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Articles 1 - 30 of 46
Full-Text Articles in Physics
More On The Demons Of Thermodynamics, Daniel P. Sheehan, Garret Moddel, James W. Lee
More On The Demons Of Thermodynamics, Daniel P. Sheehan, Garret Moddel, James W. Lee
Chemistry & Biochemistry Faculty Publications
No abstract provided.
Ds2 As Excitation Of Ads2, Florian Ecker, Daniel Grumiller, Robert Mcnees
Ds2 As Excitation Of Ads2, Florian Ecker, Daniel Grumiller, Robert Mcnees
Physics: Faculty Publications and Other Works
Title- dS2 as excitation of AdS2
We introduce a family of 2D dilaton gravity models with state-dependent constant curvature so that dS2 emerges as an excitation of AdS2. Curiously, the strong coupling region corresponds to the asymptotic region geometrically. Apart from these key differences, many features resemble the Almheiri–Polchinski model. We discuss perturbative and non-perturbative thermodynamical stability, bubble nucleation through matter shockwaves, and semiclassical backreaction effects. In some of these models, we find that low temperatures are dominated by AdS2 but high temperatures are dominated by dS2, concurrent with a recent proposal …
Symmetry And Control In Thermodynamics, Emily Adlam, L. Uribarri, N. Allen
Symmetry And Control In Thermodynamics, Emily Adlam, L. Uribarri, N. Allen
Mathematics, Physics, and Computer Science Faculty Articles and Research
We explore the relationship between symmetry and entropy, distinguishing between symmetries of state and dynamical symmetries, and in the context of quantum thermodynamics between symmetries of pure and mixed states. Ultimately, we will argue that symmetry in thermodynamics is best understood as a means of control within the control theory paradigm, and we will describe an interesting technological application of symmetry-based control in the context of a quantum coherence capacitor. Symmetry, the concept from which Noether derived the conservation laws of physics, is one of the most important guiding principles of modern physics. Moreover, symmetry is often regarded as a …
Protein Conformational Entropy Is Not Slaved To Water, Bryan S Marques, Matthew A Stetz, Christine Jorge, Kathleen G Valentine, A Joshua Wand, Nathaniel V Nucci
Protein Conformational Entropy Is Not Slaved To Water, Bryan S Marques, Matthew A Stetz, Christine Jorge, Kathleen G Valentine, A Joshua Wand, Nathaniel V Nucci
Faculty Scholarship for the College of Science & Mathematics
Conformational entropy can be an important element of the thermodynamics of protein functions such as the binding of ligands. The observed role for conformational entropy in modulating molecular recognition by proteins is in opposition to an often-invoked theory for the interaction of protein molecules with solvent water. The "solvent slaving" model predicts that protein motion is strongly coupled to various aspects of water such as bulk solvent viscosity and local hydration shell dynamics. Changes in conformational entropy are manifested in alterations of fast internal side chain motion that is detectable by NMR relaxation. We show here that the fast-internal side …
Contact In The Unitary Fermi Gas Across The Superfluid Phase Transition, S. Jensen, Christopher N. Gilbreth, Y. Alhassid
Contact In The Unitary Fermi Gas Across The Superfluid Phase Transition, S. Jensen, Christopher N. Gilbreth, Y. Alhassid
All Faculty Scholarship for the College of the Sciences
A quantity known as the contact is a fundamental thermodynamic property of quantum many-body systems with short-range interactions. Determination of the temperature dependence of the contact for the unitary Fermi gas of infinite scattering length has been a major challenge, with different calculations yielding qualitatively different results. Here we use finite-temperature auxiliary-field quantum Monte Carlo (AFMC) methods on the lattice within the canonical ensemble to calculate the temperature dependence of the contact for the homogeneous spin-balanced unitary Fermi gas. We extrapolate to the continuum limit for 40, 66, and 114 particles, eliminating systematic errors due to finite-range effects. We observe …
Testing A Thermodynamic Approach To Collective Animal Behavior In Laboratory Fish Schools, Julia A. Giannini, James G. Puckett
Testing A Thermodynamic Approach To Collective Animal Behavior In Laboratory Fish Schools, Julia A. Giannini, James G. Puckett
Physics and Astronomy Faculty Publications
Collective behaviors displayed by groups of social animals are observed frequently in nature. Understanding and predicting the behavior of complex biological systems is dependent on developing effective descriptions and models. While collective animal systems are characteristically nonequilibrium, we can employ concepts from equilibrium statistical mechanics to motivate the measurement of material-like properties in laboratory animal aggregates. Here, we present results from a new set of experiments that utilize high speed footage of two-dimensional schooling events, particle tracking, and projected static and dynamic light fields to observe and control the behavior of negatively phototaxic fish schools (Hemigrammus bleheri). First, …
Planck's And Callendar's Blackbody Radiation Formulas And Their Fitness To Experimental Data, Max Tran
Planck's And Callendar's Blackbody Radiation Formulas And Their Fitness To Experimental Data, Max Tran
Publications and Research
In this paper, we compare the blackbody radiation density formula obtained with classical physics by Hugh L Callendar and the formula obtained by Max Planck using quantization of energy. We use R and Maxima to analyze their fitness on coordinating experimental data and indicate some limitations with experiments in this area.
