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Nanoscience and Nanotechnology Commons

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2008

Purdue University

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Articles 1 - 24 of 24

Full-Text Articles in Nanoscience and Nanotechnology

Nanoantenna Array-Induced Fluorescence Enhancement And Reduced Lifetimes, Reuben M. Bakker, V. P. Drachev, Zhengtong Liu, Hsiao-Kuan Yuan, Rasmus H. Pedersen, Alexandra Boltasseva, Jiji Chen, Joseph Irudayaraj, Alexander V. Kildishev, V. M. Shalaev Dec 2008

Nanoantenna Array-Induced Fluorescence Enhancement And Reduced Lifetimes, Reuben M. Bakker, V. P. Drachev, Zhengtong Liu, Hsiao-Kuan Yuan, Rasmus H. Pedersen, Alexandra Boltasseva, Jiji Chen, Joseph Irudayaraj, Alexander V. Kildishev, V. M. Shalaev

Birck and NCN Publications

Enhanced fluorescence is observed from dye molecules interacting with optical nanoantenna arrays. Elliptical gold dimers form individual nanoantennae with tunable plasmon resonances depending upon the geometry of the two particles and the size of the gap between them. A fluorescent dye, Rhodamine 800, is uniformly embedded in a dielectric host that coats the nanoantennae. The nanoantennae act to enhance the dye absorption. In turn, emission from the dye drives the plasmon resonance of the antennae; the nanoantennae act to enhance the fluorescence signal and change the angular distribution of emission. These effects depend upon the overlap of the plasmon resonance …


Atomic-Layer-Deposited Al2o3/Gaas Metal-Oxide-Semiconductor Field-Effect Transistor On Si Substrate Using Aspect Ratio Trapping Technique, Y Q. Wu, M Xu, P. D. Ye, Z Cheng, J Li, J Park, J Hydrick, J Bai, M Carroll, J G. Fiorenza, A Lochtefeld Dec 2008

Atomic-Layer-Deposited Al2o3/Gaas Metal-Oxide-Semiconductor Field-Effect Transistor On Si Substrate Using Aspect Ratio Trapping Technique, Y Q. Wu, M Xu, P. D. Ye, Z Cheng, J Li, J Park, J Hydrick, J Bai, M Carroll, J G. Fiorenza, A Lochtefeld

Birck and NCN Publications

High quality GaAs epilayers grown by metal-organic chemical vapor deposition are demonstrated on a SiO2-patterned silicon substrate using aspect ratio trapping technique, whereby threading dislocations from lattice mismatch are largely reduced via trapping in SiO2 trenches during growth. A depletion-mode metal-oxide-semiconductor field-effect transistor (MOSFET) is demonstrated on a n-doped GaAs channel with atomic-layer deposited Al2O3 as the gate oxide. The 10 mu m gate length transistor has a maximum drain current of 88 mA/mm and a transconductance of 19 mS/mm. The surface mobility estimated from the accumulation drain current has a peak value of similar to 500 cm(2)/Vs, which is …


Transport-Based Dopant Metrology In Advanced Finfets, Gabriel P. Lansbergen, Rajib Rahman, Cameron J. Wellard, Jaap Caro, Nadine Collaert, Serge Biesemans, Gerhard Klimeck, Lloyd C. L. Hollenberg, Sven Rogge Dec 2008

Transport-Based Dopant Metrology In Advanced Finfets, Gabriel P. Lansbergen, Rajib Rahman, Cameron J. Wellard, Jaap Caro, Nadine Collaert, Serge Biesemans, Gerhard Klimeck, Lloyd C. L. Hollenberg, Sven Rogge

Other Nanotechnology Publications

Ultra-scaled FinFET transistors bear unique fingerprint-like device-to-device differences attributed to random single impurities. Through correlation of experimental data with multimillion atom simulations in NEMO 3-D, we can identify the impurity’s chemical species and determine their concentration, local electric field and depth below the Si/SiO2 interface. The ability to model the excited states rather than just the ground states is the critical need. We therefore demonstrate a new approach to atomistic impurity metrology and confirm the assumption of tunneling through individual impurity quantum states.


