Physics Commons^™

Superhalogen Properties Of Cumcln Clusters: Theory And Experiment, Y. J. Ko, H. Wang, K. Pradhan, P. Koirala, Anil K. Kandalam, K. H. Bowen, P. Jena

Physics & Engineering Faculty Publications

No abstract provided.

Dipole-Dipole Interaction Between Rubidium Rydberg Atoms, Emily Altiere, Donald P. Fahey, Michael W. Noel, Rachel J. Smith, Thomas J. Carroll

Physics and Astronomy Faculty Publications

Ultracold Rydberg atoms in a static electric field can exchange energy via the dipole-dipole interaction. The Stark effect shifts the energy levels of the atoms which tunes the energy exchange into resonance at specific values of the electric field (F¨orster resonances). We excite rubidium atoms to Rydberg states by focusing either a 480 nm beam from a tunable dye laser or a pair of diode lasers into a magneto-optical trap. The trap lies at the center of a configuration of electrodes. We scan the electric field by controlling the voltage on the electrodes while measuring the fraction of atoms that …

Equation Of State From The Potts-Percolation Model Of A Solid, Miron Kaufman

Physics Faculty Publications

We expand the Potts-percolation model of a solid to include stress and strain. Neighboring atoms are connected by bonds. We set the energy of a bond to be given by the Lennard-Jones potential. If the energy is larger than a threshold the bond is more likely to fail, whereas if the energy is lower than the threshold, the bond is more likely to be alive. In two dimensions we compute the equation of state: stress as a function of interatomic distance and temperature by using renormalization-group and Monte Carlo simulations. The phase diagram, the equation of state, and the isothermal …

Dc Pulsed Atmospheric Pressure Plasma Jet Image Information, Denis P. Dowling, F T. O'Neill, Vladimir Milosavljevic, Victor J. Law

Articles

This paper presents optical imaging and optical emission spectroscopy (OES) data of an atmospheric-pressure plasma jet. It is shown how the visual information and OES information of the air discharge are related as the blown arc extends from the nozzle (2-4 mm) with a molecular nitrogen rotational temperature on the order of 1700 K and the flowing afterglow beyond this region is dominated by the cooler (300-K) NO-O chemiluminescent reaction that produces NO₂ species.

Wave-Function Functionals For The Density, Marlina Slamet, Xiao-Yin Pan, Viraht Sahni

Publications and Research

We extend the idea of the constrained-search variational method for the construction of wave-function functionals psi[chi] of functions chi. The search is constrained to those functions chi such that psi[chi] reproduces the density rho(r) while simultaneously leading to an upper bound to the energy. The functionals are thereby normalized and automatically satisfy the electron-nucleus coalescence condition. The functionals psi[chi] are also constructed to satisfy the electron-electron coalescence condition. The method is applied to the ground state of the helium atom to construct functionals psi[chi] that reproduce the density as given by the Kinoshita correlated wave function. The expectation of single-particle …

Photoelectron Spectroscopic Study Of Iron-Pyrene Cluster Anions, Xiang Li, Kit H. Bowen Jr., Puru Jena, Anil K. Kandalam

Physics & Engineering Faculty Publications

No abstract provided.

Structural Evolution And Stabilities Of Neutral And Anionic Clusters Of Lead Sulfide: Joint Anion Photoelectron And Computational Studies, Pratik Koirala, Boggavarapu Kiran, Anil K. Kandalam, Charles A. Fancher, Helen L. De Clercq, Xiang Li, Kit H. Bowen

Physics & Engineering Faculty Publications

No abstract provided.