Sympathetic Physics: The Keely Motor And The Laws Of Thermodynamics In Nineteenth-Century Culture, Robert Macdougall
Sympathetic Physics: The Keely Motor And The Laws Of Thermodynamics In Nineteenth-Century Culture, Robert Macdougall
History Publications
In Philadelphia in the 1870s, John Worrell Keely announced the invention of a fantastic new motor that could, he promised, drive locomotives, power factories, and even defy gravity without fuel or heat. The Keely Motor became the most notorious perpetual motion scheme of the nineteenth century, attracting believers and investors for nearly thirty years. This article explores the “work” the motor performed for Keely, his supporters, and his critics—not physical work, but financial, cultural, and psychological. To investors, the Keely Motor represented a dream of riches without effort. To Keely’s critics, the motor offered an opportunity to defend the legitimacy …
Comment On "Roles Of Bulk Viscosity On Rayleigh-Taylor Instability: Non-Equilibrium Thermodynamics Due To Spatio-Temporal Pressure Fronts" Phys. Fluids 28, 094102 (2016), Robert L. Ash
Mechanical & Aerospace Engineering Faculty Publications
No abstract provided.
Student Understanding Of The Boltzmann Factor, Trevor I. Smith, Donald B. Mountcastle, John R. Thompson
Student Understanding Of The Boltzmann Factor, Trevor I. Smith, Donald B. Mountcastle, John R. Thompson
Physics and Astronomy Faculty Scholarship
We present results of our investigation into student understanding of the physical significance and utility of the Boltzmann factor in several simple models. We identify various justifications, both correct and incorrect, that students use when answering written questions that require application of the Boltzmann factor. Results from written data as well as teaching interviews suggest that many students can neither recognize situations in which the Boltzmann factor is applicable nor articulate the physical significance of the Boltzmann factor as an expression for multiplicity, a fundamental quantity of statistical mechanics. The specific student difficulties seen in the written data led us …
Identifying Student Difficulties With Heat Engines, Entropy, And The Carnot Cycle, Trevor I. Smith, Warren M. Christensen, Donald B. Mountcastle, John R. Thompson
Identifying Student Difficulties With Heat Engines, Entropy, And The Carnot Cycle, Trevor I. Smith, Warren M. Christensen, Donald B. Mountcastle, John R. Thompson
Physics and Astronomy Faculty Scholarship
We report on several specific student difficulties regarding the second law of thermodynamics in the context of heat engines within upper-division undergraduate thermal physics courses. Data come from ungraded written surveys, graded homework assignments, and videotaped classroom observations of tutorial activities. Written data show that students in these courses do not clearly articulate the connection between the Carnot cycle and the second law after lecture instruction. This result is consistent both within and across student populations. Observation data provide evidence for myriad difficulties related to entropy and heat engines, including students’ struggles in reasoning about situations that are physically impossible …
Identifying Student Difficulties With Entropy, Heat Engines, And The Carnot Cycle, Trevor I. Smith, Warren M. Christensen, Donald B. Mountcastle, John R. Thompson
Identifying Student Difficulties With Entropy, Heat Engines, And The Carnot Cycle, Trevor I. Smith, Warren M. Christensen, Donald B. Mountcastle, John R. Thompson
Faculty Scholarship for the College of Science & Mathematics
We report on several specific student difficulties regarding the second law of thermodynamics in the context of heat engines within upper-division undergraduate thermal physics courses. Data come from ungraded written surveys, graded homework assignments, and videotaped classroom observations of tutorial activities. Written data show that students in these courses do not clearly articulate the connection between the Carnot cycle and the second law after lecture instruction. This result is consistent both within and across student populations. Observation data provide evidence for myriad difficulties related to entropy and heat engines, including students’ struggles in reasoning about situations that are physically impossible …
Lectures On Thermodynamics And Statistical Mechanics, V P. Nair
Lectures On Thermodynamics And Statistical Mechanics, V P. Nair
Open Educational Resources
No abstract provided.