Full-Band And Atomisic Simulation Of Realistic 40 Nm Inas Hemt, Mathieu Luisier, Neophytos Neophytou, Neerav Kharche, Gerhard Klimeck Dec 2008

Full-Band And Atomisic Simulation Of Realistic 40 Nm Inas Hemt, Mathieu Luisier, Neophytos Neophytou, Neerav Kharche, Gerhard Klimeck

Other Nanotechnology Publications

A realistic 40 nm InAs high electron mobility transistor is studied using a two-dimensional, full-band, and atomistic Schr¨odinger-Poisson solver based on the sp3d5s∗ tightbinding model. Bandstructure non-parabolicity effects, strain, alloy disorder in the InGaAs and InAlAs barriers, as well as band-to-band tunneling in the transistor OFF-state are automatically included through the full-band atomistic model. The source and drain contact extensions are taken into account a posteriori by adding two series resistances to the device channel. The simulated current characteristics are compared to measured data and show a good quantitative agreement.


From Nemo1d And Nemo3d To Omen: Moving Towards Atomistic 3-D Quantum Transport In Nano-Scale Semiconductors, Gerhard Klimeck, Mathieu Luisier Dec 2008

From Nemo1d And Nemo3d To Omen: Moving Towards Atomistic 3-D Quantum Transport In Nano-Scale Semiconductors, Gerhard Klimeck, Mathieu Luisier

Other Nanotechnology Publications

Lessons learned in 15 years of NEMO development starting from quantitative and predictive resonant tunneling diode (RTD) to multi-million atom electronic structure modeling and the path for OMEN are laid out. The recent OMEN capabilities enable realistically large 3D atomistic nano-scale device simulation.


Optical Hyperspace For Plasmons: Dyakonov States In Metamaterials, Zubin Jacob, Evgenii E. Narimanov Dec 2008

Optical Hyperspace For Plasmons: Dyakonov States In Metamaterials, Zubin Jacob, Evgenii E. Narimanov

Birck and NCN Publications

We show that the subdiffraction imaging behavior observed in the magnifying superlens experiment, [Smolyaninov , Science 317, 1699 (2007)] is due to the hyperbolic dispersion of Dyakonov plasmons supported by the device. These states which are a special case of Dyakonov surface waves [Dyakonov, Sov. Phys. JETP 67, 714 (1988)] exist at the interface of a metal and an anisotropic dielectric giving rise to plasmon beams on resonance. Furthermore, we describe how the unique properties of metamaterial Dyakonov plasmons can be tailored for plasmonic devices.


Hydrodynamic Loading Of Microcantilevers Oscillating Near Rigid Walls, Ryan C. Tung, Jana Anirban, Arvind Raman Dec 2008

Hydrodynamic Loading Of Microcantilevers Oscillating Near Rigid Walls, Ryan C. Tung, Jana Anirban, Arvind Raman

Birck and NCN Publications

The vibrations of microcantilevers in atomic force microscopes (AFMs) or radio frequency (RF) switches are strongly influenced by the viscous hydrodynamics of the surrounding fluid in the vicinity of a rigid wall. While prior efforts to model this hydrodynamic loading have focused on squeeze film damping effects at high Knudsen and squeeze numbers, the regimes of low Knudsen and squeeze numbers are also very important for which squeeze film models need to be discarded in favor of unsteady Stokes hydrodynamics. We extend the work of Green and Sader [Phys Fluids 17, 073102 (2005); J. Appl. Phys. 98, 114913 (2005)] and …


Transformation Optics: Approaching Broadband Electromagnetic Cloaking, Alexander V. Kildishev, W Cai, U K. Chettiar, V. M. Shalaev Nov 2008

Transformation Optics: Approaching Broadband Electromagnetic Cloaking, Alexander V. Kildishev, W Cai, U K. Chettiar, V. M. Shalaev

Birck and NCN Publications

An approach to broadband cloaking of light waves is analysed for a simplified case of a scaling transformation for a general cylindrical coordinate system. The proposed approach requires metamaterials with specifically engineered dispersion. The restriction on the signs of gradients in the dispersion dependencies of the dielectric permittivity and the magnetic permeability for different operational wavelengths is revealed and is shown to cause difficulties unless additional gain-assisted compensation for losses or electromagnetically induced transparency is introduced in the cloaking system.


