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Full-Text Articles in Physics
Vibrational State Resolved Lifetimes Of The Na2 21Σ+U Double Well State, Seth T. Ashman, Lutz Huwel, Roy Anunciado, Nadeepa Jayasundara
Vibrational State Resolved Lifetimes Of The Na2 21Σ+U Double Well State, Seth T. Ashman, Lutz Huwel, Roy Anunciado, Nadeepa Jayasundara
Engineering & Physics Faculty Publications
Lifetimes of individual Na2 ro-vibrational levels of the 21Σ + u double well-state have been measured using a delayed photoionization technique. Ground state Na2 produced in a molecular beam is excited resonantly by the doubled output of a pulsed dye laser in the range 333 – 357 nm and then ionized by a 532 nm photon from a time-delayed Nd:YAG laser. By appropriate excitation laser tuning and systematic variation of the probe laser delay, ro-vibrational level resolved lifetimes are obtained for v=25- 49. The double well state lifetime values are found to decrease from about 50 ns at v=25 to …
Comparison Of Absorption, Fluorescence, And Polarization Spectroscopy Of Atomic Rubidium, Seth T. Ashman, Cayla Stifler, Joaquin Romero
Comparison Of Absorption, Fluorescence, And Polarization Spectroscopy Of Atomic Rubidium, Seth T. Ashman, Cayla Stifler, Joaquin Romero
Engineering & Physics Faculty Publications
An ongoing spectroscopic investigation of atomic rubidium utilizes a two-photon, single-laser excitation process. Transitions accessible with our tunable laser include 5P1/2 (F ′ ) ← 5S1/2 (F) and 5P3/2 (F ′ ) ← 5S1/2 (F). The laser is split into a pump and probe beam to allow for Doppler-free measurements of transitions between hyperfine levels. The pump and probe beams are overlapped in a counter-propagating geometry and the laser frequency scans over a transition. Absorption, fluorescence and polarization spectroscopy techniques are applied to this basic experimental setup. The temperature of the vapor cell and the power of the pump and …
Collisional Transfer Of Population And Orientation In Nak, Seth T. Ashman, C. M. Wolfe, J. Huennekens, B. Beser, J. Bai, A. M. Lyyra
Collisional Transfer Of Population And Orientation In Nak, Seth T. Ashman, C. M. Wolfe, J. Huennekens, B. Beser, J. Bai, A. M. Lyyra
Engineering & Physics Faculty Publications
We report current work to study transfer of population and orientation in collisions of NaK molecules with argon and potassium atoms using polarization labeling (PL) and laser- induced fluorescence (LIF) spectroscopy. In the PL experiment, a circularly polarized pump laser excites a specific NaK A1Σ +(v 0=16, J 0 ) ← X1Σ +(v 00=0, J 0 ± 1) transition, creating an orientation (non-uniform MJ0 level distribution) in both levels. The linearly polarized probe laser is scanned over various 31Π(v, J 0±1) ← A1Σ +(v 0=16, J 0 ) transitions. The probe laser passes through a crossed linear polarizer before detection, …
Experimental Studies Of The Nacs 53Π0 And 1(A)3Σ+ States, Seth T. Ashman, Brett Mcgeehan, Christopher Wolfe, Carl Faust, John Huennekens
Experimental Studies Of The Nacs 53Π0 And 1(A)3Σ+ States, Seth T. Ashman, Brett Mcgeehan, Christopher Wolfe, Carl Faust, John Huennekens
Engineering & Physics Faculty Publications
We present experimental studies of the NaCs molecule that are currently underway in our laboratory. The opticaloptical double resonance method is used to obtain Doppler-free excitation spectra for several excited states. Selected data from the 53Π0 electronic state are used to obtain Rydberg-Klein-Rees (RKR) and Inverse Perturbation Approach (IPA) potential curves. We are also mapping the repulsive wall of the 1(a) 3Σ +potential using many resolved bound-free fluorescence spectra from individual ro-vibrational levels of the 53Π0 electronic state to the 1(a) 3Σ + state. Using the determined 53Π0 state potential we fit the repulsive wall of the 1(a) 3Σ + …
Experimental Studies Of Nacs, Seth T. Ashman, C. M. Wolfe, J. P. Huennekens
Experimental Studies Of Nacs, Seth T. Ashman, C. M. Wolfe, J. P. Huennekens
Engineering & Physics Faculty Publications
We present experimental studies of excited electronic states of the NaCs molecule that are currently underway in our laboratory. The optical-optical double resonance method is used to obtain Doppler-free excitation spectra for several excited states. These data are being used to obtain RydbergKlein-Rees (RKR) or Inverse Perturbation Approach (IPA) potential curves for these states. We are also trying to map the bound portion of the 1(a) 3Σ + potential using resolved laser-induced fluorescence and Fourier transform spectroscopy to record transitions into the shallow well. Bound-free spectra from single ro-vibrational levels of electronically excited states to the repulsive wall of the …
Polarization Spectroscopy And Collisions In Nak, Seth T. Ashman, C. M. Wolfe, J. Huennekens, B. Beser, J. Bai, A. M. Lyyra
Polarization Spectroscopy And Collisions In Nak, Seth T. Ashman, C. M. Wolfe, J. Huennekens, B. Beser, J. Bai, A. M. Lyyra
Engineering & Physics Faculty Publications
We report current work to study transfer of population and orientation in collisions of NaK molecules with argon and potassium atoms using polarization labeling (PL) and laser-induced fluorescence (LIF) spectroscopy. In the PL experiment, a circularly polarized pump laser excites a specific NaK A1Σ +(v=16, J) ← X1Σ +(v=0, J ± 1) transition, creating an orientation (non-uniform MJ level distribution) in both levels. The linear polarized probe laser is scanned over various 3 1Π(v=8, J 0 ± 1) ← A1Σ +(v=16, J 0 ) transitions. The probe laser passes through a crossed linear polarizer before detection, and signal is recorded …