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Articles 31 - 60 of 74
Full-Text Articles in Physics
Volatile Products Controlling Titan’S Tholins Production, N. Carrasco, T. Gautier, Et. Es-Sebbar, P. Pernot, G. Cernogora
Volatile Products Controlling Titan’S Tholins Production, N. Carrasco, T. Gautier, Et. Es-Sebbar, P. Pernot, G. Cernogora
Dr. Et-touhami Es-sebbar
A quantitative agreement between nitrile relative abundances and Titan’s atmospheric composition was recently shown with a reactor simulating the global chemistry occurring in Titan’s atmosphere [Gautier et al. (2011) Icarus, 213: 625]. Here we present a complementary study on the same reactor using an in-situ diagnostic of the gas phase composition. Various initial N2-CH4 gas mixtures (methane varying from 1 to 10%) are studied, with a monitoring of the methane consumption and of the stable gas neutrals by in-situ mass spectrometry. Atomic hydrogen is also measured by optical emission spectroscopy. A positive correlation is found between atomic hydrogen abundance and …
Vuv Photoionization Of Acetamide Studied By Electron / Ion Coincidence Spectroscopy In The 8-24 Ev Photon Energy Range, M. Schwell, Y. Bénilan, N. Fray, M.-C Gazeau, Et. Es-Sebbar, Gustavo A. Garcia, L. Nahon, N. Champion, S. Leach
Vuv Photoionization Of Acetamide Studied By Electron / Ion Coincidence Spectroscopy In The 8-24 Ev Photon Energy Range, M. Schwell, Y. Bénilan, N. Fray, M.-C Gazeau, Et. Es-Sebbar, Gustavo A. Garcia, L. Nahon, N. Champion, S. Leach
Dr. Et-touhami Es-sebbar
A VUV photoionization study of acetamide was carried out over the 8-24 eV photon energy range using synchrotron radiation and photoelectron/photoion coincidence (PEPICO) spectroscopy. Threshold photoelectron photoion coincidence (TPEPICO) measurements were also made. Photoion yield curves and branching ratios were measured for the parent ion and six fragment ions. The adiabatic ionization energy of acetamide was determined as I.E (12A’) = (9.71±0.02) eV, in agreement with an earlier reported photoionization mass spectrometry (PIMS) value. The adiabatic energy of the first excited state of the ion, 12A”, was determined to be ≈ 10.1 eV. Assignments of the fragment ions and the …
Hydrogen Production From Biogas By Oxy-Reforming: Reaction System Analysis, Aleksandra Terlecka, Wojciech M. Budzianowski
Hydrogen Production From Biogas By Oxy-Reforming: Reaction System Analysis, Aleksandra Terlecka, Wojciech M. Budzianowski
Wojciech Budzianowski
Oxy-reforming is emerging as an interesting alternative to conventional methods of hydrogen generation. The current article characterises this process through analysis of individual reactions: SMR (steam methane reforming), WGS (water gas shift) and CPO (catalytic partial oxidation). Analyses relate to optimisation of thermal conditions thus enabling cost-effectivenes of the process.
Vuv Absorption Cross Section Of Benzene, Relevance For Titan’S Atmosphere, F-J. Capalbo, Y. Bénilan, N. Fray, M. Schwell, Et. Es-Sebbar, N. Champion, T. Koskinen, R. Yelle
Vuv Absorption Cross Section Of Benzene, Relevance For Titan’S Atmosphere, F-J. Capalbo, Y. Bénilan, N. Fray, M. Schwell, Et. Es-Sebbar, N. Champion, T. Koskinen, R. Yelle
Dr. Et-touhami Es-sebbar
Saturn's largest satellite, Titan, is the only one in the Solar System known to have a thick N2/CH4, planet like atmosphere. The dissociation of these principal components and the recombination of the products make this atmosphere to be rich in organic compounds of high interest for astrobiology. Solar and stellar occultations observed by the Ultraviolet Imaging Spectrograph (UVIS) on board the Cassini spacecraft can be used to characterize the composition of Titan’s upper atmosphere (400 – 1400 km). The results depend strongly on the knowledge of the molecular absorption cross sections of the atmospheric constituents (Ferradaz et al. 2009). This …
Bistability In A Simple Fluid Network Due To Viscosity Contrast, John B. Geddes, Brian D. Storey, David Gardner, Russell T. Carr
Bistability In A Simple Fluid Network Due To Viscosity Contrast, John B. Geddes, Brian D. Storey, David Gardner, Russell T. Carr
John B. Geddes
We study the existence of multiple equilibrium states in a simple fluid network using Newtonian fluids and laminar flow. We demonstrate theoretically the presence of hysteresis and bistability, and we confirm these predictions in an experiment using two miscible fluids of different viscosity—sucrose solution and water. Possible applications include blood flow, microfluidics, and other network flows governed by similar principles.
