Physics Commons^™

Photoelectric Characterization Of Bacteriorhodopsin Reconstituted In Lipid Bilayer Membrane, Joel Kamwa

Graduate Theses and Dissertations

The objective of this work was to conduct basic research in biologically inspired energy conversion solutions. A photosynthetic protein (Bacteriorhodopsin) was reconstituted in a bi-layer membrane. Then, when a laser beam was shined on the membrane, the photon energy was used by the protein to pump protons across the membrane. The translocation of protons across the membrane was measured as photocurrent. For this purpose, a system was built to characterize the lipid bilayer membranes and to measure the photocurrent. The lipid bilayer membrane was characterized by its capacitance and resistance. A picoampere photocurrent was observed when Bacteriorhodopsin protein was present …

Nuclear Magnetic Resonance Studies On Lithium And Sodium Electrode Materials For Rechargeable Batteries, Tetiana Nosach

Dissertations, Theses, and Capstone Projects

In this thesis, Nuclear Magnetic Resonance (NMR) spectroscopic techniques are used to study lithium and sodium electrode materials for advanced rechargeable batteries. Three projects are described in this thesis. The first two projects involve 6Li, 7Li and 31P NMR studies of two cathode materials for advanced rechargeable batteries. The third project is a study of sodium titanate cathode materials for Na-ion batteries, where 1H, 7Li, and 23Na static and magic angle spinning NMR were used in order to obtain detailed information on the chemical environments.

Optical Resonators And Fiber Tapers As Transducers For Detection Of Nanoparticles And Bio-Molecules, Huzeyfe Yilmaz

McKelvey School of Engineering Theses & Dissertations

In recent years, detection of biological interactions on single molecule level has aspired many researchers to investigate several optical, chemical, electrical and mechanical sensing tools. Among these tools, toroidal optical resonators lead the way in detection of the smallest particle/molecule with the real time measurements. In this work, bio-sensing capabilities of toroidal optical resonators are investigated. Bio-sensing is realized via measuring the analyte-antigen interaction while the antigen is immobilized through a novel functionalization method.

Not long ago, detection of single nanoparticles using optical resonators has been accomplished however the need for cost-effective and practical transducers demands simpler tools. A tapered …

Propagation Of An Optical Vortex In Fiber Arrays With Triangular Lattices, Muhammad Abdulrahman Mushref

Theses and Dissertations

The propagation of optical vortices (OVs) in linear and nonlinear media is an important field of research in science and engineering. The most important goal is to explore the properties of guiding dynamics for potential applications such as sensing, all-optical switching, frequency mixing and modulation. In this dissertation, we present analytical methods and numerical techniques to investigate the propagation of an optical vortex in fiber array waveguides. Analytically, we model wave propagation in a waveguide by coupled mode Equations as a simplified approximation. The beam propagation method (BPM) is also employed to numerically solve the paraxial wave Equation by finite …

Quantum Levitation Using Metamaterials, Venkatesh K. Pappakrishnan

Doctoral Dissertations

The emergence of an attractive vacuum force (Casimir force) between two purely dielectric materials can lead to an increase in the friction and the stiction effects in nanoscale devices, resulting in degradation or decreased performance. Thus, it is of high practical importance that the conditions for the reversal of the Casimir force from attractive to repulsive are identified. Although the repulsive Casimir force has been considered for high dielectric materials as an intermediate (between the plates) medium, so far no realistic system has been proposed that can demonstrate quantum levitation with air/vacuum as a host medium. Since air is the …

On Electromagnetic And Quantum Invisibility, Pattabhiraju Chowdary Mundru

Doctoral Dissertations

The principle objective of this dissertation is to investigate the fundamental properties of electromagnetic wave interactions with artificially fabricated materials i.e., metamaterials for application in advanced stealth technology called electromagnetic cloaking. The main goal is to theoretically design a metamaterial shell around an object that completely eliminates the dipolar and higher order multipolar scattering, thus making the object invisible.

