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Full-Text Articles in Physical Sciences and Mathematics

Interband Transitions And Critical Points Of Single-Crystal Thoria Compared With Urania, Christina Dugan, Lu Wang, Kai Zhang, James M. Mann, Martin M. Kimani, Wai-Ning Mei, Peter A. Dowben, James C. Petrosky Nov 2022

Interband Transitions And Critical Points Of Single-Crystal Thoria Compared With Urania, Christina Dugan, Lu Wang, Kai Zhang, James M. Mann, Martin M. Kimani, Wai-Ning Mei, Peter A. Dowben, James C. Petrosky

Faculty Publications

The interband transitions of UO2 are validated independently through cathode luminescence. A picture emerges consistent with density functional theory. While theory is generally consistent with experiment, it is evident from the comparison of UO2 and ThO2 that the choice of functional can significantly alter the bandgap and some details of the band structure, in particular at the conduction band minimum. Strictly ab initio predictions of the optical properties of the actinide compounds, based on density functional theory alone, continue to be somewhat elusive.


Probing Free Nucleons With (Anti)Neutrinos, Roberto Petti Nov 2022

Probing Free Nucleons With (Anti)Neutrinos, Roberto Petti

Faculty Publications

We discuss a method to study free protons and neutrons using ν()-hydrogen (H) Charged Current (CC) inelastic interactions, together with various precision tests of the isospin (charge) symmetry using ν and CC interactions on both H and nuclear targets. Probing free nucleons with (anti)neutrinos provides information about their partonic structure, as well as a crucial input for the modeling of ν(⊽)-nucleus (A) interactions. Such measurements concurrently represent a valuable tool to address the main limitations of accelerator-based neutrino scattering experiments on nuclear targets, originating from the combined effect of the unknown (anti)neutrino energy and of the …


Separation Of Track- And Shower-Like Energy Deposits In Protodune-Sp Using A Convolutional Neural Network, A. Abed Abud, B. Abi, R, Acciarri, M. A. Acero, M. R. Adames, G. Adamov, M. Adamowski, D. Adams, M. Adinolfi, A. Aduszkiewicz, M. Andreotti, M. Andrews, F. Andrianala, S. Andringa, N. Anfimov, A. Ankowski, M. Antoniassi, M. Antonova, A. Antoshkin, S. Antusch, Roberto Petti, Et. Al. Oct 2022

Separation Of Track- And Shower-Like Energy Deposits In Protodune-Sp Using A Convolutional Neural Network, A. Abed Abud, B. Abi, R, Acciarri, M. A. Acero, M. R. Adames, G. Adamov, M. Adamowski, D. Adams, M. Adinolfi, A. Aduszkiewicz, M. Andreotti, M. Andrews, F. Andrianala, S. Andringa, N. Anfimov, A. Ankowski, M. Antoniassi, M. Antonova, A. Antoshkin, S. Antusch, Roberto Petti, Et. Al.

Faculty Publications

Liquid argon time projection chamber detector technology provides high spatial and calorimetric resolutions on the charged particles traversing liquid argon. As a result, the technology has been used in a number of recent neutrino experiments, and is the technology of choice for the Deep Underground Neutrino Experiment (DUNE). In order to perform high precision measurements of neutrinos in the detector, final state particles need to be effectively identified, and their energy accurately reconstructed. This article proposes an algorithm based on a convolutional neural network to perform the classification of energy deposits and reconstructed particles as track-like or arising from electromagetic …


Tau Neutrinos In The Next Decade: From Gev To Eev, Roshan Mammen Abraham, Jamie Alvarez-Muñiz, Carlos A. Argüelles, Akitaka Ariga, Tomoko Ariga, Adam Aurisano, Dario Autiero, Mary Bishai, Nilay Bostan, Mauricio Bustamante, Austin Cummings, Valentin Decoene, André De Gouvêa, Giovanni De Lellis, Albert De Roeck, Peter B. Denton, Antonia Di Crescenzo, Milind V. Diwan, Yasaman Farzan, Anatoli Fedynitch, Jonathan L. Feng, Laura J. Fields, Alfonso Garcia, Maria Vittoria Garzelli, Julia Gehrlein, Christian Glaser, Katarzyna Grzelak, Steffen Hallmann, Jeremy Hewes, D Indumathi, Ahmed Ismail, Sudip Jana, Yu Seon Jeong, Kevin J. Kelly, Spencer R. Klein, Felix Kling, Thomas Kosc, Umut Kose, D Jason Koskinen, John Krizmanic, Jeff Lazar, Yichen Li, Ivan Martinez-Soler, Irina Mocioiu, Jiwoo Nam, Valentin Niess, Nepomuk Otte, Sameer Patel, Roberto Petti, Et. Al. Oct 2022

