Engineering Commons^™

The Advancement Of Experimental And Computation Tools For The Study Of Molten Salt Chemistry To Facilitate The Extraction Of Strategic Elements In Nuclear Applications, Michael Stoddard

Theses and Dissertations

Nuclear energy presents environmental benefits, yet the challenge of radioactive waste management persists. Advanced solutions, such as Molten Salt Reactors (MSRs), require a more profound understanding of molten salt chemistry. This research aims to develop tools, including a depletion simulator, molten salt electrochemical simulator, and a fluoride-based thermodynamic reference electrode for electrochemical purification. The computationally inexpensive depletion simulator allows for exploration into extraction and processing strategies for molten salt reactors. An illustrative case study on Mo-99 production from MSRs demonstrates the practical application of the theoretical framework, emphasizing the need for optimization in extraction effectiveness and separation difficulty. The electrochemical …

Uncertainty Quantification Framework For Design Optimization, Austin Ryan Williams

Masters Theses

Difficulty to obtain neutron sources of interest have driven the need for optimization
techniques to tailor a neutron generator as a replacement. A proposed solution uses
off-the-shelf neutron sources coupled with an energy-tuning assembly to mimic the
source of interest (i.e. AmLi, AmBe, thermonuclear fission spectra, etc.). These
energy-tuning assemblies have been designed with complex optimization algorithms
coupled with Monte Carlo simulations. These new system surrogate designs often
do not have an experimental counterpart for validation and comparison, and lack
non-statistical uncertainties. This work aims to improve confidence in the predictions
by providing a tool for fast uncertainty quantification to …

Remote Laboratory For Nuclear Security Education, Anthony R. Galindo, Craig Marianno

International Journal of Nuclear Security

Laboratory experiences for online students are very limited. To fill this gap, educators in the Department of Nuclear Engineering at Texas A&M University developed a series of radiation detection experiments for their remote students. Radiation detection is only one piece of nuclear security. The objective of the current research is to describe the development and execution of three online laboratories that investigate the basic application of physical security sensors that use light, ultrasonics, and heat to detect adversaries. This laboratory complements lecture material from the department’s Nuclear Security System and Design course. Using the Remote Desktop Application, students connect to …

Selection Of Materials For A Nuclear Rocket Engine, Marcos Fernandez-Tous

AI Assignment Library

Selection of materials which will be used in the construct of a nuclear reactor for a space rocket.

Fabrication, Measurements, And Modeling Of Semiconductor Radiation Detectors For Imaging And Detector Response Functions, Corey David Ahl

Doctoral Dissertations

In the first part of this dissertation, we cover the development of a diamond semiconductor alpha-tagging sensor for associated particle imaging to solve challenges with currently employed scintillators. The alpha-tagging sensor is a double-sided strip detector made from polycrystalline CVD diamond. The performance goals of the alpha-tagging sensor are 700-picosecond timing resolution and 0.5 mm spatial resolution. A literature review summarizes the methodology, goals, and challenges in associated particle imaging. The history and current state of alpha-tagging sensors, followed by the properties of diamond semiconductors are discussed to close the literature review. The materials and methods used to calibrate the …

Total Absorption Spectroscopy Of Mo-106 And Tc-106, Michael Cooper

Doctoral Dissertations

Total absorption spectroscopy is a method of gamma-ray spectroscopy that has gained prominence in the past several decades, as nuclear data revisions are performed on older nuclear data, which is often incomplete. A strong understanding of underlying nuclear data, particularly fission and beta decay data, is essential for nuclear reactors and nuclear fuel decay heat. This PhD work involves the analysis of fission fragments 106Mo [Mo-106] and 106Tc [Tc-106]. These neutron rich isotopes contribute upwards of 6% of the cumulative fission yield of 241Pu [Pu-241] fission, and 4% of 239Pu [Pu-239] fission. Prior data for these two fission fragments only …

Examination Of Hypothetical Transportation Accidents For Transportable Nuclear Power Plants, Richard Louis Calvin