Hydrogen Donors And Ti3+ Ions In Reduced Tio2 Crystals, A. T. Brant, Shan Yang (杨山), Nancy C. Giles, Larry E. Halliburton

Faculty Publications

Electron paramagnetic resonance (EPR) and electron-nuclear double resonance (ENDOR) are used to identify and characterize the neutral hydrogen donor in TiO₂ crystals having the rutile structure. These spectra are best observed near 5 K. The neutral donors are present without photoexcitation in crystals that have been slightly reduced at high temperature in a nitrogen atmosphere. The same defects can be photoinduced at low temperature in oxidized crystals. The neutral hydrogen donor in this lattice consists of a substitutional Ti³⁺ ion adjacent to a substitutional OH^– molecular ion. The axis of the OH^– molecule lies in the …

The Role Of Llnl's Fast Calibration Facility In Diagnosing Nif Fusion Plasmas, Joshua G. Thompson, Carey Scott, Greg V. Brown

STAR Program Research Presentations

The Fusion and Astrophysics (FAST) Calibration and Diagnostic Facility uses the original Electron Beam Ion Trap (EBIT-I) to profile x-ray filters that are used in the Dante Soft X-Ray Diagnostic at the National Ignition Facility (NIF). FAST has an advantage over any other facility not only for its high accuracy, but also for its proximity to NIF in the Lawrence Livermore National Laboratory (LLNL). This makes for highly accurate and near-instantaneous filter calibration turnover.

EBIT-I was first constructed to create, trap, and observe static highly charged ions (HCIs) and conduct experimental astrophysics (creating an x-ray spectroscopy catalogue of ions). To …

Laboratory Astrophysics: Using Ebit Measurements To Interpret High Resolution Spectra From Celestial Sources, Carey Scott, Joshua Thompson, N. Hell, Greg V. Brown

STAR Program Research Presentations

Astrophysicists use radiation to investigate the physics controlling a variety of celestial sources, including stellar atmospheres, black holes, and binary systems. By measuring the spectrum of the emitted radiation, astrophysicists can determine a source’s temperature and composition. Accurate atomic data are needed for reliably interpreting these spectra. Here we present an overview of how LLNL’s EBIT facility is used to put the atomic data on sound footing for use by the high energy astrophysics community.

Laser-Wakefield Accelerators: Glass-Guiding Benefits, Donald P. Umstadter

Donald Umstadter Publications

A main attraction of laser-driven electron accelerators is their absence of cavity walls, which can break down in the presence of intense electric fields. Now it seems that the inclusion of a hollow glass fibre cavity could lead to more efficient acceleration at lower laser intensities. ... Further research will reveal which of the above methods for guiding light will ultimately prove best for future accelerator designs. In any case, although it is perhaps ironic that the relatively old technology of glass waveguides may benefit next-generation accelerators, it is nonetheless satisfying to see such a classic photonic solution come to …

Top Quark Rapidity Distribution And Forward-Backward Asymmetry, Nikolaos Kidonakis

Faculty and Research Publications

I present results for the top quark rapidity distribution at Large Hadron Collider and Tevatron energies, including higher-order corrections from threshold resummation. Approximate next-to-next-to-leading-order (NNLO) results are obtained by adding the NNLO soft-gluon corrections at next-to-next-to-leading-logarithm level to the exact next-to-leading-order calculation. Theoretical predictions are shown for the rapidity distribution, including the scale dependence of the distributions. The forward-backward asymmetry at the Tevatron is also calculated.

Causality And Relativistic Localization In One-Dimensional Hamiltonians, R E. Wagner, B T. Shields, M R. Ware, Qichang Su, Rainer Grobe

Faculty publications – Physics

We compare the relativistic time evolution of an initially localized quantum particle obtained from the relativistic Schrodinger, the Klein-Gordon and the Dirac equations. By computing the amount of the spatial probability density that evolves outside the light cone we quantify the amount of causality violation for the relativistic Schrodinger Hamiltonian. We comment on the relationship between quantum field theoretical transition amplitudes, commutators of the fields and their bilinear combinations outside the light cone as indicators of a possible causality violation. We point out the relevance of the relativistic localization problem to this discussion and comment on ideas about the supposed …

Photoassociative Spectroscopy Of Ultracold Metastable Argon, M. K. Shaffer, G. Ranjit, C. I. Sukenik, M. Walhout