Tau Neutrinos In The Next Decade: From Gev To Eev, Roshan Mammen Abraham, Jamie Alvarez-Muñiz, Carlos A. Argüelles, Akitaka Ariga, Tomoko Ariga, Adam Aurisano, Dario Autiero, Mary Bishai, Nilay Bostan, Mauricio Bustamante, Austin Cummings, Valentin Decoene, André De Gouvêa, Giovanni De Lellis, Albert De Roeck, Peter B. Denton, Antonia Di Crescenzo, Milind V. Diwan, Yasaman Farzan, Anatoli Fedynitch, Jonathan L. Feng, Laura J. Fields, Alfonso Garcia, Maria Vittoria Garzelli, Julia Gehrlein, Christian Glaser, Katarzyna Grzelak, Steffen Hallmann, Jeremy Hewes, D Indumathi, Ahmed Ismail, Sudip Jana, Yu Seon Jeong, Kevin J. Kelly, Spencer R. Klein, Felix Kling, Thomas Kosc, Umut Kose, D Jason Koskinen, John Krizmanic, Jeff Lazar, Yichen Li, Ivan Martinez-Soler, Irina Mocioiu, Jiwoo Nam, Valentin Niess, Nepomuk Otte, Sameer Patel, Roberto Petti, Et. Al.

Faculty Publications

Tau neutrinos are the least studied particle in the standard model. This whitepaper discusses the current and expected upcoming status of tau neutrino physics with attention to the broad experimental and theoretical landscape spanning long-baseline, beam-dump, collider, and astrophysical experiments. This whitepaper was prepared as a part of the NuTau2021 Workshop.


Solvation Of Large Polycyclic Aromatic Hydrocarbons In Helium: Cationic And Anionic Hexabenzocoronene, Miriam Kappe, Florent Calvo, Johannes Schöntag, Holger F. Bettinger, Serge Krasnokutski, Martin Kuhn, Elisabeth Gruber, Fabio Zappa, Paul Scheier, Olof E. Echt Oct 2022

Solvation Of Large Polycyclic Aromatic Hydrocarbons In Helium: Cationic And Anionic Hexabenzocoronene, Miriam Kappe, Florent Calvo, Johannes Schöntag, Holger F. Bettinger, Serge Krasnokutski, Martin Kuhn, Elisabeth Gruber, Fabio Zappa, Paul Scheier, Olof E. Echt

Faculty Publications

The adsorption of helium on charged hexabenzocoronene (Hbc, C42H18), a planar polycyclic aromatic hydrocarbon (PAH) molecule of D6h symmetry, is investigated by a combination of high-resolution mass spectrometry and classical and quantum computational methods. The ion abundance of HenHbc+ complexes versus size n features prominent local anomalies at n = 14, 38, 68, 82, and a weak one at 26, indicating that for these “magic” sizes the helium evaporation energies are relatively large. Surprisingly, mass spectra of anionic HenHbc complexes feature a different set of anomalies, namely at …


Oxygen Vacancies In Lib3O5 Crystals And Their Role In Nonlinear Absorption, Brian C. Holloway, Christopher A. Lenyk, Timothy D. Gustafson, Nancy C. Giles Oct 2022

Oxygen Vacancies In Lib3O5 Crystals And Their Role In Nonlinear Absorption, Brian C. Holloway, Christopher A. Lenyk, Timothy D. Gustafson, Nancy C. Giles

Faculty Publications

LiB3O5 (LBO) crystals are used to generate the second, third, and fourth harmonics of near-infrared solid-state lasers. At high power levels, the material’s performance is adversely affected by nonlinear absorption. We show that as-grown crystals contain oxygen and lithium vacancies. Transient absorption bands are formed when these intrinsic defects serve as traps for “free” electrons and holes created by x rays or by three- and four-photon absorption processes. Trapped electrons introduce a band near 300 nm and trapped holes produce bands in the 500-600 nm region. Electron paramagnetic resonance (EPR) is used to identify and characterize the …


Deep-Turbulence Phase Compensation Using Tiled Arrays, Mark F. Spencer, Terry J. Brennan Sep 2022

Deep-Turbulence Phase Compensation Using Tiled Arrays, Mark F. Spencer, Terry J. Brennan

Faculty Publications

Tiled arrays use modulo-2π phase compensation and coherent beam combination to correct for the effects of deep turbulence. As such, this paper uses wave-optics simulations to compare the closed-loop performance of tiled arrays to a branch-point-tolerant phase reconstructor known as LSPV+7 [Appl. Opt. 53, 3821 (2014) [CrossRef] ]. The wave-optics simulations make use of a point-source beacon and are setup with weak-to-strong scintillation conditions. This setup enables a trade-space exploration in support of a power-in-the-bucket comparison with LSPV+7. In turn, the results show that tiled arrays outperform LSPV+7 when transitioning from weak-to-strong scintillation conditions. These results are both …


Resonant Plasmonic–Biomolecular Chiral Interactions In The Far-Ultraviolet: Enantiomeric Discrimination Of Sub-10 Nm Amino Acid Films, Tiago Ramos Leite, Lin Zschiedrich, Orhan Kizilkaya, Kevin M. Mcpeak Sep 2022