In this context, we developed a quasi-effective medium theory that determines the optical properties of multi-layered-composites beyond the quasi-static limit. The proposed theory exactly reproduces the far-field scattering/extinction cross sections through an iterative process in which mode-dependent quasi-effective impedances of the …

Investigation And Optimization Of A New Compact Superconducting Cavity For Deflecting And Crabbing Applications, Subashini Uddika De Silva

Physics Theses & Dissertations

Deflecting and crabbing structures have many applications in current accelerator systems. The primary use of a deflecting cavity is to separate a single beam into multiple beams. A crabbing cavity enables the head-on collision at the interaction point in particle colliders in order to increase the luminosity. The early uses of the deflecting structures have been in the early 1960s: these structures were disk loaded structures operating at room temperature. The crabbing structure which was installed at the NEK electron-positron collider was the first and only operational superconducting cavity of that kind. The most common design of superconducting deflecting and …

Properties Of Multiferroic Bifeo3 From First Principles, Dovran Rahmedov

Graduate Theses and Dissertations

In this dissertation, a first-principle-based approach is developed to study magnetoelectric effect in multiferoic materials. Such approach has a significant predictive power and might serve as a guide to new experimental works. As we will discuss in the course of this work, it also gives an important insight to the underlying physics behind the experimentally observed phenomena.

We start by applying our method to investigate properties of a generic multiferroic material. We observe how magnetic susceptibility of such materials evolves with temperature and compare this evolution with the characteristic behavior of magnetic susceptibility for pure magnetic systems. Then we focus …

Frequency Selective Detection Of Infrared Radiation In Uncooled Optical Nano-Antenna Array, Sushrut Modak

Electronic Theses and Dissertations

Mid-infrared (mid-IR) detection and imaging over atmospheric transparent 3-5 μm and 8-12 μm bands are increasingly becoming important for various space, defense and civilian applications. Various kinds of microbolometers offer uncooled detection of IR radiation. However, broadband absorption of microbolometers makes them less sensitive to spectrally resolved detection of infrared radiation and the fabrication is also very tedious involving multiple complex lithography steps. In this study, we designed an optical nano-antenna array based detector with narrow frequency band of operation. The structure consists of a two-element antenna array comprised of a perforated metallic hole array coupled with an underneath disk …

Self-Heating Control Of Edge Emitting And Vertical Cavity Surface Emitting Lasers, Yu Zhang

Electronic Theses and Dissertations

Self-heating leads to temperature rise of laser diode and limits the output power, efficiency and modulation bandwidth due to increased loss and decreased differential gain. The main heat sources in laser diode during continuous wave operation are Joule heating and free carrier absorption loss. To control device self-heating, the epi structure needs to be designed with low electrical resistance and low absorption loss, while the heat flux must spread out of the device efficiently. This dissertation presents the control of self-heating of both edge emitting laser diodes and vertical cavity surface emitting lasers (VCSELs). For the 980nm high power edge …

Distribution Of Laser Induced Heating In Multi-Component Chalcogenide Glass And Its Associated Effects, Laura Sisken

Electronic Theses and Dissertations

Chalcogenide glasses are well known to have good transparency into the infrared spectrum. These glasses though tend to have low thresholds as compared to oxide glasses for photo-induced changes and thermally-induced changes. Material modification such as photo-induced darkening, bleaching, refractive index change, densification or expansion, ablation of crystallization have been demonstrated, and are typically induced by a thermal furnace-based heat treatment, an optical source such as a laser, or a combination of photo-thermal interactions. Solely employing laser-based heating has an advantage over a furnace, since one has the potential to be able to spatially modify the materials properties with much …

Highly-Sensitive Stoichiometric Analysis Of Yag Ceramics Using Laser-Induced Breakdown Spectroscopy (Libs), Jahromi, Ali Kazemi

Electronic Theses and Dissertations

Transparent ceramics are an important class of optical materials with applications in high-strength windows, radiation detectors and high-power lasers. Despite the many successful developments of the past decades, their challenging fabrication still needs to be perfected to achieve a better consistency in optical quality. In particular, ternary phase materials such as Yttrium Aluminum Garnet (YAG, Y3Al5O12), a long standing high-power laser host, require a precise control of stoichiometry, often beyond the precision of current analytical techniques, in order to reduce scattering losses and the presence of deleterious point defects. This work explores the potential of Laser-Induced Breakdown Spectroscopy (LIBS) for …