Masters Theses

The reintroduction of Transportable Nuclear Power Plants (TNPPs) opens the doors for potential accidents which have not been previously considered under current licensing standards. TNPPs transported via truck, rail, aircraft, or boat may be involved in various hypothetical transportation accidents. 10 CFR 71, Packaging and Transportation of Radioactive Material, regulatorily addresses various accident scenarios. However, when applying logistics and design constraints alternative methods to license and transport these TNPPs will be required. These alternative methods require the use of Probabilistic Risk Assessments, modeling of accident scenarios, and experimental data to demonstrate an equivalent level of safety to 10 CFR 71. …

Determination Of Near-Sol Carbon Impurity Content Due To Divertor Target Leakage Using Carbon-13 Tracers Via Methane Injection On The Diii-D Tokamak, Jonah David Duran

Doctoral Dissertations

Experiments with outer strike point injection of isotopically enriched methane (¹³CD­₄) in DIII-D L-mode discharges have demonstrated the ability to infer near scrape-off-layer (SOL) impurity density profiles based on: far-SOL collector probe (CP) measurements; a stable isotopic mixing model; and SOL impurity transport modelling. This work enables one of the first in-depth investigations on the source and transport of SOL impurities which could hinder performance of future fusion devices. Modelling by DIVIMP and 3DLIM of ¹³C SOL evolution is consistent with diagnostic observations and indicates that the buildup of injected impurities on plasma-facing surfaces must …

Multi-Objective Optimization Of The Fast Neutron Source By Machine Learning, John L. Pevey

Doctoral Dissertations

The design and optimization of nuclear systems can be a difficult task, often with prohibitively large design spaces, as well as both competing and complex objectives and constraints. When faced with such an optimization, the task of designing an algorithm for this optimization falls to engineers who must apply engineering knowledge and experience to reduce the scope of the optimization to a manageable size. When sufficient computational resources are available, unsupervised optimization can be used.

The optimization of the Fast Neutron Source (FNS) at the University of Tennessee is presented as an example for the methodologies developed in this work. …

A Bulk Driven Transimpedance Cmos Amplifier For Sipm Based Detection, Shahram Hatefi Hesari

Masters Theses

The contribution of this work lies in the development of a bulk driven operational
transconducctance amplifier which can be integrated with other analog circuits and
photodetectors in the same chip for compactness, miniaturization and reducing the
power. Silicon photomultipliers, also known as SiPMs, when coupled with scintillator materials are used in many imaging applications including nuclear detection. This thesis discuss the design of a bulk-driven transimpedance amplifier suitable for detectors where the front end is a SiPM. The amplifier was design and fabricated in a standard standard CMOS process and is suitable for integration with CMOS based SiPMs and commercially …

Design And Evaluation Of A Unique Weighted-Sum-Based Anger Camera, Matthew W. Seals

Masters Theses

Anger camera imaging technology has become widely popular for neutron diffraction imaging due to recent shortages in Helium-3 (He-3). Research into neutron diffraction optimized Anger camera by the Oak Ridge National Laboratory (ORNL) detectors group has provided an alternative to He-3 Tube-based detectors with a high-resolution Anger camera. However, the cost of these high-resolution Anger camera technology can make it less attractive than He-3 tubes when a large Field of View (FOV) is desired. Currently, there is a need for a lower-cost alternative to this high-resolution anger camera. Further applications for Anger camera have become of interest with the advent …

Enigma - Ongoing Development Towards Novel Beta-Decay Spectroscopy Station At Isolde, Philipp Wagenknecht

Masters Theses

Beta decay and collinear laser spectroscopy are proven efficient tools to study nuclear structure far from stability. Two areas of significance are investigations into nuclear deformation and shape coexistence, as well as delayed neutron emissions used in nuclear energy applications. This contribution presents the ongoing development towards a novel beta-decay spectroscopy station for the VITO experiment at CERN’s radioactive ion beam facility ISOLDE. The setup will utilize both collinear laser spectroscopy and beta-decay spectroscopy to measure the energy and spin-parities of the ground and excited states of radioactive beams. Initial designs of the support structure, magnetic field, and detector array …