Resonant Plasmonic–Biomolecular Chiral Interactions In The Far-Ultraviolet: Enantiomeric Discrimination Of Sub-10 Nm Amino Acid Films, Tiago Ramos Leite, Lin Zschiedrich, Orhan Kizilkaya, Kevin M. Mcpeak

Faculty Publications

Resonant plasmonic–molecular chiral interactions are a promising route to enhanced biosensing. However, biomolecular optical activity primarily exists in the far-ultraviolet regime, posing significant challenges for spectral overlap with current nano-optical platforms. We demonstrate experimentally and computationally the enhanced chiral sensing of a resonant plasmonic–biomolecular system operating in the far-UV. We develop a full-wave model of biomolecular films on Al gammadion arrays using experimentally derived chirality parameters. Our calculations show that detectable enhancements in the chiroptical signals from small amounts of biomolecules are possible only when tight spectral overlap exists between the plasmonic and biomolecular chiral responses. We support this conclusion …


Adsorption Of Helium And Hydrogen On Triphenylene And 1,3,5-Triphenylbenzene, Bergmeister Bergmeister, Kollotzek Kollotzek, Florent Calvo, Elisabeth Gruber, Fabio Zappa, Paul Scheier, Olof E. Echt Aug 2022

Adsorption Of Helium And Hydrogen On Triphenylene And 1,3,5-Triphenylbenzene, Bergmeister Bergmeister, Kollotzek Kollotzek, Florent Calvo, Elisabeth Gruber, Fabio Zappa, Paul Scheier, Olof E. Echt

Faculty Publications

The adsorption of helium or hydrogen on cationic triphenylene (TPL, C18H12), a planar polycyclic aromatic hydrocarbon (PAH) molecule, and of helium on cationic 1,3,5-triphenylbenzene (TPB, C24H18), a propeller-shaped PAH, is studied by a combination of high-resolution mass spectrometry and classical and quantum computational methods. Mass spectra indicate that HenTPL+ complexes are particularly stable if n = 2 or 6, in good agreement with the quantum calculations which show that for these sizes the helium atoms are strongly localized on either side of the central carbon ring for n = …


Measurement Of The Branching Fractions Of The B+Η′ℓ+Νℓ And B+Η′ℓ+Νℓ Decays With Signal-Side Only Reconstruction In The Full Q2 Range, U. Gebauer, C. Beleño, A. Frey, I. Adachi, K. Adamczyk, H. Aihara, S. Al Said, D. M. Asner, H. Atmacan, T. Aushev, R. Ayad, V. Babu, S. Bahinipati, P. Behera, K. Belous, J. Bennett, M. Bessner, V. Bhardwaj, B. Bhuyan, Milind Purohit, Et. Al. Aug 2022

Measurement Of The Branching Fractions Of The B+ → Η′ℓ+Νℓ And B+ → Η′ℓ+Νℓ Decays With Signal-Side Only Reconstruction In The Full Q2 Range, U. Gebauer, C. Beleño, A. Frey, I. Adachi, K. Adamczyk, H. Aihara, S. Al Said, D. M. Asner, H. Atmacan, T. Aushev, R. Ayad, V. Babu, S. Bahinipati, P. Behera, K. Belous, J. Bennett, M. Bessner, V. Bhardwaj, B. Bhuyan, Milind Purohit, Et. Al.

Faculty Publications

The branching fractions of the decays B+ηl+νl and B+ηl+νl are measured, where l is either an electron or a muon, using a data sample of 711 fb−1 containing 772 × 106 BB̅ pairs collected at the ϒ(4S) resonance with the Belle detector at the KEKB asymmetric-energy e+e collider. To reduce the dependence of the result on the form factor model, the measurement is performed over the entire q2 range. The resulting branching fractions are B(B+η ℓ + ν ℓ)=(2.83 …


Measurement Of The Branching Fractions Of The B+ → Ηl+ Νl And B+ → Η0l+ Νl Decays With Signal-Side Only Reconstruction In The Full Q2 Range, U. Gebauer, C. Beleño, A. Frey, I. Adachi, K. Adamczyk, H. Aihara, S. Al Said, D. M. Asner, H. Atmacan, T. Aushev, R. Ayad, V. Babu, S. Bahinipati, P. Behera, K. Belous, J. Bennett, M. Bessner, V. Bhardwaj, B. Bhuyan, Milind Purohit, Et. Al. Aug 2022

Measurement Of The Branching Fractions Of The B+ → Ηl+ Νl And B+ → Η0l+ Νl Decays With Signal-Side Only Reconstruction In The Full Q2 Range, U. Gebauer, C. Beleño, A. Frey, I. Adachi, K. Adamczyk, H. Aihara, S. Al Said, D. M. Asner, H. Atmacan, T. Aushev, R. Ayad, V. Babu, S. Bahinipati, P. Behera, K. Belous, J. Bennett, M. Bessner, V. Bhardwaj, B. Bhuyan, Milind Purohit, Et. Al.

