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Full-Text Articles in Physics
Structural Distortion-Induced Magnetoelastic Locking In Sr2Iro4 Revealed Through Nonlinear Optical Harmonic Generation, D. H. Torchinsky, H. Chu, L. Zhao, N. B. Perkins, Y. Sizyuk, T. Qi, Gang Cao, D. Hsieh
Structural Distortion-Induced Magnetoelastic Locking In Sr2Iro4 Revealed Through Nonlinear Optical Harmonic Generation, D. H. Torchinsky, H. Chu, L. Zhao, N. B. Perkins, Y. Sizyuk, T. Qi, Gang Cao, D. Hsieh
Physics and Astronomy Faculty Publications
We report a global structural distortion in Sr2IrO4 using spatially resolved optical second and third harmonic generation rotational anisotropy measurements. A symmetry lowering from an I41/acd to I41/a space group is observed both above and below the Néel temperature that arises from a staggered tetragonal distortion of the oxygen octahedra. By studying an effective superexchange Hamiltonian that accounts for this lowered symmetry, we find that perfect locking between the octahedral rotation and magnetic moment canting angles can persist even in the presence of large noncubic local distortions. Our results …
Harmonic Generation In Thin Films And Multilayers, William S. Kolthammer '04, Dustin Barnard '03, Nicole Carson, Aaron D. Edens '00, Nathan A. Miller '01, Peter N. Saeta
Harmonic Generation In Thin Films And Multilayers, William S. Kolthammer '04, Dustin Barnard '03, Nicole Carson, Aaron D. Edens '00, Nathan A. Miller '01, Peter N. Saeta
All HMC Faculty Publications and Research
A general method for computing harmonic generation in reflection and transmission from planar nonmagnetic multilayer structures is described. The method assumes plane waves and treats harmonic generation in the parametric approximation. The method is applied in studying the second- and third-harmonic generation properties of thin crystal silicon layers surrounded by thermal oxide. Most independent components of the nonlinear susceptibility tensor have unique signatures with silicon layer thickness d, allowing their strength to be determined in principle by measuring harmonic generation as a function of d. Surface and bulk contributions to third-harmonic generation are cleanly distinguished, with the bulk signal dominating. …