Physical Sciences and Mathematics Commons^™

Observation Of In-Plane Magnetic Field Induced Phase Transitions In Fese, Jong Mok Ok, Chang Il Kwon, Yoshimitsu Kohama, Jung Sang You, Sun Kyu Park, Ji-Hye Kim, Y.J. Jo, E.S. Choi, Koichi Kindo, Woun Kang, Ki-Seok Kim, E. G. Moon, Alex Gurevich, Jun Sung Kim

Physics Faculty Publications

We investigate thermodynamic properties of FeSe under in-plane magnetic fields using torque magnetometry, specific heat, and magnetocaloric measurements. Below the upper critical field H_c2, we observed the field induced anomalies at H₁ ∼ 15 T and H₂ ∼ 22 T near H ∥ ab and below a characteristic temperature T* ∼ 2 K. The transition magnetic fields H₁ and H₂ exhibit negligible dependence on both temperature and field orientation. This contrasts to the strong temperature and angle dependence of H_c2, suggesting that these anomalies are attributed to the field induced phase transitions, …

Dynamic Pair-Breaking Current, Critical Superfluid Velocity, And Nonlinear Electromagnetic Response Of Nonequilibrium Superconductors, Ahmad Sheikhzada, Alex Gurevich

Physics Faculty Publications

We report numerical calculations of a dynamic pair-breaking current density J_d and a critical superfluid velocity v_d in a nonequilibrium superconductor carrying a uniform, large-amplitude AC current density J(t)=J_asinΩt with Ω well below the gap frequency Ω ≪ Δ₀/h. The dependencies J_d(Ω,T) and v_d(Ω,T) near the critical temperature T_cwere calculated from either the full time-dependent nonequilibrium equations for a dirty s-wave superconductor or the time-dependent Ginzburg-Landau (TDGL) equations for a gapped superconductor, taking into account the GL relaxation time of the order parameter GL …

Superconductivity In La₂Ni₂In, Jannis Maiwald, Igor I. Mazin, Alex Gurevich, Meigan Aronson

Physics Faculty Publications

We report here the properties of single crystals of La₂Ni₂In. Electrical resistivity and specific heat measurements concur with the results of density functional theory calculations, finding that La₂Ni₂In is a weakly correlated metal, where the Ni magnetism is almost completely quenched, leaving only a weak Stoner enhancement of the density of states. Superconductivity is observed at temperatures below 0.9 K. A detailed analysis of the field and temperature dependencies of the resistivity, magnetic susceptibility, and specific heat at the lowest temperatures reveals that La₂Ni₂In is a dirty type-II …

Heisenberg Model Analysis On Inelastic Powder Neutron Scattering Data Using Parent And K Doped Bamn2as2 Samples, Mehmet Ramazanoglu, Aashish Sapkota, Abhishek Pandey, Jagat Lamsal, Douglas L. Abernathy, Jennifer L. Niedziela, Matthew B. Stone, R. Salci, D. A. Acar, F. O. Oztirpan, Şener Ozonder, Andreas Kreyssig, Alan I. Goldman, David C. Johnston, Robert J. Mcqueeney

A. I. Goldman

Low temperature powder inelastic neutron scattering measurements were performed on three different powder samples; parent BaMn2As2,12.5% K-doped Ba0.875K0.125Mn2As2 and 25% K-doped Ba(0.75)K0.25Mn2As2. The Heisenberg Model involving J1‐J2‐Jz coupling constants were compared to the data by a powder integration routine using Monte Carlo integration methods. The best magnetic parameters were selected using a chi-square test where model intensities were compared to the full (q,E) dependence of magnetic scattering. A key step to this analysis is the characterization of the background which is formed mostly by phonon scattering intensities along with other sources including the magnetic impurity scattering events. The calculated powder …

Loop Currents And Anomalous Hall Effect From Time-Reversal Symmetry-Breaking Superconductivity On The Honeycomb Lattice, P.M.R. Brydon, D.S.L. Abergel, Daniel Agterberg, Victor M. Yakovenko