Characterization Of Continuous Vacuum Ultraviolet Lamps-Implication On The Study Of Methane Photolysis At Lyman Alpha (121.6 Nm), M-C. Gazeau, Y. Benilan, Et. Es-Sebbar, A. Jolly, E. Arzoumanian, N. Fray, H. Cottin
Characterization Of Continuous Vacuum Ultraviolet Lamps-Implication On The Study Of Methane Photolysis At Lyman Alpha (121.6 Nm), M-C. Gazeau, Y. Benilan, Et. Es-Sebbar, A. Jolly, E. Arzoumanian, N. Fray, H. Cottin
Dr. Et-touhami Es-sebbar
Low-temperature hydrogen plasmas are widely used as continuous vacuum ultraviolet irradiation sources in photochemical studies and, in particular, in laboratory simulations of planetary atmospheres. One of the most challenging objectives of such experiments is to retrieve accurate quantitative laboratory data allowing a reliable comparison with theoretical and/or observational ones. This task can only be achieved when the irradiation source delivers a well characterised radiation in terms of flux and wavelength dependency. As an example, we will present a study, developed in the frame of a program dedicated to simulations of Titan’s atmosphere, on methane photolysis at Lyman alpha (121.6 nm). …
Formation Of Hcn And Nh3 As Primary Compounds Of Titan’S Atmosphere Simulations Using N2-Ch4 Afterglow Plasma’’, M-C. Gazeau, Y. Bénilan, E. Arzoumanian, Et. Es-Sebbar, A. Jolly, C.D. Pintassilgo
Formation Of Hcn And Nh3 As Primary Compounds Of Titan’S Atmosphere Simulations Using N2-Ch4 Afterglow Plasma’’, M-C. Gazeau, Y. Bénilan, E. Arzoumanian, Et. Es-Sebbar, A. Jolly, C.D. Pintassilgo
Dr. Et-touhami Es-sebbar
No abstract provided.
Argon Rectification And The Cause Of Light Emission In Single-Bubble Sonoluminescence, Brian D. Storey, Andrew J. Szeri
Argon Rectification And The Cause Of Light Emission In Single-Bubble Sonoluminescence, Brian D. Storey, Andrew J. Szeri
Brian Storey
In single-bubble sonoluminescence, repeated brief flashes of light are produced in a gas bubble strongly driven by a periodic acoustic field. A startling hypothesis has been made by Lohse and co-workers [Phys. Rev. Lett. 78, 1359 (1997)] that the non-noble gases in an air bubble undergo chemical reaction into soluble products, leaving only argon. In the present work, this dissociation hypothesis is supported by simulations, although the associated temperatures of about 7000 K seem too low for bremsstrahlung, which has been proposed as the dominant light emission mechanism. This suggests that emission from water vapor and its reaction products, heretofore …
Shape Stability Of Sonoluminescence Bubbles: Comparison Of Theory To Experiments, Brian D. Storey
Shape Stability Of Sonoluminescence Bubbles: Comparison Of Theory To Experiments, Brian D. Storey
Brian Storey
Single bubble sonoluminescence (SBSL) is the brief flash of light emitted from a single, stable, acoustically forced bubble. In experiments, the maximum pressure amplitude with which a bubble may be forced is limited by considerations of spherical stability. The traditional linear stability analysis predicts a threshold for SBSL at a much lower pressure amplitude than experimental observations. This work shows that if one constructs an accurate model of the radial dynamics, the traditional linear stability analysis predicts a boundary that is in excellent agreement with experimental data.
