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2013

Australian Institute for Innovative Materials - Papers

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Full-Text Articles in Physical Sciences and Mathematics

Single-Pulse Terahertz Coherent Control Of Spin Resonance In The Canted Antiferromagnet Yfeo3, Mediated By Dielectric Anisotropy, Zuanming Jin, Zoltan Mics, Guohong Ma, Zhenxiang Cheng, Mischa Bonn, Dmitry Turchinovich Jan 2013

Single-Pulse Terahertz Coherent Control Of Spin Resonance In The Canted Antiferromagnet Yfeo3, Mediated By Dielectric Anisotropy, Zuanming Jin, Zoltan Mics, Guohong Ma, Zhenxiang Cheng, Mischa Bonn, Dmitry Turchinovich

Australian Institute for Innovative Materials - Papers

We report on the coherent control of terahertz (THz) spin waves in a canted antiferromagnet yttrium orthoferrite, YFeO3, associated with a quasiferromagnetic (quasi-FM) spin resonance at a frequency of 0.3 THz, using a single-incident THz pulse. The spin resonance is excited impulsively by the magnetic field component of the THz pulse. The intrinsic dielectric anisotropy of YFeO3 in the THz range allows for coherent control of both the amplitude and the phase of the excited spin wave. The coherent control is based on simultaneous generation of two interfering phase-shifted spin waves whose amplitudes and relative phase, dictated by the dielectric …


The Flux Pinning Mechanism, And Electrical And Magnetic Anisotropy In Fe1.04te0.6se0.4 Superconducting Single Crystal, Mahboobeh Shahbazi-Manshadi, Xiaolin Wang, S X. Dou, H Fang, C T. Lin Jan 2013

The Flux Pinning Mechanism, And Electrical And Magnetic Anisotropy In Fe1.04te0.6se0.4 Superconducting Single Crystal, Mahboobeh Shahbazi-Manshadi, Xiaolin Wang, S X. Dou, H Fang, C T. Lin

Australian Institute for Innovative Materials - Papers

The temperature and magnetic field dependences of the magnetization and critical current density of Fe1.04Te0.6Se0.4 single crystals have been investigated, and the flux pinning mechanism has been analysed. The normalized pinning force (fp Fp/F p,max) vs. h(H/Hirr) curves, are scaled using the Dew-Hughes theory, f(h) ≈ hp(1 - h)q with p 1.35 and q 3.06. The angular dependence of the resistivity under different magnetic fields shows a dip-like structure, below the superconducting transition temperature. The anisotropic value of 2 was obtained using Ginzburg-Landau theory.


Spin Switching And Magnetization Reversal In Single-Crystal Ndfeo3, S J. Yuan, W Ren, F Hong, Y B. Wang, J C. Zhang, L Bellaiche, S X. Cao, G Cao Jan 2013

Spin Switching And Magnetization Reversal In Single-Crystal Ndfeo3, S J. Yuan, W Ren, F Hong, Y B. Wang, J C. Zhang, L Bellaiche, S X. Cao, G Cao

Australian Institute for Innovative Materials - Papers

We report an experimental and computational study of single-crystal NdFeO3, which features two inequivalent magnetic sublattices, namely, Fe and Nd sublattices that are coupled in an antiparallel fashion. This paper reveals that a strong interaction between 3d and 4f electrons of the two sublattices along with a spin-lattice coupling drives an extremely interesting magnetic state that is highly sensitive to the orientation and history of weak magnetic field. The following phenomena are particularly remarkable: (1) sharply contrasting magnetization M(T) along the a and c axes; (2) a first-order spin switching along the a axis below 29 K when the system …


Direct Observation Of Liquid-Like Behavior Of A Single Au Grain Boundary, Gilberto Casillas, Arturo Ponce, Jesus Velazquez-Salazar, M Jose-Yacaman Jan 2013

Direct Observation Of Liquid-Like Behavior Of A Single Au Grain Boundary, Gilberto Casillas, Arturo Ponce, Jesus Velazquez-Salazar, M Jose-Yacaman

Australian Institute for Innovative Materials - Papers

Behavior of matter at the nanoscale differs fromthat of the bulk due to confinement and surface effects. Here, we report a direct observation of liquid-like behavior of a single grain boundary formed by cold-welding Au nanoparticles, 40 nm in size, by mechanical manipulation in situ TEM. The grain boundary rotates almost freely due to the free surfaces and can rotate about 90 degrees. The grain boundary sustains more stress than the bulk, confirming a strong bonding between the nanoparticles.Moreover, this technique allows the measurement of the surface diffusion coefficient from experimental observations, which we compute for the Au nanoparticles. This …


