Physics Commons^™

Analysis, Prototyping, And Design Of An Ionization Profile Monitor For The Spallation Neutron Source Accumulator Ring, Dirk A. Bartkoski

Doctoral Dissertations

The Spallation Neutron Source (SNS) located in the Oak Ridge National Laboratory is comprised of a 1 GeV linear H^- [H^-] accelerator followed by an accumulator ring that delivers high intensity 1 μs [microsecond] long pulses of 1.5x10¹⁴ [1.5x10^14] protons to a liquid mercury target for neutron production by spallation reaction. With its strict 0.01% total beam loss condition, planned power upgrade, and proposed second target station, SNS ring beam-profile diagnostics capable of monitoring evolving beam conditions during high-power conditions are crucial for efficient operation and improvement. By subjecting ionized electrons created during beam interactions with the residual …

Tracking Real-Time Nanoparticle Positions And Measuring Three-Dimensional Solution Flow With A Four-Focus Confocal Microscope, James Andrew Germann

Doctoral Dissertations

This dissertation presents the development of instrumentation for measuring the position of a single emitter within the sample volume of a confocal fluorescence microscope with sub-diffraction limited precision in three dimensions together with applications for determining solution flow and for tracking a fluorescent nanoparticle as it undergoes Brownian diffusion. The localization method is based on comparing photon counts from alternating excitation of the emitter by four laser beams, which are focused at slightly offset positions in a tetrahedral pattern within the confocal volume. Two experimental set-ups are constructed. In the first, the four beams are from a femtosecond laser, which …

A Viscous Flow Analog To Prandtl’S Optimized Lifting Line Theory Utilizing Rotating Biquadratic Bodies Of Revolution, Mark Nathaniel Callender

Doctoral Dissertations

Prandtl’s lifting line theory expanded the Kutta-Joukowski theorem to calculate the lift and induced drag of finite wings. The circulation distribution about a real wing was represented by a superposition of infinitesimal vortex filaments. From this theory, the optimum distribution of circulation was determined to be elliptical. A consequence of this theory led to the prediction that the elliptical chord distribution on a real fixed wing would provide the elliptical circulation distribution. The author applied the same line of reasoning to lift-producing rotating cylinders in order to determine the cylindrical geometry that would theoretically produce an elliptical circulation distribution. The …

Numerical Study Of Hubbard Model For Iron-Based Superconductors, Qinlong Luo

Doctoral Dissertations

This thesis addresses the numerical and analytical study of the iron-based superconductors, mainly using the multi-orbital Hubbard model and Hartree-Fock approximation. The text starts with an introduction to the new iron-based superconductors, followed by a theoretical description of the multi-orbital Hubbard model and Hartree-Fock approximations. The numerical study of the Hubbard model in momentum space is described next, where the phase diagrams for three- and five-orbital Hubbard models are provided. The physically ``realistic" regime of couplings is highlighted, to guide future theoretical work into the proper region of parameters of Hubbard models for iron-based superconductors. What goes next is the …

A Holographic Model Of Striped Superconductors, Suman Ganguli

Doctoral Dissertations

One of the most prominent distinguishing features in strongly correlated electron systems, such as the high Tc (critical temperature) cuprates and the most recent iron pnictides, is the presence of "competing orders" that are related to the breaking of the lattice symmetries. Does the ubiquitous presence of such inhomogeneous orders in strongly correlated superconductors have a deep connection to superconductivity? The answer to this question is crucial for identifying the mechanism of superconductivity, at least in the cuprates. Amidst serious difficulties within conventional theoretical framework to deal with strongly interacting degrees of freedom at finite density, "AdS/CFT correspondence" or "gauge/gravity …

Experimental And Statistical Techniques To Probe Extraordinary Electronic Properties Of Molecules, Byron Hager Smith

Doctoral Dissertations

The existence of an additional electron or hole in the presence of an electric monopole is a well understood physical system, but this ideality is far from the true physical properties of many molecules. Examples of such irregular electronic states include the attachment of an excess charge to a molecule's dipole moment, electronic correlation spanning a molecule, or attachment of multiple excess charges. Current theoretical and experimental interpretations widely vary for these states and further elucidation of the nature of irregular electronic structure may provide solutions to unexplained observations and the impetus for industrial application. For example, in the case …

Measurement Of The Prompt Double J/Psi Production Cross Section In Pp Collisions At Sqrt(S) = 7 Tev, Andrew David York

Doctoral Dissertations

The simultaneous production of two J/psi mesons has been significantly observed in proton-proton collisions at a center-of-mass energy of 7 TeV with the CMS detector. The two J/psi mesons are fully reconstructed in their decay to muons. The signal yield is extracted with an extended maximum likelihood fit based on four event variables. A method was developed to correct for detector acceptances and efficiencies based on the measured momenta of the J/psi and their decay muons to maintain the least model dependence possible.

