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Temporal Coherent Control Of Resonant Two-Photon Double Ionization Of The Hydrogen Molecule Via Doubly Excited States, Jean Marcel Ngoko Djiokap, Anthony F. Starace

Anthony F. Starace Publications

We use time-delayed, counter-rotating, circularly polarized few-cycle attosecond nonoverlapping pulses to study the temporal coherent control of the resonant process of two-photon double ionization (TPDI) of hydrogen molecule via doubly excited states for pulse propagation direction along ˆk either parallel or perpendicular to the molecular axis ˆR. For ˆk ‖ ˆR and a pulse carrier frequency of 36 eV resonantly populating the Q₂ 1∏ ⁺ _u (1) doubly excited state as well as other 1∏ ⁺ _u doubly excited states, we find that the indirect ionization pathway through these doubly excited states changes the character of the kinematical vortex-shaped …