Solutions In Folded Geometries, And Associated Cloaking Due To Anomalous Resonance, Graeme W. Milton, Nicolae-Alexandru P. Nicorovici, Ross C. Mcphedran, Kirill Cherednichenko, Zubin Jacob Nov 2008

Solutions In Folded Geometries, And Associated Cloaking Due To Anomalous Resonance, Graeme W. Milton, Nicolae-Alexandru P. Nicorovici, Ross C. Mcphedran, Kirill Cherednichenko, Zubin Jacob

Birck and NCN Publications

Solutions for the fields in a coated cylinder where the core radius is bigger than the shell radius are seemingly unphysical, but can be given a physical meaning if one transforms to an equivalent problem by unfolding the geometry. In particular, the unfolded material can act as an impedance matched hyperlens, and as the loss in the lens goes to zero finite collections of polarizable line dipoles lying within a critical region surrounding the hyperlens are shown to be cloaked having vanishingly small dipole moments. This cloaking, which occurs both in the folded geometry and the equivalent unfolded one, is …


Toward Nanowire Electronics, Joerg Appenzeller, Joachim Knoch, Mikael Bjoerk, Heike Riel, Heinz Schmid, Walter Riess Nov 2008

Toward Nanowire Electronics, Joerg Appenzeller, Joachim Knoch, Mikael Bjoerk, Heike Riel, Heinz Schmid, Walter Riess

Other Nanotechnology Publications

This paper discusses the electronic transport properties of nanowire field-effect transistors (NW-FETs). Four different device concepts are studied in detail: Schottky-barrier NW-FETs with metallic source and drain contacts, conventional-type NW-FETs with doped NW segments as source and drain electrodes, and, finally, two new concepts that enable steep turn-on characteristics, namely, NW impact ionization FETs and tunnel NW-FETs. As it turns out, NW-FETs are, to a large extent, determined by the device geometry, the dimensionality of the electronic transport, and the way of making contacts to the NW. Analytical as well as simulation results are compared with experimental data to explain …


Structures And Energetics Of Silicon Nanotubes From Molecular Dynamics And Density Functional Theory, Amritanshu Palaria, Gerhard Klimeck, Alejandro Strachan Nov 2008

Structures And Energetics Of Silicon Nanotubes From Molecular Dynamics And Density Functional Theory, Amritanshu Palaria, Gerhard Klimeck, Alejandro Strachan

PRISM: NNSA Center for Prediction of Reliability, Integrity and Survivability of Microsystems

We use molecular dynamics with a first-principles-based force field and density functional theory to predict the atomic structure, energetics, and elastic properties of Si nanotubes. We find various low-energy and low-symmetry hollow structures with external diameters of about 1 nm. These are the most stable structures in this small-diameter regime reported so far and exhibit properties very different from the bulk. While the cohesive energies of the four most stable nanotubes reported here are similar (from 0.638 to 0.697 eV above bulk Si), they have disparate Young's moduli (from 72 to 123 GPa).


