Physics Commons^™

Exciton Coherence In 1d Phthalocyanine Based Organic Crystalline Thin Films, Kimngan Burrill

Graduate College Dissertations and Theses

Quantum coherence plays a vital role in the excitonic properties of organic semiconductors. Several theoretical and experimental studies have shown an unprecedented role of coherence in charge transfer and transport processes, which in turn can improve the performance of electronic devices. Specifically, an enhancement of exciton coherence size can result in fast energy transport and efficient charge separation. The ability to tailor the design and performance of organic electronics based on exciton coherence effects represents the possibility of ultrafast electronic applications in communication and information technology.

The objective of this thesis is the excitonic coherence studies of 1D crystalline thin …

Generating Electromagnetic Schell-Model Sources Using Complex Screens With Spatially Varying Auto- And Cross-Correlation Functions, Milo W. Hyde Iv

Faculty Publications

We present a method to generate any physically realizable electromagnetic Schell-model source. Our technique can be directly implemented on existing vector-beam generators that utilize spatial light modulators for coherence control, beam shaping, and relative phasing. This work significantly extends published research on the subject, where control over the partially coherent source’s cross-spectral density matrix was limited. We begin by presenting the statistical optics theory necessary to derive and implement our method. We then apply our technique, both analytically and in simulation, to produce two electromagnetic Schell-model sources from the literature. We demonstrate control over the full cross-spectral density matrices of …

Digital Holography Efficiency Experiments For Tactical Applications, Douglas E. Thornton

Theses and Dissertations

Digital holography (DH) uses coherent detection and offers direct access to the complex-optical field to sense and correct image aberrations in low signal-to-noise environments, which is critical for tactical applications. The performance of DH is compared to a similar, well studied deep-turbulence wavefront sensor, the self-referencing interferometer (SRI), with known efficiency losses. Wave optics simulations with deep-turbulence conditions and noise were conducted and the results show that DH outperforms the SRI by 10's of dB due to DH's strong reference. Additionally, efficiency experiments were conducted to investigate DH system losses. The experimental results show that the mixing efficiency (37%) is …

Near-Field Effects On Partially Coherent Light Scattered By An Aperture, Milo W. Hyde Iv, Michael J. Havrilla

Faculty Publications

We investigate how the near field affects partially coherent light scattered from an aperture in an opaque screen. Prior work on this subject has focused on the role of surface plasmons, and how they affect spatial coherence is well documented. Here, we consider other near-field effects that might impact spatial coherence. We do this by examining the statistics of the near-zone field scattered from an aperture in a perfect electric conductor plane—a structure that does not support surface plasmons. We derive the near-field statistics (in particular, cross-spectral density functions) by applying electromagnetic equivalence theorems and the Method of Moments. We …

Free Electron Sources And Diffraction In Time, Eric R. Jones

Department of Physics and Astronomy: Dissertations, Theses, and Student Research

The quantum revolution of the last century advanced synergistically with technology, for example, with control of the temporal and spatial coherence, and the polarization state of light. Indeed, experimental confirmation of the quirks of quantum theory, as originally highlighted by Einstein, Podolsky, and Rosen, through Bohm, and then Bell, have been performed with photons, i.e., electromagnetic wave packets prepared in the same quantum states. Experimental tests of quantum mechanics with matter wave packets have been limited due to challenges in preparing all of the packets with similar quantum states. While great strides have been made for trapped atoms and Bose-Einstein …

Shaping The Far-Zone Intensity, Degree Of Polarization, Angle Of Polarization, And Ellipticity Angle Using Vector Schell-Model Sources, Milo W. Hyde Iv

Faculty Publications

This paper presents a method to control both the shape and polarization of a beam in the far field using a vector Schell-model source. Given a desired far-zone beam shape and polarization, and applying Fourier and statistical optics theory, we derive the requisite second-order moments of said source, discuss what aspects of the far-zone beam can be controlled, and develop a step-by-step procedure for synthesizing the required random vector field instances. We validate this approach with Monte-Carlo wave-optics simulations. The results are found to be in very good agreement with the desired far-zone beam characteristics. The beam-shaping technique developed in …

Power-Law Schell-Model Sources, Milo W. Hyde Iv

Faculty Publications

A new type of Schell-model source is developed that has a spectral degree of coherence, or spatial power spectrum, which is described by a power-law function. These power-law sources generally produce cusped, or peaked far-zone spectral density patterns making them potentially useful in directed energy applications. The spectral degrees of coherence, spatial power spectra, and spatial coherence radii for power-law sources are derived and discussed. Two power-law sources are then synthesized in the laboratory using a liquid crystal spatial light modulator. The experimental spectral densities are compared to the corresponding theoretical predictions to serve as a proof of concept.

