Physical Sciences and Mathematics Commons^™

Supercontinuum Light Generation Via Non-Linear Effects In Hollow-Core Fiber, Skyler Gulati

Physics Student Works

The field of non-linear optics has gained traction in the last couple decades due to the variable generation of wavelengths which are less deterministic than within traditional optics. Using non-linear mediums, including hollow-core fibers (HCF), generation of wavelengths spanning into the vacuum ultraviolet (VUV) wavelength range is possible. These short wavelengths can be utilized within electron spectroscopy-based methods of material science like angle-resolved photoemission spectroscopy (ARPES). This technique most often uses specific photoemission lines of atoms in discharge lamps, however, with the frequency dispersion capabilities of HCF, broad band creation can allow for variable wavelength selection through filtering specific wavelengths …

Whispering Gallery Modes Of A Triatomic Photonic Molecule, Vladimir Shuvayev, Stanislav Kreps, Tal Carmon, Lev Deych

Publications and Research

In this paper, we present the results of numerical simulations of the optical spectra of a three-sphere photonic molecule. The configuration of the system was continuously modified from linear to triangular, in-plane with the fundamental mode excited in one of the spheres and perpendicular to it. We found the relative insensitivity of the spectra to the in-plane deviation from the linear arrangement up to about 110°. For larger angles, the spectra show significant modification consisting of the major spectral peaks splitting and shifting. On the contrary, the spectra are quite sensitive to out-of-plane molecule deviation, even at small angles. Thus, …

Helium Nanodroplets As An Efficient Tool To Investigate Hydrogen Attachment To Alkali Cations, Siegfried Kollotzek, José Campos-Martínez, Massimiliano Bartolomei, Fernando Pirani, Lukas Tiefenthaler, Marta I. Hernández, Teresa Lázaro, Eva Zunzunegui-Bru, Tomás González-Lezana, José Bretón, Javier Hernández-Rojas, Olof E. Echt, Paul Scheier

Faculty Publications

We report a novel method to reversibly attach and detach hydrogen molecules to positively charged sodium clusters formed inside a helium nanodroplet host matrix. It is based on the controlled production of multiply charged helium droplets which, after picking up sodium atoms and exposure to H₂ vapor, lead to the formation of Na_m⁺(H₂)_n clusters, whose population was accurately measured using a time-of-flight mass spectrometer. The mass spectra reveal particularly favorable Na⁺(H₂)_n and Na₂⁺(H₂)_n clusters for specific “magic” numbers of attached hydrogen molecules. …

An Interactive Simulation And Visualization Tool For Conventional And Aberration-Corrected Transmission Electron Microscopy, Xingzhong Li

Nebraska Center for Materials and Nanoscience: Faculty Publications

Contrast transfer function (CTF) is a vital function in transmission electron microscopy (TEM). It expresses to what extent amplitudes converted from the phase changes of the diffracted waves contribute to the TEM image, including the effects of lens aberrations. Simulation is very helpful to understand the application of the function thoroughly. In this work, we develop the CTFscope as a component in the Landyne software suite, to calculate the CTF with temporal and spatial dumping envelopes for conventional TEM and to extend it to various aberrations (up to fifth order) for aberration-corrected (AC)- TEM. It also includes effects on the …

Remote Surface Optical Phonon Scattering In Ferroelectric Ba0.6Sr0.4Tio3 Gated Graphene, Hanying Chen, Tianlin Li, Yifei Hao, Anil Rajapitamahuni, Zhiyong Xiao, Stefan Schoeche, Mathias Schubert, Xia Hong

Xia Hong Publications

We report the effect of remote surface optical (RSO) phonon scattering on carrier mobility in monolayer graphene gated by ferroelectric oxide. We fabricate monolayer graphene transistors back-gated by epitaxial (001) Ba0.6Sr0.4TiO3 films, with field effect mobility up to 23,000 cm² V⁻¹ s⁻¹ achieved. Switching ferroelectric polarization induces nonvolatile modulation of resistance and quantum Hall effect in graphene at low temperatures. Ellipsometry spectroscopy studies reveal four pairs of optical phonon modes in Ba_0.6Sr_0.4TiO₃, from which we extract RSO phonon frequencies. The temperature dependence of resistivity in graphene can be well accounted for …

Solvation Of Large Polycyclic Aromatic Hydrocarbons In Helium: Cationic And Anionic Hexabenzocoronene, Miriam Kappe, Florent Calvo, Johannes Schöntag, Holger F. Bettinger, Serge Krasnokutski, Martin Kuhn, Elisabeth Gruber, Fabio Zappa, Paul Scheier, Olof E. Echt