Cosmological Constant As Confining U(1) Charge In Two-Dimensional Dilaton Gravity, Daniel Grumiller, Robert A. Mcnees Iv, Jakob Salzer
Cosmological Constant As Confining U(1) Charge In Two-Dimensional Dilaton Gravity, Daniel Grumiller, Robert A. Mcnees Iv, Jakob Salzer
Physics: Faculty Publications and Other Works
The cosmological constant is treated as a thermodynamical parameter in the framework of two-dimensional dilaton gravity. We find that the cosmological constant behaves as a U(1) charge with a confining potential, and that such potentials require a novel Born-Infeld boundary term in the action. The free energy and other thermodynamical quantities of interest are derived, from first principles, in a way that is essentially model independent. We discover that there is always a Schottky anomaly in the specific heat and explain its physical origin. Finally, we apply these results to specific examples, like anti-de Sitter–Schwarzschild–Tangherlini black holes, Bañados-Teitelboim-Zanelli black holes …
Hydration Of The Sulfuric Acid−Methylamine Complex And Implications For Aerosol Formation, Danielle J. Bustos, Berhane Temelso, George C. Shields
Hydration Of The Sulfuric Acid−Methylamine Complex And Implications For Aerosol Formation, Danielle J. Bustos, Berhane Temelso, George C. Shields
Faculty Journal Articles
The binary H2SO4−H2O nucleation is one of the most important pathways by which aerosols form in the atmosphere, and the presence of ternary species like amines increases aerosol formation rates. In this study, we focus on the hydration of a ternary system of sulfuric acid (H2SO4), methylamine (NH2CH3), and up to six waters to evaluate its implications for aerosol formation. By combining molecular dynamics (MD) sampling with high-level ab initio calculations, we determine the thermodynamics of forming H2SO4(NH2CH3)(H …
Approximate Equations Of State In Two-Temperature Plasma Mixtures, John D. Ramshaw, Andrew W. Cook
Approximate Equations Of State In Two-Temperature Plasma Mixtures, John D. Ramshaw, Andrew W. Cook
Physics Faculty Publications and Presentations
Approximate thermodynamic state relations for multicomponent atomic and molecular gas mixtures are often constructed by artificially partitioning the mixture into its constituent materials and requiring the separated materials to be in temperature and pressure equilibrium. Iterative numerical algorithms have been employed to enforce this equilibration and compute the resulting approximate state relations in single-temperature mixtures. In partially ionized gas mixtures, there is both theoretical and empirical evidence that equilibrating the chemical potentials, number densities, or partial pressures of the free electrons is likely to produce more accurate results than equilibrating the total pressures. Moreover, in many situations of practical interest …
Size-Induced Chemical And Magnetic Ordering In Individual Fe–Au Nanoparticles, Pinaki Mukherjee, Priyanka Manchanda, Pankaj Kumar, Lin Zhou, Matthew J. Kramer, Arti Kashyap, Ralph Skomski, David J. Sellmyer, Jeffrey E. Shield
Size-Induced Chemical And Magnetic Ordering In Individual Fe–Au Nanoparticles, Pinaki Mukherjee, Priyanka Manchanda, Pankaj Kumar, Lin Zhou, Matthew J. Kramer, Arti Kashyap, Ralph Skomski, David J. Sellmyer, Jeffrey E. Shield
David Sellmyer Publications
Formation of chemically ordered compounds of Fe and Au is inhibited in bulk materials due to their limited mutual solubility. However, here we report the formation of chemically ordered L12-type Fe3Au and FeAu3 compounds in Fe–Au sub-10 nm nanoparticles, suggesting that they are equilib-rium structures in size-constrained systems. The stability of these L12-ordered Fe3Au and FeAu3 com-pounds along with a previously discovered L10-ordered FeAu has been explained by a size-dependent equilibrium thermodynamic model. Furthermore, the spin ordering of these three com-pounds has been computed using ab initio first-principle calculations. All ordered compounds exhibit a …
Dynamical (E,2e) Studies Of Tetrahydropyran And 1,4-Dioxane, J. D. Builth-Williams, G. Da Silva, L. Chiari, D. B. Jones, Hari Chaluvadi, Don H. Madison, M. J. Brunger
Dynamical (E,2e) Studies Of Tetrahydropyran And 1,4-Dioxane, J. D. Builth-Williams, G. Da Silva, L. Chiari, D. B. Jones, Hari Chaluvadi, Don H. Madison, M. J. Brunger
