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Full-Text Articles in Physics

Determining Magnetic Nanoparticle Size Distributions From Thermomagnetic Measurements., R. S. Dipietro, H. G. Johnson, S. P. Bennett, T. J. Nummy, L. H. Lewis, D. Heiman Dec 2011

Determining Magnetic Nanoparticle Size Distributions From Thermomagnetic Measurements., R. S. Dipietro, H. G. Johnson, S. P. Bennett, T. J. Nummy, L. H. Lewis, D. Heiman

Donald Heiman

Thermomagnetic measurements are used to obtain the size distribution and anisotropy of magnetic nanoparticles. An analytical transformation method is described which utilizes temperature-dependent zero-field cooling magnetization data to provide a quantitative measurement of the average diameter and relative abundance of superparamagnetic nanoparticles. Applying this method to self-assembled MnAs nanoparticles in MnAs–GaAs composite films reveals a log-normal size distribution and reduced anisotropy for nanoparticles compared to bulk materials. This analytical technique holds promise for rapid assessment of the size distribution of an ensemble of superparamagnetic nanoparticles.


Magnetotransport Properties Of Mn-Si-C Based Nanostructures, Sungmu Kang, Greg A. Brewer, Battogtokh Jugdersuren, Robert Dipietro, Don Heiman, Andrew C. Buechele, David A. Mckeown, Ian L. Pegg, John Philip Dec 2011

Magnetotransport Properties Of Mn-Si-C Based Nanostructures, Sungmu Kang, Greg A. Brewer, Battogtokh Jugdersuren, Robert Dipietro, Don Heiman, Andrew C. Buechele, David A. Mckeown, Ian L. Pegg, John Philip

Donald Heiman

Boron-incorporated Mn5SiC nanowires were grown using chemical vapor deposition method. The nanowire cluster exhibits magnetic hysteresis loops at room temperature and the strength of the magnetic behavior depends on the concentration of the boron incorporation. Mn5SiC nanowire-based devices exhibit spin dependent transport properties which shows significant changes with boron content. Large magnetoresistance is observed in lightly boron-incorporated nanowire devices and it decreases with increase in boron content.


Magnetic Signature Of Symmetry Reduction In Epitaxial La₀.₆₇Sr₀.₃₃Mno₃ Films, Radhika Barua, L. H. Lewis, D. Heiman Dec 2011

Magnetic Signature Of Symmetry Reduction In Epitaxial La₀.₆₇Sr₀.₃₃Mno₃ Films, Radhika Barua, L. H. Lewis, D. Heiman

Donald Heiman

The magnetic properties of epitaxially grown La0.67Sr0.33MnO3 perovskite thin films were investigated to elucidate an unexpected broken symmetry between orthogonal [100] and [010] inplane directions, resulting from the magnetostructural coupling between the film and the cubic SrTiO3 (001) substrate. The films were synthesized by molecular beam epitaxy with either complete or zero A-site cation disorder. Magnetization measured in [100] and [010] directions shows differences that signal a reduction of the in-plane cubic symmetry only for T < 290 K. The magnetization asymmetry is more robust in the film with complete A-site disorder. These results are attributed to a dominant Mn3+ character …


Universal Properties Of Linear Magnetoresistance In Strongly Disordered Mnas-Gaas Composite Semiconductors, H. Johnson, S. Bennett, R. Barua, L. Lewis, D. Heiman Dec 2011

Universal Properties Of Linear Magnetoresistance In Strongly Disordered Mnas-Gaas Composite Semiconductors, H. Johnson, S. Bennett, R. Barua, L. Lewis, D. Heiman

Donald Heiman

Linear magnetoresistance (LMR) occurs in semiconductors as a consequence of strong electrical disorder and is characterized by nonsaturating magnetoresistance that is proportional to the applied magnetic field. By investigating a disordered MnAs-GaAs composite material, it is found that the magnitude of the LMR is numerically equal to the carrier mobility over a wide range and is independent of carrier density. This behavior is complementary to the Hall effect that is independent of the mobility and dependent on the carrier density. Moreover, the LMR appears to be insensitive to the details of the disorder and points to a universal explanation of …


Large Low Field Magnetoresistance In La₀.₆₇Sr₀.₃₃Mno₃ Nanowire Devices, Battogtokh Jugdersuren, Sungmu Kang, Robert S. Dipietro, Don Heiman, David Mckeown, Ian L. Pegg, John Philip Dec 2011

Large Low Field Magnetoresistance In La₀.₆₇Sr₀.₃₃Mno₃ Nanowire Devices, Battogtokh Jugdersuren, Sungmu Kang, Robert S. Dipietro, Don Heiman, David Mckeown, Ian L. Pegg, John Philip

Donald Heiman

Large low field magnetoresistance (LFMR) of about 28% is observed in La0.67Sr0.33MnO3 nanowires with 80 nm in diameter at T = 300 K. A gradual decrease in the LFMR has been found with increase in wire diameter. The LFMR drops to zero for wires above 280 nm in diameter. The nanowires are grown by means of electrospinning process and exhibit distorted orthorhombic crystal structure. The large LFMR is considered as a grain boundary effect as observed in several perovskite systems. The large LFMR observed in these manganites with reduced dimensions may be useful for room temperature device applications.


Large Coercivity In Nanostructured Rare-Earth-Free Mnxga Films, Don Heiman, Tom Nummy, Steve Bennett, Tom Cardinal Dec 2011

Large Coercivity In Nanostructured Rare-Earth-Free Mnxga Films, Don Heiman, Tom Nummy, Steve Bennett, Tom Cardinal

Donald Heiman

The magnetic hysteresis of MnxGa films exhibit remarkably large coercive fields as high as HC=2.5 T when fabricated with nanoscale particles of a suitable size and orientation. This coercivity is an order of magnitude larger than in well-ordered epitaxial film counterparts and bulk materials. The enhanced coercivity is attributed to the combination of large magnetocrystalline anisotropy and ~50-100 nm size nanoparticles. The large coercivity is also replicated in the electrical properties through the anomalous Hall effect. The magnitude of the coercivity approaches that found in rare-earth magnets, making them attractive for rare-earth-free magnet applications.


Determining Magnetic Nanoparticle Size Distributions From Thermomagnetic Measurements, R. S. Dipietro, H. G. Johnson, S. P. Bennett, T. J. Nummy, L. H. Lewis, D. Heiman Jan 2011

Determining Magnetic Nanoparticle Size Distributions From Thermomagnetic Measurements, R. S. Dipietro, H. G. Johnson, S. P. Bennett, T. J. Nummy, L. H. Lewis, D. Heiman

Donald Heiman

Thermomagnetic measurements are used to obtain the size distribution and anisotropy of magnetic nanoparticles. An analytical transformation method is described which utilizes temperature-dependent zero-field cooling (ZFC) magnetization data to provide a quantitative measurement of the average diameter and relative abundance of superparamagnetic nanoparticles. Applying this method to self-assembled MnAs nanoparticles in MnAs-GaAs composite films reveals a log-normal size distribution and reduced anisotropy for nanoparticles compared to bulk materials. This analytical technique holds promise for rapid assessment of the size distribution of an ensemble of superparamagnetic nanoparticles.