Faculty Publications

The adsorption of helium on charged hexabenzocoronene (Hbc, C₄₂H₁₈), a planar polycyclic aromatic hydrocarbon (PAH) molecule of D_6h symmetry, is investigated by a combination of high-resolution mass spectrometry and classical and quantum computational methods. The ion abundance of He_nHbc⁺ complexes versus size n features prominent local anomalies at n = 14, 38, 68, 82, and a weak one at 26, indicating that for these “magic” sizes the helium evaporation energies are relatively large. Surprisingly, mass spectra of anionic He_nHbc^– complexes feature a different set of anomalies, namely at …

Search For A W' Boson Decaying To A Vector-Like Quark And A Top Or Bottom Quark In The All-Jets Final State At √S = 13 Tev, The Cms Collaboration

Department of Physics and Astronomy: Faculty Publications

A search is presented for a heavy W0 boson resonance decaying to a B or T vector-like quark and a t or a b quark, respectively. The analysis is performed using protonproton collisions collected with the CMS detector at the LHC. The data correspond to an integrated luminosity of 138 fb⁻¹ at a center-of-mass energy of 13TeV. Both decay channels result in a signature with a t quark, a Higgs or Z boson, and a b quark, each produced with a significant Lorentz boost. The all-hadronic decays of the Higgs or Z boson and of the t quark are …

Degree Of Linear Polarization: An Indicator Of Optical Vortex Beam Entanglement, Ella James

Summer Community of Scholars Posters (RCEU and HCR Combined Programs)

No abstract provided.

Enabling Rapid Chemical Analysis Of Plutonium Alloys Via Machine Learning-Enhanced Atomic Spectroscopy Techniques, Ashwin P. Rao

Theses and Dissertations

Analytical atomic spectroscopy methods have the potential to provide solutions for rapid, high fidelity chemical analysis of plutonium alloys. Implementing these methods with advanced analytical techniques can help reduce the chemical analysis time needed for plutonium pit production, directly enabling the 80 pit-per-year by 2030 manufacturing goal outlined in the 2018 Nuclear Posture Review. Two commercial, handheld elemental analyzers were validated for potential in situ analysis of Pu. A handheld XRF device was able to detect gallium in a Pu surrogate matrix with a detection limit of 0.002 wt% and a mean error of 8%. A handheld LIBS device was …

Developing Optical Devices And Projects For Teaching Engineering, Nathan D. Lemke, John Mccauley, Tristan E. Noble, Grace Riermann, Ellesa St. George, Nathan C. Lindquist, Keith R. Stein, Karen Irene Rogers

Physics and Engineering Faculty Publications

We are creating a suite of tools and techniques based on optics to be used for teaching a variety of engineering topics. Each tool is intended for non-expert use and without the need for high-end equipment such as vibration-free optical tables. Here we report progress on three such tools: image-plane digital holography for measuring mechanical deformation; schlieren imaging of convective flows using a smart phone; and a simple optical communication protocol using LabVIEW. We will present the designs of the tools and preliminary results from teaching engineering labs and projects with these tools. Specific courses impacted to date include Fluid …

Adsorption Of Helium And Hydrogen On Triphenylene And 1,3,5-Triphenylbenzene, Bergmeister Bergmeister, Kollotzek Kollotzek, Florent Calvo, Elisabeth Gruber, Fabio Zappa, Paul Scheier, Olof E. Echt

Faculty Publications

The adsorption of helium or hydrogen on cationic triphenylene (TPL, C₁₈H₁₂), a planar polycyclic aromatic hydrocarbon (PAH) molecule, and of helium on cationic 1,3,5-triphenylbenzene (TPB, C₂₄H₁₈), a propeller-shaped PAH, is studied by a combination of high-resolution mass spectrometry and classical and quantum computational methods. Mass spectra indicate that He_nTPL⁺ complexes are particularly stable if n = 2 or 6, in good agreement with the quantum calculations which show that for these sizes the helium atoms are strongly localized on either side of the central carbon ring for n = …

Using Optical Tweezersto Probe Dna Polymerase Kappa’S Binding Mechanism To Dna, Joshua Watts

Honors Program Theses and Projects

The integrity of our DNA is constantly under threat from many internal and external factors. If the cell cannot properly protect the integrity of DNA, errors (lesions) in DNA may form which can lead to cancer. Most of these lesions serve as a roadblock to the protein, DNA polymerase (Pol), that replicates the DNA during cell division. The mechanism that is employed to read through these errors is called translesion DNA synthesis (TLS). During this process, a special class of DNA polymerases known as TLS DNA Pols that can tolerate and bypass the lesions in DNA are employed by the …