Field-Amplified Sample Stacking And Focusing In Nanofluidic Channels, Jess M. Sustarich, Brian D. Storey, Sumita Pennathur
Field-Amplified Sample Stacking And Focusing In Nanofluidic Channels, Jess M. Sustarich, Brian D. Storey, Sumita Pennathur
Brian Storey
Nanofluidic technology is gaining popularity for bioanalytical applications due to advances in both nanofabrication and design. One major obstacle in the widespread adoption of such technology for bioanalytical systems is efficient detection of samples due to the inherently low analyte concentrations present in such systems. This problem is exacerbated by the push for electronic detection, which requires an even higher sensor-local sample concentration than optical detection. This paper explores one of the most common preconcentration techniques, field-amplified sample stacking, in nanofluidic systems in efforts to alleviate this obstacle. Holding the ratio of background electrolyte concentrations constant, the parameters of channel …
Rayleigh-Taylor Instability Of Violently Collapsing Bubbles, Hao Lin, Brian D. Storey, Andrew J. Szeri
Rayleigh-Taylor Instability Of Violently Collapsing Bubbles, Hao Lin, Brian D. Storey, Andrew J. Szeri
Brian Storey
In a classical paper Plesset has determined conditions under which a bubble changing in volume maintains a spherical shape. The stability analysis was further developed by Prosperetti to include the effects of liquid viscosity on the evolving shape modes. In the present work the theory is further modified to include the changing density of the bubble contents. The latter is found to be important in violent collapses where the densities of the gas and vapor within a bubble may approach densities of the liquid outside. This exerts a stabilizing influence on the Rayleigh–Taylor mechanism of shape instability of spherical bubbles. …
Electrohydrodynamic Instabilities In Microchannels With Time Periodic Forcing, David A. Boy, Brian D. Storey
Electrohydrodynamic Instabilities In Microchannels With Time Periodic Forcing, David A. Boy, Brian D. Storey
Brian Storey
In microfluidic applications it has been observed that flows with spatial gradients in electrical conductivity are unstable under the application of sufficiently strong electric fields. These electrohydrodynamic instabilities can drive a nonlinear flow despite the low Reynolds number. Such flows hold promise as a simple mechanism for mixing fluids. In this work, the effect of a time periodic electric field on the instability is explored. The case where an electric field is applied across a diffuse interface of two fluids with varying electrical conductivity is considered. Frequency-dependent behavior is found only in the regime where the instability growth rates are …
Bistability In A Simple Fluid Network Due To Viscosity Contrast, John B. Geddes, Brian D. Storey, David Gardner, Russell T. Carr
Bistability In A Simple Fluid Network Due To Viscosity Contrast, John B. Geddes, Brian D. Storey, David Gardner, Russell T. Carr
Brian Storey
We study the existence of multiple equilibrium states in a simple fluid network using Newtonian fluids and laminar flow. We demonstrate theoretically the presence of hysteresis and bistability, and we confirm these predictions in an experiment using two miscible fluids of different viscosity—sucrose solution and water. Possible applications include blood flow, microfluidics, and other network flows governed by similar principles.
Bulk Electroconvective Instability At High Péclet Numbers, Brian D. Storey, Boris Zaltzman, Isaak Rubinstein
Bulk Electroconvective Instability At High Péclet Numbers, Brian D. Storey, Boris Zaltzman, Isaak Rubinstein
Brian Storey
Bulk electroconvection pertains to flow induced by the action of a mean electric field upon the residual space charge in the macroscopic regions of a locally quasielectroneutral strong electrolyte. For a long time, controversy has existed in the literature as to whether quiescent electric conduction from such an electrolyte into a uniform charge-selective solid, such as a metal electrode or ion exchange membrane, is stable with respect to bulk electroconvection. While it was recently claimed that bulk electroconvective instability could not occur, this claim pertained to an aqueous, low-molecular-weight electrolyte characterized by an order-unity electroconvection Péclet number. In this paper, …
Instability Of Electro-Osmotic Channel Flow With Streamwise Conductivity Gradients, J. Jobim Santos, Brian D. Storey
Instability Of Electro-Osmotic Channel Flow With Streamwise Conductivity Gradients, J. Jobim Santos, Brian D. Storey
Brian Storey