Physics Faculty Articles

We study a tight-binding model on the honeycomb lattice of chiral d-wave superconductivity that breaks time-reversal symmetry. Because of its nontrivial sublattice structure, we show that it is possible to construct a gauge-invariant time-reversal-odd bilinear of the pairing potential. The existence of this bilinear reflects the sublattice polarization of the pairing state. We show that it generates persistent loop current correlations around each lattice site and opens a topological mass gap at the Dirac points, resembling Haldane’s model of the anomalous quantum Hall effect. In addition to the usual chiral d-wave edge states, there also exist electronlike edge …

Ternary Inorganic Electrides With Mixed Bonding, Junjie Wang, Qiang Zhu, Zhenhai Wang, Hideo Hosono

Physics & Astronomy Faculty Research

A high-throughput screening based on first-principles calculations was performed to search for new ternary inorganic electrides. From the available materials database, we identified three new thermodynamically stable materials (Li12Mg3Si4, NaBa2O, and Ca5Ga2N4) as potential electrides made by main group elements, in addition to the well known mayenite based electride (C12A7:e−). Different from those conventional inorganic electrides in which the excess electrons play only the role of anions, the three new materials, resembling the electrides found in simple metals under high pressure, possess mixed ionic and metallic bonding. The interplay between two competing mechanisms, together with the different crystal packing motifs, …

Argon Metastable And Resonant Level Densities In Ar And Ar/Cl² Discharges Used For The Processing Of Bulk Niobium, Jeremy Peshl, Roderick Mcneill, Charles I. Sukenik, Milka Nikolić, Svetozar Popović, Leposava Vŭsković

Physics Faculty Publications

A comparative analysis of two popular spectroscopy techniques is conducted in a coaxial cylindrical capacitively coupled discharge designed for the plasma processing of superconducting radio frequency (SRF) cavities. The density of the metastable and resonant levels in Ar is measured in both Ar and Ar/Cl₂ discharges to properly characterize the unique discharge system and aid in the development of a cavity etching routine. The first method, deemed the “branching fraction method,” utilizes the sensitivity of photon reabsorption of radiative decay to measure the lower state (metastable and resonant) densities by taking ratios of spectral lines with a common upper …

Heat Flux Capacity Measurement And Improvement For The Test Of Superconducting Logic Circuits In Closed-Cycle Cryostats, Sasan Razmkhah, Ali̇ Bozbey

Turkish Journal of Electrical Engineering and Computer Sciences

With the current progress of superconducting integrated circuits, circuit complexities have reached more than 100,000 Josephson junctions. At the laboratory environment, circuit tests are generally being conducted at liquid Helium environments. With the commercialization of the superconducting integrated circuit-based systems and/or price increase of liquid Helium, utilization of the closed-cycle systems will be inevitable. Even though it is possible to implement closed-cycle systems with quite substantial excess cooling powers after all the wirings and peripheral circuits, one point not to be overlooked is the power density at the superconducting chips. We have observed that the circuits designed for operation at …

Scanning Tunneling Spectroscopy Investigations Of Superconducting-Doped Topological Insulators: Experimental Pitfalls And Results, Stefan Wilfert, Paolo Sessi, Zhiwei Wang, Henrik Schmidt, M. Carmen Martínez-Velarte, Seng Huat Lee, Yew San Hor, Alexander F. Otte, Yoichi Ando, Weida Wu, Matthias Bode

Physics Faculty Research & Creative Works

Recently, the doping of topological insulators has attracted significant interest as a potential route towards topological superconductivity. Because many experimental techniques lack sufficient surface sensitivity, however, definite proof of the coexistence of topological surface states and surface superconductivity is still outstanding. Here we report on highly surface sensitive scanning tunneling microscopy and spectroscopy experiments performed on Tl-doped Bi₂Te₃, a three-dimensional topological insulator which becomes superconducting in the bulk at T_C=2.3 K. Landau level spectroscopy as well as quasiparticle interference mapping clearly demonstrated the presence of a topological surface state with a Dirac point energy …

Current Induced Depairing And Mixed State Behavior In The Bite/Fete Interfacial Superconductor, Charles Louis Dean Ii

