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Full-Text Articles in Nuclear Engineering
Real-Time Identification Of Oxygen Vacancy Centers In Linbo₃ And Srtio₃ During Irradiation With High Energy Particles, Miguel L. Crespillo, Joseph T. Graham, Fernando Agulló-López, Yanwen Zhang, William J. Weber
Real-Time Identification Of Oxygen Vacancy Centers In Linbo₃ And Srtio₃ During Irradiation With High Energy Particles, Miguel L. Crespillo, Joseph T. Graham, Fernando Agulló-López, Yanwen Zhang, William J. Weber
Nuclear Engineering and Radiation Science Faculty Research & Creative Works
Oxygen vacancies are known to play a central role in the optoelectronic properties of oxide perovskites. A detailed description of the exact mechanisms by which oxygen vacancies govern such properties, however, is still quite incomplete. The unambiguous identification of oxygen vacancies has been a subject of intense discussion. Interest in oxygen vacancies is not purely academic. Precise control of oxygen vacancies has potential technological benefits in optoelectronic devices. In this review paper, we focus our attention on the generation of oxygen vacancies by irradiation with high energy particles. Irradiation constitutes an efficient and reliable strategy to introduce, monitor, and characterize …
Recent Advances On Carrier And Exciton Self-Trapping In Strontium Titanate: Understanding The Luminescence Emissions, Miguel L. Crespillo, Joseph T. Graham, Fernando Agullo-Lopez, Yanwen Zhang, William J. Weber
Recent Advances On Carrier And Exciton Self-Trapping In Strontium Titanate: Understanding The Luminescence Emissions, Miguel L. Crespillo, Joseph T. Graham, Fernando Agullo-Lopez, Yanwen Zhang, William J. Weber
Nuclear Engineering and Radiation Science Faculty Research & Creative Works
An up-to-date review on recent results for self-trapping of free electrons and holes, as well as excitons, in strontium titanate (STO), which gives rise to small polarons and self-trapped excitons (STEs) is presented. Special attention is paid to the role of carrier and exciton self-trapping on the luminescence emissions under a variety of excitation sources with special emphasis on experiments with laser pulses and energetic ion-beams. In spite of the extensive research effort, a definitive identification of such localized states, as well as a suitable understanding of their operative light emission mechanisms, has remained lacking or controversial. However, promising advances …
Neutron Irradiation Effects On Domain Wall Mobility And Reversibility In Lead Zirconate Titanate Thin Films, Joseph T. Graham, Geoff L. Brennecka, Paulo Ferreira, Leo Small, David Duquette, Christopher Apblett, Sheldon Landsberger, Jon F. Ihlefeld
Neutron Irradiation Effects On Domain Wall Mobility And Reversibility In Lead Zirconate Titanate Thin Films, Joseph T. Graham, Geoff L. Brennecka, Paulo Ferreira, Leo Small, David Duquette, Christopher Apblett, Sheldon Landsberger, Jon F. Ihlefeld
Nuclear Engineering and Radiation Science Faculty Research & Creative Works
The effects of neutron-induced damage on the ferroelectric properties of thin film lead zirconate titanate (PZT) were investigated. Two sets of PbZr0.52Ti0.48O3 films of varying initial quality were irradiated in a research nuclear reactor up to a maximum 1 MeV equivalent neutron fluence of (5.16± 0.03) x 1015 cm-2. Changes in domain wall mobility and reversibility were characterized by polarization-electric field measurements, Rayleigh analysis, and analysis of first order reversal curves (FORC). With increasing fluence, extrinsic contributions to the small-signal permittivity diminished. Additionally, redistribution of irreversible hysterons towards higher coercive fields was …