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Full-Text Articles in Science and Technology Studies
Continuous Biotransformation Of Bisphenol A And Diclofenac By Laccase In An Enzymatic Membrane Reactor, Ngoc Luong Nguyen, Faisal I. Hai, William Price, Frederic Leusch, Felicity Roddick, Ewan J. Mcadam, Saleh Faraj Magram, Long D. Nghiem
Continuous Biotransformation Of Bisphenol A And Diclofenac By Laccase In An Enzymatic Membrane Reactor, Ngoc Luong Nguyen, Faisal I. Hai, William Price, Frederic Leusch, Felicity Roddick, Ewan J. Mcadam, Saleh Faraj Magram, Long D. Nghiem
Faisal I Hai
A novel enzymatic membrane reactor (EMR) was explored for continuous removal of two trace organic contaminatnts (TrOCs) ubiquitously detected in wastewater - namely bisphenol A (BPA and diclofnac (DCF) - by a commercially available laccase from aspergillus oryzae.
Enhancement Of Removal Of Trace Organic Contaminants By Powdered Activated Carbon Dosing Into Membrane Bioreactors, Ngoc Luong Nguyen, Faisal Ibney Hai, Long Nghiem, Jinguo Kang, William Price, Chul Park, Kazuo Yamamoto
Enhancement Of Removal Of Trace Organic Contaminants By Powdered Activated Carbon Dosing Into Membrane Bioreactors, Ngoc Luong Nguyen, Faisal Ibney Hai, Long Nghiem, Jinguo Kang, William Price, Chul Park, Kazuo Yamamoto
Faisal I Hai
This study compared the removal efficiency of 22 widespread trace organic contaminants by a laboratory-scale membrane bioreactor (MBR) with and without direct addition of powdered activated carbon (PAC) into the activated sludge reactor over a period of 312 days. The removal of hydrophilic and biologically persistent trace organic contaminants was immediately improved to above 95% after the addition of PAC into MBR. However, a compound-specific gradual decrease in removal underscored the requirement for the addition of fresh PAC. Adsorption onto PAC-added sludge appeared to play a significant role in the relatively more effective aqueous phase removal of a few resistant …
Introduction - A Review Of Membrane Reactors, Fausto Gallucci, Angelo Basile, Faisal Ibney Hai
Introduction - A Review Of Membrane Reactors, Fausto Gallucci, Angelo Basile, Faisal Ibney Hai
Faisal I Hai
In the last decades, membrane catalysis has been studied by several research and the significant progress in this field is summarized in several review articles (Armor 1998, Lin 2001, Lu 2007, Mcleary 2006, Sanchez 2002, Saracco 1994, Shu 1991). Considering a IUPAC definition (Koros 1996), a membrane reactor (MR) is a device for simultaneously performing a reaction (steam reforming, dry reforming, autothermal reforming, etc.) and a membrane-based separation in the same physical device. Therefore, the membrane not only plays the role of a separator, but also takes place in the reaction itself. The term Membrane Bioreactor (MBR), on the other …
Comparison Between Sequential And Simultaneous Application Of Activated Carbon With Membrane Bioreactor For Trace Organic Contaminant Removal, Luong N. Nguyen, Faisal I. Hai, Jinguo Kang, Long D. Nghiem, William E. Price, Wenshan Guo, Huu H. Ngo, Kuo-Lun Tung
Comparison Between Sequential And Simultaneous Application Of Activated Carbon With Membrane Bioreactor For Trace Organic Contaminant Removal, Luong N. Nguyen, Faisal I. Hai, Jinguo Kang, Long D. Nghiem, William E. Price, Wenshan Guo, Huu H. Ngo, Kuo-Lun Tung
Faisal I Hai
The removal efficiency of 22 selected trace organic contaminants by sequential application of granular activated carbon (GAC) and simultaneous application of powdered activated carbon (PAC) with membrane bioreactor (MBR) was compared in this study. Both sequential application of GAC following MBR treatment (MBR–GAC) and simultaneous application of PAC within MBR (PAC–MBR) achieved improved removal (over 95%) of seven hydrophilic and biologically persistent compounds, which were less efficiently removed by MBR-only treatment (negligible to 70%). However, gradual breakthrough of these compounds occurred over an extended operation period. Charged compounds, particularly, fenoprop and diclofenac, demonstrated the fastest breakthrough (complete and 50–70%, in …
Coupling Granular Activated Carbon Adsorption With Membrane Bioreactor Treatment For Trace Organic Contaminant Removal: Breakthrough Behaviour Of Persistent And Hydrophilic Compounds, Luong N. Nguyen, Faisal I. Hai, William E. Price, Jinguo Kang, Long D. Nghiem
Coupling Granular Activated Carbon Adsorption With Membrane Bioreactor Treatment For Trace Organic Contaminant Removal: Breakthrough Behaviour Of Persistent And Hydrophilic Compounds, Luong N. Nguyen, Faisal I. Hai, William E. Price, Jinguo Kang, Long D. Nghiem
Faisal I Hai
