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Measurements Of The Hyperpolarizability Tensor By Means Of Hyper-Rayleigh Scattering, Liang-Chy Chien, V. Ostroverkhova, R. G. Petschek, K. D. Singer, L. Sukhomlinova, R. J. Twieg, S.-X. Wang
Measurements Of The Hyperpolarizability Tensor By Means Of Hyper-Rayleigh Scattering, Liang-Chy Chien, V. Ostroverkhova, R. G. Petschek, K. D. Singer, L. Sukhomlinova, R. J. Twieg, S.-X. Wang
Liang-Chy Chien
We describe improvements to a previously reported hyper-Rayleigh scattering technique [J. Opt. Sec. Am. B 15, 289 (1998)], for measuring all rotational invariants of the first hyperpolarizability tensor. The full hyper-Rayleigh scattering tensor is expressed in terms of its rotationally invariant components leading to a figures of merit corresponding to each of the rotationally invariant tensors. With elliptically polarized incident light, the polarization state and the intensity of the harmonic light are measured at a scattering angle of 45 degrees. A new analytical fitting method is applied to the signal for two polarization measurements to yield the invariants. We have …