University Faculty Publications and Creative Works

We present results of photoassociative spectroscopy performed on ultracold metastable argon atoms in a magneto-optical trap. Ion spectra are obtained with laser detuning up to a few gigahertz below the 4s[3/2]2→4p[5/2] 3 trapping transition at 811 nm and with intensities in a range of ∼(102-105)ISat. We also compute dipole-dipole potentials for both singly and doubly excited diatomic molecules and use a Leroy-Bernstein analysis to determine the approximate vibrational spacings in the (s+p) and (p+p) manifolds. Based on this theoretical framework, we explain a broad background feature in our data and suggest that double-excitation mechanisms are likely responsible for sharp dips …

Next-To-Next-To-Leading-Order Collinear And Soft Gluon Corrections For T-Channel Single Top Quark Production, Nikolaos Kidonakis

Faculty and Research Publications

I present the resummation of collinear and soft-gluon corrections to single top quark production in the t channel at next-to-next-to-leading logarithm accuracy using two-loop soft anomalous dimensions. The expansion of the resummed cross section yields approximate next-to-next-to-leading-order cross sections. Numerical results for t-channel single top quark (or single antitop) production at the Tevatron and the LHC are presented, including the dependence of the cross sections on the top quark mass and the uncertainties from scale variation and parton distributions. Combined results for all single top quark production channels are also given.

Electron-Positron Pair Creation Induced By Quantum-Mechanical Tunneling, M Jiang, W Su, X Lu, Z M. Sheng, Y T. Li, J Zhang, Rainer Grobe, Qichang Su

Faculty publications – Physics

We study the creation of electron-positron pairs from the vacuum induced by two spatially displaced static electric fields. The strength and spatial width of each localized field is less than required for pair creation. If, however, the separation between the fields is less than the quantum-mechanical tunneling length associated with the corresponding quantum scattering system, the system produces a steady flux of electron-positron pairs. We compute the time dependence of the pair-creation probability by solving the Dirac equation numerically for various external field sequences. For the special case of two very narrow fields we provide an analytical expression for the …

The Economics Of The Atomic Bomb: Cost And Utilization, Jonathan M. Davis Mr.

Senior Honors Theses

Few moments in human history can be compared to the culmination of events that brought the atomic bomb into creation. It is incredible to contemplate that while a nation was fighting a two front war that spanned from Europe into the Pacific, that the United States was able to utilize the time, energy, brains, materials, manpower, and capital to complete a project in four years. That under any other circumstances would have taken greater than half a century to complete.

First, this thesis will discuss breakthroughs in research that led scientists to believe that the atomic weapons could be built, …

Oxygen Vacancies Adjacent To Cu(2+) Ions In Tio(2) (Rutile) Crystals, A. T. Brant, Shan Yang (杨山), Nancy C. Giles, Zafar Iqbal, A. Manivannan, Larry E. Halliburton

Faculty Publications

Electron paramagnetic resonance (EPR) and electron-nuclear double resonance (ENDOR) are used to characterize Cu²⁺ ions substituting for Ti⁴⁺ ions in nominally undoped TiO₂ crystals having the rutile structure. Illumination at 25 K with 442 nm laser light reduces the concentration of Cu²⁺ ions by more than a factor of 2. The laser light also reduces the EPR signals from Fe³⁺ and Cr³⁺ ions and introduces signals from Ti³⁺ ions. Warming in the dark to room temperature restores the crystal to its preilluminated state. Monitoring the recovery of the photoinduced changes in the Cu …

Local Origins Of Volume Fraction Fluctuations In Dense Granular Materials, James G. Puckett, Frederic Lechenault, Karen E. Daniels

Physics and Astronomy Faculty Publications

Fluctuations of the local volume fraction within granular materials have previously been observed to decrease as the system approaches jamming.We experimentally examine the role of boundary conditions and interparticle friction μ on this relationship for a dense granular material of bidisperse particles driven under either constant volume or constant pressure.Using a radicalVorono¨ı tessellation, we find the variance of the local volume fraction φ monotonically decreases as the system becomes more dense, independent of boundary condition and μ. We examine the universality and origins of this trend using experiments and the recent granocentric model, modified to draw particle locations from an …

Increased Power And Detuning Of Diode Lasers For Magneto-Optical Trap Of Lithium, Jami Johnson