This study investigated the removal of trace organic contaminants by a combined membrane bioreactor - granular activated carbon (MBR-GAC) system over a period of 196 days. Of the 22 compounds investigated here, all six hydrophilic compounds with electron-withdrawing functional groups (i.e., metronidazole, carbamazepine, ketoprofen, naproxen, fenoprop and diclofenac) exhibited very low removal efficiency by MBR-only treatment. GAC post-treatment initially complemented MBR treatment very well; however, a compound-specific gradual deterioration of the removal of the above-mentioned problematic compounds was noted. While a 20% breakthrough of all four negatively charged compounds namely ketoprofen, naproxen, fenoprop and diclofenac occurred within 1000-3000 bed volumes …
Coupling Powdered Activated Carbon (Pac) Adsorption With Membrane Bioreactor (Mbr) Treatment For Enhanced Removal Of Trace Organics, Luong Nguyen, Faisal Ibney Hai, Long Nghiem, Jinguo Kang, William Price
Coupling Powdered Activated Carbon (Pac) Adsorption With Membrane Bioreactor (Mbr) Treatment For Enhanced Removal Of Trace Organics, Luong Nguyen, Faisal Ibney Hai, Long Nghiem, Jinguo Kang, William Price
Faisal I Hai
the occurrence of trace organics such as pesticides, pharmaceutically active compounds, natural and synthetic hormones as well as varous industrial compounds in the aquatic environment is of great concern due to their potential adverse effects on human health and those of other biota. Therefore, the removal of these compounds from wastewater is an important consideration to ensure safe drinking water and better protection of the environment. In the literature, several techniques have been explored for trace organics removal, namely, conventional activated sludge, membrane bioreactors (MBRs), and absorptioin. However it has been found that neither MBR nor activated carbon on its …
Rejection And Fate Of Trace Organic Compounds (Trocs) During Membrane Distillation, Kaushalya Wijekoon, Faisal Ibney Hai, Jinguo Kang, William E. Price, Tzahi Cath, Long D. Nghiem
Rejection And Fate Of Trace Organic Compounds (Trocs) During Membrane Distillation, Kaushalya Wijekoon, Faisal Ibney Hai, Jinguo Kang, William E. Price, Tzahi Cath, Long D. Nghiem
Faisal I Hai
In this study, we examined the feasibility of membrane distillation (MD) for removing trace organic compounds (TrOCs) during water and wastewater treatment. A set of 29 compounds was selected to represent major TrOC groups, including pharmaceuticals, steroid hormones, phytoestrogens, UV-filters, industrial chemicals, and pesticides that occur ubiquitously in municipal wastewater. Results reported here suggest that rejection and fate and transport of TrOC during MD are governed by their volatility and, to a lesser extent, hydrophobicity. All TrOCs with pKH > 9 (which can be classified as non-volatile) were well removed by MD. Among the 29 TrOCs investigated in this study, three …
High Retention Membrane Bioreactors: Challenges And Opportunities, Wenhai Luo, Faisal Ibney Hai, William Price, Wenshan Guo, Hao H. Ngo, Kazuo Yamamoto, Long Nghiem
High Retention Membrane Bioreactors: Challenges And Opportunities, Wenhai Luo, Faisal Ibney Hai, William Price, Wenshan Guo, Hao H. Ngo, Kazuo Yamamoto, Long Nghiem
Faisal I Hai
Extensive research has focussed on the development of novel high retention membrane bioreactor (HR-MBR) systems for wastewater reclamation in recent years. HR-MBR integrates high rejection membrane separation with conventional biological treatment in a single step. High rejection membrane separation processes currently used in HR-MBR applications include nanofiltration, forward osmosis, and membrane distillation. In these HR-MBR systems, organic contaminants can be effectively retained, prolonging their retention time in the bioreactor and thus enhancing their biodegradation. Therefore, HR-MBR can offer a reliable and elegant solution to produce high quality effluent. However, there are several technological challenges associated with the development of HR-MBR, …
Removal Of Bisphenol A And Diclofenac By A Novel Fungal Membrane Bioreactor Operated Under Non-Sterile Conditions, Shufan Yang, Faisal I. Hai, Long D. Nghiem, Luong N. Nguyen, Felicity Roddick, William E. Price
Removal Of Bisphenol A And Diclofenac By A Novel Fungal Membrane Bioreactor Operated Under Non-Sterile Conditions, Shufan Yang, Faisal I. Hai, Long D. Nghiem, Luong N. Nguyen, Felicity Roddick, William E. Price
Faisal I Hai
Previous studies have confirmed significant removal of various trace organic contaminants (TrOCs) by white-rot fungal cultures under sterile batch test conditions. However, little is known about TrOC removal in continuous flow fungal reactors in a non-sterile environment. This study reports the removal of two TrOCs, namely, bisphenol A and diclofenac, by a fungal membrane bioreactor (MBR).