Faculty Publications

The branching fractions of the decays B+ → ηl+νl and B+ → η0 lþνl are measured, where l is either an electron or a muon, using a data sample of 711 fb−1 containing 772 × 106 BB̅ pairs collected at the ϒ(4S) resonance with the Belle detector at the KEKB asymmetric-energy e+e collider. To reduce the dependence of the result on the form factor model, the measurement is performed over the entire q2 range. The resulting branching fractions are B(B+ → ηlþνl)=(2.83 ± 0.55(stat.) ± 0.34(syst.) )× 10 …


Improved Measurement Of Neutrino Oscillation Parameters By The Nova Experiment, M. A. Acero, P. Adamson, L. Aliaga, N. Anfimov, A. Antoshkin, E. Arrieta-Diaz, L. Asquith, A. Aurisano, A. Back, C. Backhouse, M. Baird, N. Balashov, P. Baldi, B. A. Bambah, S. Bashar, K. Bays, R. Bernstein, V. Bhatnagar, D. Bhattarai, B. Bhuyan, Roberto Petti, Et. Al. Aug 2022

Improved Measurement Of Neutrino Oscillation Parameters By The Nova Experiment, M. A. Acero, P. Adamson, L. Aliaga, N. Anfimov, A. Antoshkin, E. Arrieta-Diaz, L. Asquith, A. Aurisano, A. Back, C. Backhouse, M. Baird, N. Balashov, P. Baldi, B. A. Bambah, S. Bashar, K. Bays, R. Bernstein, V. Bhatnagar, D. Bhattarai, B. Bhuyan, Roberto Petti, Et. Al.

Faculty Publications

We present new νμ → νe, νμ → νμ, μe, and μμ oscillation measurements by the NOvA experiment, with a 50% increase in neutrino-mode beam exposure over the previously reported results. The additional data, combined with previously published neutrino and antineutrino data, are all analyzed using improved techniques and simulations. A joint fit to the νe, νμ, e, and μ candidate samples within the 3-flavor neutrino oscillation framework continues to yield a best-fit point in the normal mass …


Search For The Radiative Penguin Decays B0 → K 0 SK 0 S Γ In The Belle Experiment, H. B. Jeon, K. H. Kang, H. Park, I. Adachi, H. Aihara, S. Al Said, D. M. Asner, H. Atmacan, T. Aushev, R. Ayad, V. Babu, S. Bahinipati, P. Behera, K. Belous, J. Bennett, F. Bernlochner, M. Bessner, V. Bhardwaj, B. Bhuyan, Milind Purohit, Et. Al. Jul 2022

Search For The Radiative Penguin Decays B0 → K 0 SK 0 S Γ In The Belle Experiment, H. B. Jeon, K. H. Kang, H. Park, I. Adachi, H. Aihara, S. Al Said, D. M. Asner, H. Atmacan, T. Aushev, R. Ayad, V. Babu, S. Bahinipati, P. Behera, K. Belous, J. Bennett, F. Bernlochner, M. Bessner, V. Bhardwaj, B. Bhuyan, Milind Purohit, Et. Al.

Faculty Publications

We report results from the first search for the rare penguin-dominated decay mode B0→K 0 S K 0 Sγ, which can result from the production of tensor mesons f(1270) and f'(1525) in association with a photon. The search uses the full data sample of 772×106  BB̅ pairs collected with the Belle detector at the KEKB asymmetric-energy e+e collider. No statistically significant signals are observed in the K 0 S K 0 S invariant mass range 1  GeV/c2K 0 S K 0 S/c2, and the following upper …


Scintillation Light Detection In The 6-M Drift-Length Protodune Dual Phase Liquid Argon Tpc, A. Abed, B. Abi, R. Acciarri, M. A. Acero, M. R. Adames, G. Adamov, M. Adamowski, D. Adams, M. Adinolfi, A. Aduszkiewicz, J. Aguilar, Z. Ahmad, J. Ahmed, B. Aimard, B. Ali-Mohammadzadeh, T. Alion, K. Allison, S. Alonso Monsalve, M. Alrashed, C. Alt, Roberto Petti, Et. Al. Jul 2022

Scintillation Light Detection In The 6-M Drift-Length Protodune Dual Phase Liquid Argon Tpc, A. Abed, B. Abi, R. Acciarri, M. A. Acero, M. R. Adames, G. Adamov, M. Adamowski, D. Adams, M. Adinolfi, A. Aduszkiewicz, J. Aguilar, Z. Ahmad, J. Ahmed, B. Aimard, B. Ali-Mohammadzadeh, T. Alion, K. Allison, S. Alonso Monsalve, M. Alrashed, C. Alt, Roberto Petti, Et. Al.

