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Full-Text Articles in Atmospheric Sciences

The Aging And Impacts Of Atmospheric Soot: Closing The Gap Between Experiments And Models, Ogochukwu Yvonne Enekwizu Dec 2020

The Aging And Impacts Of Atmospheric Soot: Closing The Gap Between Experiments And Models, Ogochukwu Yvonne Enekwizu

Dissertations

The main goal of this dissertation is to generate data and parameterizations to accurately represent soot aerosols in atmospheric models. Soot from incomplete combustion of fossil fuels and biomass burning is a major air pollutant and a significant contributor to climate warming. The environmental impacts of soot are strongly dependent on the particle morphology and mixing state, which evolve continuously during atmospheric transport via a process known as aging. To make predictions of soot impacts on the environment, most atmospheric models adopt simplifications of particle structure and mixing state, which lead to substantial uncertainties. Using an experimentally constrained modeling approach, …


Morphology And Mixing State Of Atmospheric Particles: Links To Optical Properties And Cloud Processing, Swarup China Jan 2014

Morphology And Mixing State Of Atmospheric Particles: Links To Optical Properties And Cloud Processing, Swarup China

Dissertations, Master's Theses and Master's Reports - Open

Atmospheric particles are ubiquitous in Earth’s atmosphere and impact the environment and the climate while affecting human health and Earth’s radiation balance, and degrading visibility. Atmospheric particles directly affect our planet’s radiation budget by scattering and absorbing solar radiation, and indirectly by interacting with clouds. Single particle morphology (shape, size and internal structure) and mixing state (coating by organic and inorganic material) can significantly influence the particle optical properties as well as various microphysical processes, involving cloud-particle interactions and including heterogeneous ice nucleation and water uptake. Conversely, aerosol cloud processing can affect the morphology and mixing of the particles. For …


Detailed Modeling Of Soot Size Distribution Evolution And Pollutant Formation Inside Aircraft And Diesel Engines, Chowdhury Golam Moniruzzaman Jan 2012

Detailed Modeling Of Soot Size Distribution Evolution And Pollutant Formation Inside Aircraft And Diesel Engines, Chowdhury Golam Moniruzzaman

Legacy Theses & Dissertations (2009 - 2024)

Combustion emission of soot and pollutant gas species contributes to poor regional air quality near emission sources and to climate change. It is important to understand the formation mechanism and time evolution of these pollutants inside the combustion engine, through detailed modeling of combustion chemistry and microphysics as well as comparison with observation. In this thesis, two multi-zone gas parcel combustion engine models, one for aircraft engines and another for diesel engines, have been developed to study soot size distribution evolution and pollutant formation inside the engines as well as emissions. The models take into account size-resolved (sectional) soot aerosol …