Degradation Of Azo Dye Acid Orange 7 In A Membrane Bioreactor By Pellets And Attached Growth Of Coriolus Versicolour, Faisal I. Hai, Kazuo Yamamoto, Fumiyuki Nakajima, Kensuke Fukushi, Long D. Nghiem, William E. Price, Bo Jin
Degradation Of Azo Dye Acid Orange 7 In A Membrane Bioreactor By Pellets And Attached Growth Of Coriolus Versicolour, Faisal I. Hai, Kazuo Yamamoto, Fumiyuki Nakajima, Kensuke Fukushi, Long D. Nghiem, William E. Price, Bo Jin
Faisal I Hai
The aim of this study was to systematically compare the degradation of azo dye acid orange 7 by spongy pellets and attached biofilm of Coriolus versicolour (NBRC 9791) in a membrane bioreactor (MBR) under non-sterile conditions. Mild stirring (35 rpm) resulted in spherical (φ = 0.5 cm), spongy pellets and concomitantly triggered high enzymatic activity of the fungus, allowing for excellent decolouration (>99%) of a synthetic wastewater containing the dye. However, bacterial contamination eventually damaged the fungus pellets, leading to decreased decolouration efficiency. Promotion of attached growth on a plastic support along with formation of spherical spongy pellets allowed …
Coupling Granular Activated Carbon Adsorption With Membrane Bioreactor Treatment For Trace Organic Contaminant Removal: Breakthrough Behaviour Of Persistent And Hydrophilic Compounds, Luong N. Nguyen, Faisal I. Hai, William E. Price, Jinguo Kang, Long D. Nghiem
Coupling Granular Activated Carbon Adsorption With Membrane Bioreactor Treatment For Trace Organic Contaminant Removal: Breakthrough Behaviour Of Persistent And Hydrophilic Compounds, Luong N. Nguyen, Faisal I. Hai, William E. Price, Jinguo Kang, Long D. Nghiem
William E. Price
This study investigated the removal of trace organic contaminants by a combined membrane bioreactor - granular activated carbon (MBR-GAC) system over a period of 196 days. Of the 22 compounds investigated here, all six hydrophilic compounds with electron-withdrawing functional groups (i.e., metronidazole, carbamazepine, ketoprofen, naproxen, fenoprop and diclofenac) exhibited very low removal efficiency by MBR-only treatment. GAC post-treatment initially complemented MBR treatment very well; however, a compound-specific gradual deterioration of the removal of the above-mentioned problematic compounds was noted. While a 20% breakthrough of all four negatively charged compounds namely ketoprofen, naproxen, fenoprop and diclofenac occurred within 1000-3000 bed volumes …
Changes In Surface Properties And Separation Efficiency Of A Nanofiltration Membrane After Repeated Fouling And Chemical Cleaning Cycles, Alexander Simon, William E. Price, Long D. Nghiem
Changes In Surface Properties And Separation Efficiency Of A Nanofiltration Membrane After Repeated Fouling And Chemical Cleaning Cycles, Alexander Simon, William E. Price, Long D. Nghiem
William E. Price
The aim of this study was to evaluate the changes in membrane surface properties and solute separation by a nanofiltration membrane during repetitive membrane fouling and chemical cleaning. Secondary treated effluent and model fouling solutions containing humic acids, sodium alginate, or silica colloids were used to simulate membrane fouling. Chemical cleaning was carried out using a commercially available caustic cleaning formulation. Carbamazepine and sulfamethoxazole were selected to examine the filtration behaviour of neutral and negatively charged organic compounds, respectively. Results show that the impact of membrane fouling on solute rejection is governed by pore blocking, modification of the membrane surface …
Comparison Between Sequential And Simultaneous Application Of Activated Carbon With Membrane Bioreactor For Trace Organic Contaminant Removal, Luong N. Nguyen, Faisal I. Hai, Jinguo Kang, Long D. Nghiem, William E. Price, Wenshan Guo, Huu H. Ngo, Kuo-Lun Tung
Comparison Between Sequential And Simultaneous Application Of Activated Carbon With Membrane Bioreactor For Trace Organic Contaminant Removal, Luong N. Nguyen, Faisal I. Hai, Jinguo Kang, Long D. Nghiem, William E. Price, Wenshan Guo, Huu H. Ngo, Kuo-Lun Tung
William E. Price