Physics Faculty Research & Creative Works
We present experimental and theoretical results for the electron-impact ionization of the highest occupied molecular orbitals of tetrahydropyran and 1,4-dioxane. Using an (e,2e) technique in asymmetric coplanar kinematics, angular distributions of the slow ejected electron, with an energy of 20 eV, are measured when incident electrons at 250 eV ionize the target and scatter through an angle of either -10° or -15°. The data are compared with calculations performed at the molecular 3-body distorted wave level. Fair agreement between the theoretical model and the experimental measurements was observed. The similar structures for these targets provide key insights for assessing the …
Entropy Driven Crystal Formation On Highly Strained Substrates, John R. Savage, Stefan F. Hopp, Rajesh Ganapathy, Sharon J. Gerbode, Andreas Heuer, Itai Cohen
Entropy Driven Crystal Formation On Highly Strained Substrates, John R. Savage, Stefan F. Hopp, Rajesh Ganapathy, Sharon J. Gerbode, Andreas Heuer, Itai Cohen
All HMC Faculty Publications and Research
In heteroepitaxy, lattice mismatch between the deposited material and the underlying surface strongly affects nucleation and growth processes. The effect of mismatch is well studied in atoms with growth kinetics typically dominated by bond formation with interaction lengths on the order of one lattice spacing. In contrast, less is understood about how mismatch affects crystallization of larger particles, such as globular proteins and nanoparticles, where interparticle interaction energies are often comparable to thermal fluctuations and are short ranged, extending only a fraction of the particle size. Here, using colloidal experiments and simulations, we find particles with short-range attractive interactions form …
Non-Fermi Liquid Transport And "Universal" Ratios In Quantum Griffiths Phases, David Nozadze, Thomas Vojta
Non-Fermi Liquid Transport And "Universal" Ratios In Quantum Griffiths Phases, David Nozadze, Thomas Vojta
Physics Faculty Research & Creative Works
We use the semi-classical Boltzmann equation to investigate transport properties such as electrical resistivity, thermal resistivity, thermopower, and the Peltier coefficient of disordered metals close to an antiferromagnetic quantum phase transition. In the quantum Griffiths phase, the electrons are scattered by spin-fluctuations in the rare regions. This leads to singular temperature dependencies not just at the quantum critical point, but in the entire Griffiths phase. We show that the resulting non-universal power-laws in transport properties are controlled by the same Griffiths exponent λ which governs the thermodynamics. λ takes the value zero at the quantum critical point and increases throughout …
Transcendental Thermodynamics, Richard E. Morel, George Fleck
Transcendental Thermodynamics, Richard E. Morel, George Fleck
Kahn Institute Projects
Thermodynamics is often viewed as a narrow, introspective discipline, trapped by its origins in the 18th and 19th centuries. By dramatic contrast, we show that the Fourth Law of Thermodynamics provides explanations and interpretations of all natural events, extending across artificial boundaries of tradition- al academic disciplines. The Fourth Law of Thermodynamics states that far-from-equilibrium systems increase entropy at the maximum rate available to them. This broadly inclusive paradigm applies to systems from molecules, to organisms, to the biosphere. The Fourth Law is the Law of Evolution. All systems that communicate with their environment exhibit self-organization and self-optimization, enabling the …
Exact Results In Model Statistical Systems, Peter H. Kleban
Exact Results In Model Statistical Systems, Peter H. Kleban
University of Maine Office of Research Administration: Grant Reports
Intellectual merit: This project focuses on continued research on the exact study of the statistical mechanics of model systems. The research concentrates on two areas:
1) critical percolation in two dimensions, an important and very extensively studied model system, to which we are bringing new and unexpected approaches, and
2) the thermodynamics of the Farey fraction spin chain, a set of one dimensional models with interesting phase transition behavior and connections to multifractals, and dynamical systems.
