Nuclear Engineering Commons^™

Modeling Of Laser-Produced Plasma Plumes: Expansion, Chemistry, And Thin-Film Deposition, Edmund Tsiri Semaha, Edmund Tsiri Semaha

Theses and Dissertations

Abstract

Laser-assisted material processing involves coupled plasma expansion, chemical reactions, and particle transport that govern the quality of thin-film deposition. This dissertation presents a comprehensive computational investigation of these processes using the OpenFOAM framework. First, the performance of the twoPhaseEulerFoam (tPEF), rhoCentralFoam (rCF), and sonicFoam (sF) solvers is evaluated for modeling laser-produced plasma plume expansion under atmospheric conditions, demonstrating that tPEF accurately captures shock-wave propagation, hydrodynamic behavior, and multispecies interactions. Building on this validation, the reactingFoam (rF) solver is employed to investigate the chemistry of aluminum plasma expanding into an air environment (Al–N₂–O₂). The model incorporates appropriate thermodynamic, transport, and …

Investigating The Impact Of Forest Vegetation On Nuclear Weapon Prompt Radiation Energy Deposition, Paul A. Clement

Theses and Dissertations

This work seeks to answer the unstudied questions “Does a layer of vegetation impact the prompt radiation energy deposition in the soil from an atmospheric nuclear detonation?” and “If yes, by how much?” A new methodology was developed to repeatably automate and streamline a process of generating a three-dimensional geometry for subsequent radiation transport simulations and statistical analysis. The methodology streamlined three diverse applications: a three-dimensional mesh generator, a radiation transport simulation code, and a sensitivity analysis & uncertainty quantification software. The methodology was tested by simulating the quantitative influence that vegetation has on changing the energy deposition into the …

Isotope Production Modeling In Sodium-Cooled Fast Reactors, Aaron W. Burkhardt

Theses and Dissertations

The accurate prediction of isotopic compositions in Sodium-Cooled Fast Reactors (SFRs) is essential for nuclear forensic analyses and international nuclear treaty monitoring, particularly with the increased global deployment of Generation-IV reactors. This research developed and validated a detailed computational model tailored specifically to the Prototype Fast Breeder Reactor (PFBR), employing advanced Monte Carlo neutron transport methods, sophisticated burnup modeling, and variance reduction techniques. Validation against empirical data from the Experimental Breeder Reactor-II confirmed the model’s accuracy, producing a comprehensive database of isotopic compositions across 301 assembly locations and 580 isotopes through the reactor’s initial operation and equilibrium cycle. The model …

Constraining Nuclear Data Uncertainty Requirements For The 19F(A, N)22Na Reaction For Non-Proliferation Applications, Tyler R. M. Smith

Theses and Dissertations

This thesis explores the requirements on nuclear data uncertainties needed for the use of the ¹⁹F(α, n)²²Na reaction for nuclear non-proliferation applications. An overview of how neutrons are produced from alpha decays in a UF₆ medium is discussed. Calculation demonstrate the role nuclear data uncertainties effect the neutron yield and energy spectra as a function of enrichment.

Hybrid Machine Learning And Comparison Error Minimization For Frequency Domain-Based Rapid State Estimation In Structures Subjected To High-Rate Boundary Change, James Scheppegrell

Theses and Dissertations

Dynamic forces and evolving structural boundary conditions pose challenges for various structural systems such as aircraft, orbital infrastructure, and energy harvesting devices. The design, evaluation, and functionality, of such systems can be aided through the collection and analysis of data. However, real-time decision-making for systems experiencing high-rate changes can pose unique challenges, if assessments are to be made accurately and rapidly enough to be relevant. In cases where the systems are well-defined and thoroughly understood, monitoring the frequency response can be instrumental in determining the state of structures subjected to high-rate structural boundary condition changes. This study focuses on investigating …

Assessing The Feasibility Of Transportable Nuclear Reactors: A Radiological Risk Case Study, Robert John Demuth

Theses and Dissertations

The feasibility of a truly transportable nuclear reactor presents significant radiological challenges that must be addressed to ensure compliance with regulatory limits and operational safety. This study evaluates the radiological constraints associated with the transportability of the Transportable Helium-cooled One-megawatt Reactor (THOR), focusing on neutron activation, shielding performance, and external radiation exposure. Using advanced radiation transport and activation modeling within the SCALE framework, a comprehensive analysis was conducted to quantify dose rates during operation, post-shutdown, and transport. A key aspect of this work involved assessing activation products in core materials, auxiliary components, and surrounding environments to determine their contribution to …

