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Full-Text Articles in Physics

Conducting Polyelectrolyte Complexes: Assembly, Structure, And Transport, Michael A. Leaf Nov 2017

Conducting Polyelectrolyte Complexes: Assembly, Structure, And Transport, Michael A. Leaf

Doctoral Dissertations

Decades of progress have yielded a tremendous variety of organic electronics, with great strides in the development of photovoltaics, thermoelectrics and other flexible devices. Ubiquitous in these research areas are films of poly(3,4-ethylenedioxythiophene): poly(styrenesulfonic acid) (PEDOT: PSS), a complex of oppositely-charged polyelectrolytes initially suspended in water before film formation. This material has high electronic conductivity and good water processability. Pristine film conductivity is somewhat low, but is dramatically enhanced through simple treatments like ionic liquid addition or shear. Can this enhancement be understood so that further optimization might render PEDOT: PSS commercially viable? PEDOT: PSS is a complicated material, with …


Angular Distribution Of Single-Photon Superradiance In A Dilute And Cold Atomic Ensemble, A. S. Kuraptsev, I. M. Sokolov, M. D. Havey Aug 2017

Angular Distribution Of Single-Photon Superradiance In A Dilute And Cold Atomic Ensemble, A. S. Kuraptsev, I. M. Sokolov, M. D. Havey

Physics Faculty Publications

On the basis of a quantum microscopic approach we study the dynamics of the afterglow of a dilute Gaussian atomic ensemble excited by pulsed radiation. Taking into account the vector nature of the electromagnetic field we analyze in detail the angular and polarization distribution of single-photon superradiance of such an ensemble. The dependence of the angular distribution of superradiance on the length of the pulse and its carrier frequency as well as on the size and the shape of the atomic clouds is studied. We show that there is substantial dependence of the superradiant emission on the polarization and the …