This work considers the stability of an electro-osmotic microchannel flow with streamwise electrical conductivity gradients, a configuration common in microfluidic applications such as field amplified sample stacking. Previous work on such flows has focused on how streamwise conductivity gradients set a nonuniform electro-osmotic velocity which results in dispersion of the conductivity field. However, it has been known for many years that electric fields can couple with conductivity gradients to generate unstable flows. This work demonstrates that at high electric fields such an electrohydrodynamic instability arises in this configuration and the basic mechanisms are explored through numerical simulations. The instability is …
Steric Effects On Ac Electro-Osmosis In Dilute Electrolytes, Brian D. Storey, Lee R. Edwards, Mustafa Sabri Kilic, Martin Z. Bazant
Steric Effects On Ac Electro-Osmosis In Dilute Electrolytes, Brian D. Storey, Lee R. Edwards, Mustafa Sabri Kilic, Martin Z. Bazant
Brian Storey
The current theory of alternating-current electro-osmosis (ACEO) is unable to explain the experimentally observed flow reversal of planar ACEO pumps at high frequency (above the peak, typically 10–100 kHz), low salt concentration (1–1000 μM), and moderate voltage (2–6 V), even taking into account Faradaic surface reactions, nonlinear double-layer capacitance, and bulk electrothermal flows. We attribute this failure to the breakdown of the classical Poisson-Boltzmann model of the diffuse double layer, which assumes a dilute solution of pointlike ions. In spite of low bulk salt concentration, the large voltage induced across the double layer leads to crowding of the ions and …
A Depth-Averaged Electrokinetic Flow Model For Shallow Microchannels, Hao Lin, Brian D. Storey, Juan G. Santiago
A Depth-Averaged Electrokinetic Flow Model For Shallow Microchannels, Hao Lin, Brian D. Storey, Juan G. Santiago
Brian Storey
Electrokinetic flows with heterogeneous conductivity configuration occur widely in microfluidic applications such as sample stacking and multidimensional assays. Electromechanical coupling in these flows may lead to complex flow phenomena, such as sample dispersion due to electro-osmotic velocity mismatch, and electrokinetic instability (EKI). In this work we develop a generalized electrokinetic model suitable for the study of microchannel flows with conductivity gradients and shallow-channel geometry. An asymptotic analysis is performed with the channel depth-to-width ratio as a smallness parameter, and the three-dimensional equations are reduced to a set of depth-averaged equations governing in-plane flow dynamics. The momentum equation uses a Darcy–Brinkman–Forchheimer-type …
Reverse Logic - Safety Of Spent Nuclear Fuel Disposal, Antti Lempinen, Marianne Silvan-Lempinen
Reverse Logic - Safety Of Spent Nuclear Fuel Disposal, Antti Lempinen, Marianne Silvan-Lempinen
Antti Lempinen
No abstract provided.
Absolute Ground-State Nitrogen Atom Density In A N2/Ch4 Late Afterglow: Talif Experiments And Modelling Studies, Et. Es-Sebbar, M.-C. Gazeau, Y. Benilan, A. Jolly, C D. Pintassilgo
Absolute Ground-State Nitrogen Atom Density In A N2/Ch4 Late Afterglow: Talif Experiments And Modelling Studies, Et. Es-Sebbar, M.-C. Gazeau, Y. Benilan, A. Jolly, C D. Pintassilgo
Dr. Et-touhami Es-sebbar
Following a first study on a late afterglow in flowing pure nitrogen post discharge, we report new two-photon absorption laser-induced fluorescence (TALIF) measurements of the absolute ground-state atomic nitrogen density N(4S) and investigate the influence of methane introduced downstream from the discharge by varying the CH4 mixing ratio from 0% up to 50%. The N (4S) maximum density is about 2.2 × 1015 cm−3 in pure N2 for a residence time of 22 ms and does not change significantly for methane mixing ratio up to ~15%, while above, a drastic decrease is observed. The influence of the residence time has …
Experimental And Theoretical Studies On Nitrogen Plasma And Methane Photolysis: Implications For Laboratory Simulations Of Titan’S Atmosphere, M-C. Gazeau, Y. Benilan, E. Arzoumanian, Et. Es-Sebbar, A. Jolly
Experimental And Theoretical Studies On Nitrogen Plasma And Methane Photolysis: Implications For Laboratory Simulations Of Titan’S Atmosphere, M-C. Gazeau, Y. Benilan, E. Arzoumanian, Et. Es-Sebbar, A. Jolly
Dr. Et-touhami Es-sebbar
No abstract provided.
Spectroscopic Studies Applied To Uvis Observations Of Titan, Y. Benilan, F. Capalbo, Et. Es-Sebbar, N. Fray, A. Jolly, M-C. Gazeau, J-C. Guillemin, M. Schwell
Spectroscopic Studies Applied To Uvis Observations Of Titan, Y. Benilan, F. Capalbo, Et. Es-Sebbar, N. Fray, A. Jolly, M-C. Gazeau, J-C. Guillemin, M. Schwell
Dr. Et-touhami Es-sebbar
No abstract provided.