The measurement is performed in an acceptance region defined by the individual J/psi transverse momentum and rapidity. …

Magneto-Optical Properties Of Complex Oxides, Peng Chen

Doctoral Dissertations

Complex oxides give rise to rich physics and exotic cross-coupled electronic and magnetic properties. This is because of the competing interaction between charge, structure, and magnetism in the materials. In this dissertation I present a spectroscopic investigation of several model complex oxides under external stimuli of magnetic field and temperature. The compounds of interest include BiFeO₃ [bismuth ferrite] nanoparticles and tetragonal film, Bi_1-xNd_xFeO₃ [neodymium doped bismuth ferrite], α-Fe₂O₃ [hematite], Ni₃V₂O₈ [nickel vanadate], and RIn_1-xMn_xO₃ [manganese doped rare earth indium oxide]. …

A Study Of The Optical And Negative Ion Properties Of Selected Chiral Molecules, Jason Michael Lambert

Doctoral Dissertations

Chirality is subtle geometric property where objects lack reflection plane symmetry. In this thesis I study three chiral molecules using a combination of experimental and theoretical methods to elucidate the relationships between conformation freedom, solvent choice, and temperature. The importance of nuclear motion when predicting the optical rotation is explored. For carvone, corrections with each nuclear mode coordinate is important. Predictions of the ORD have the incorrect sign without the inclusion of vibrational corrections. For the case of two newly synthesized amino acid derivatives the vibrational corrections did not correct the sign of the calculated ORD to bring it into …

Measurement Of [Special Characters Omitted] (Pp[Special Characters Omitted]Tt) In The[Special Characters Omitted]+ Jets Channel Using 4.7 Fb-1 Of Data From The Atlas Experiment Of The Large Hadron Collider, Anirvan Sircar

Doctoral Dissertations

The top quark is the heaviest of the known elementary particles in the Standard Model. Top quark decay can result into various final states; therefore, careful study of its production rate and other properties is very important for particle physics. With the shutdown of the Tevatron, The Large Hadron Collider (LHC) is the only facility currently capable of studying top quark properties. The data obtained by proton-proton collisions in the LHC is recorded by two general purpose detectors, ATLAS and CMS. The results in the dissertation are from the ATLAS detector. A new measurement is reported of &sgr;(pp [special …

Three-Dimensional Electrokinetic Trapping Of A Single Fluorescent Nanoparticle In Solution, Jason Keith King

Doctoral Dissertations

This dissertation presents the development of an instrument for effectively trapping a single fluorescent nanoparticle that is freely diffusing in solution in all three dimensions. The instrument is expected to have applications for studies of single nanoparticles or molecules for which prolonged observations are required, but without immobilization or proximity to a surface, which may alter behavior. The trapping technique depends on rapid three-dimensional position measurements of the nanoparticle with sub-micron precision, which are used for real-time control of induced electrokinetic motion, so as to counteract Brownian motion. While anti-Brownian electrokinetic trapping experiments in one and two dimensions have previously …

Fully Coupled Fluid And Electrodynamic Modeling Of Plasmas: A Two-Fluid Isomorphism And A Strong Conservative Flux-Coupled Finite Volume Framework, Richard Joel Thompson

Doctoral Dissertations

Ideal and resistive magnetohydrodynamics (MHD) have long served as the incumbent framework for modeling plasmas of engineering interest. However, new applications, such as hypersonic flight and propulsion, plasma propulsion, plasma instability in engineering devices, charge separation effects and electromagnetic wave interaction effects may demand a higher-fidelity physical model. For these cases, the two-fluid plasma model or its limiting case of a single bulk fluid, which results in a single-fluid coupled system of the Navier-Stokes and Maxwell equations, is necessary and permits a deeper physical study than the MHD framework. At present, major challenges are imposed on solving these physical models …