Faculty Publications

DUNE is a dual-site experiment for long-baseline neutrino oscillation studies, neutrino astrophysics and nucleon decay searches. ProtoDUNE Dual Phase (DP) is a 6×6×6 m3 liquid argon time-projection-chamber (LArTPC) that recorded cosmic-muon data at the CERN Neutrino Platform in 2019–2020 as a prototype of the DUNE Far Detector. Charged particles propagating through the LArTPC produce ionization and scintillation light. The scintillation light signal in these detectors can provide the trigger for non-beam events. In addition, it adds precise timing capabilities and improves the calorimetry measurements. In ProtoDUNE-DP, scintillation and electroluminescence light produced by cosmic muons in the LArTPC is collected …


Search For Multimessenger Signals In Nova Coincident With Ligo/Virgo Detections, M. A. Acero, P. Adamson, L. Aliaga, T. Alion, V. Alakhberdian, N. Anfimov, A. Antoshkin, L. Asquith, A. Aurisano, A. Back, C. Backhouse, M. Biard, N. Balashov, P. Baldi, B. A. Bambah, S. Bashar, K. Bays, S. Bending, R. Bernstein, V. Bhatnagar, Roberto Petti, Et. Al. Jun 2022

Search For Multimessenger Signals In Nova Coincident With Ligo/Virgo Detections, M. A. Acero, P. Adamson, L. Aliaga, T. Alion, V. Alakhberdian, N. Anfimov, A. Antoshkin, L. Asquith, A. Aurisano, A. Back, C. Backhouse, M. Biard, N. Balashov, P. Baldi, B. A. Bambah, S. Bashar, K. Bays, S. Bending, R. Bernstein, V. Bhatnagar, Roberto Petti, Et. Al.

Faculty Publications

Using the NOvA neutrino detectors, a broad search has been performed for any signal coincident with 28 gravitational wave events detected by the LIGO/Virgo Collaboration between September 2015 and July 2019. For all of these events, NOvA is sensitive to possible arrival of neutrinos and cosmic rays of GeV and higher energies. For five (seven) events in the NOvA Far (Near) Detector, timely public alerts from the LIGO/Virgo Collaboration allowed recording of MeV-scale events. No signal candidates were found.


Improving On Atmospheric Turbulence Profiles Derived From Dual Beacon Hartmann Turbulence Sensor Measurements, Alexander S. Boeckenstedt, Jack E. Mccrae, Santasri Bose-Pillai, Benjamin Wilson Jun 2022

Improving On Atmospheric Turbulence Profiles Derived From Dual Beacon Hartmann Turbulence Sensor Measurements, Alexander S. Boeckenstedt, Jack E. Mccrae, Santasri Bose-Pillai, Benjamin Wilson

Faculty Publications

Atmospheric turbulence is an inevitable source of wavefront distortion in all fields of long range laser propagation and sensing. However, the distorting effects of turbulence can be corrected using wavefront sensors contained in adaptive optics systems. Such systems also provide deeper insight into surface layer turbulence, which is not well understood. A unique method of profile generation by a dual source Hartmann Turbulence Sensor (HTS) technique is introduced here. Measurements of optical turbulence along a horizontal path were taken to create C2n profiles. Two helium-neon laser beams were directed over an inhomogeneous horizontal path and captured by the HTS. The …


Feasibility Of Obtaining Surface Layer Moisture Flux Using An Ir Thermometer, Steven T. Fiorino, Lance Todorowski, Jaclyn Schmidt, Yogendra Raut, Jacob Margraf May 2022

Feasibility Of Obtaining Surface Layer Moisture Flux Using An Ir Thermometer, Steven T. Fiorino, Lance Todorowski, Jaclyn Schmidt, Yogendra Raut, Jacob Margraf

Faculty Publications

This paper evaluates the feasibility of a method using a single hand-held infrared (IR) thermometer and a mini tower of wet and dry paper towels to psychometrically obtain surface layer temperature and moisture gradients and fluxes. Sling Psychrometers have long been standard measuring devices for quantifying the thermodynamics of near-surface atmospheric gas–vapor mixtures, specifically moisture parameters. However, these devices are generally only used to measure temperature and humidity at one near-surface level. Multiple self-aspirating psychrometers can be used in a vertical configuration to measure temperature and moisture gradients and fluxes in the first 1–2 m of the surface layer. This …


Electron Traps In Ag-Doped Li2B4O7 Crystals: The Role Of Ag Interstitial Ions, Timothy D. Gustafson, Brant E. Kananen, Nancy C. Giles, Brian C. Holloway, Volodymyr T. Adamiv, Ihor M. Teslyuk, Yaroslav V. Burak, Larry E. Halliburton May 2022

Electron Traps In Ag-Doped Li2B4O7 Crystals: The Role Of Ag Interstitial Ions, Timothy D. Gustafson, Brant E. Kananen, Nancy C. Giles, Brian C. Holloway, Volodymyr T. Adamiv, Ihor M. Teslyuk, Yaroslav V. Burak, Larry E. Halliburton

