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Articles 1 - 7 of 7
Full-Text Articles in Physics
Photoemission Investigation Of Topological Quantum Materials, Klauss M. Dimitri
Photoemission Investigation Of Topological Quantum Materials, Klauss M. Dimitri
Honors Undergraduate Theses
Topological insulators (TIs) are a class of quantum materials, which behave as insulators in the bulk, yet possess gapless spin-polarized surface states, which are robust against nonmagnetic impurities. The unique properties of TIs make them attractive not only for studying various fundamental phenomena in condensed matter and particle physics, but also as promising candidates for applications ranging from spintronics to quantum computation. Within the topological insulator realm, a great deal of focus has been placed on discovering new quantum materials, however, ideal multi-modal quantum materials have yet to be found. Here we study alpha-PdBi2, KFe2Te2, and DySb compounds including others …
Resonant Anisotropic Emission In Rabbitt Spectroscopy, Bejan M. Ghomashi
Resonant Anisotropic Emission In Rabbitt Spectroscopy, Bejan M. Ghomashi
Honors Undergraduate Theses
A variant of RABBITT pump-probe spectroscopy in which the attosecond pulse train comprises both even and odd harmonics of the fundamental IR probe frequency is explored to measure time-resolved photoelectron emission in systems that exhibit autoionizing states. It is shown that the group delay of both one-photon and two-photon resonant transitions is directly encoded in the energy-resolved photoelectron anisotropy as a function of the pump-probe time-delay. This principle is illustrated for a 1D model with symmetric zero-range potentials that supports both bound states and shape-resonances. The model is studied using both perturbation theory and solving the time-dependent Schodinger equation on …
Micro-Spectroscopy Of Bio-Assemblies At The Single Cell Level, Jeslin Kera
Micro-Spectroscopy Of Bio-Assemblies At The Single Cell Level, Jeslin Kera
Honors Undergraduate Theses
In this thesis, we investigate biological molecules on a micron scale in the ultraviolet spectral region through the non-destructive confocal absorption microscopy. The setup involves a combination of confocal microscope with a UV light excitation beam to measure the optical absorption spectra with spatial resolution of 1.4 μm in the lateral and 3.6 μm in the axial direction. Confocal absorption microscopy has the benefits of requiring no labels and only low light intensity for excitation while providing a strong signal from the contrast generated by the attenuation of propagating light due to absorption. This enables spatially resolved measurements of single …
Synchrotron Based Infrared Microspectroscopy Of Carbonaceous Chondrites., Mehmet Yesiltas
Synchrotron Based Infrared Microspectroscopy Of Carbonaceous Chondrites., Mehmet Yesiltas
Electronic Theses and Dissertations
Relationships between organic molecules and inorganic minerals are investigated in five carbonaceous chondrites, Northwest Africa 852 (CR2), Tagish Lake (C2-ungroupped), Orgueil (CI1), Sutter's Mill (CM), and Murchison (CM2), with micron spatial resolution using synchrotron-based imaging micro-FTIR spectroscopy. Correlations based on absorption strength for various constituents are determined using statistical correlation analysis. Silicate band is found to be positively correlated with stretching modes of aliphatic hydrocarbons in NWA 852 and Tagish Lake. The former is highly correlated with the hydration band in all meteorites. Negative correlation is observed between water+organics and carbonate bands in all meteorites. Two dimensional infrared maps for …
Characterization And Application Of Isolated Attosecond Pulses, Michael Chini
Characterization And Application Of Isolated Attosecond Pulses, Michael Chini
Electronic Theses and Dissertations
Tracking and controlling the dynamic evolution of matter under the influence of external fields is among the most fundamental goals of physics. In the microcosm, the motion of electrons follows the laws of quantum mechanics and evolves on the timescale set by the atomic unit of time, 24 attoseconds. While only a few time-dependent quantum mechanical systems can be solved theoretically, recent advances in the generation, characterization, and application of isolated attosecond pulses and few-cycle femtosecond lasers have given experimentalists the necessary tools for dynamic measurements on these systems. However, pioneering studies in attosecond science have so far been limited …
Random Transformations Of Optical Fields And Applications, Thomas Kohlgraf-Owens
Random Transformations Of Optical Fields And Applications, Thomas Kohlgraf-Owens
Electronic Theses and Dissertations
The interaction of optical waves with material systems often results in complex, seemingly random fields. Because the fluctuations of such fields are typically difficult to analyze, they are regarded as noise to be suppressed. Nevertheless, in many cases the fluctuations of the field result from a linear and deterministic, albeit complicated, interaction between the optical field and the scattering system. As a result, linear systems theory (LST) can be used to frame the scattering problem and highlight situations in which useful information can be extracted from the fluctuations of the scattered field. Three fundamental problems can be posed in LST …
Molecular Structure-Nonlinear Optical Property Relationships For A Series Of Polymethine And Squaraine Molecules, Jie Fu
Electronic Theses and Dissertations
This dissertation reports on the investigation of the relationships between molecular structure and two-photon absorption (2PA) properties for a series of polymethine and squaraine molecules. Current and emerging applications exploiting the quadratic dependence upon laser intensity, such as two-photon fluorescence imaging, three-dimensional microfabrication, optical data storage and optical limiting, have motivated researchers to find novel materials exhibiting strong 2PA. Organic materials are promising candidates because their linear and nonlinear optical properties can be optimized for applications by changing their structures through molecular engineering. Polymethine and squaraine dyes are particularly interesting because they are fluorescent and showing large 2PA. We used …