Neutron Scattering Study Of The Iron Based Superconductors, Miaoyin Wang

Doctoral Dissertations

In most iron-based and copper-oxide superconductors, the T_c [superconducting critical temperature] gradually increases upon charge carrier doping or isovalent doping. In the under-doped regime of electron-doped BaFe₂As₂ [Barium Iron 2 Arsenic 2], the superconductivity appears before the complete suppression of AF [antiferromagnetic] long-range order, creating a SC-AF [superconducting-antiferromagnetic] coexisting area. The interplay between long-range magnetic order and superconductivity was studied using a triple-axis thermal neutron spectrometer under an in-plane magnetic field. The suppression of superconductivity and the enhancement of long-range AF order were discovered under 11 Tesla, suggesting the competing nature of these two phases and …

The Study Of Nuclear Structure Of Neutron-Rich 81ge And Its Contribution In The R-Process Via The Neutron Transfer Reaction 80ge(D,P), Sunghoon Ahn

Doctoral Dissertations

The study of low-lying levels of nuclei near closed shells not only elucidates the evolution of nuclear shell structure far from stability, but also affects estimates of heavy element nucleosynthesis in supernova explosions. Especially, the properties of the low-lying levels in ⁸¹Ge[Germanium 81] are important because the sensitivity study of the r-process pointed out that the properties of the nucleus can affect the final bundance pattern. Also, the spins and parities measurements of the states are essential to understand the shape coexistence in odd-mass N = 49 isotones.

This work describes the study of the odd-mass N = …

Complex Magnetism In Noncentrosymmetric Magnets, Nirmal Jeevi Ghimire

Doctoral Dissertations

Broken inversion symmetry in a crystal lattice allows an extra term called the Dzyaloshinskii-Moriya (DM) interaction in the magnetic Hamiltonian. The DM interaction tends to align spins in perpendicular orientation and therefore competes with the exchange interaction that favors collinear spins. This competition results in different modulated chiral magnetic structures depending on the relative strength of the two interactions. Skyrmion, soliton and magnetic blue phases are some of the anticipated structures. This dissertation extends the search for these exotic magnetic structures using various techniques to study the magnetism in the noncentrosymmetric magnets Cr₁₁Ge₁₉ [chromium eleven germanium nineteen], …

Investigation Of Time And Position Resolved Alpha Transducers For Multi-Modal Imaging With A D-T Neutron Generator, Joshua William Cates

Doctoral Dissertations

Deuterium-Tritium (D-T) neutron generators have been used as an active interrogation source for associated particle imaging (API) techniques. The D-T reaction yields a 14.1 MeV neutron and a 3.5 MeV alpha (or assoicated) particle, projected nearly back-to-back. The kinetics of the reaction allow the direction and initial time of the neutron to be determined utilizing position sensitive detectors for both the alpha and neutron. This information facilitates multi-modal fast neutron imaging of inspection objects and closed containers to infer the geometry within them and the presence of special nuclear material (SNM). Since position and time of interaction of the alpha …

Neutron Scintillation Detectors Based On Polymers Containing Lithium-6 For Radiation Portal Monitor Applications, Andrew Neil Mabe

Doctoral Dissertations

The work presented herein describes an investigation of four main types of thin film polymer scintillators containing ⁶Li [lithium-6] for neutron detection: polystyrene containing ⁶LiF [lithium-6 fluoride] and a preblended fluor mixture comprising 2,5-diphenyloxazole and 1,4-bis(5-phenyloxazol-2-yl)benzene; poly(styrene-co-lithium maleate) containing salicylic acid; poly[styrene-co-lithium maleate-co-2-phenyl-5-(4-vinylphenyl)oxazole]; and poly(styrene-co-lithium 4-vinylbenzoate). A variety of chemical and physical characterizations as well as optical and scintillation characterizations were performed to guide the development of optimized compositions of each type of polymer film. The scintillation performances of optimized compositions of each type of polymer film were calibrated using …

The Measurement Of The Dielectric Constant Of Concrete Pipes And Clay Pipes, David Mcgraw