The 'Quantal Newtonian' First Law: A Complementary Perspective To The Stationary-State Quantum Theory Of Electrons, Viraht Sahni

Publications and Research

A complementary perspective to the Göttingen-Copenhagen interpretation of stationary-state quantum theory of electrons in an electromagnetic field is described. The perspective, derived from Schrödinger-Pauli theory, is that of the individual electron via its equation of motion or ‘Quantal Newtonian’ First Law. The Law is in terms of ‘classical’ fields experienced by each electron: the sum of the external and internal fields vanishes. The external field is a sum of the electrostatic and Lorentz fields. The internal field is a sum of fields’ representative of Pauli and Coulomb correlations; kinetic effects; electron density; and internal magnetic component. The energy is obtained …

Studying The Synthesis Of 196Hg At Astrophysically Relevant Energies Through The Measurement Of Capture Reaction Cross-Sections Of (P, Γ) (P, N) And (P, Α) Reactions, Khushi Bhatt

Dissertations

Understanding the origin of all the chemical elements is an important question for the nuclear-astrophysics community. There are many unanswered questions like: What astrophysical events are responsible for the synthesis of what particular chemical elements? How many different elements were made in total? What is the abundance of each synthesized element? etc. Currently, scientists are largely depending upon theory and simulations to define nuclear and astrophysical reaction. This makes it critical to have accurate experimental nuclear physics data to input in astrophysical theoretical models. However, out of more than 20000 reactions involved in these calculations, only a very few are …

Probing The Equation Of State Of Neutron Stars With Heavy Ion Collisions, Om Bhadra Khanal

Dissertations

The equation of state (EOS) is a fundamental property of nuclear matter, important for studying the structure of systems as diverse as the atomic nucleus and the neutron star. Nuclear reactions, especially heavy-ion collisions in the laboratories, can produce the nuclear matter similar to those contained in neutron stars. The density and the momentum dependence of the EOS of asymmetric nuclear matter, especially the symmetry energy term, is widely unconstrained. Finding appropriate constrains, especially at higher densities of the nuclear matter, requires the development of new devices, new experimental measurements as well as advances in theoretical understanding of nuclear collisions …

Using Coherence And Interference To Study The Few Body Dynamics In Simple Atomic Collisions Systems, Sujan Bastola

Doctoral Dissertations

"Atomic Collision experiments are best suited to sensitively test the few-body dynamics of simple systems. The few-body dynamics, in turn, can be sensitively affected by interference effects. However, an important requirement to observe interference effects in atomic scattering experiments is that the incoming projectile beam must be coherent. The coherence properties of the incoming projectile can be controlled by the geometry of the collimating slit placed before the target. We performed a kinematically complete experiment where a 75 keV proton beam is crossed with a molecular hydrogen beam to study the dissociative capture process. The motivation for this project was …

Quantum Dots In Two-Dimensional Tungsten Diselenide, Jeb Allen Michael Stacy

Graduate Theses and Dissertations

This work focuses on the investigation of single and double quantum dots in two-dimensional transition metal dichalcogenide tungsten diselenide (WSe_2) as a means to evaluate the valley degree of freedom as a potential qubit and ambipolar tungsten diselenide monolayers as single photon sources. Gate-defined quantum dots in monolayer and bilayer WSe_2 were fabricated and characterized. Single dot devices are gated from above and below the WSe_2 to accumulate a hole gas. Temperature dependence of Coulomb-blockade peak height is consistent with single-level transport. Excited-state transport in the quantum dot is shown for both monolayer and bilayer devices. Magnetic field dependence of …

Hierarchically Structured Photoelectrodes Via Atomic Layer Deposition, Justin Rowan Reed Demoulpied

Graduate Theses and Dissertations

In the search for a sustainable method to meet increasing energy needs, solar energy emerges as an underutilized, plentiful resource. Solar intermittency and requirements for transportation necessitate storing solar energy in the form of chemical bonds via artificial photosynthesis. Photoelectrochemical (PEC) water splitting generates hydrogen fuel from solar energy and water. A semiconducting material that successfully meets the complex requirements for building an industrially scalable PEC device has yet to emerge. This is leading to a reevaluation of materials previously overlooked within PEC research, mainly materials with limitations such as minimal charge carrier mobility and propensity to corrosion under illumination …