Synthesizing Time-Evolving Partially-Coherent Schell-Model Sources, Noah R. Van Zandt, Milo W. Hyde Iv, Santasri Bose-Pillai, David G. Voelz, Xifeng Xiao, Steven T. Fiorino

Faculty Publications

Time-evolving simulation of sources with partial spatial and temporal coherence is sometimes instructive or necessary to explain optical coherence effects. Yet, existing time-evolving synthesis techniques often require prohibitive amounts of computer memory. This paper discusses three methods for the synthesis of continuous or pulsed time-evolving sources with nearly arbitrary spatial and temporal coherence. One method greatly reduces computer memory requirements, making this type of synthesis more practical. The utility of all three methods is demonstrated via a modified form of Young's experiment. Numerical simulation and laboratory results for time-averaged irradiance are presented and compared with theory to validate the synthesis …

Quantum Coherence And Entanglement In Open Quantum Systems, Yiteng Zhang

Open Access Dissertations

We humans always want to believe that we can overpower nature. However, the reality is that nature outperforms humans in many aspects. Animals' abilities to navigate/orient and photosynthesis are two excellent examples in these aspects. However, the mechanisms underlying them are still unknown. For decades, scientists and researchers have made a lot of efforts to reveal these mysteries in nature.

Recently, quantum coherence and entanglement are believed to play a crucial role in such biological systems–avian compass and photosynthesis. Thus, nature might know more tricks to utilize quantum mechanics than humans. Studies on the mechanisms underlying avian compass and photosynthesis …

Quantum And Classical Optics–Emerging Links, Joseph H. Eberly, Xiao-Feng Qian, Asma Al Qasimi, Hazrat Ali, M. A. Alonso, R Gutiérrez-Cuevas, Bethany Little, John C. Howell, Tanya Malhotra, A. N. Vamivakas

Mathematics, Physics, and Computer Science Faculty Articles and Research

Quantum optics and classical optics are linked in ways that are becoming apparent as a result of numerous recent detailed examinations of the relationships that elementary notions of optics have with each other. These elementary notions include interference, polarization, coherence, complementarity and entanglement. All of them are present in both quantum and classical optics. They have historic origins, and at least partly for this reason not all of them have quantitative definitions that are universally accepted. This makes further investigation into their engagement in optics very desirable. We pay particular attention to effects that arise from the mere co-existence of …

The Quest For High Power Lasers: Forcing Mutual Coherence In Broad Area Diode Lasers, Jonathan R. Wurtz

Student Research Projects

This poster explains efforts to improve spatial beam quality of diode array stacks using an external optical feedback system to force coherence of individual diodes.

Quantumness And Coherence In Photosynthesis, Brian Doolittle

Honors Theses

Long-lived oscillations lasting up to 1800 fs have been observed in the Fenna--Mathews--Olsen (FMO) Pigment-Protein complex. It is unclear if the oscillations are quantum or classical in origin. Quantized intra-pigment normal modes are responsible for these long-lived oscillations. In this thesis we simulate a bacteriachlorophyll dimer in the FMO Complex at physiological conditions. Our model describes two electronically coupled pigments coupled to the vibrational protein environment. Our goal is to find system parameters that allow long-lived quantum coherences to exist in photosynthetic complexes. We calculate the time evolution of our system's density matrix using the numerically exact quantum adiabatic path …

Forcing Mutual Coherence In Diode Laser Stacks, Jonathan R. Wurtz

Honors Theses and Capstones

This paper will discuss both theoretical and experimental attempts to improve the spatial beam quality of diode laser stacks using an external optical system. An overview and derivation of the mathematics of both the optical system and diode lasers will be discussed. The experimental setup will be presented, as well as the fundamental theoretical and experimental results that suggest the external optical system used for this thesis fails to improve the beam quality of a diode laser stack.

