoscience: Faculty Publications
Here we report on the structural and magnetic properties of Ni0.2Mn3.2Ga0.6 melt- spun ribbons. The as-spun ribbons were found to exhibit mixed cubic phases that transform to non-cubic structure upon annealing. Additionally, an amorphous phase was found to co-exist in all ribbons. The SEM images show that minor grain forma- tion occurs on the as-spun ribbons. However, the formation of extensive nano-grains was observed on the surfaces of the annealed ribbons. While the as-spun ribbons exhibit predominantly paramagnetic behavior, the ribbons annealed under various thermal conditions were found to be ferromagnetic with a Curie temperature …
Effect Of Fe Substitution On The Structural, Magnetic And Electron-Transport Properties Of Half-Metallic Co2tisi, Y. Jin, J. Waybright, P. Kharel, I. Tutic, J. Herran, P. Lukashev, S. Valloppilly, D. J. Sellmyer
Effect Of Fe Substitution On The Structural, Magnetic And Electron-Transport Properties Of Half-Metallic Co2tisi, Y. Jin, J. Waybright, P. Kharel, I. Tutic, J. Herran, P. Lukashev, S. Valloppilly, D. J. Sellmyer
Nebraska Center for Materials and Nanoscience: Faculty Publications
The structural, magnetic and electron-transport properties of Co2Ti1-xFexSi (x = 0, 0.25, 0.5) ribbons prepared by arc-melting and melt-spinning were investi- gated. The rapidly quenched Co2Ti0.5Fe0.5Si crystallized in the cubic L21 structure whereas Co2Ti0.75Fe0.25Si and Co2TiFe0Si showed various degrees of B2-type disorder. At room temperature, all the samples are ferromagnetic, and the Curie tem- perature increased from 360 K for Co2TiSi to about 800 K for Co2Ti0.5Fe0.5Si. The measured …