Study Of Single-Photon Wave-Packets With Atomically Thin Nonlinear Mirrors, Christopher Klenke

Graduate Theses and Dissertations

A novel controlled phase gate for photonic quantum computing is proposed by exploiting the powerful nonlinear optical responses of atomically thin transition metal dichalcogenides (TMDs) and it is shown that such a gate could elicit a π-rad phase shift in the outgoing electric field only in the case of two incident photons and no other cases. Firstly, the motivation for such a gate is developed and then the implementation of monolayer TMDs is presented as a solution to previous realization challenges. The single-mode case of incident photons upon a TMD is derived and is then used to constrain the more …

Development Of High Quantum Efficiency Strained Superlattice Spin Polarized Photocathodes Via Metal Organic Chemical Vapor Deposition, Benjamin Belfore

Electrical & Computer Engineering Theses & Dissertations

Spin polarized photocathodes are necessary to examine parity violations and other fundamental phenomena in the field of high energy physics. To create these devices, expensive and complicated growth processes are necessary. While integral to accelerator physics, spin polarized electrons could have other exciting applications in materials science and other fields of physics. In order to explore these other applications feasibly, the relative supply of spin polarized photocathodes with a high rate of both polarization and photoemission needs to be increased. One such way to increase this supply is to develop the means to grow them faster and at a larger …

Resonant Energy Exchange In Ultracold Rydberg Atoms, Samantha Grubb, Alan Okinaka

Physics and Astronomy Summer Fellows

Ultracold Rydberg atoms serve as good systems in which resonant dipole-dipole interactions can be observed. The goal of our work is to design a simulation in which energy exchange among many nearly evenly spaced energy levels is observed. These observations are useful for understanding the time evolution of complicated quantum systems, and have applications in quantum computing and simulating. We are utilizing a supercomputer to run our simulation as well as studying the system experimentally. Once we obtain simulated results, we plan to compare them with the results obtained in a lab.

Weakness Of Weak Values: Incompatibility Of Anomalous Pulse-Spectrum Amplification And Optical Frequency Combs, John C. Howell

Mathematics, Physics, and Computer Science Faculty Articles and Research

We probe the use of optical frequency combs to place lower bounds on anomalous amplification of a weak-value-measured pulse delay, potentially reaching a theoretical temporal resolution of better than 10⁻³⁴ s. Owing to the interferometric behavior of weak values, we show that anomalous weak value amplification of a time delay is not equivalent to a temporal linear phase ramp. We show that the anomalous weak value is a rearrangement of amplitudes that generates an apparent shift that can be measured in direct detection, but does not change the actual frequency offset of a spectral distribution measurable in coherent detection. …

Atomic Gradiometry Based On The Interference Of Microwave Optical Sidebands, Kaleb L. Campbell

Optical Science and Engineering ETDs

We describe a novel pulsed magnetic gradiometer based on the optical interference of sidebands generated using two spatially separated alkali vapor cells. The sidebands are produced with high efficiency using parametric frequency conversion of a probe beam interacting with Rubiduim 87 atoms in a coherent superposition of magnetically sensitive hyperfine ground states. First, experimental evidence of the sideband process is described for both steady-state and pulsed operation. Then, a theoretical framework is developed that accurately models sideband generation based on density matrix formalism. The gradiometer is then constructed using two spatially separated vapor cells, and a beat-note is generated. The …

Neutron Interferometry Using A Single Modulated Phase Grating, Ivan J. Hidrovo Giler

LSU Master's Theses

Neutron grating interferometry provides information on phase and small-angle scatter in addition to attenuation. Previously, phase grating moiré interferometers (PGMI) with two or three phase gratings have been developed. These phase-grating systems use the moiré far-field technique to avoid the need for high-aspect absorption gratings used in Talbot-Lau interferometers (TLI) which reduce the neutron flux reaching the detector. We demonstrate through simulations a novel phase grating interferometer system for cold neutrons that requires a single modulated phase grating (MPG) for phase-contrast imaging, as opposed to the two or three phase gratings in previously employed PGMI systems. We compare the MPG …

Characterization Of Electrophoretic Deposited Zinc Oxide Nanopartices For The Fabrication Of Next-Generation Nanoscale Electronic Applications, Fawwaz Abduh A. Hazzazi

LSU Doctoral Dissertations

Several reports state that it is crucial to analyze nanoscale semiconductor materials and devices with potential benefits to meet the need for next-generation nanoelectronics, bio, and nanosensors. The progress in the electronics field is as significant now, with modern technology constantly evolving and a greater focus on more efficient robust optoelectronic applications. This dissertation focuses on the study and examination of the practicality of Electrophoretic Deposition (EPD) of zinc oxide (ZnO) nanoparticles (NPs) for use in semiconductor applications.