Radiation Assessment And Distribution In Changing Atmospheric Structures And Turbulence (Radcast), Steven B. Hernandez

Theses and Dissertations

The accessibility of materials and online information has made radiological dispersal devices (RDDs) a more probable threat than conventional nuclear weapons. This study analyzed five datasets from three test periods, using a correlation analysis between optical turbulence, aerosol concentration, and environmental parameters, and geometric mean diameter (GMD) calculations. The correlation analysis failed to yield meaningful insights, prompted a transition to the GMD analysis, which produced clearer results. Findings show GMD ranged from 38–41 nm, increasing at night and during neutral events as reduced vertical motion and boundary layer contraction correlated with optical turbulence. An alternative GMD dataset, calculated by the …

Measurements Of The Radioisotope Production Cross Section Of 193Ir(N,N')193mIr Between 0.5–9 Mev, Ronnie P. Rera

Theses and Dissertations

This thesis covers a measurements of the radioisotope production cross section of ¹⁹³Ir(n,n′) ^193mIr between 0.5–9 MeV is discussed. The experiment was performed at the University of Notre Dame St.ANA 5U accelerator laboratory. Experimental planning, data collection, analysis, results, and impacts are discussed.

Characterization Of The Neutron Spectrum Produced By A Pulsed Power Generator, Daniel S. Godlasky

Theses and Dissertations

Neutron time-of-flight, activation foils, and spectral unfolding software were used to characterize the energy and fluence of the neutron spectrum created by the Gamble II pulsed power generator. Gamble II is a pulsed power generator that delivers a 1 MV to 2.2 MV and 800 kA electrical pulse peaking at 50 ns. This electrical release creates deuterium ions in the diode that are accelerated to a neutron converter covered with a novel lithium fluoride or deuterated polyethylene to create primarily ⁷Li(d,n) or D(d,n) and ¹²C(d,n) nuclear reactions. In October 2024, two D(d,n) shots occurred, and in November 2024, …

Design, Simulation, And Characterization Of A Deuterated Plastic Scintillator For A Portable Neutron Spectrometer, Anders M. Kinney Ii

Theses and Dissertations

This thesis examines the design, simulation, and experimental characterization of a novel deuterated plastic scintillator for portable neutron spectroscopy applications related to homeland security and nuclear non-proliferation. Using Monte Carlo N-Particle (MCNP) simulations and experimental tests with gamma-ray (¹³⁷Cs) and neutron sources (AmBe, ²⁵²Cf), this research shows that deuterium substitution in scintillators significantly enhances pulse shape discrimination (PSD) and neutron energy spectrum unfolding capabilities. Although deuterated scintillators demonstrate reduced overall light output, their higher stopping power and increased ionization quenching lead to superior neutron event differentiation, particularly between (α, n) and spontaneous fission neutrons critical for detecting …

Multiphysics Modeling Of Material Response To High-Intensity X-Ray And Laser Pulses: Heating, Ablation, And Plasma Expansion, Youssef Abouhussien

Theses and Dissertations

This dissertation presents a computational framework to investigate material response under high-intensity X-ray fluxes produced by an exo-atmospheric nuclear detonation and laser-material irradiations, with a focus on heating, ablation, and plasma expansion phenomena relevant to satellite vulnerability and high-energy-density environments. A hybrid Monte Carlo and Two-Temperature Model (MC-TTM) was developed to simulate X-ray and laser energy deposition and thermal relaxation in metals and semiconductors across a range of X-ray and laser pulse durations from femtoseconds to nanoseconds. Results demonstrate distinct thermal behavior between materials, with ablation thresholds and phase transitions captured in good agreement with experimental data.

In parallel, a …

Hafnium Oxide-Based Nanoheterostructures For Catalytic Radiosensitization And Enhanced X-Ray Radiotherapy, Marlen Dariela Calix Quezada

Theses and Dissertations

Orthovoltage X-ray beams are attractive for surface and intra-operative radiotherapy. Yet, their clinical utility is constrained by rapid attenuation and the limited dose that can be delivered without harming healthy tissue. High-Z hafnium oxide (HfO₂) nanoparticles can boost local energy deposition through the photoelectric effect, while catalytic surface defects accelerate water radiolysis. Harnessing both mechanisms in a single nano-heterostructure could enable potent radiosensitization at diagnostic-range energies.