This project aims at new results and insights in both these areas. Research on the Farey models illuminates an interesting borderline case in the …
Numerical Study Of The Thermodynamics Of Clinoatacamite, Ehsan Khatami, Joel Helton, Marcos Rigol
Numerical Study Of The Thermodynamics Of Clinoatacamite, Ehsan Khatami, Joel Helton, Marcos Rigol
Faculty Publications
We study the thermodynamic properties of the clinoatacamite compound, Cu2(OH)3Cl, by considering several approximate models. They include the Heisenberg model on (i) the uniform pyrochlore lattice, (ii) a very anisotropic pyrochlore lattice, and (iii) a kagome lattice weakly coupled to spins that sit on a triangular lattice. We utilize the exact diagonalization of small clusters with periodic boundary conditions and implement a numerical linked-cluster expansion approach for quantum lattice models with reduced symmetries, which allows us to solve model (iii) in the thermodynamic limit. We find a very good agreement between the experimental uniform susceptibility and the numerical results for …
Computational Study Of The Hydration Of Sulfuric Acid Dimers: Implications For Acid Dissociation And Aerosol Formation, Berhane Temelso, Thuong Ngoc Phan, George C. Shields
Computational Study Of The Hydration Of Sulfuric Acid Dimers: Implications For Acid Dissociation And Aerosol Formation, Berhane Temelso, Thuong Ngoc Phan, George C. Shields
Faculty Journal Articles
We have investigated the thermodynamics of sulfuric acid dimer hydration using ab initio quantum mechanical methods. For (H2SO4)2(H2O)n where n = 0−6, we employed high-level ab initio calculations to locate the most stable minima for each cluster size. The results presented herein yield a detailed understanding of the first deprotonation of sulfuric acid as a function of temperature for a system consisting of two sulfuric acid molecules and up to six waters. At 0 K, a cluster of two sulfuric acid molecules and one water remains undissociated. Addition of a second …
Thermodynamics And Phase Transitions For The Heisenberg Model On The Pinwheel Distorted Kagome Lattice, Ehsan Khatami, Rajiv Singh, Marcos Rigol
Thermodynamics And Phase Transitions For The Heisenberg Model On The Pinwheel Distorted Kagome Lattice, Ehsan Khatami, Rajiv Singh, Marcos Rigol
Faculty Publications
We study the Heisenberg model on the pinwheel distorted kagome lattice as observed in the material Rb2Cu3SnF12. Experimentally relevant thermodynamic properties at finite temperatures are computed utilizing numerical linked-cluster expansions. We also develop a Lanczos-based, zero-temperature, numerical linked-cluster expansion to study the approach of the pinwheel distorted lattice to the uniform kagome-lattice Heisenberg model. We find strong evidence for a phase transition before the uniform limit is reached, implying that the ground state of the kagome-lattice Heisenberg model is likely not pinwheel dimerized and is stable to finite pinwheel-dimerizing perturbations.