Particle Swarm Optimization For Critical Experiment Design, Cole Michael Kostelac

Masters Theses

“Critical experiments are used by nuclear data evaluators and criticality safety engineers to validate nuclear data and computational methods. Many of these experiments are designed to maximize the sensitivity to a certain nuclide-reaction pair in an energy range of interest. Traditionally, a parameter sweep is conducted over a set of experimental variables to find a configuration that is critical and maximally sensitive. As additional variables are added, the total number of configurations increases exponentially and quickly becomes prohibitively computationally expensive to calculate, especially using Monte Carlo methods.

This work presents the development of a particle swarm optimization algorithm to design …

Modeling Pa-233 Generation In Thorium-Fueled Reactors For Safeguards, Victoria Davis

Theses and Dissertations

Thorium has been researched for many decades as a possible alternative to uranium nuclear fuel. Thorium can be implemented in many different reactor designs including pressurized water reactors (PWRs), pressurized heavy water reactors (PHWRs), and molten salt reactors (MSRs). Its abundance in the earth, decreased long-lived transuranic waste, and claims that there are fewer proliferation concerns contribute to the attractiveness of using thorium as alternative nuclear fuel. However, possible proliferation pathways have been noted and must be investigated, particularly the potential diversion of ²³³Pa which can then decay to ²³³U – special fissionable material that should be under …

Feasibility Of A Critical Experiment Utilizing Uranium Dioxide-Beryllium Oxide With Neutron Spectrum Shifting Capabilities, Ashley Rachel Raster

Masters Theses

“The goal of this project is to determine the feasibility of utilizing Annular Core Research Reactor (ACRR) fuel in core design with Sandia Pulse Reactor Facility’s (SPRF) Seven Percent Critical Experiment (7uPCX) fuel rods as driver fuel for a critical experiment facility to support future critical and benchmark experiments for the International Criticality Safety Benchmark Evaluation Project (ICSBEP) handbook. This is part of the Critical Experiment Design (CED) process for future criticality experiments. These criticality experiment designs have the main goal of being performed in the same facility at different neutron energy ranges. To test the feasibility of this experiment …

Purification Of I-129 From Spent Pwr Fuel, Sydney B. Whitaker, Kaitlyn Pierson, Kaylie Richard, Samantha Cahill

Chancellor’s Honors Program Projects

No abstract provided.

Surrogate Optimization Model For An Integrated Regenerative Methanol Transcritical Cycle, Yili Zhang

All Graduate Theses and Dissertations, Spring 1920 to Summer 2023

In order to reduce the cost ($) per megawatts hour (MWh) of electrical energy generated by a nuclear power cycle with a novel small modular reactor (SMR), a new SMR-based nuclear power cycle with Methanol as working fluid was designed. It was built virtually with the Python & Coolprop software based on all components’ physical properties, and it is therefore called the physics-based model. The physics-based model would require seven user-defined values as input for the seven free design parameters, respectively. The physics-based model outcomes include LCOE (the cost per megawatts hour of electrical energy generated by the …

Equations Of State For Warm Dense Carbon From Quantum Espresso, Derek J. Schauss

Theses and Dissertations

Warm dense plasma is the matter that exists, roughly, in the range of 10,000 to 10,000,000 Kelvin and has solid-like densities, typically between 0.1 and 10 grams per centimeter. Warm dense fluids like hydrogen, helium, and carbon are believed to make up the interiors of many planets, white dwarfs, and other stars in our universe. The existence of warm dense matter (WDM) on Earth, however, is very rare, as it can only be created with high-energy sources like a nuclear explosion. In such an event, theoretical and computational models that accurately predict the response of certain materials are thus very …

Structural Health Monitoring Of Pipelines In Radioactive Environments Through Acoustic Sensing And Machine Learning, Michael Thompson