Theses and Dissertations

The Bi2Te3/FeTe heterostructure intersects several phenomena and key classes of materials in condensed matter physics: topological insulators, superconductivity, magnetism, and the physics of interfaces. While neither the topological insulator (BiTe) nor the iron chalcogenide (FeTe) are themselves superconductors, superconductivity forms in a thin 7nm interfacial layer between the two. The restricted dimensionality and the extraordinarily conductive normal state, possibly sourced by the topologically protected surface states, have led to the observation of novel phenomena such as the Likharev vortex explosion and transitions in behavior resulting from the interplay between current induced depairing and the Berezinski-Kosterlitz-Thouless regime. The measured depairing current …

Non-Centrosymmetric Superconductivity And Magnetism In The Presence Of Broken Symmetries, Mojammel Alam Khan

LSU Doctoral Dissertations

Non-centrosymmetric (NC) superconducting and magnetic compounds have been synthesized and investigated using magnetic, specific heat, and transport measurements, as well as by neutron scattering and quantum oscillations. The crystal structures of NC compounds are defined by the lack of an inversion center. In NC superconductors, a finite antisymmetric spin orbit coupling originating from broken inversion symmetry results in unconventional Cooper pairing. Instead of a single spin channel, the order parameter is a mixture of spin-singlet and spin-triplet states. For NC magnetic compounds, the antisymmetric and isotropic spin interactions compete, leading to a helical ground state.

We have studied the NC …

Calorimetric Measurements Of Magnetic-Field-Induced Inhomogeneous Superconductivity Above The Paramagnetic Limit, Charles C. Agosta, Nathanael Alexander Fortune, Scott T. Hannahs, Shuyao Gu, Lucy Liang, Ju-Hyun Park, John A. Schleuter

Physics: Faculty Publications

We report the first magnetocaloric and calorimetric observations of a magnetic-field-induced phase transition within a superconducting state to the long-sought exotic Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) superconducting state, first predicted over 50 years ago. Through the combination of bulk thermodynamic calorimetric and magnetocaloric measurements in the organic superconductor κ−(BEDT−TTF)2Cu(NCS)2 as a function of temperature, magnetic field strength, and magnetic field orientation, we establish for the first time that this field-induced first-order phase transition at the paramagnetic limit Hp is a transition to a higher-entropy superconducting phase, uniquely characteristic of the FFLO state. We also establish that this high-field superconducting state displays the bulk …

Nonlinear Dynamics Of Vortices In Different Types Of Grain Boundaries, Ahmad K. Sheikhzada

Physics Theses & Dissertations

As a major component of linear particle accelerators, superconducting radio-frequency (SRF) resonator cavities are required to operate with lowest energy dissipation and highest accelerating gradient. SRF cavities are made of polycrystalline materials in which grain boundaries can limit maximum RF currents and produce additional power dissipation sources due to local penetration of Josephson vortices. The essential physics of vortex penetration and mechanisms of dissipation of vortices driven by strong RF currents along networks of grain boundaries and their contribution to the residual surface resistance have not been well understood. To evaluate how GBs can limit the performance of SRF materials, …

Crabbing System For An Electron-Ion Collider, Alejandro Castilla

Physics Theses & Dissertations

As high energy and nuclear physicists continue to push further the boundaries of knowledge using colliders, there is an imperative need, not only to increase the colliding beams’ energies, but also to improve the accuracy of the experiments, and to collect a large quantity of events with good statistical sensitivity. To achieve the latter, it is necessary to collect more data by increasing the rate at which these pro- cesses are being produced and detected in the machine. This rate of events depends directly on the machine’s luminosity. The luminosity itself is proportional to the frequency at which the beams …

Exact Numerical Study Of Disordered Systems, Conrad Wilson Moore

LSU Doctoral Dissertations

This thesis presents work on the development of new techniques to study the problem of localization in various models of disordered systems with the goal of being able to extend these model calculations to real materials where these various mechanisms of disorder can all be present. I consider the Anderson Model with diagonal, off-diagonal disorder, multiple bands and superconductivity is included at the level of a Bogoliubov - De Gennes mean field (superconductivity is considered by adding the symmetries of the Bogoliubov - De Gennes Hamiltonian on top of the disordered lattice Hamiltonian). The localization of electrons is studied with …