Faculty Publications

Electron paramagnetic resonance (EPR) is used to establish models for electron traps in Ag-doped lithium tetraborate (Li2B4O7) crystals. When exposed at room temperature to ionizing radiation, electrons are trapped at interstitial Ag+ ions and holes are trapped at Ag+ ions on Li+ sites. The trapped electrons occupy a 5s1 orbital on the interstitial Ag ions (some of the unpaired spin density is also on neighboring ions). Three EPR spectra are assigned to electrons trapped at interstitial Ag ions. Their g values are near 1.99 and they have resolved hyperfine structure …


Stabilization Of Phenanthrene Anions In Helium Nanodroplets, Siegfried Kollotzek, Farhad Izadi, Miriam Meyer, Stefan Bergmeister, Fabio Zappa, Stephan Denifl, Olof E. Echt, Paul Scheier, Elisabeth Gruber May 2022

Stabilization Of Phenanthrene Anions In Helium Nanodroplets, Siegfried Kollotzek, Farhad Izadi, Miriam Meyer, Stefan Bergmeister, Fabio Zappa, Stephan Denifl, Olof E. Echt, Paul Scheier, Elisabeth Gruber

Faculty Publications

It has been debated for years if the polycyclic aromatic hydrocarbon phenanthrene exists in its anionic form, or, in other words, if its electron affinity (EA) is positive or negative. In this contribution we confirm that the bare phenanthrene anion Ph- created in a binary collision with an electron at room temperature has a lifetime shorter than microseconds. However, the embedding of neutral phenanthrene molecules in negatively charged helium nanodroplets enables the formation of phenanthrene anions by charge transfer processes and the stabilization of the latter in the ultracold environment. Gentle shrinking of the helium matrix of phenanthrene-doped HNDs …


Particle-In-Cell Simulations Of Ion Dynamics In A Pinched-Beam Diode, Jesse C. Foster, John W. Mcclory, S. B. B. Swanekamp, D. D. Hinshelwood, A. S. Richardson, Paul E. Adamson, J. W. Schumer, R. W. James, P. F. Ottinger, D. Mosher May 2022

Particle-In-Cell Simulations Of Ion Dynamics In A Pinched-Beam Diode, Jesse C. Foster, John W. Mcclory, S. B. B. Swanekamp, D. D. Hinshelwood, A. S. Richardson, Paul E. Adamson, J. W. Schumer, R. W. James, P. F. Ottinger, D. Mosher

Faculty Publications

article-in-cell simulations of a 1.6 MV, 800 kA, and 50 ns pinched-beam diode have been completed with emphasis placed on the quality of the ion beams produced. Simulations show the formation of multiple regions in the electron beam flow characterized by locally high charge and current density (“hot spots”). As ions flow through the electron-space-charge cloud, these hot spots electrostatically attract ions to produce a non-uniform ion current distribution. The length of the cavity extending beyond the anode-to-cathode gap (i.e., behind the cathode tip) influences both the number and amplitude of hot spots. A longer cavity length increases the number …


Hands-On Stem: Chemistry, Physics, And Other Science Resources For K-12 Education, Lisa Ahlberg, G. Brendan Cross May 2022

Hands-On Stem: Chemistry, Physics, And Other Science Resources For K-12 Education, Lisa Ahlberg, G. Brendan Cross

Faculty Publications

No abstract provided.


Search For An Axionlike Particle In B Meson Decays, J. P. Lees, V. Poireau, V. Tisserand, E. Grauges, A. Palano, G. Eigen, D. N. Brown, Yu. G. Kolomensky, M. Fritsch, H. Koch, T. Schroeder, R. Cheaib, C. Hearty, T. S. Mattison, J. A. Mckenna, R. Y. So, V. E. Blinov, A. R. Buzykaev, Milind Purohit, Et. Al. Apr 2022

Search For An Axionlike Particle In B Meson Decays, J. P. Lees, V. Poireau, V. Tisserand, E. Grauges, A. Palano, G. Eigen, D. N. Brown, Yu. G. Kolomensky, M. Fritsch, H. Koch, T. Schroeder, R. Cheaib, C. Hearty, T. S. Mattison, J. A. Mckenna, R. Y. So, V. E. Blinov, A. R. Buzykaev, Milind Purohit, Et. Al.