Talif Investigation And Modelling Of The Absolute N(4s) Density In A N2-Ch4 Late Afterglow, C.D. Pintassilgo, Et. Es-Sebbar, Y. Benilan, M-C. Gazeau, A. Jolly
Talif Investigation And Modelling Of The Absolute N(4s) Density In A N2-Ch4 Late Afterglow, C.D. Pintassilgo, Et. Es-Sebbar, Y. Benilan, M-C. Gazeau, A. Jolly
Dr. Et-touhami Es-sebbar
The purpose of the present work is the experimental and numerical study of the absolute ground-state nitrogen atoms density N(4S) in the late afterglow of a pure N2 flowing microwave discharge in which different amounts of CH4 have been injected at 25 cm downstream from the nitrogen discharge. The absolute N(4S) concentrations have been measured using Two-photon Absorption Laser-Induced Fluorescence (TALIF), while a detailed kinetic model has been developed to simulate both the discharge and the post-discharge regions. Theoretical predictions are then compared to experimental measurements.
Combined Experimental And Theoretical Studies On Methane Photolysis At 121.6 Nm And 248 Nm- Implications On A Program Of Laboratory Simulations Of Titan’S Atmosphere, C. Romanzin, E. Arzoumanian, Et. Es-Sebbar, A. Jolly, S. Perrier, M.-C. Gazeau, Y. Bénilan
Combined Experimental And Theoretical Studies On Methane Photolysis At 121.6 Nm And 248 Nm- Implications On A Program Of Laboratory Simulations Of Titan’S Atmosphere, C. Romanzin, E. Arzoumanian, Et. Es-Sebbar, A. Jolly, S. Perrier, M.-C. Gazeau, Y. Bénilan
Dr. Et-touhami Es-sebbar
Methane is, together with N2, the main precursor of Titan’s atmospheric chemistry. In our laboratory, we are currently developing a program of laboratory simulations of Titan’s atmosphere, where methane is intended to be dissociated by multiphotonic photolysis at 248 nm. A preliminary study has shown that multiphotonic absorption of methane at 248 nm is efficient and leads to the production of hydrocarbons such as C2H2 (Romanzin et al., 2008). Yet, at this wavelength, little is known about the branching ratios of the hydrocarbon radicals (CH3, CH2 and CH) and their following photochemistry. This paper thus aims at investigating methane photochemistry …
Temperature-Dependent Photoabsorption Cross-Section Of Cyano-Diacetylene In The Vacuum Uv, N. Fray, Y. Bénilan, M.-C. Gazeau, A. Jolly, M. Schwell, E. Arzoumanian, Et. Es-Sebbar, T. Ferradaz, J.- C. Guillemin
Temperature-Dependent Photoabsorption Cross-Section Of Cyano-Diacetylene In The Vacuum Uv, N. Fray, Y. Bénilan, M.-C. Gazeau, A. Jolly, M. Schwell, E. Arzoumanian, Et. Es-Sebbar, T. Ferradaz, J.- C. Guillemin
Dr. Et-touhami Es-sebbar
Using synchrotron radiation as a tunable VUV light source, we have measured, for the first time, the absolute photoabsorption cross sections of HC5N with a spectral resolution of 0.05 nm in the region between 80 and 205 nm from 233 to 298 K. The measured cross sections are used to predict the HC5N photodestruction rate in the solar system and to model a transmission spectrum in Titan's atmosphere. Comparing the latter with that acquired by the Ultraviolet Imaging Spectrograph on board the Cassini spacecraft, we have determined an upper limit of 2.7 × 10−5 on the HC5N abundance at 1100 …
Absolute Nitrogen Atom Density Measurements By Two-Photon Laser-Induced Fluorescence Spectroscopy In Atmospheric Pressure Dielectric Barrier Discharges Of Pure Nitrogen, Et-Touhami Es-Sebbar, Christian Sarra-Bournet, Nicolas Naudé, Françoise Massines, Nicolas Gherardi
Absolute Nitrogen Atom Density Measurements By Two-Photon Laser-Induced Fluorescence Spectroscopy In Atmospheric Pressure Dielectric Barrier Discharges Of Pure Nitrogen, Et-Touhami Es-Sebbar, Christian Sarra-Bournet, Nicolas Naudé, Françoise Massines, Nicolas Gherardi
Dr. Et-touhami Es-sebbar
In this paper, two-photon absorption laser induced fluorescence spectroscopy is used to follow the nitrogen atom density in flowing dielectric barrier discharges fed with pure nitrogen and operating at atmospheric pressure. Two different dielectric barrier discharge regimes are investigated: the Townsend regime, which is homogeneous although operating at atmospheric pressure, and the more common filamentary regime. In both regimes, densities as high as 3x1014 /cm3 are detected. However, the N atoms kinetic formation depends on the discharge regime. The saturation level is reached more rapidly with a filamentary discharge. For a given discharge regime, the N atom density depends strongly …
Contributions To The Development Of The S.E.T.U.P. (Experimental And Theoretical Simulations Useful For Planetology) Project, E. Arzoumanian, C. Romanzin, M-C. Gazeau, Et. Es-Sebbar, A. Jolly, S. Perrier, Y. Benilan
Contributions To The Development Of The S.E.T.U.P. (Experimental And Theoretical Simulations Useful For Planetology) Project, E. Arzoumanian, C. Romanzin, M-C. Gazeau, Et. Es-Sebbar, A. Jolly, S. Perrier, Y. Benilan
Dr. Et-touhami Es-sebbar
No abstract provided.