Rotational Symmetry Breaking In A Trigonal Superconductor Nb-Doped Bi₂Se₃, T. Asaba, B. J. Lawson, C. Tinsman, L. Chen, P. Corbae, G. Li, Y. Qiu, Yew San Hor, L. Fu, L. Li

Physics Faculty Research & Creative Works

The search for unconventional superconductivity has been focused on materials with strong spin-orbit coupling and unique crystal lattices. Doped bismuth selenide (Bi₂Se₃) is a strong candidate, given the topological insulator nature of the parent compound and its triangular lattice. The coupling between the physical properties in the superconducting state and its underlying crystal symmetry is a crucial test for unconventional superconductivity. In this paper, we report direct evidence that the superconducting magnetic response couples strongly to the underlying trigonal crystal symmetry in the recently discovered superconductor with trigonal crystal structure, niobium (Nb)-doped Bi₂Se_{3 …}

Power Distribution Of Terahertz Emission From Hexagonal Bscco Microstrip Antennas, Andrew E. Davis

Honors Undergraduate Theses

We analyze the distribution of coherent terahertz radiation from a regular hexagonal microstrip antenna (MSA) made from the high-T_c superconductor Bi₂Sr₂CaCu₂O_8+x (BSCCO). We discuss the C_6v symmetry of the solutions of the wave equation on a hexagonal domain and distinguish between the closed-form and non-closed-form solutions. The closed-form wavefunctions of the transverse magnetic (TM) electromagnetic cavity modes are presented and formulas for the radiated power arising from the uniform part of the AC Josephson current and from the resonant cavity modes are derived. The wavefunctions and angular distribution of radiation from …

Cryogenic Rf Test Of The First Srf Cavity Etched In An Rf Ar/Cl2 Plasma, J. Upadhyay, A. Palczewski, S. Popovic, A.-M. Valente-Feliciano, Do Im, H. L. Phillips, L. Vuskovic

Physics Faculty Publications

An apparatus and a method for etching of the inner surfaces of superconducting radio frequency (SRF) accelerator cavities are described. The apparatus is based on the reactive ion etching performed in an Ar/Cl₂ cylindrical capacitive discharge with reversed asymmetry. To test the effect of the plasma etching on the cavity rf performance, a 1497 MHz single cell SRF cavity was used. The single cell cavity was mechanically polished and buffer chemically etched and then rf tested at cryogenic temperatures to provide a baseline characterization. The cavity's inner wall was then exposed to the capacitive discharge in a mixture of …

Exact Solution Of Quadratic Fermionic Hamiltonians For Arbitrary Boundary Conditions, Abhijeet Alase, Emilio Cobanera, Gerardo Ortiz, Lorenza Viola

Dartmouth Scholarship

We present a procedure for exactly diagonalizing finite-range quadratic fermionic Hamiltonians with arbitrary boundary conditions in one of D dimensions, and periodic in the remaining D−1. The key is a Hamiltonian-dependent separation of the bulk from the boundary. By combining information from the two, we identify a matrix function that fully characterizes the solutions, and may be used to construct an efficiently computable indicator of bulk-boundary correspondence. As an illustration, we show how our approach correctly describes the zero-energy Majorana modes of a time-reversal-invariant s-wave two-band superconductor in a Josephson ring configuration, and predicts that a fractional 4π-periodic Josephson effect …

Vortices And Quasiparticles In Superconducting Microwave Resonators, Ibrahim Nsanzineza

Dissertations - ALL

Superconducting resonators with high quality factors are of great interest in many areas. However, the quality factor of the resonator can be weakened by many dissipation channels including trapped magnetic flux vortices and nonequilibrium quasiparticles which can significantly impact the performance of superconducting microwave resonant circuits and qubits at millikelvin temperatures. Quasiparticles result in excess loss, reducing resonator quality factors and qubit lifetimes. Vortices trapped near regions of large microwave currents also contribute excess loss. However, vortices located in current-free areas in the resonator or in the ground plane of a device can actually trap quasiparticles and lead to a …