Honors Student Works

Precision experiments such as laser cooling and trapping using diode laser systems are increasingly prevalent in the fields of modern atomic, molecular and optical physics. Multiple laser diodes of precise frequencies and significant output power are often needed for such research. Here, a method for injection locking a slave laser to a master laser stabilized to an atomic line of lithium is described.The slave laser is a free running diode that is injection-locked by a small portion (2 mW) of the frequency shifted master laser light. Evidence of incomplete injection locking is described, in addition to a technique for improving …

Phase Sensitive Detection: Frequency Locking Of A Laser Diode For Lithium Cooling And Trapping, Brandon Peplinski

Honors Student Works

The frequency of a laser-diode can be locked by providing a negative feedback voltage to the piezo-electric transducer in the laser cavity. By phase-modulating the light and placing side bands on the carrier frequency, the fluorescence of the atoms is modulated. The signal from this fluorescence is phase-sensitively compared with a phase-locked reference signal in a lock-in amplifier, and an asymmetric error signal is produced. With this feedback method a laser-diode is locked within a 75 Mhz doppler-broadened spectroscopic line width. The lock is robust enough to last a few hours at a time and is impervious to high amplitude, …

Structures And Photoelectron Spectroscopy Of Cun(Bo2)M− (N, M = 1, 2) Clusters: Observation Of Hyperhalogen Behavior, Yuan Feng, Hong-Guang Xu, Weijun Zheng, Hongmin Zhao, Anil K. Kandalam, Puru Jena

Physics & Engineering Faculty Publications

No abstract provided.

Superlattice Ultrasonic Generation, Thomas E. Wilson, M. Oehme, E. Kasper, H-J. L. Gossmann

Physics Faculty Research

We report the first experimental evidence for the resonant excitation of coherent high-frequency acoustic phonons in semiconducting doping superstructures by far-infrared laser radiation. After a grating-coupled delta-doped silicon doping superlattice is illuminated with ~1 kW/mm² nanosecond-pulsed 246 GHz laser radiation, a delayed nanosecond pulse is detected by a superconducting bolometer at a time corresponding to the appropriate time-of-flight for ballistic longitudinal acoustic phonons across the (100) silicon substrate. The absorbed phonon power density in the microbolometer is observed to be ~10 μW/mm², in agreement with theory. The phonon pulse duration also matches the laser pulse duration. The …

Evidence For The Generation Of Coherent Longitudinal Acoustic Phonons Through The Resonant Absorption Of Pulsed Far-Infrared Laser Radiation In Silicon Doping Superlattices, Thomas E. Wilson

Physics Faculty Research

We report the first experimental evidence for the direct excitation of coherent high-frequency acoustic phonons in semiconducting doping superstructures by electromagnetic fields of the same frequency. Nanosecond pulses of acoustic phonons have been detected by a superconducting bolometer at the appropriate time-of-flight across a (100) silicon substrate for ballistic longitudinal phonons when a silicon doping superlattice is illuminated with grating-coupled nanosecond-pulsed 246-GHz laser radiation with power density of ∼1 kW/mm². The absorbed phonon power density in the microbolometer is estimated to be ∼ 10/Wmm², in agreement with theory. The phonon pulse duration matches the laser pulse …

Raman Scattering Analysis Of Silicon Dioxide Single Crystal Treated By Direct Current Plasma Discharge, Dusan M. Poparic, Vladimir Milosavljevic, Andrijana Zekic, N Romcevic, Steven Daniels

Articles

Low-k materials such as silicon dioxide (SiO2) play an important role in the semiconductor industry. Plasma has become indispensable for advanced materials processing. In this work a treatment of SiO2single crystal by direct current plasma discharge is studied in detail. Offline metrology is conducted for silicon dioxide wafers by Raman scattering, energy-dispersive x-ray spectroscopy, and ellipsometry. Broad Raman peak at around 2800 cm−1 is observed for the treatedSiO2 wafers. Effects of plasma treatment on position of this peak are reported in the paper. An analysis of this correlation could be a framework for creating virtual etch rate sensors, which might …