Multiwavelength Studies For Titan's Atmospheric Composition Analysis, Y. Benilan, Et. Es-Sebbar, N. Fray, M-C. Gazeau, A. Jolly, M. Schwell, J. Guillemin
Multiwavelength Studies For Titan's Atmospheric Composition Analysis, Y. Benilan, Et. Es-Sebbar, N. Fray, M-C. Gazeau, A. Jolly, M. Schwell, J. Guillemin
Dr. Et-touhami Es-sebbar
Titan's atmosphere mainly made of nitrogen and methane is rich in organic molecules. Hydrocarbons are formed from the photolytic dissociation of CH4 and nitriles are created by dissociation of N2 followed by reactions with hydrocarbons. In order to understand the physicochemical mechanisms responsible for the evolution of Titan's atmosphere, photochemical models are built. The latter need constrains for vertical profiles of organic compounds from the high thermosphere down to the low stratosphere as well as photodissociation rates. Those profiles over the entire atmosphere can be retrieved from Cassini observations, in particular by limb sounding, coupling infrared and ultraviolet spectroscopy. However, …
Vuv Photostability Of Prebiotic Species, M. Schwell, Y. Bénilan, M.-C. Gazeau, N. Fray, A. Jolly, Et. Es-Sebbar, N. Champion, S. Leach, H. W Jochims, H. Baumgärtel, E. Rühl
Vuv Photostability Of Prebiotic Species, M. Schwell, Y. Bénilan, M.-C. Gazeau, N. Fray, A. Jolly, Et. Es-Sebbar, N. Champion, S. Leach, H. W Jochims, H. Baumgärtel, E. Rühl
Dr. Et-touhami Es-sebbar
No abstract provided.
S.E.T.U.P. Experimental And Theoretical Simulations Useful For Planetology- Related Studies In The Frame Of A Program Of Titan’S Atmosphere Laboratory Simulations, M.-C. Gazeau, Et. Es-Sebbar, E. Arzoumanian, C. Romanzin, A. Jolly, S. Perrier, Y. Bénilan
S.E.T.U.P. Experimental And Theoretical Simulations Useful For Planetology- Related Studies In The Frame Of A Program Of Titan’S Atmosphere Laboratory Simulations, M.-C. Gazeau, Et. Es-Sebbar, E. Arzoumanian, C. Romanzin, A. Jolly, S. Perrier, Y. Bénilan
Dr. Et-touhami Es-sebbar
No abstract provided.
Characterization Of An N2 Flowing Microwave Post-Discharge By Oes Spectroscopy And Determination Of Absolute Ground-State Nitrogen Atom Densities By Talif, Et. Es-Sebbar, Y. Benilan, A. Jolly, M-C. Gazeau
Characterization Of An N2 Flowing Microwave Post-Discharge By Oes Spectroscopy And Determination Of Absolute Ground-State Nitrogen Atom Densities By Talif, Et. Es-Sebbar, Y. Benilan, A. Jolly, M-C. Gazeau
Dr. Et-touhami Es-sebbar
A flowing microwave post-discharge source sustained at 2.45 GHz in pure nitrogen has been investigated by optical emission spectroscopy (OES) and two-photon absorption laser-induced fluorescence (TALIF) spectroscopy. Variations of the optical emission along the post-discharge (near, pink and late afterglow) have been studied and the gas temperature has been determined. TALIF spectroscopy has been used in the late afterglow to determine the absolute ground-state nitrogen atomic densities using krypton as a reference gas. Measurements show that the microwave flowing post-discharge is an efficient source of N (4S) atoms in late afterglow. In our experimental conditions, the maximum N (4S) density …