This thesis develops and evaluates HfO₂-based nanoheterostructures, both bare and Au-decorated, as catalytic radiosensitizers.

Two types of HfO₂ were evaluated, one was synthesized following a specific route and the …

Advanced Air Preheater Sealing Systems For Enhanced Efficiency And Reliability In Thermal Power Plants, Pavan Kumar Ravulaparthy

Theses and Dissertations

Global electricity generation still relies heavily on thermal power plants, which consume vast amounts of fuel and emit significant amounts of carbon dioxide. A major but often overlooked source of inefficiency in these plants lies within the rotary regenerative air preheater (RAPH), a critical heat-exchange component where air leakage can exceed 20% in aging units. This leakage increases fuel consumption, parasitic fan power, and CO₂ emissions, while degrading boiler reliability.

This research introduces advanced adaptive sealing systems designed to mitigate these losses by dynamically compensating for rotor eccentricity, thermal distortion, and wear under harsh operating conditions. Brush seals, composed of …

Laser Ablation-Induced Corrosion Resistance For Molten Salt Equipment Materials Evaluated Utilizing Electrochemical And Spectroscopic Analysis, Peggy Milota

Theses and Dissertations

Advanced reactors and used nuclear fuel separation (i.e. pyroprocessing technology) utilize high temperature salt as a thermal storage medium as well as an ionic solution for electrochemical processes. The use of these aggressive molten chloride and fluoride mediums requires specific materials or additional system alterations to extend the lifetime and structural integrity of equipment due to corrosion. Some materials, in the presence of inherently impure salt, will corrode and form oxide films in a specific formation that decreases corrosion rate by electrochemically and physically preventing elemental movement to the material surface. This is referred to as a passivation layer. However, …

Generation And Implementation Of Mixed Radiation From Laser Interactions On A Liquid Target, Benjamin M. Knight

Theses and Dissertations

The simultaneous generation of different forms of radiation from the same source is highly desirable but technically challenging. We present the generation of D-D fusion neutrons and >MeV-energy x-rays from extreme intensity (∼ 10¹⁹ W/cm² ), high repetition-rate (1 kHz) laser pulses on a thin liquid target. Total neutron fluxes of ∼ 105 neutrons/s and x-ray exposure rates up to ∼ 200 R/hr at 74 cm are measured. Evidence of D-D fusion is verified with a measurement suite including three independent neutron detection systems: an EJ-309 organic scintillator, a ³He proportional counter, and a set of 36 …

Synergistic Effects Of Neutron And Gamma Radiations On The Electrical Properties Of Mosfets, Jackson T. Piechowski

Theses and Dissertations

In many radiation environments, electronic assets are exposed to a wide variety of species of radiation. This thesis studies the effect of sequential exposure of MOSFETs to neutron and gamma radiation. 27 Goford Semiconductor GT060N04T MOSFETs with gate thickness ∼500 nm were exposed to gamma radiation from a Cesium-137 source and mixed gamma and neutron radiation from a Californium-252 source with total amounts of ionizing radiation dose, neutron fluence, and order of irradiation varied to determine if synergistic effects of neutron and gamma irradiation can be measured. Neutron fluence values as low as 3.45x10⁹ and as high as 3.40x10 …

Neutron Spectrum Unfolding From Activation Foils Irradiated In Gamble Ii Using Deuterated Polyethylene Anodes, Christopher J. Smith

Theses and Dissertations

Neutrons can cause irreparable harm to electronics, and experiments are needed to understand their effects fully. This work explores using pulsed power, which is low-cost compared to other sources, to create a useful neutron-rich environment. Deuterated polyethylene was used as anode and catcher material to generate the neutrons from the Deuterium-Deuterium (DD) fusion reaction. A simple, effective, and repeatable method was employed to directly cast deuterated polyethylene onto polyethylene sheets to fabricate the anode and catcher. The DD reactions were made by an ion beam-driven pulsed power generator, Gamble II, with the catcher located in the cathode. Zinc, copper, aluminum, …

Gamma Protection Factor For A Surrogate Armored Vehicle Exposed To The Us Army Fast Burst Reactor, Ian J. Poropat

Theses and Dissertations

This work measures the Gamma Protection Factor (GPF) of a steel cube, which is meant to serve as a surrogate for armored vehicles. The GPF is measured at the White Sands Missile Range Fast Burst Reactor (FBR) and is modeled using MCNP® v6.2 transport simulation software. When exposed to the FBR, the GPF is found to depend roughly linearly on the distance between the reactor core and steel cube. The GPF is determined to be 1.176 ± 0.00067 at 9.21 m, 1.098 ± 0.0011 at 26.16 m, and 1.033 ± 0.00082 at 42.92 m. MCNP® estimates the GPF for the …