FIU Electronic Theses and Dissertations

Structural health monitoring (SHM) comprises multiple methodologies for the detection and characterization of stress, damage, and aberrations in engineering structures and equipment. Although, standard commercial engineering operations may freely adopt new technology into everyday operations, the nuclear industry is slowed down by tight governmental regulations and extremely harsh environments. This work aims to investigate and evaluate different sensor systems for real-time structural health monitoring of piping systems and develop a novel machine learning model to detect anomalies from the sensor data. The novelty of the current work lies in the development of an LSTM-autoencoder neural network to automate anomaly detection …

Introducing The Journal Of Nuclear Engineering: An Interdisciplinary Open Access Journal Dedicated To Publishing Research In Nuclear And Radiation Sciences And Applications, Dan Gabriel Cacuci

Faculty Publications

Note: In lieu of an abstract, this is an excerpt from the first page.

In 1938, Strassmann, Hahn and Meitner discovered neutron-induced nuclear fission in uranium, forever changing our world and opening multiple paths to developing nuclear energy, nuclear medicine, instrumentation, space propulsion, environmental monitoring, remediation and nuclear security [...]

Mechanical Properties Of Permanent Foaming Fixatives For Deactivation & Decommissioning Activities, Tristan Maximilian Simoes-Ponce

FIU Electronic Theses and Dissertations

The Department of Energy is investigating fixative technologies that encapsulate and/or immobilize residual contamination in voids during deactivation and decommissioning (D&D). These technologies must have adequate mechanical and adhesion properties to withstand seismic activity that may occur. One solution is the implementation of polyurethane foams used as permanent foaming fixatives (PFF), specifically intumescent foams that contain expandable graphite, making them fire resistant when exposed to extreme heat conditions.

Tensile, compression, seismic, and tensile adhesion testing was done on six commercial-off-the-self polyurethane foams to determine if the expandable graphite and other filler intumescent technologies improve its mechanical limits. It was found …

Automatic Ventricular Nuclear Magnetic Resonance Image Processing With Deep Learning, Binbin Yong, Chen Wang, Jun Shen, Fucun Li, Hang Yin

Faculty of Engineering and Information Sciences - Papers: Part A

Cardiovascular diseases (CVD) seriously threaten the health of human beings, and they have caused widespread concern in recent years. At present, the diagnosis of CVD is mainly conducted by computed tomography (CT), echocardiography and nuclear magnetic resonance (NMR) technologies. NMR imaging technology is widely used in medical applications owing to its characteristics of high resolution and very low radiation. However, manual NMR image segmentation is time-consuming and error-prone, which has led to the research on automatic NMR image segmentation technologies. Researchers tend to explore the ventricular NRM image segmentation to improve the accuracy of CVD diagnosis. In this study, based …

Reducing Material Attractiveness Utilizing Pu-238 And U-232, Cody Lloyd

Theses and Dissertations

Decreasing the material attractiveness of uranium and plutonium materials is crucial to nuclear nonproliferation. The International Atomic Energy Agency (IAEA) implements safeguards across the world on a limited budget. Not only does decreasing material attractiveness reduce the possibility of proliferation, but also may lighten the financial burden on the IAEA if safeguards can be reduced. Two particular isotopes that have negative material attractiveness traits are ²³⁸Pu and ²³²U. Without isotopic separation technology, these isotopes cannot be removed from plutonium and uranium materials respectively. Both ²³⁸Pu and ²³²U produce large quantities of heat by alpha decay. High …

The Cuntz–Toeplitz Algebras Have Nuclear Dimension One, Philip Easo, Esperanza Garijo, Sarunas Kaubrys, David Nkansah, Martin Vrabec, David Watt, Cameron Wilson, Christian Bonicke, Samuel Evington, Marzieh Forough, Sergio Giron Pacheco, Nicholas Seaton, Stuart White, Michael F. Whittaker, Joachim Zacharias

Faculty of Engineering and Information Sciences - Papers: Part B

We prove that unital extensions of Kirchberg algebras by separable stable AF algebras have nuclear dimension one. The title follows.