Bright-Field Analysis Of Phi29 Dna Packaging Motor Using A Magnetomechanical System, Chun-Li Chang, Hui Zhang, Dan Shu, Peixuan Guo, Cagri A. Savran Oct 2008

Bright-Field Analysis Of Phi29 Dna Packaging Motor Using A Magnetomechanical System, Chun-Li Chang, Hui Zhang, Dan Shu, Peixuan Guo, Cagri A. Savran

Birck and NCN Publications

We report a simple and robust magnetomechanical system for direct visual observation of the DNA packaging behavior of the bacteriophage phi29 in real time. The system comprises a micron-sized magnetic bead attached to the free end of the viral DNA, a magnet and a bright-field microscope. We show that the phi29 DNA packaging activity can be observed and dynamically analyzed at the single molecular level in bright field with a relatively simple system. With this system we also visually demonstrate the phi29 motor transporting a cargo 10 000 times the viral size.


A Parallel Spectral Element Method For Dynamic Three-Dimensional Nonlinear Elasticity Problems, S. Dong, Z. Yosibash Sep 2008

A Parallel Spectral Element Method For Dynamic Three-Dimensional Nonlinear Elasticity Problems, S. Dong, Z. Yosibash

PRISM: NNSA Center for Prediction of Reliability, Integrity and Survivability of Microsystems

We present a high-order method employing Jacobi polynomial-based shape functions, as an alternative to the typical Legendre polynomial-based shape functions in solid mechanics, for solving dynamic three-dimensional geometrically nonlinear elasticity problems. We demonstrate that the method has an exponential convergence rate spatially and a second-order accuracy temporally for the four classes of problems of linear/geometrically nonlinear elastostatics/elastodynamics. The method is parallelized through domain decomposition and message passing interface (MPI), and is scaled to over 2000 processors with high parallel performance.


Level Spectrum Of Single Gated As Donors, Gabriel P. Lansbergen, Rajib Rahman, J. Caro, N. Collaert, S. Biesemans, Gerhard Klimeck, S. Rogge, L.C. L. Hollenberg Jul 2008

Level Spectrum Of Single Gated As Donors, Gabriel P. Lansbergen, Rajib Rahman, J. Caro, N. Collaert, S. Biesemans, Gerhard Klimeck, S. Rogge, L.C. L. Hollenberg

Other Nanotechnology Publications

We study the electrical transport through single As donors incorporated in the channel of a FinFET, i.e. a donor in a three-terminal geometry. By means of spectroscopic measurements in conjuction with a NEMO-3D model, we can identify the excited states and associate them with either the donors Coulomb potential, a triangular well at the interface or a hybridized combination of the two. The correspondence between the transport measurements, the theoretical model and the local environment provides an atomic understanding of actual gated donors in a nanostructure.


Release Of Hydrophobic Molecules From Polymer Micelles Into Cell Membranes Revealed By Forster Resonance Energy Transfer Imaging, Hongtao Chen, Sungwon Kim, Shuyi Wang, Kinam Park, Ji-Xin Cheng May 2008

Release Of Hydrophobic Molecules From Polymer Micelles Into Cell Membranes Revealed By Forster Resonance Energy Transfer Imaging, Hongtao Chen, Sungwon Kim, Shuyi Wang, Kinam Park, Ji-Xin Cheng

Other Nanotechnology Publications

it is generally assumed that polymeric micelles, upon administration into the blood stream, carry drug molecules until they are taken up into cells followed by intracellular release. The current work revisits this conventional wisdom. The study using dual-labeled micelles containing fluorescently labeled copolymers and hydrophobic fluorescent probes entrapped in the polymeric micelle core showed that cellular uptake of hydrophobic probes was much faster than that of labeled copolymers. This result implies that the hydrophobic probes in the core are released from micelles in the extracellular space. Forster resonance energy transfer (FRET) imaging and spectroscopy were used to monitor this process …


Structures And Energetics Of Si Nanotubes From Molecular Dynamics And Density Functional Theory, Amritanshu Palaria, Gerhard Klimeck, Alejandro Strachan May 2008

Structures And Energetics Of Si Nanotubes From Molecular Dynamics And Density Functional Theory, Amritanshu Palaria, Gerhard Klimeck, Alejandro Strachan

Birck and NCN Publications

We use molecular dynamics (MD) with a first principles-based force field (ReaxFF) and density functional theory (DFT) to predict the atomic structure, energetics and elastic propoerties of Si nanotubes. We find various low-energy and low-symmetry hollow structures with external diameters of about 1 nm. These are the most stable structures in this small-diameter regime reported so far and exhibit properties very different from the bulk. While the cohesive energies of the four most stable nanotubes reported here are similar (from 0.638 to 0.697 eV above bulk Si), they have disparate Young's moduli (from 72 to 123 GPa).