Thermodynamics Of Strongly Interacting Fermions In Two-Dimensional Optical Lattices, Ehsan Khatami, Marcos Rigol
Thermodynamics Of Strongly Interacting Fermions In Two-Dimensional Optical Lattices, Ehsan Khatami, Marcos Rigol
Faculty Publications
We study finite-temperature properties of strongly correlated fermions in two-dimensional optical lattices by means of numerical linked cluster expansions, a computational technique that allows one to obtain exact results in the thermodynamic limit. We focus our analysis on the strongly interacting regime, where the on-site repulsion is of the order of or greater than the band width. We compute the equation of state, double occupancy, entropy, uniform susceptibility, and spin correlations for temperatures that are similar to or below the ones achieved in current optical lattice experiments. We provide a quantitative analysis of adiabatic cooling of trapped fermions in two …
Thermodynamics Of Magnetic Multilayers, Tathagata Mukherjee
Thermodynamics Of Magnetic Multilayers, Tathagata Mukherjee
Department of Physics and Astronomy: Dissertations, Theses, and Student Research
Our interest in thermodynamics of magnetic thin film heterostructure began by exploring the possibility to use magnetic nanostructures in the search for optimized magnetocaloric materials for potential room temperature refrigeration. In the present thesis magnetic thin film heterostructures are experimentally realized by Molecular Beam Epitaxy (MBE) and Pulsed Laser Deposition (PLD). Co/Cr and Fe/Cr superlattices were fabricated using mean-field theoretical concepts as guiding principles. The potential of artificial antiferromagnets for near room-temperature refrigeration is explored. Magnetocaloric properties are deduced from measurements of the temperature and field dependence of the magnetization of our samples. The effects of intra-plane and inter-plane exchange …
Scaling Properties At Freeze-Out In Relativistic Heavy-Ion Collisions, M. M. Aggarwal, Z. Ahammed, A. V. Alakhverdyants, I. Alekseev, J. Alford, B. D. Anderson, S. Bueltmann, I. Koralt, D. Plyku, Star Collaboration
Scaling Properties At Freeze-Out In Relativistic Heavy-Ion Collisions, M. M. Aggarwal, Z. Ahammed, A. V. Alakhverdyants, I. Alekseev, J. Alford, B. D. Anderson, S. Bueltmann, I. Koralt, D. Plyku, Star Collaboration
Physics Faculty Publications
Identified charged pion, kaon, and proton spectra are used to explore the system size dependence of bulk freeze-out properties in Cu+Cu collisions at √sNN=200 and 62.4 GeV. The data are studied with hydrodynamically motivated blast-wave and statistical model frameworks in order to characterize the freeze-out properties of the system. The dependence of freeze-out parameters on beam energy and collision centrality is discussed. Using the existing results from Au + Au and pp collisions, the dependence of freeze-out parameters on the system size is also explored. This multidimensional systematic study furthers our understanding of the QCD phase diagram revealing the importance …
Structure-Property Maps And Optimal Inversion In Configurational Thermodynamics, Gus L. W. Hart, Björn Arnold, Alejandro Díaz Ortiz, Helmut Dosch
Structure-Property Maps And Optimal Inversion In Configurational Thermodynamics, Gus L. W. Hart, Björn Arnold, Alejandro Díaz Ortiz, Helmut Dosch
Faculty Publications
Cluster expansions of first-principles density-functional databases in multicomponent systems are now used as a routine tool for the prediction of zero- and finite-temperature physical properties. The ability of producing large databases of various degrees of accuracy, i.e., high-throughput calculations, makes pertinent the analysis of error propagation during the inversion process. This is a very demanding task as both data and numerical noise have to be treated on equal footing. We have addressed this problem by using an analysis that combines the variational and evolutionary approaches to cluster expansions. Simulated databases were constructed ex professo to sample the configurational space in …
Classical Thermodynamics Of Particles In Harmonic Traps, Martin K. Ligare
Classical Thermodynamics Of Particles In Harmonic Traps, Martin K. Ligare
Faculty Journal Articles
No abstract provided.