Platinum Electrodeposition On Unsupported Single Wall Carbon Nanotubes And Its Application As Methane Sensing Material, Enid Contes-De Jesus, Diana Santiago, Gilberto Casillas, Alvaro Mayoral, Cesar Magen, Miguel Jose-Yacaman, Jing Li, Carlos R. Cabrera Jan 2013

Platinum Electrodeposition On Unsupported Single Wall Carbon Nanotubes And Its Application As Methane Sensing Material, Enid Contes-De Jesus, Diana Santiago, Gilberto Casillas, Alvaro Mayoral, Cesar Magen, Miguel Jose-Yacaman, Jing Li, Carlos R. Cabrera

Australian Institute for Innovative Materials - Papers

This paper reports the decoration of single wall carbon nanotubes (SWCNTs) with platinum (Pt) nanoparticles using an electrochemical technique, rotating disk slurry electrode (RoDSE). Pt/SWCNTs were electrochemically characterized by cyclic voltammetry technique (CV) and physically characterized through the use of transmission electron microscopy (TEM), energy dispersive spectroscopy - X-ray florescence (EDS-XRF) and X-ray diffraction (XRD). After characterization it was found that electrodeposited nanoparticles had an average particle size of 4.1 ± 0.8 nm. Pt/SWCNTs were used as sensing material for methane (CH4) detection and showed improved sensing properties in a range of concentration from 50 ppm to 200 ppm parts …


Flux Pinning Mechanism In Bafe1.9ni0.1as2 Single Crystals: Evidence For Fluctuation In Mean Free Path Induced Pinning, M Shahbazi-Manshadi, X L Wang, K Y Choi, S X. Dou Jan 2013

Flux Pinning Mechanism In Bafe1.9ni0.1as2 Single Crystals: Evidence For Fluctuation In Mean Free Path Induced Pinning, M Shahbazi-Manshadi, X L Wang, K Y Choi, S X. Dou

Australian Institute for Innovative Materials - Papers

The flux pinning mechanism of BaFe1.9Ni0.1As2 superconducting crystals have been investigated systematically by magnetic measurements up to 13 T at various temperatures. The field dependence of the critical current density, Jc, was analysed within the collective pinning model. A remarkably good agreement between the experimental results and theoretical dl pinning curve is obtained, which indicates that pinning in BaFe1.9Ni0.1As2 crystal originates from spatial variation of the mean free path. Moreover, the normalized pinning force density, Fp, curves versus h1/4B/Birr (Birr is the irreversibility field) were scaled using the Dew-Hughes model. Analysis suggests that point pinning alone cannot explain the observed …


Magnetic Field Induced Discontinuous Spin Reorientation In Erfeo3 Single Crystal, Hui Shen, Zhenxiang Cheng, Fang Hong, Jiayue Xu, Shujuan Yuan, Shixun Cao, Xiaolin Wang Jan 2013

Magnetic Field Induced Discontinuous Spin Reorientation In Erfeo3 Single Crystal, Hui Shen, Zhenxiang Cheng, Fang Hong, Jiayue Xu, Shujuan Yuan, Shixun Cao, Xiaolin Wang

Australian Institute for Innovative Materials - Papers

The spin reorientation of ErFeO3 that spontaneously occurs at low temperature has been previously determined to be a process involving the continuous rotation of Fe3þ spins. In this work, the dynamic process of spin reorientation in ErFeO3 single crystal has been investigated by AC susceptibility measurements at various frequencies and static magnetic fields. Interestingly, two completely discontinuous steps are induced by a relatively large static magnetic field due to the variation in the magnetic anisotropy during this process. It provides deeper insights into the intriguing magnetic exchange interactions which dominate the sophisticated magnetic phase transitions in the orthoferrite systems.


Crystal Growth, Structure And Thermal Properties Of Noncentrosymmetric Single Crystals Prca4o(Bo3)3+, Fapeng Yu, Shujun Zhang, Xiufeng Cheng, Xiulan Duan, Tingfeng Ma, Xian Zhao Jan 2013

Crystal Growth, Structure And Thermal Properties Of Noncentrosymmetric Single Crystals Prca4o(Bo3)3+, Fapeng Yu, Shujun Zhang, Xiufeng Cheng, Xiulan Duan, Tingfeng Ma, Xian Zhao

Australian Institute for Innovative Materials - Papers

Noncentrosymmetric praseodymium calcium oxyborate single crystals, PrCa4O(BO3)3 (PrCOB), were grown by the Czochralski technique. The monoclinic unit cell parameters were found to be a = 8.177 Å, b = 16.157 Å, c = 3.629 Å and Z = 2 with space group Cm. Crystal density was measured using the Archimedes method, being on the order of 3.47 g cm-3. Thermal properties of PrCOB were investigated, where the specific heat was found to be 0.63 J g-1 °C-1 at room temperature, increasing to 0.85 J g-1°C-1 at 700°C. The thermal expansion coefficients were measured to be α11 = 7.99, α22 = …