Gold Nanorod-Mediated Photothermolysis Induces Apoptosis To Macrophages Via Damage Of Mitochondria, Ling Tong, Ji-Xin Cheng Apr 2008

Gold Nanorod-Mediated Photothermolysis Induces Apoptosis To Macrophages Via Damage Of Mitochondria, Ling Tong, Ji-Xin Cheng

Birck Poster Sessions

Alterations in macrophage functions contribute to a variety of autoimmune and inflammatory diseases. Diagnosis and eradication of activated macrophages is becoming a valid pharmaceutical target. In this work, gold nanorods conjugated with arginine-rich peptides were applied as theragonosis agents to detect activated macrophages via two-photon luminescence (TPL) and subsequent eradicate through optical hyperthermia. Functionalized gold nanorods could be selectively internalized by activated macrophages in live animals 0.5 h after intraperitoneal (i.p.) injection. Apoptosis of macrophage was induced under proper irradiation conditions to reduce secondary inflammation, through mitochondria-dependent pathway.


Water-Soluble Iron Oxide Nanoparticles For Nanomedicine, Christy L. Cooper, Lisa M. Reece, J Key, Donald E. Bergstrom, James F. Leary Apr 2008

Water-Soluble Iron Oxide Nanoparticles For Nanomedicine, Christy L. Cooper, Lisa M. Reece, J Key, Donald E. Bergstrom, James F. Leary

Birck Poster Sessions

Monodisperse iron oxide nanoparticles (MION) are easily synthesized in organic solvents for industrial applications. However, biological applications require that the particles by readily dispersed in aqueous solutions. To improve their dispersion in aqueous solution, MION particles can be conjugated to water soluble polymers. These water soluble particles can then be used for nanomedicine, which utilizes nanometer scale constructs to treat diseases at the cellular level. Here we report the synthesis of a monodisperse iron oxide nanoparticle construct for breast cancer applications.


Outperforming The Conventional Scaling Rules In The Quantum-Capacitance Limit, Joachim Knoch, W Riess, Joerg Appenzeller Apr 2008

Outperforming The Conventional Scaling Rules In The Quantum-Capacitance Limit, Joachim Knoch, W Riess, Joerg Appenzeller

Other Nanotechnology Publications

We present a study on the scaling behavior of field-effect transistors in the quantum-capacitance limit (QCL). It will be shown that a significant performance improvement in terms of the power delay product can be obtained in devices scaled toward the QCL. As a result, nanowires or nanotubes exhibiting a 1-D transport are a premier choice as active channel materials for transistor devices since the QCL can be attained in such systems.


Determination Of The Eigenstates And Wavefunctions Of A Single Gated As Donor, Gabriel P. Lansbergen, R. Rahman, C. J. Wellard, P. E. Rutten, J. Caro, I. Woo, N. Colleart, S. Biersemans, Gerhard Klimeck Feb 2008

Determination Of The Eigenstates And Wavefunctions Of A Single Gated As Donor, Gabriel P. Lansbergen, R. Rahman, C. J. Wellard, P. E. Rutten, J. Caro, I. Woo, N. Colleart, S. Biersemans, Gerhard Klimeck

Other Nanotechnology Publications

Current semiconductor devices have been scaled to such dimensions that we need take atomistic approach to understand their operation for nano-electronics. From a bottomsup perspective, the smallest functional element within a nanodevice would be a single (dopant) atom itself. Control and understanding over the eigenenergies and wavefunctions of a single dopant could prove a key ingredient for device technology beyond-CMOS. Here, we will discuss the eigenlevels of a single As donor in a three terminal configuration. The donor is incorporated in the channel of prototype transistors called FinFETs. The measured eigenlevels are shown to consist of levels associated with the …