High Resolution Time-Resolved Imaging System In The Vacuum Ultraviolet Region, Yuseong Jang

Electronic Theses and Dissertations

High-power debris-free vacuum ultraviolet (VUV) light sources have applications in several scientific and engineering areas, such as high volume manufacturing lithography and inspection tools in the semiconductor industry, as well as other applications in material processing and photochemistry. For the past decades, the semiconductor industry has been driven by what is called "Moore's Law". The entire semiconductor industry relies on this rule, which requires chip makers to pack transistors more tightly with every new generation of chips, shrinking the size of transistors. The ability to solve roadmap challenges is, at least partly, proportional to our ability to measure them. The …

High Performance Three-Dimensional Display Based On Polymer-Stabilized Blue Phase Liquid Crystal, Yifan Liu

Electronic Theses and Dissertations

Autostereoscopic 2D/3D (two-dimension/three-dimension) switchable display has been attracting great interest in research and practical applications for several years. Among different autostereoscopic solutions, direction-multiplexed 3D displays based on microlens array or parallax barrier are viewed as the most promising candidates, due to their compatibility with conventional 2D display technologies. These 2D/3D switchable display system designs rely on fast switching display panels and photonics devices, including adaptive focus microlens array and switchable slit array. Polymer-stabilized blue phase liquid crystal (PS-BPLC) material provides a possible solution to meet the aforementioned fast response time requirement. However, present display and photonic devices based on blue …

Holographic Recording And Applications Of Multiplexed Volume Bragg Gratings In Photo-Thermo-Refractive Glass, Daniel Ott

Electronic Theses and Dissertations

Recent developments in holographic recording of volume Bragg gratings (VBGs) in photo-thermo-refractive (PTR) glass have demonstrated their utility as components in high power laser systems for spectral narrowing, transverse mode control, beam combining, and pulse stretching/compression. VBG structures are capable of diffracting incident light into a single diffraction order with high efficiency given the Bragg condition is met. The Bragg condition depends on both the wavelength and angle of the incident light making VBGs useful for filtering and manipulating both the wavelength and angular spectrum of a source. This dissertation expands upon previous research in PTR VBGs by investigating multiplexed …

Entangled Photon Pairs In Disordered Photonic Lattices, Lane Martin

Electronic Theses and Dissertations

Photonic lattices consisting of arrays of evanescently coupled waveguides fabricated with precisely controlled parameters have enabled the study of discrete optical phenomena, both classical and quantum, and the simulation of other physical phenomena governed by the same dynamics. In this dissertation, I have experimentally demonstrated transverse Anderson localization of classical light in arrays with off-diagonal coupling disorder and investigated theoretically and experimentally the propagation of entangled photon pairs through such disordered systems. I discovered a new phenomenon, Anderson co-localization, in which a spatially entangled photon pair in a correlated transversally extended state localizes in the correlation space, though neither photon …

Injection-Locked Vertical Cavity Surface Emitting Lasers (Vcsels) For Optical Arbitrary Waveform Generation, Sharad Bhooplapur

Electronic Theses and Dissertations

Complex optical pulse shapes are typically generated from ultrashort laser pulses by manipulating the optical spectrum of the input pulses. This generates complex but periodic time-domain waveforms. Optical Arbitrary Waveform Generation (OAWG) builds on the techniques of ultrashort pulse-shaping, with the goal of making non-periodic, truly arbitrary optical waveforms. Some applications of OAWG are coherently controlling chemical reactions on a femtosecond time scale, improving the performance of LADAR systems, high-capacity optical telecommunications and ultra wideband signals processing. In this work, an array of Vertical Cavity Surface Emitting Lasers (VCSELs) are used as modulators, by injection-locking each VCSEL to an individual …

Nonlinear Integrated Photonics On Silicon And Gallium Arsenide Substrates, Jichi Ma

Electronic Theses and Dissertations

Silicon photonics is nowadays a mature technology and is on the verge of becoming a blossoming industry. Silicon photonics has also been pursued as a platform for integrated nonlinear optics based on Raman and Kerr effects. In recent years, more futuristic directions have been pursued by various groups. For instance, the realm of silicon photonics has been expanded beyond the well-established near-infrared wavelengths and into the mid-infrared (3 - 5 µm). In this wavelength range, the omnipresent hurdle of nonlinear silicon photonics in the telecommunication band, i.e., nonlinear losses due to two-photon absorption, is inherently nonexistent. With the lack of …

