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Full-Text Articles in Physics
Coupling Nuclear Induced Phonon Propagation With Conversion Electron Mössbauer Spectroscopy, Michael J. Parker
Coupling Nuclear Induced Phonon Propagation With Conversion Electron Mössbauer Spectroscopy, Michael J. Parker
Theses and Dissertations
Mössbauer spectroscopy is a very sensitive measurement technique (10-8 eV) which prompted motivation for the experiment described in this thesis. Namely, can a sensitive detection system be developed to detect nuclear recoils on the order of 10 to 100 of eVs? The hypothesis that this thesis tests is: Nuclear induced phonon bursts caused by Rutherford scattered alphas, decayed from 241Am, in a type-310 stainless steel material can couple with 7.3 keV conversion electron Mössbauer events at the other end of the material which will have a statistically significant effect on a Mössbauer spectrum. The phonon bursts produced by …
Interstitial Silicon Ions In Rutile Tio2 Crystals, Eric M. Golden, Nancy C. Giles, Shan Yang, Larry E. Halliburton
Interstitial Silicon Ions In Rutile Tio2 Crystals, Eric M. Golden, Nancy C. Giles, Shan Yang, Larry E. Halliburton
Faculty Publications
Electron paramagnetic resonance (EPR) is used to identify a new and unique photoactive silicon-related point defect in single crystals of rutile TiO2. The importance of this defect lies in its assignment to interstitial silicon ions and the unexpected establishment of silicon impurities as a major hole trap in TiO2. Principal g values of this new S=1/2 center are 1.9159, 1.9377, and 1.9668 with principal axes along the [¯110],[001], and [110] directions, respectively. Hyperfine structure in the EPR spectrum shows the unpaired spin interacting equally with two Ti nuclei and unequally with two Si nuclei. These silicon …
Theoretical Investigation Of Stabilities And Optical Properties Of Si12C12 Clusters, Xiaofeng F. Duan, Larry W. Burggraf
Theoretical Investigation Of Stabilities And Optical Properties Of Si12C12 Clusters, Xiaofeng F. Duan, Larry W. Burggraf
Faculty Publications
By sorting through hundreds of globally stable Si12C12 isomers using a potential surface search and using simulated annealing, we have identified low-energy structures. Unlike isomers knit together by Si–C bonds, the lowest energy isomers have segregated carbon and silicon regions that maximize stronger C–C bonding. Positing that charge separation between the carbon and silicon regions would produce interesting optical absorption in these cluster molecules, we used time-dependent density functional theory to compare the calculated optical properties of four isomers representing structural classes having different types of silicon and carbon segregation regions. Absorptions involving charge transfer between segregated …