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Tailoring Optical And Plasmon Resonances In Core-Shell And Core-Multishell Nanowires, Sarath Ramadurgam Jan 2016

Tailoring Optical And Plasmon Resonances In Core-Shell And Core-Multishell Nanowires, Sarath Ramadurgam

Open Access Dissertations

Semiconductor nanowires (NWs) are sub-wavelength structures which exhibit strong optical (Mie) resonances in the visible range. In addition to such optical resonances, the localized surface plasmon resonances (LSPR) in metal and semiconductor (or dielectric) based core-shell (CS) and core-multishell (CMS) NWs can be tailored to achieve novel negative-index metamaterials (NIM), extreme absorbers, invisibility cloaks and sensors. Particularly, in this dissertation, the versatility of CS and CMS NWs for the design of negative-index metamaterials in the visible range and, plasmonic light harvesting in ultrathin photocatalyst layers for water splitting are studied.

Utilizing the LSPR in the metal layer and the magnetic ...


Semiconductor Nanowires: Optical Properties And All-Optical Switching, Brian Edward Piccione Jan 2012

Semiconductor Nanowires: Optical Properties And All-Optical Switching, Brian Edward Piccione

Publicly Accessible Penn Dissertations

The optical properties of semiconductor nanowires are both important from a fundamental materials physics standpoint and necessary to understand in engineering applications: nanowire photovoltaic devices, sensors, and lasers, among others, could all benefit. Unfortunately, these optical properties are not easy to ascertain. Transmission times are short, in-coupling of white probe light is difficult, and the angle-resolved measurements typically used to determine material dispersion relations in bulk materials are hindered by diffraction effects at subwavelength nanowire end facets.

Here, we present a series of experimental techniques and theoretical models developed to study of the optical properties of active nanowire waveguides. Beginning ...