Photonic Filtering For Applications In Microwave Generation And Metrology, Marcus Bagnell

Electronic Theses and Dissertations

This work uses the photonic filtering properties of Fabry-Perot etalons to show improvements in the electrical signals created upon photodetection of the optical signal. First, a method of delay measurement is described which uses multi-heterodyne detection to find correlations in white light signals at 20 km of delay to sub millimeter resolution. By filtering incoming white light with a Fabry-Perot etalon, the pseudo periodic signal is suitable for measurement by combining and photodetecting it with an optical frequency comb. In this way, optical data from a large bandwidth can be downconverted and sampled on low frequency electronics. Second, a high …

Multifunctional, Multimaterial Particle Fabrication Via An In-Fiber Fluid Instability, Joshua Kaufman

Electronic Theses and Dissertations

Spherical micro- and nano-particles have found widespread use in many various applications from paint to cosmetics to medicine. Due to the multiplicity of desired particle material(s), structure, size range, and functionality, many approaches exist for generating such particles. Bottom-up methods such as chemical synthesis have a high yield and work with a wide range of materials; however, these processes typically lead to large polydispersity and cannot produce structured particles. Top-down approaches such as microfluidics overcome the polydispersity issue and may produce a few different structures in particles, but at lower rates and only at the micro-scale. A method that can …

Large Area Conformal Infrared Frequency Selective Surfaces, Jeffrey D'Archangel

Electronic Theses and Dissertations

Frequency selective surfaces (FSS) were originally developed for electromagnetic filtering applications at microwave frequencies. Electron-beam lithography has enabled the extension of FSS to infrared frequencies; however, these techniques create sample sizes that are seldom appropriate for real world applications due to the size and rigidity of the substrate. A new method of fabricating large area conformal infrared FSS is introduced, which involves releasing miniature FSS arrays from a substrate for implementation in a coating. A selective etching process is proposed and executed to create FSS particles from crossed-dipole and square-loop FSS arrays. When the fill-factor of the particles in the …

Broad Bandwidth, All-Fiber, Thulium-Doped Photonic Crystal Fiber Amplifier For Potential Use In Scaling Ultrashort Pulse Peak Powers, Alex Sincore

Electronic Theses and Dissertations

Fiber based ultrashort pulse laser sources are desirable for many applications; however generating high peak powers in fiber lasers is primarily limited by the onset of nonlinear effects such as self-phase modulation, stimulated Raman scattering, and self-focusing. Increasing the fiber core diameter mitigates the onset of these nonlinear effects, but also allows unwanted higher-order transverse spatial modes to propagate. Both large core diameters and single-mode propagation can be simultaneously attained using photonic crystal fibers. Thulium-doped fiber lasers are attractive for high peak power ultrashort pulse systems. They offer a broad gain bandwidth, capable of amplifying sub-100 femtosecond pulses. The longer …

Laser Filamentation - Beyond Self-Focusing And Plasma Defocusing, Khan Lim

Electronic Theses and Dissertations

Laser filamentation is a highly complex and dynamic nonlinear process that is sensitive to many physical parameters. The basic properties that define a filament consist of (i) a narrow, high intensity core that persists for distances much greater than the Rayleigh distance, (ii) a low density plasma channel existing within the filament core, and (iii) a supercontinuum generated over the course of filamentation. However, there remain many questions pertaining to how these basic properties are affected by changes in the conditions in which the filaments are formed; that is the premise of the work presented in this dissertation. To examine …

Multimaterial Fibers In Photonics And Nanotechnology, Guangming Tao

Electronic Theses and Dissertations

Recent progress in combing multiple materials with distinct optical, electronic, and thermomechanical properties monolithically in a kilometer-long fiber drawn from a preform offers unique multifunctionality at a low cost. A wide range of unique in-fiber devices have been developed in fiber form-factor using this strategy. Here, I summary my recent results in this nascent field of 'multimaterial fibers'. I will focus on my achievements in producing robust infrared optical fibers and in appropriating optical fiber production technology for applications in nanofabrication. The development of optical components suitable for the infrared (IR) is crucial for applications in this spectral range to …