Faculty Publications

Axionlike particles (ALPs) are predicted in many extensions of the standard model, and their masses can naturally be well below the electroweak scale. In the presence of couplings to electroweak bosons, these particles could be emitted in flavor-changing B meson decays. We report herein a search for an ALP, a, in the reaction B ±→K ± a, aγ γ using data collected by the BABAR experiment at SLAC. No significant signal is observed, and 90% confidence level upper limits on the ALP coupling to electroweak bosons are derived as a function of ALP mass, improving current …


Possible Studies On Generalized Parton Distributions And Gravitational Form Factors In Neutrino Reactions, Shunzo Kumano, Roberto Petti Mar 2022

Possible Studies On Generalized Parton Distributions And Gravitational Form Factors In Neutrino Reactions, Shunzo Kumano, Roberto Petti

Faculty Publications

Spacelike and timelike generalized parton distributions (GPDs) have been investigated in charged-lepton scattering and electron-positron collisions via deeply virtual Compton scattering and two-photon processes, respectively. Furthermore, we expect that hadron-accelerator-facility measurements will be performed in future. The GPDs will play a crucial role in clarifying the origins of hadron spins and masses in terms of quarks and gluons. It is also possible to probe internal pressure within hadrons for understanding their stability. Gravitational form factors of hadrons used to be considered as a purely academic subject because gravitational interactions are too weak to be measured in microscopic systems. However, due …


Search For Lepton Flavor Violation In ϒ(3S) → E±Μ, J. P. Lees, V. Tisserand, A. Palano, G. Eigen, D. N. Brown, Yu. G. Kolomensky, M. Fritsch, H. Koch, T. Schroeder, R. Cheaib, C. Hearty, T. S. Mattison, J. A. Mckenna, R. Y. So, V. E. Blinov, A. R. Buzykaev, V. P. Druzhinin, V. B. Golubev, E. A. Kozyrev, Milind Purohit, Et. Al. Mar 2022

Search For Lepton Flavor Violation In ϒ(3S) → E±Μ∓, J. P. Lees, V. Tisserand, A. Palano, G. Eigen, D. N. Brown, Yu. G. Kolomensky, M. Fritsch, H. Koch, T. Schroeder, R. Cheaib, C. Hearty, T. S. Mattison, J. A. Mckenna, R. Y. So, V. E. Blinov, A. R. Buzykaev, V. P. Druzhinin, V. B. Golubev, E. A. Kozyrev, Milind Purohit, Et. Al.

Faculty Publications

We report on the first search for electron-muon lepton flavor violation (LFV) in the decay of a b quark and b antiquark bound state. We look for the LFV decay ϒ(3S) → e ± μ in a sample of 118 million ϒ(3S) mesons from 27 fb−1 of data collected with the BABAR detector at the SLAC PEP-II e+e collider operating with a 10.36 GeV center-of-mass energy. No evidence for a signal is found, and we set a limit on the branching fraction B[ϒ(3S) → e ± μ]< 3.6 × 10−7 …


Thermo-Fluidic Transport Process In A Novel M-Shaped Cavity Packed With Non-Darcian Porous Medium And Hybrid Nanofluid: Application Of Artificial Neural Network (Ann), Dipak Kumar Mandal, Nirmalendu Biswas, Nirmal K. Manna, Dilip Kumar Gayen, Rama S. R. Gorla, Ali J. Chamkha Mar 2022

Thermo-Fluidic Transport Process In A Novel M-Shaped Cavity Packed With Non-Darcian Porous Medium And Hybrid Nanofluid: Application Of Artificial Neural Network (Ann), Dipak Kumar Mandal, Nirmalendu Biswas, Nirmal K. Manna, Dilip Kumar Gayen, Rama S. R. Gorla, Ali J. Chamkha

Faculty Publications

In this work, an attempt has been made to explore numerically the thermo-fluidic transport process in a novel M-shaped enclosure filled with permeable material along with Al2O3-Cu hybrid nanoparticles suspended in water under the influence of a horizontal magnetizing field. To exercise the influence of geometric parameters, a classical trapezoidal cavity is modified with an inverted triangle at the top to construct an M-shaped cavity. The cavity is heated isothermally from the bottom and cooled from the top, whereas the inclined sidewalls are insulated. The role of geometric parameters on the thermal performance is scrutinized thoroughly …


Utilization And Efficient Computation Of Polarization Factor Q For Fast, Accurate Brdf Modeling, Samuel D. Butler, Michael A. Marciniak Feb 2022

Utilization And Efficient Computation Of Polarization Factor Q For Fast, Accurate Brdf Modeling, Samuel D. Butler, Michael A. Marciniak

Faculty Publications

The Bidirectional Reflectance Distribution Function (BRDF) is of substantial use in remote sensing, scene generation, and computer graphics, to describe optical scatter off realistic surfaces. This paper begins by summarizing our prior work in relating wave optics and geometric optics models, culminating with the Modified Cook-Torrance (MCT) model. The MCT model is evaluated here against aluminum, Infragold, and silver paint at various wavelengths in the IR. In each case, the MCT model is shown to outperform a standard microfacet model. Then, this paper shows a non-trivial method of computing the primary new term, the polarization factor Q. This optimization …


Phenanthrene: Establishing Lower And Upper Bounds To The Binding Energy Of A Very Weakly Bound Anion, Elisabeth Gruber, Siegfried Kollotzek, Stefan Bergmeister, Fabio Zappa, Milan Ončák, Paul Scheier, Olof E. Echt Feb 2022