The feasibility of several synthesized electrolytes, with and without surfactants and APTES surface functionalization, is discussed. The primary objective of this study …

Surpassing The Standard Quantum Limit Using An Optical Spring, Torrey Cullen

LSU Doctoral Dissertations

In 1916, Albert Einstein predicted the existence of gravitational waves based on his new theory of general relativity. He predicted an accelerating mass with a non-zero quadrupole moment would emit energy in the form of gravitational waves. Often referred to as ripples in space-time, gravitational waves are extremely small by the time reach Earth, potentially having traveled hundreds of megaparsecs. It is common for these ripples in space-time to stretch and squeeze matter 1000 times smaller than the width of a proton.
Laser interferometer observatories were first built in the 1990s in the US and Europe, and as sensitivity improvements …

Localized Surface Plasmon Resonance Of Copper Nanoparticles Using Finite Element Method, Samaya El Samad, Salem Marhaba

BAU Journal - Science and Technology

The aim of this paper is to study the interaction of the electromagnetic wave with plasmonic nanoparticles. Localized Surface Plasmon resonance (LSPR) characteristics are governed by the intrinsic properties of the nanoparticle (size, shape and dielectric environment). The extinction cross-section spectra of Cu nanoparticles are calculated using finite element method (FEM). By increasing both the size of the nanoparticle and the dielectric environment, the simulations show a red-shifting and broadening on the LSPR spectrum with enhancement of the spectral amplitude. The extinction cross section spectra are calculated using polarized light for non-spherical or assembled nanoparticles. We investigated the LSPR of …

Ultrafast Electron Diffraction: Visualizing Dynamic States Of Matter, D. Filipetto, P. Musumed, R. K. Li, B. J. Siwick, M. R. Otto, Martin Centurion, J. P.F. Nunes

Martin Centurion Publications

Since the discovery of electron-wave duality, electron scattering instrumentation has developed into a powerful array of techniques for revealing the atomic structure of matter. Beyond detecting local lattice variations in equilibrium structures with the highest possible spatial resolution, recent research efforts have been directed towards the long sought-after dream of visualizing the dynamic evolution of matter in real-time. The atomic behavior at ultrafast timescales carries critical information on phase transition and chemical reaction dynamics, the coupling of electronic and nuclear degrees of freedom in materials and molecules, the correlation between structure, function and previously hidden metastable or nonequilibrium states of …

Ultra-High Carrier Mobilities In Ferroelectric Domain Wall Corbino Cones At Room Temperature, Conor J. Mccluskey, Matthew G. Colbear, James P.V. Mcconville, Shane J. Mccartan, Jesi R. Maguire, Michele Conroy, Kalani Moore, Alan Harvey, Felix Trier, Ursel Bangert, Alexei Gruverman, Manuel Bibes, Amit Kumar, Raymong G.P. Mcquaid, J. Marty Gregg

Alexei Gruverman Publications

Recently, electrically conducting heterointerfaces between dissimilar band-insulators (such as lanthanum aluminate and strontium titanate) have attracted considerable research interest. Charge transport has been thoroughly explored and fundamental aspects of conduction firmly established. Perhaps surprisingly, similar insights into conceptually much simpler conducting homointerfaces, such as the domain walls that separate regions of different orientations of electrical polarisation within the same ferroelectric band-insulator, are not nearly so well-developed. Addressing this disparity, we herein report magnetoresistance in approximately conical 180° charged domain walls, which occur in partially switched ferroelectric thin film single crystal lithium niobate. This system is ideal for such measurements: firstly, …

Applications Of Machine Learning Algorithms In Materials Science And Bioinformatics, Mohammed Quazi

Mathematics & Statistics ETDs

The piezoelectric response has been a measure of interest in density functional theory (DFT) for micro-electromechanical systems (MEMS) since the inception of MEMS technology. Piezoelectric-based MEMS devices find wide applications in automobiles, mobile phones, healthcare devices, and silicon chips for computers, to name a few. Piezoelectric properties of doped aluminum nitride (AlN) have been under investigation in materials science for piezoelectric thin films because of its wide range of device applicability. In this research using rigorous DFT calculations, high throughput ab-initio simulations for 23 AlN alloys are generated.

This research is the first to report strong enhancements of piezoelectric properties …