Wavelet Transform Of Optical Conductivity Of Bi2sr2cacu2o8+X In The Normal And Superconducting State, Patrick Janovick

Williams Honors College, Honors Research Projects

This paper compares the wavelet transform of the optical conductivity of Bi₂Sr₂CaCu₂O_8+x in both the normal and the superconducting state. The wavelet transforms of the normal and superconducting state are also compared with wavelet transforms of the Drude model as well as the Lorentz model. The wavelet transform of the collected data for Bi₂Sr₂CaCu₂O_8+x is similar in shape to the Drude model. The wavelet transform of the collected data in the normal state corresponds to the Drude model with a high scattering rate and the collected …

Tuning Superconductivity In Fese Thin Films Via Magnesium Doping, Wenbin Qiu, Zongqing Ma, Yongchang Liu, Md Shahriar Hossain, Xiaolin Wang, Chuanbing Cai, S X. Dou

Australian Institute for Innovative Materials - Papers

In contrast to its bulk crystal, the FeSe thin film or layer exhibits better superconductivity performance, which recently attracted much interest in its fundamental research as well as in potential applications around the world. In the present work, tuning superconductivity in FeSe thin films was achieved by magnesium-doping technique. Tc is significantly enhanced from 10.7 K in pure FeSe films to 13.4 K in optimized Mg-doped ones, which is approximately 1.5 times higher than that of bulk crystals. This is the first time achieving the enhancement of superconducting transition temperature in FeSe thin films with practical thickness (120 nm) via …

Interface-Enhanced Electron-Phonon Coupling And High-Temperature Superconductivity In Potassium-Coated Ultrathin Fese Films On Srtio3, Chenjia Tang, Chong Liu, Guanyu Zhou, Fangsen Li, Hao Ding, Zhi Li, Ding Zhang, Zheng Li, Canli Song, Shuaihua Ji, Ke He, Lili Wang, Xucan Ma, Qi-Kun Xue

Australian Institute for Innovative Materials - Papers

Alkali-metal (potassium) adsorption on FeSe thin films with thickness from 2 unit cells (UC) to 4 UC on SrTiO3 grown by molecular beam epitaxy is investigated with a low-temperature scanning tunneling microscope. At appropriate potassium coverage (0.20-0.25 monolayer), the tunneling spectra of the films all exhibit a superconductinglike gap which is overall larger than 11 meV (five times the gap value of bulk FeSe) and decreases with increasing thickness, and two distinct features of characteristic phonon modes at ∼11 and ∼21 meV. The results reveal the critical role of the interface-enhanced electron-phonon coupling for possible high-temperature superconductivity in ultrathin FeSe …

The Effect Of Impurities On The Superconductivity Of Bscco-2212, John Vastola

Honors Undergraduate Theses

BSCCO-2212 is a high-temperature cuprate superconductor whose microscopic behavior is currently poorly understood. In particular, it is unclear whether its order parameter is consistent with s-wave or d-wave symmetry. It has been suggested that its order parameter might take one of several forms that are consistent with d-wave behavior. We present some calculations using the many-body theory approach to superconductivity that suggest that such order parameters would lead to a suppression of the critical temperature in the presence of impurities. Because some experiments have suggested the critical temperature of BSCCO-2212 is relatively independent of the concentration of impurities, this lends …

Anisotropic Thermodynamic And Transport Properties Of Single-Crystalline Cakfe4As4, W. R. Meier, T. Kong, U. S. Kaluarachchi, V. Taufour, N. H. Jo, G. Drachuck, A. E. Böhmer, S. M. Saunders, A. Sapkota, A. Kreyssig, M. A. Tanatar, R. Prozorov, A. I. Goldman, Fedor F. Balakirev, Alex Gurevich, S. L. Bud'ko, P. C. Canfield