Reference Compensation For Localized Surface-Plasmon Resonance Sensors, Neha Nehru

Theses and Dissertations--Electrical and Computer Engineering

Noble metal nanoparticles supporting localized surface plasmon resonances (LSPR) have been extensively investigated for label free detection of various biological and chemical interactions. When compared to other optical sensing techniques, LSPR sensors offer label-free detection of biomolecular interactions in localized sensing volume solutions. However, these sensors also suffer from a major disadvantage – LSPR sensors remain highly susceptible to interference because they respond to both solution refractive index change and non-specific binding as well as specific binding of the target analyte. These interactions can severely compromise the measurement of the target analyte in a complex unknown media and hence limit …

Techniques For Characterization Of Third Order Optical Nonlinearities, Manuel Ferdinandus

Electronic Theses and Dissertations

This dissertation describes the development of novel techniques for characterization of nonlinear properties of materials. The dissertation is divided into two parts, a background and theory section and a technique development section. In the background and theory section we explain the origins of the nonlinear optical response of materials across many different spatial and temporal scales. The mechanisms that we are most interested in are the electronic nuclear and reorientational responses, which occur on the range of sub-femtosecond to several picoseconds. The electronic mechanism is due to the electrons of a material experiencing a non-parabolic potential well due a strong …

Advanced Liquid Crystal Materials For Display And Photonic Applications, Yuan Chen

Electronic Theses and Dissertations

Thin-film-transistor (TFT) liquid crystal display (LCD) has been widely used in smartphones, pads, laptops, computer monitors, and large screen televisions, just to name a few. A great deal of effort has been delved into wide viewing angle, high resolution, low power consumption, and vivid color. However, relatively slow response time and low transmittance remain as technical challenges. To improve response time, several approaches have been developed, such as low viscosity liquid crystals, overdrive and undershoot voltage schemes, thin cell gap with a high birefringence liquid crystal, and elevated temperature operation. The state-of-the-art gray-to-gray response time of a nematic LC device …

Generation And Characterization Of Sub-70 Isolated Attosecond Pulses, Qi Zhang

Electronic Theses and Dissertations

Dynamics occurring on microscopic scales, such as electronic motion inside atoms and molecules, are governed by quantum mechanics. However, the Schroedinger equation is usually too complicated to solve analytically for systems other than the hydrogen atom. Even for some simple atoms such as helium, it still takes months to do a full numerical analysis. Therefore, practical problems are often solved only after simplification. The results are then compared with the experimental outcome in both the spectral and temporal domain. For accurate experimental comparison, temporal resolution on the attosecond scale is required. This had not been achieved until the first demonstration …

Lp Fiber Mode Converters Using Holographic Phase Mask In Photo-Thermo-Refractive Glass, Aniket Patil

Electronic Theses and Dissertations

In this study, an investigation was undertaken to research the use of holographic phase masks (HPMs) in photo-thermo-refractive (PTR) glass as mode converters for linearly polarized (LP) fiber modes. A Spatial Light Modulator (SLM) was used to generate higher-order transverse fiber modes LPm,n. Under proper incidence condition on the holographic device, LPm,n modes are diffracted and simultaneously converted into higher order or lower order LP modes. The process was analyzed by imaging the far field on a CCD camera. It is demonstrated that using this novel method of converting transverse fiber modes several combinations of LP modes can be converted …

Particle Manipulation Via Optical Forces And Engineering Soft-Matter Systems With Tunable Nonlinearities., Shima Fardad

Electronic Theses and Dissertations

One of the most intriguing properties of light-matter interaction is the ability of an electromagnetic field to exert mechanical forces on polarizable objects. This phenomenon is a direct consequence of the fact that light carries momentum, which in turn can be transferred to matter. Mediated by scattering, this interaction usually manifests itself as a “pushing force” in the direction of beam propagation. However, it is possible to judiciously engineer these optical forces, either by tailoring particle polarizability, and/or by structuring the incident light field. As a simple example, a tightly focused laser beam demonstrates strong gradient forces, which may attract …