Phenanthrene: Establishing Lower And Upper Bounds To The Binding Energy Of A Very Weakly Bound Anion, Elisabeth Gruber, Siegfried Kollotzek, Stefan Bergmeister, Fabio Zappa, Milan Ončák, Paul Scheier, Olof E. Echt

Faculty Publications

Quite a few molecules do not form stable anions that survive the time needed for their detection; their electron affinities (EA) are either very small or negative. How does one measure the EA if the anion cannot be observed? Or, at least, can one establish lower and upper bounds to their EA? We propose two approaches that provide lower and upper bounds. We choose the phenanthrene (Ph) molecule whose EA is controversial. Through competition between helium evaporation and electron detachment in HenPh- clusters, formed in helium nanodroplets, we estimate the lower bound of the vertical detachment energy …


Measurement Of The Nucleon F N2 / F P2 Tructure Function Ratio By The Jefferson Lab Marathon Tritium/Helium-3 Deep Inelastic Scattering Experiment, D. Abrams, H. Albataineh, B. S. Aljawrneh, S. Alsalmi, D. Androic, K. Aniol, W. Armstrong, J. Arrington, H. Atac, T. Averett, C. Ayerbe Gayoso, X. Bai, J. Bane, S. Barcus, A. Beck, V. Bellini, H. Bhatt, D. Bhetuwal, D. Biswas, D. Blyth, Roberto Petti, Et. Al. Feb 2022

Measurement Of The Nucleon F N2 / F P2 Tructure Function Ratio By The Jefferson Lab Marathon Tritium/Helium-3 Deep Inelastic Scattering Experiment, D. Abrams, H. Albataineh, B. S. Aljawrneh, S. Alsalmi, D. Androic, K. Aniol, W. Armstrong, J. Arrington, H. Atac, T. Averett, C. Ayerbe Gayoso, X. Bai, J. Bane, S. Barcus, A. Beck, V. Bellini, H. Bhatt, D. Bhetuwal, D. Biswas, D. Blyth, Roberto Petti, Et. Al.

Faculty Publications

The ratio of the nucleon F2 structure functions, F n2 / F p2 is determined by the MARATHON experiment from measurements of deep inelastic scattering of electrons from 3H and 3He nuclei. The experiment was performed in the Hall A Facility of Jefferson Lab using two high-resolution spectrometers for electron detection, and a cryogenic target system which included a low-activity tritium cell. The data analysis used a novel technique exploiting the mirror symmetry of the two nuclei, which essentially eliminates many theoretical uncertainties in the extraction of the ratio. The results, which cover the Bjorken …


Cu2+ And Cu3+ Acceptors In Β-Ga2O3 Crystals: A Magnetic Resonance And Optical Absorption Study, Timothy D. Gustafson, Nancy C. Giles, Brian C. Holloway, Christopher A. Lenyk, J. Jesenovec, J. S. Mccloy, M. D. Mccluskey, Larry E. Halliburton Feb 2022

Cu2+ And Cu3+ Acceptors In Β-Ga2O3 Crystals: A Magnetic Resonance And Optical Absorption Study, Timothy D. Gustafson, Nancy C. Giles, Brian C. Holloway, Christopher A. Lenyk, J. Jesenovec, J. S. Mccloy, M. D. Mccluskey, Larry E. Halliburton

Faculty Publications

Electron paramagnetic resonance (EPR) and optical absorption are used to characterize Cu2+ (3d9) and Cu3+ (3d8) ions in Cu-doped β-Ga2O3. These Cu ions are singly ionized acceptors and neutral acceptors, respectively (in semiconductor notation, they are Cu and Cu0 acceptors). Two distinct Cu2+ EPR spectra are observed in the as-grown crystals. We refer to them as Cu2+(A) and Cu2+(B). Spin-Hamiltonian parameters (a g matrix and a 63,65Cu hyperfine matrix) are obtained from the angular dependence of each spectrum. Additional electron-nuclear double resonance …


Connecting Ansatz Expressibility To Gradient Magnitudes And Barren Plateaus, Zoe Holmes, Kunal Sharma, M Cerezo, Patrick Coles Jan 2022

Connecting Ansatz Expressibility To Gradient Magnitudes And Barren Plateaus, Zoe Holmes, Kunal Sharma, M Cerezo, Patrick Coles

Faculty Publications

Parametrized quantum circuits serve as ansatze for solving variational problems and provide a flexible paradigm for the programming of near-term quantum computers. Ideally, such ansatze should be highly expressive, so that a close approximation of the desired solution can be accessed. On the other hand, the ansatz must also have sufficiently large gradients to allow for training. Here, we derive a fundamental relationship between these two essential properties: expressibility and trainability. This is done by extending the well-established barren plateau phenomenon, which holds for ansatze that form exact 2-designs, to arbitrary ansatze. Specifically, we calculate the variance in the cost …