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Performance Limiting Factors Of Cu2znsn(Sxse1-X)4 Solar Cells Prepared By Thermal Evaporation, Sandip Das, Raghu N. Bhattacharya, Krishna C. Mandal
Performance Limiting Factors Of Cu2znsn(Sxse1-X)4 Solar Cells Prepared By Thermal Evaporation, Sandip Das, Raghu N. Bhattacharya, Krishna C. Mandal
Faculty and Research Publications
Cu2ZnSn(SxSe1−x)4 (CZTSSe) thin film solar cells have been prepared by vacuum-based thermal evaporation of metal and binary sulfide precursors followed by annealing in a mixed chalcogen vapor at 550 °C for one hour. The Zn/Sn ratio in the precursor was varied from 0.75 to 1.50 keeping the Cu/(Zn+Sn) ratio constant at 0.7. The best performing solar cell was obtained with a final film composition of Cu/(Zn+Sn)=0.77 and Zn/Sn=1.13 corresponding to a Zn/Sn ratio of 0.9 in the precursor. The champion cell exhibited an open-circuit voltage (VOC) of 506 mV, short-circuit current density (J …