Physics Faculty Publications

Single-crystalline, single-phase CaKFe₄As₄ has been grown out of a high-temperature, quaternary melt. Temperature-dependent measurements of x-ray diffraction, anisotropic electrical resistivity, elastoresistivity, thermoelectric power, Hall effect, magnetization, and specific heat, combined with field-dependent measurements of electrical resistivity and field and pressure-dependent measurements of magnetization indicate that CaKFe₄As₄ is an ordered, stoichiometric, Fe-based superconductor with a superconducting critical temperature, T_c = 35.0 ± 0.2 K. Other than superconductivity, there is no indication of any other phase transition for 1.8K ≤ T ≤ 300 K. All of these thermodynamic and transport data reveal striking similarities to …

Anyonic Superconductivity In A Modified Large-U Hubbard Model, Asim Gangopadhyaya, Prasanta Panigrahi

Asim Gangopadhyaya

A modified large-U Hubbard model at half filling is analyzed by a mean-field approach. Preserving a local U(1) symmetry of the action, the fluctuations about half filling are studied in the spirit of the commensurate-flux-phase condition. The fluctuations then contribute a Chern-Simons term to the tree-level Lagrangian with a coefficient appropriate to that of a half fermion. With the Coulomb repulsion term, we study the low-energy excitations of the model and show the existence of superconductivity in the presence of a four-Fermi interaction term.

Enhanced Magnetism In Dy And Tb At Extreme Pressure, Jinhyuk Lim

Arts & Sciences Electronic Theses and Dissertations

At ambient pressure all lanthanide metals order magnetically at temperatures at or below ambient. The magnetic ordering is known to result from the indirect exchange interaction between localized 4f magnetic moments mediated by the surrounding conduction electrons, the so-called Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction. With the RKKY interaction the magnetic ordering temperature To is expected to be proportional to the de Gennes factor which is a function of the Landé g factor gJ and the total angular momentum J. For example, Gd has the highest value of To, 292 K, at ambient pressure as it has the largest de Gennes factor of …

Prospective Solid-State Photonic Cryocooler Based On The “Phonon-Deficit Effect”, Gurgen Melkonyan, Armen Gulian

Mathematics, Physics, and Computer Science Faculty Articles and Research

In this design microwave photons are propagating in a sapphire rod, and are being absorbed by a superconductor deposited on the surface of the rod. The frequency of the radiation is tuned to be less than the energy gap in the superconductor, so that the pair breaking is not taking place. This photon pumping redistributes the electron-hole quasiparticles: their distribution function is non-equilibrium, and the “phonon-deficit effect” takes place. There is a dielectric material deposited on top of superconductor, which serves asthe “cold finger” of the cooler. Its “acoustical density” is supposed to be smaller than that of the superconducting …

Flux-Tunable Superconducting Transmons For Quantum Information Processing, Matthew Ware

Dissertations - ALL

In this thesis, I describe a series of experiments using flux-tunable transmon qubits for quantum information processing. These qubits are designed with different levels of Josephson junction asymmetry. The first two chapters of this thesis will introduce the reader to superconducting qubits and circuit quantum electrodynamics. I will present experiments using the cQED architecture to implement fast photon swapping between an asymmetric qubit and a superconducting resonator using flux-driven sidebands. This is the first experimental observation of flux-driven sidebands in a superconducting system. This process also allows photon swaps between qubit and resonator to first order in the qubit-resonator coupling …

Dynamical Generation Of Floquet Majorana Flat Bands In S-Wave Superconductors, A. Poudel, G. Ortiz, L. Viola

Dartmouth Scholarship

We present quantum control techniques to engineer flat bands of symmetry-protected Majorana edge modes in s -wave superconductors. Specifically, we show how periodic control may be employed for designing time-independent effective Hamiltonians, which support Floquet Majorana flat bands, starting from equilibrium conditions that are either topologically trivial or only support individual Majorana pairs. In the first approach, a suitable modulation of the chemical potential simultaneously induces Majorana flat bands and dynamically activates a pre-existing chiral symmetry which is responsible for their protection. In the second approach, the application of effective parity kicks dynamically generates a desired chiral symmetry by suppressing …