Generation Of Mid-Ir Wavelengths, Deborah Robinson, Robert Hartsock, Kelly Gaffney

STAR Program Research Presentations

Generation of mid-IR wavelengths

Deborah Robinson, Robert Hartsock, and Kelly Gaffney

Abstract

Research to determine basic molecular properties utilizing pump/probe experiments is an on going effort at SLAC. Here we have been given the task to generate mid-IR laser pulses and commission a mid-IR detector for said experiments and research. The mid-IR pulses will be used to probe the changes in molecular properties induced by exciting the electrons in molecules with visible pump pulses. In order to accomplish this, an optical parametric amplifier (OPA) has been set-up and aligned. The pump beam for the OPA is a 40 femtosecond 800nm …

Magnetism Of Cluster-Deposited Y–Co Nanoparticles, Balamuruga Balamurugan, Ralph Skomski, Xingzhong Li, V. R. Shah, George C. Hadjipanayis, Jeffrey E. Shield, David J. Sellmyer

Nebraska Center for Materials and Nanoscience: Faculty Publications

Nanoparticles of YCo₂, YCo_3, and YCo₅ are produced by cluster-deposition and investigated both structurally and magnetically. The nanoparticles have sizes of less than 10 nm and are superparamagnetic at 300 K, irrespective of stoichiometry. As-produced nanoparticles exhibit disordered structures with magnetic properties differing from those of the bulk particles. The temperature-dependent magnetization curves of the nanoparticles reveal blocking temperatures from 110 to 250 K, depending on stoichiometry. The magnetic anisotropy constant K₁ of disordered YCo₅ nanoparticles of 7.8 nm in size is 3.5×10⁶ergs/cm³, higher than those of the disordered YCo …

Structure And Magnetism Of Mnau Nanoclusters, X. Wei, Damien Le Roy, Ralph Skomski, Xingzhong Li, Zhiguang Sun, Jeffrey E. Shield, M. J. Kramer, David J. Sellmyer

Nebraska Center for Materials and Nanoscience: Faculty Publications

Equiatomic MnAu clusters with average sizes of 4 and 10 nm are produced by inert-gas condensation. As-produced clusters are used to form both dense cluster films and films with clusters embedded in a W matrix with a cluster volume fraction of 25%. Both structure and magnetism are size-dependent. Structural analysis of the 10 nm clusters indicate a distorted tetragonal body-centered cubic structure with lattice parameters a=0.315 and c=0.329 nm. The 4 nm clusters have a partially ordered tetragonal L10 structure with lattice parameters a=0.410 nm and c=0.395 nm. Magnetic properties of the clusters show evidence at …

In Vitro Analysis Of Immersed Human Tissues By Raman Microspectroscopy, Franck Bonnier, A. Mehmood, Peter Knief, Aidan Meade, Helen Lambkin, Kathleen Flynn, V. Mcdonagh, C. Healy, T. C. Lee, Fiona Lyng, Hugh Byrne

Articles

Raman microspectroscopy is a powerful tool for the analysis of tissue sections, providing a molecular map of the investigated samples. Nevertheless, data pre-processing and, particularly, the removal of the broad background to the spectra remain problematic. Indeed, the physical origin of the background has not been satisfactorily determined. Using 785 nm as source in a confocal geometry, it is demonstrated for the example of the protein kappa-elastin that the background and resulting quality of the recorded spectrum are dependent on the morphology of the sample. Whereas a fine powder yields a dominant broad background, compressed pellets and solution-cast thin films …

In Memoriam: Robert Katz (1917–2011), M. P. R. Waligorski, Francis A. Cucinotta

Robert Katz Publications

Bob Katz will be well remembered for his enthusiasm and strong personality. In a scientific dispute, few indeed could match his wit or his sense of humor or survive the cutting logic of his arguments. To those who had appreciation for his science and his personality, he was truly a great scientist and a master teacher. There are many people around the world who will remember Bob Katz for what he offered them and for the way he showed them what truth in science is.

The Katz Model, developed at that time for solid-state detectors and for cell cultures, relates …