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Atomic, Molecular and Optical Physics

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Rydberg atoms

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Density Dependence And Dynamics Of Dipole-Dipole Interactions Among Rydberg Atoms, Hannah Conley Jul 2023

Density Dependence And Dynamics Of Dipole-Dipole Interactions Among Rydberg Atoms, Hannah Conley

Physics and Astronomy Summer Fellows

After trapping atoms, exciting them to an initial high-energy Rydberg state, and allowing them a brief time to exchange energy with each other through dipole-dipole interactions, we observe how their energies are redistributed among various energy levels. The measurements we make in this physical experiment do not give insight into how individual atoms interact or metrics like fidelity and entanglement entropy, which impact our results. For this reason, it is useful to compare our results from the physical experiment to those of our simulation on a supercomputer, in which we can track the final and initial energy of individual atoms …


Time Dependence Of Few-Body Forster Interactions Among Ultracold Rydberg Atoms, Zhimin Cheryl Liu, Nina P. Inman, Thomas J. Carroll, Michael W. Noel Mar 2020

Time Dependence Of Few-Body Forster Interactions Among Ultracold Rydberg Atoms, Zhimin Cheryl Liu, Nina P. Inman, Thomas J. Carroll, Michael W. Noel

Physics and Astronomy Faculty Publications

Rubidium Rydberg atoms in either |mj| sublevel of the 36p3/2 state can exchange energy via Stark-tuned Förster resonances, including two-, three-, and four-body dipole-dipole interactions. Three-body interactions of this type were first reported and categorized by Faoro et al. [Nat. Commun. 6, 8173 (2015)] and their Borromean nature was confirmed by Tretyakov et al. [Phys. Rev. Lett. 119, 173402 (2017)]. We report the time dependence of the N-body Förster resonance N×36p3/2,|mj|=1/2→36s1/2+37s1/2+(N−2)×36p3/2,|mj|=3/2, for N=2, 3, …


Improving The State Selectivity Of Field Ionization With Quantum Control, Vincent C. Gregoric, Jason Bennett, Bianca R. Gualtieri, Ankitha Kannad, Zhimin Cheryl Liu, Zoe A. Rowley, Thomas J. Carroll, Michael W. Noel Dec 2018

Improving The State Selectivity Of Field Ionization With Quantum Control, Vincent C. Gregoric, Jason Bennett, Bianca R. Gualtieri, Ankitha Kannad, Zhimin Cheryl Liu, Zoe A. Rowley, Thomas J. Carroll, Michael W. Noel

Physics and Astronomy Faculty Publications

The electron signals from the field ionization of two closely spaced Rydberg states of rubidium-85 are separated using quantum control. In selective field ionization, the state distribution of a collection of Rydberg atoms is measured by ionizing the atoms with a ramped electric field. Generally, atoms in higher energy states ionize at lower fields, so ionized electrons which are detected earlier in time can be correlated with higher energy Rydberg states. However, the resolution of this technique is limited by the Stark effect. As the electric field is increased, the electron encounters numerous avoided Stark level crossings which split the …


Catalysis Of Stark-Tuned Interactions Between Ultracold Rydberg Atoms, A. L. Win, W. D. Williams, Thomas J. Carroll, C. I. Sukenik Sep 2018

Catalysis Of Stark-Tuned Interactions Between Ultracold Rydberg Atoms, A. L. Win, W. D. Williams, Thomas J. Carroll, C. I. Sukenik

Physics and Astronomy Faculty Publications

We have experimentally investigated a catalysis effect in the resonant energy transfer between ultracold 85Rb Rydberg atoms. We studied the time dependence of the process, 34p + 34p → 34s + 35s, and observed an enhancement of 34s state population when 34d state atoms are added.We have also performed numerical model simulations, which are in qualitative agreement with experiment and indicate that the enhancement arises from a redistribution of p-state atoms due to the presence of the d-state atoms.


Detecting Rydberg Interactions With Controlled Ionization, Lauren Yoast Jul 2018

Detecting Rydberg Interactions With Controlled Ionization, Lauren Yoast

Physics and Astronomy Summer Fellows

Rydberg atoms, which have a highly excited outer electron, are easily manipulated by electric fields. Using a magneto-optical trap, we cool Rubidium atoms to a few hundred millionths of a Kelvin above absolute zero and then excite to Rydberg states. Our first project looks at the dipole-dipole interactions of two atoms starting in the 33p state and ending in the 34s and 33s states. The standard technique is to apply an increasing electric field that ionizes the Rydberg electron and sends it to a detector, but unfortunately the signals overlap. A genetic algorithm is used to separate the signals by …


Optimizing An Electron's Path To Ionization Using A Genetic Algorithm, Jason Bennett, Kevin Choice Jul 2017

Optimizing An Electron's Path To Ionization Using A Genetic Algorithm, Jason Bennett, Kevin Choice

Physics and Astronomy Summer Fellows

A Rydberg atom is an atom with a highly excited and weakly bound valence electron. A widespread method of studying quantum mechanics with Rydberg atoms is to ionize the electron and measure its arrival time. We use a Genetic Algorithm (GA) to control the electron's path to ionization. The Rydberg electron's energy levels are strongly shifted by the presence of an electric field. The energy levels shift and curve, but never cross. At an avoided crossing the electron can jump from one level to the next. By engineering the electric field's time dependence, we thereby control the path to ionization. …


Quantum Interference In The Field Ionization Of Rydberg Atoms, Rachel Feynman, Jacob A. Hollingsworth, Michael Vennettilli, Tamas Budner, Ryan Zmiewski, Donald P. Fahey, Thomas J. Carroll, Michael W. Noel Oct 2015

Quantum Interference In The Field Ionization Of Rydberg Atoms, Rachel Feynman, Jacob A. Hollingsworth, Michael Vennettilli, Tamas Budner, Ryan Zmiewski, Donald P. Fahey, Thomas J. Carroll, Michael W. Noel

Physics and Astronomy Faculty Publications

We excite ultracold rubidium atoms in a magneto-optical trap to a coherent superposition of the three |mj | sublevels of the 37d5/2 Rydberg state. After some delay, during which the relative phases of the superposition components can evolve, we apply an electric field pulse to ionize the Rydberg electron and send it to a detector. The electron traverses many avoided crossings in the Stark levels as it ionizes. The net effect of the transitions at these crossings is to mix the amplitudes of the initial superposition into the same final states at ionization. Similar to a Mach-Zehnder interferometer, the three …


Simulations Of The Dipole-Dipole Interaction Between Two Spatially Separated Groups Of Rydberg Atoms, Thomas J. Carroll, Christopher Daniel, Leah Hoover, Timothy Sidie, Michael W. Noel Nov 2009

Simulations Of The Dipole-Dipole Interaction Between Two Spatially Separated Groups Of Rydberg Atoms, Thomas J. Carroll, Christopher Daniel, Leah Hoover, Timothy Sidie, Michael W. Noel

Physics and Astronomy Faculty Publications

The dipole-dipole interaction among ultracold Rydberg atoms is simulated. We examine a general interaction scheme in which two atoms excited to the x and x states are converted to y and y states via a Förster resonance. The atoms are arranged in two spatially separated groups, each consisting of only one species of atom. We monitor the state mixing by recording the fraction of atoms excited to the y state as the distance between the two groups is varied. With zero detuning a many-body effect that relies on always resonant interactions causes the state mixing to have a finite range. …