Scan-Based Near-Field Acoustical Holography On Partially Correlated Sources, Michael D. Gardner

Theses and Dissertations

Scan-based near-field acoustical holography (NAH) is applied to partially correlated sources. Partial field decomposition via the virtual coherence method is used to implement the scan-based NAH. The background and theory of these methods are developed. Multiple stationary reference microphones are required for the partial field decomposition. Guidelines for reference microphone placement in the literature thus far have been limited. Improved guidelines for reference microphones are given after the results of two sets of experiments. The first set involves discrete, partially correlated sources, both physical and numerical. The second set of experiments is strictly numerical and involves continuous sources. Fewer microphones …

Effects Of Polarization And Coherence On The Propagation And The Detection Of Stochastic Electromagnetic Beams, Mohamed Fouad Salem

Electronic Theses and Dissertations

Most of the physically realizable optical sources are radiating in a random manner given the random nature of the radiation of a large number of atoms that constitute the source. Besides, a lot of natural and synthetic materials are fluctuating randomly. Hence, the optical fields that one encounters, in most of the applications are fluctuating and must be treated using random or stochastic functions. Within the framework of the scalar-coherence theory, one can describe changes of the properties of any stochastic field such as the spectral density and the spectral degree of coherence on propagation in any linear medium, deterministic …

On The Use Of Variable Coherence In Inverse Scattering Problems, Erwan Baleine

Electronic Theses and Dissertations

Even though most of the properties of optical fields, such as wavelength, polarization, wavefront curvature or angular spectrum, have been commonly manipulated in a variety of remote sensing procedures, controlling the degree of coherence of light did not find wide applications until recently. Since the emergence of optical coherence tomography, a growing number of scattering techniques have relied on temporal coherence gating which provides efficient target selectivity in a way achieved only by bulky short pulse measurements. The spatial counterpart of temporal coherence, however, has barely been exploited in sensing applications. This dissertation examines, in different scattering regimes, a variety …

Diffuse Light Scattering Dynamics Under Conditions Of Electromagnetically Induced Transparency, V. M. Datsyuk, I. M. Sokolov, D. V. Kupriyanov, M. D. Havey

Physics Faculty Publications

We show that under conditions of electromagnetically induced transparency (EIT) in an ultracold atomic sample in a magneto-optical trap, a significant portion of the incident probe pulse is transferred into Rayleigh and Raman scattering channels. The light scattered into the Rayleigh channel emerges from the sample with an EIT time delay. We show that a proper description of the probe light propagation in the sample should include, in the diffusion dynamics, a spin polariton generated by the two-photon EIT process. The results have important implications for studies of weak light localization and for manipulation of single and few photon states …

Coherence Properties Of Optical Near-Fields, Adela Apostol

Electronic Theses and Dissertations

Next generation photonics-based technologies will ultimately rely on novel materials and devices. For this purpose, phenomena at subwavelength scales are being studied to advance both fundamental knowledge and experimental capabilities. In this dissertation, concepts specific to near-field optics and experimental capabilities specific to near-field microscopy are used to investigate various aspects of the statistical properties of random electromagnetic fields in the vicinity of optically inhomogeneous media which emit or scatter radiation. The properties of such fields are being characterized within the frame of the coherence theory. While successful in describing the far-field properties of optical fields, the fundamental results of …

Multiple Scattering Of Light In Inhomogeneous Media And Applications, Claudia Mujat

Electronic Theses and Dissertations

Light scattering-based techniques are being developed for non-invasive diagnostics of inhomogeneous media in various fields, such as medicine, biology, and material characterization. However, as most media of interest are highly scattering and have a complex structure, it is difficult to obtain a full analytical solution of the scattering problem without introducing approximations and assumptions about the properties of the system under consideration. Moreover, most of the previous studies deal with idealized scattering situations, rarely encountered in practice. This dissertation provides new analytical, numerical, and experimental solutions to describe subtle effects introduced by the properties of the light sources, and by …

Polarimetric Characterization Of Random Electromagnetic Beams And Applications, Mircea Mujat

Electronic Theses and Dissertations

Polarimetry is one of the principal means of investigating the interaction of light with matter. Theoretical models and experimental techniques are presented in this dissertation for polarimetric characterization of random electromagnetic beams and of signatures of random media in different scattering regimes and configurations. The degree of polarization rather than the full description of the state of polarization is of interest in multiple scattering and free space propagation where the statistical nature and not the deterministic component of light bears the relevant information. A new interferometric technique for determining the degree of polarization by measuring the intensity fluctuations in a …

A Simple Description Of Coherence, William Moebs, Jeff Sanny

Physics Faculty Works

No abstract provided.