Analysis Of Energy Economy In Muon Catalyzed Fusion Considering External X-Ray Reactivation, Nishant Raghav Pillai

Masters Theses

"An analysis of the energy economy of a theoretical muon-catalyzed nuclear fusion system has been made by invoking the use of point kinetic equations, Monte Carlo radiation transport simulations, and from a review of existing literature on muon-catalyzed fusion. An external X-ray reactivation source is proposed as a novel way to increase the number of fusions per muon and thereby overcome the so-called alpha sticking problem that has long been considered the primary impediment to breakeven muon-catalyzed fusion power. Free electron lasers, synchrotrons and Wakefield accelerators are discussed as possible bright X-ray photon sources. The addition of an intense external …

A Case Study: The First Coastal Nuclear Decommissioning Project In California, Willie Aaron Quiros

Construction Management

San Onofre Nuclear Generating System (SONGS) is one of two nuclear power plants in California. Since the shut down in 2012, there is only one actively remaining, Diablo Canyon Nuclear Power Plant, which is set to shut down in 2024. This paper will examine the decommissioning of SONGS thus far; the first coastal nuclear decommissioning project in California’s stringent permitting process. This project was awarded as a joint venture to AECOM and Energy Solutions, both having experiencing in the field of nuclear decommissioning. This paper will outline what nuclear decommissioning challenges have been in the past; general steps of decommissioning …

The Effect Of Flinak Molten Salt Corrosion On The Hardness Of Hastelloy N, David Kok

Scholar Week 2016 - present

The Molten Salt Reactor (MSR) has been identified as a promising candidate to replace aging nuclear reactors around the world. However, a suitable combination of molten salt and container material needs to be found in order to reduce the potential for corrosion in the MSR before it can be considered commercially viable. FLiNaK molten salt and the nickel-based alloy Hastelloy N have been identified as prime candidates for this function, but the severity of FLiNaK corrosion in Hastelloy N requires additional study before this combination can be used in the operation of a MSR. In this study, Hastelloy N samples …

The Effect Of Flinak Molten Salt Corrosion On The Hardness Of Hastelloy N, David Kok

Honors Program Projects

The desire to reduce pollution caused by electricity production has led to a call for the replacement of conventional fossil fuel power plants. In order to fulfill this goal, a large amount of new nuclear reactors is required, and this provides the opportunity to put new and innovative reactor designs into production. The Molten Salt Reactor (MSR) is one of the most promising concepts, but a suitable combination of molten salt and container material needs to be found to reduce the potential for corrosion before the concept can be put into production. FLiNaK molten salt and the nickel-based alloy Hastelloy …

Electrochemical Separation Of Multivalent Species On A Liquid Bismuth Cathode In Licl-Kcl Eutectic For Used Nuclear Fuel Reprocessing, Michael Woods

Theses and Dissertations

The presence of group I/II fission products (Cs-137, Sr-90, and Ba-137) within molten salt nuclear processes degrades operational efficiencies by contributing to increased radiation levels in the case of material handling processes or to loss of criticality in the case of a reactor. While methods such as zone freezing and ion exchange have been proven for the separation of these fission products in LiCl-KCl salts, they require extra equipment and processing steps. Addition of a liquid metal electrode to molten salt media, such as the electrorefiner of a pyroprocessing scheme or the salt cleaning stage of a molten salt fast …

A Security Approach For The Example Sodium Fast Reactor, Christian X. Young, Robert S. Bean

The Summer Undergraduate Research Fellowship (SURF) Symposium

Increases in the spread of nuclear technology and the rise of non-state terrorism in the modern era has proved the need for effective security approaches to new nuclear facilities. Many documents about security approaches for nuclear plants are non-public material, however, making it difficult to teach others about the basics of security design. To alleviate this issue, we used available texts in the security realm to design a security approach for the Generation IV International Forum’s Example Sodium Fast Reactor. Our approach utilized infrared, microwave, fiber optic, and other advanced technologies to provide security for the special nuclear material present. …