Nanopatterning Using Nsom Probes Integrated With High Transmission Nanoscale Bowtie Aperture, Nicholas Murphy-Dubay, Liang Wang, Edward C. Kinzel, Sreemanth Mv Uppuluri, Xianfan Xu Feb 2008

Nanopatterning Using Nsom Probes Integrated With High Transmission Nanoscale Bowtie Aperture, Nicholas Murphy-Dubay, Liang Wang, Edward C. Kinzel, Sreemanth Mv Uppuluri, Xianfan Xu

Birck and NCN Publications

Nanoscale ridge aperture antennas have been shown to have high transmission efficiency and confined nanoscale radiation in the near field region compared with regularly-shaped apertures. The radiation enhancement is attributed to the fundamental electric-magnetic field propagating in the TE10 mode concentrated in the gap between the ridges. This paper reports experimental demonstration of field enhancement using such ridge antenna apertures in a bowtie shape for the manufacture of nanometer size structures using an NSOM (near field scanning optical microscopy) probe integrated with nanoscale bowtie aperture. Consistent lines with width of 59 nm and as small as 24 nm have be …


Externally Assembled Gate-All-Around Carbon Nanotube Field-Effect Transistor, Zhihong Chen, Damon Farmer, Sheng Xu, Roy Gordon, Phaedon Avouris, Joerg Appenzeller Feb 2008

Externally Assembled Gate-All-Around Carbon Nanotube Field-Effect Transistor, Zhihong Chen, Damon Farmer, Sheng Xu, Roy Gordon, Phaedon Avouris, Joerg Appenzeller

Other Nanotechnology Publications

In this letter, we demonstrate a gate-all-around single-wall carbon nanotube field-effect transistor. This is the first successful experimental implementation of an off-chip gate and gate-dielectric assembly with subsequent deposition on a suitable substrate. The fabrication process and device measurements are discussed in the letter. We also argue in how far charges in the gate oxide are responsible for the observed nonideal device performance.


Carbon Nanotubes For High-Performance Electronics - Progress And Prospect, Joerg Appenzeller Feb 2008

Carbon Nanotubes For High-Performance Electronics - Progress And Prospect, Joerg Appenzeller

Other Nanotechnology Publications

Carbon nanotube devices offer intrinsic advantages for high-performance logic device applications. The ultrasmall body of a carbon nanotube-the tube diameter-is the key feature that should allow aggressive channel length scaling, while the intrinsic transport properties of the nanotube ensure at the same time high on-currents. in addition, the narrowness of the tube is critical to implementation of novel device concepts like the tunneling transistor. By understanding the unique capabilities of carbon nanotubes and using them in unconventional designs, novel nanoelectronic applications may become feasible. However, much better control of materials quality must be obtained, and new fabrication processes must be …


Influence Of Phonon Scattering On The Performance Of P-I-N Band-To-Band Tunneling Transistors, Siyuranga O. Koswatta, Mark S. Lundstrom, Dmitri E. Nikonov Jan 2008

Influence Of Phonon Scattering On The Performance Of P-I-N Band-To-Band Tunneling Transistors, Siyuranga O. Koswatta, Mark S. Lundstrom, Dmitri E. Nikonov

Other Nanotechnology Publications

Power dissipation has become a major obstacle in performance scaling of modern integrated circuits and has spurred the search for devices operating at lower voltage swing. In this letter, we study p-i-n band-to-band tunneling field effect transistors taking semiconducting carbon nanotubes as the channel material. The on current of these devices is mainly limited by the tunneling barrier properties, and phonon-scattering has only a moderate effect. We show, however, that the off current is limited by phonon absorption assisted tunneling, and thus is strongly temperature dependent. Subthreshold swings below the 60 mV/decade conventional limit can be readily achieved even at …