Personal Dosimeter Testing For High Altitude Air Crew, Seth D. Bacon

Theses and Dissertations

In 2014 the Thermo Scientific N2 electronic personal dosimeter became the aircrews’ sole means to record ionizing radiation dose. The production of this dosimeter was discontinued in July of 2021, motivating the Air Force to seek a flight-certifiable replacement. The Thermo Scientific Trudose NG, Mirion DMC 3000, and Fuji NRF-51 electronic personal dosimeters, as well as the Landauer InLight optically stimulated luminescent dosimeter, were subjected to mixed gamma and fast neutron fields simulating a high-altitude flight environment. Dosimeters are evaluated on their consistency and accuracy in reporting dose and compared to the current N2 dosimeter’s reported dose.

Applying X-Ray Fluorescence With Monte Carlo Methods For Analysis Of Surface Defects On Coated Zr4, James Tyler Cahill

Theses and Dissertations

Chromium-coated Zircaloy-4 cladding represents a novel solution for creating nuclear cladding that has passive safety features. This and related developments aimed at improving nuclear safety are broadly categorized as accident-tolerant fuel and cladding. However, implementing this material presents practical challenges such as the vulnerability that cladding has to surface damage such as fretting wear. This research aims to determine if the pre-existing technique of X-ray fluorescence analysis is applicable for detecting these defects on the surface of the cladding. This was done by developing Monte Carlo N-Particle Transport models of a handheld device, the XL-5, alongside experimental measurements using this …

Modeling Of Macroscopic Melt Splashing On Beryllium First Wall Panels Of Fusion Tokamaks Under Off-Normal Events, Cheng Zhang

Theses and Dissertations

Beryllium (Be) is a material which is used as a plasma facing component in tokamak reactors due to its unique properties of high thermal conductivity, low density, and high strength. However, under extreme conditions of high temperature and pressure, Be can melt on the surface of armor tiles and molten droplets can be ejected into the reactor chamber leading to disruption of fusion plasma. The variations of pressure, mass density, velocity, and temperature of Be vapor on the surface of melt layer as well as magnetic field strength and direction can influence the splashing of Be melt and their effects …

Modeling The Radiation Shielding Effectiveness Of Hafnium Diboride Reinforced Epoxy Composites Using Mcnp, Randolph Snook

Theses and Dissertations

This thesis uses MCNP simulations to evaluate the performance of a radiation shielding material consisting of Hafnium Diboride (HfB₂) powder in an epoxy matrix. Comparing the results to previously measured data against both gamma and neutron sources, suitability for other applications can be confirmed. The model simulated the epoxy material with different weight percentages of HfB₂ and thicknesses. It was compared to other shielding materials such as pure epoxy and 5% Borated High Density Polyethylene (HDPE-B). The HfB₂-epoxy composite was tested against a wide energy range gamma spectrum from a ¹⁵²Eu source, and neutrons …

Openfoam Computational Fluid Dynamic Modeling Of Plasma Expansion Into Vacuum, Robert B. Padgett

Theses and Dissertations

Nuclear weapons, and their effects, have been heavily studied with decades of data and information to create simulations and quantify the risks of their use. However, in the modern day, nuclear strikes pose new risks to precision electronics, power systems, and vital infrastructure. As such, simulations of nuclear weapon use are required due to nuclear weapon testing being prohibited. These simulations can incorporate testing practices, such as laboratory lasers, and computer simulation technology, such as OpenFOAM Computational Fluid Dynamics (CFD). The use of OpenFOAM CFD allows testing in an area that has never been tested with nuclear weapons before, specifically …

Fluid Flow And Thermal Performance Investigation Of Twisted Elliptical Tubes For Use In High Prandtl Number Systems, Connor F. Donlan

Theses and Dissertations

The development of clean energy systems is paramount to reducing mankind's climate impact. These clean energy systems include solar, wind, and nuclear power where nuclear power shows a reduced lifetime carbon dioxide footprint per kilowatt hour compared to other sources [102]. Advanced nuclear reactors, fusion energy systems, and concentrated solar power designers are looking at using molten salt heat transfer fluids and improved heat exchanger design to increase power production and efficiency of clean energy systems. The improving heat transfer within the main heat transfer components within advanced nuclear reactors will enable increased efficiencies and power production.