The removal efficiency of 22 selected trace organic contaminants by sequential application of granular activated carbon (GAC) and simultaneous application of powdered activated carbon (PAC) with membrane bioreactor (MBR) was compared in this study. Both sequential application of GAC following MBR treatment (MBR–GAC) and simultaneous application of PAC within MBR (PAC–MBR) achieved improved removal (over 95%) of seven hydrophilic and biologically persistent compounds, which were less efficiently removed by MBR-only treatment (negligible to 70%). However, gradual breakthrough of these compounds occurred over an extended operation period. Charged compounds, particularly, fenoprop and diclofenac, demonstrated the fastest breakthrough (complete and 50–70%, in …
Removal Of N-Nitrosamines By An Aerobic Membrane Bioreactor, Kaushalya C. Wijekoon, Takahiro Fujioka, James A. Mcdonald, Stuart J. Khan, Faisal I. Hai, William E. Price, Long D. Nghiem
Removal Of N-Nitrosamines By An Aerobic Membrane Bioreactor, Kaushalya C. Wijekoon, Takahiro Fujioka, James A. Mcdonald, Stuart J. Khan, Faisal I. Hai, William E. Price, Long D. Nghiem
William E. Price
This study investigated the fate of eight N-nitrosamines during membrane bioreactor (MBR) treatment. The results suggest that biodegradation is mainly responsible for the removal of N-nitrosamines during MBR treatment. Other removal mechanisms were insignificant (e.g. adsorption to sludge) or not expected (e.g. photolysis and volatilization) given the experimental conditions and physicochemical properties of the N-nitrosamines studied here. N-nitrosamine removal efficiencies were from 24% to 94%, depending on their molecular properties. High removal of N-nitrosamines such as N-nitrosodimethylamine and N-nitrosodiethylamine could be explained by the presence of strong electron donating functional groups (EDG) in their structure. In contrast, N-nitrosomorpholine possessing the …
Enhanced Biological Phosphorus Removal And Its Modeling For The Activated Sludge And Membrane Bioreactor Processes, M F. R Zuthi, W S. Guo, H H. Ngo, L D. Nghiem, F I. Hai
Enhanced Biological Phosphorus Removal And Its Modeling For The Activated Sludge And Membrane Bioreactor Processes, M F. R Zuthi, W S. Guo, H H. Ngo, L D. Nghiem, F I. Hai
Faisal I Hai
A modified activated sludge process (ASP) for enhanced biological phosphorus removal (EBPR) needs to sustain stable performance for wastewater treatment to avoid eutrophication in the aquatic environment. Unfortunately, the overall efficiency of the EBPR in ASPs and membrane bioreactors (MBRs) is frequently hindered by different operational/system constraints. Moreover, although phosphorus removal data from several wastewater treatment systems are available, a comprehensive mathematical model of the process is still lacking. This paper presents a critical review that highlights the core issues of the biological phosphorus removal in ASPs and MBRs while discussing the inhibitory process requirements for other nutrients' removal. This …
Removal Of N-Nitrosamines By An Aerobic Membrane Bioreactor, Kaushalya C. Wijekoon, Takahiro Fujioka, James A. Mcdonald, Stuart J. Khan, Faisal I. Hai, William E. Price, Long D. Nghiem
Removal Of N-Nitrosamines By An Aerobic Membrane Bioreactor, Kaushalya C. Wijekoon, Takahiro Fujioka, James A. Mcdonald, Stuart J. Khan, Faisal I. Hai, William E. Price, Long D. Nghiem
Faisal I Hai
This study investigated the fate of eight N-nitrosamines during membrane bioreactor (MBR) treatment. The results suggest that biodegradation is mainly responsible for the removal of N-nitrosamines during MBR treatment. Other removal mechanisms were insignificant (e.g. adsorption to sludge) or not expected (e.g. photolysis and volatilization) given the experimental conditions and physicochemical properties of the N-nitrosamines studied here. N-nitrosamine removal efficiencies were from 24% to 94%, depending on their molecular properties. High removal of N-nitrosamines such as N-nitrosodimethylamine and N-nitrosodiethylamine could be explained by the presence of strong electron donating functional groups (EDG) in their structure. In contrast, N-nitrosomorpholine possessing the …