Heat transfer improvements …

Direct Measurement Of The 114cd(N, Gamma)115cd Cross Section In The 1 Ev To 300 Kev Energy Range, Kofi Tutu Addo Assumin-Gyimah

Theses and Dissertations

The large thermal cross section of cadmium makes it ideal for many practical applications where screening of thermal neutrons is desired. For example, in non-destructive assay techniques, or for astrophysical studies of the s-process. All such applications require precise knowledge of the neutron-capture cross section on cadmium. Although there are some data on neutron-capture cross sections particularly at thermal energies and at energies relevant for astrophysics, there is very little data at most other energies. Further, the evaluated cross sections from the ENDF and JENDL databases disagree at high energies. Therefore, there is a critical need for precise knowledge of …

Conceptual Design And Preliminary Safety Analysis Of A Proposed Nuclear Microreactor For Mobile Application, A. S. M. Fakhrul Islam

Theses and Dissertations

Conceptual design and preliminary safety analysis of a proposed helium-cooled Micro Nuclear reactor In ONe megawatt (MINION) thermal output is done through three-dimensional computational analysis. Compared with the conventional high temperature gas-cooled reactors (HTGR) that use tri-structural or bi-structural isotropic (TRISO or BISO) fuel particles, MINION uses traditional clad fuel pellets. This greatly simplifies the core design and allows for a substantially more compact design thanks to the fuel’s signif-icantly higher U-235 atom density. Uranium carbide (UC) enriched up to 19.75% in U-235 is used as fuel. In the power-flattened design, U-235 enrichment varies radially between 19.75% and 10.5% in …

Automated Additive Layering Of Vat Polymerized Plastic Organic Scintillators, Chandler J. Moore

Theses and Dissertations

The current technology for fast neutron detection imaging is limited in achieving the required high spatial resolution, strong neutron discrimination, and practical time of manufacturing. Traditional fabrication methods require days of thermal polymerization and hundreds of man-hours to produce average resolution pixelated scintillator arrays. The present work helps to eliminate this limitation by developing an additive manufacturing technique to construct such detectors for use in in dual particle imaging applications. In this work, fast-, light-curing resins are used in a prototype automated assembly machine, capable of layering of individual light-cured resin layers and optical segmentation with a self-bonded specular reflector, …

Angle Resolved Photoelectron Spectroscopy Study Of Germanium Tin: Experimentally Determined Electronic Band Gap And Surface Analysis, Jeremy M. Hunter

Theses and Dissertations

The germanium tin band gap is responsive to wavelengths in the mid to near infrared spectrum; this shows promise in meeting the detection demands of the next generation infrared detectors. Recent developments in germanium tin (GeSn) alloy growth techniques have peaked the scientific community’s interest in GeSn based optoelectrical and detection devices. Detection materials made entirely of group IV elements are compatible with complementary metal-oxide semiconductor manufacturing techniques. Understanding the surface chemistry of this alloy is fundamental for solid state device design and must be analyzed to optimize device performance. Studies have shown that with the addition of tin, the …

Fast Engineering Model For Defect Production In Magnesium Oxide, Henry R. Little

Theses and Dissertations

Defect production from irradiation of materials with thicknesses much less than the mean free path for neutron interaction is explored. A model is developed using the Monte Carlo N-Particle transport code from Los Alamos National Laboratory, experimental data from irradiations at the Oak Ridge High Flux Isotope Reactor, defect production theory, and atomistic simulation results to predict the total number of F-centers resulting from neutron irradiation of a MgO rod. This model accurately predicts the concentration of atomic defects under conditions closely matching experiments at long timescales, for large geometries, and requiring only 6.9 minutes on a single CPU. Results …

Fabrication And Testing Of A Novel Layered Metascintillator For Neutron And Gamma Discrimination, Evan W. Threlkeld

Theses and Dissertations

By leveraging new developments in fast-curing of plastic scintillators, it is possible to fabricate multi-material plastic scintillators, or metascintillators, which offer improved and/or novel capabilities for radiation detection. This document proposes one geometry of metascintillator that uses layers of green and blue scintillating material to discriminate neutron/gamma radiation, details the devices necessary to fabricate it, and analyzes the metascintillator’s response to radiation. A model of the metascintillator using Geant4 and Python suggested that spectral-based neutron/gamma event discrimination is possible with 63% of gamma events and only 1% of neutron events being multi-color. Fabrication of a 500 µm per layer metascintillator …