Doctoral Dissertations

To optimize the effectiveness of the rehabilitation of underground utilities, taking in consideration limitation of available resources, there is a need for a cost effective and efficient sensing systems capable of providing effective, in real time and in situ, measurement of infrastructural characteristics. To carry out accurate non-destructive condition assessment of buried and above ground infrastructure such as sewers, bridges, pavements and dams, an advanced ultra-wideband (UWB) based radar was developed at Trenchless Technology Centre (TTC) and Centre for Applied Physics Studies (CAPS) at Louisiana Tech University (LTU). One of the major issues in designing the FCC compliant UWB radar …

Generalized Finite-Difference Time-Domain Schemes For Solving Nonlinear Schrödinger Equations, Frederick Ira Moxley Iii

Doctoral Dissertations

The nonlinear Schrödinger equation (NLSE) is one of the most widely applicable equations in physical science, and characterizes nonlinear dispersive waves, optics, water waves, and the dynamics of molecules. The NLSE satisfies many mathematical conservation laws. Moreover, due to the nonlinearity, the NLSE often requires a numerical solution, which also satisfies the conservation laws. Some of the more popular numerical methods for solving the NLSE include the finite difference, finite element, and spectral methods such as the pseudospectral, split-step with Fourier transform, and integrating factor coupled with a Fourier transform. With regard to the finite difference and finite element methods, …

Application Of Computational Molecular Biophysics To Problems In Bacterial Chemotaxis, Davi Ortega

Doctoral Dissertations

The combination of physics, biology, chemistry, and computer science constitutes the promising field of computational molecular biophysics. This field studies the molecular properties of DNA, protein lipids and biomolecules using computational methods. For this dissertation, I approached four problems involving the chemotaxis pathway, the set of proteins that function as the navigation system of bacteria and lower eukaryotes.

In the first chapter, I used a special-purpose machine for molecular dynamics simulations, Anton, to simulate the signaling domain of the chemoreceptor in different signaling states for a total of 6 microseconds. Among other findings, this study provides enough evidence to propose …

Novel Bimetallic Plasmonic Nanomaterials, Ritesh Sachan

Doctoral Dissertations

Plasmonic nanomaterials have attracted a lot of attention recently due to their application in various fields such as chemical and biological sensing, catalysis, energy harvesting and optical devices. However, there is a need to address several outstanding issues with these materials, including cost-effective synthesis, tunability in plasmonic characteristics, and long term stability. In this thesis, we have focused on bimetallic nanoparticles (NPs) of Ag and Co due to their immiscibility as well as their individual properties. First, a pulsed laser induced dewetting route was used to synthesize Ag-Co bimetallic plasmonic NPs. An synthesis parameter space was derived to show the …

Femtosecond Laser Patterned Templates And Imprinted Polymer Structures, Deepak Rajput

Doctoral Dissertations

Femtosecond laser machining is a direct-write lithography technique by which user-defined patterns are efficiently and rapidly generated at the surface or within the bulk of transparent materials. When femtosecond laser machining is performed with tightly focused amplified pulses in single-pulse mode, transparent substrates like fused silica can be surface patterned with high aspect ratio (>10:1) and deep (>10 μm) nanoholes. The main objective behind this dissertation is to develop single-pulse amplified femtosecond laser machining into a novel technique for the production of fused silica templates with user-defined patterns made of high aspect ratio nanoholes. The size of the …

Quantitative Techniques For Pet/Ct: A Clinical Assessment Of The Impact Of Psf And Tof, Joshua Donald Schaefferkoetter

Doctoral Dissertations

Tomographic reconstruction has been a challenge for many imaging applications, and it is particularly problematic for count-limited modalities such as Positron Emission Tomography (PET). Recent advances in PET, including the incorporation of time-of-flight (TOF) information and modeling the variation of the point response across the imaging field (PSF), have resulted in significant improvements in image quality. While the effects of these techniques have been characterized with simulations and mathematical modeling, there has been relatively little work investigating the potential impact of such methods in the clinical setting. The objective of this work is to quantify these techniques in the context …

Haldane Pseudopotentials And Landau Level Mixing In The Quantum Hall Effect, Rachel Elizabeth Wooten

Doctoral Dissertations

The discovery of the quantum Hall effect in 1980 opened to physics one of the simplest systems for studying many-body correlations. Numerical techniques and trial wavefunctions have proven useful for describing the novel collective behavior of the electrons, but have not fully explained all features of the fractional quantum Hall effect. For example, it is predicted that Landau level mixing should have a moderate effect on the system for all but the very strongest magnetic fields, but this effect has not been extensively studied. Among the tools most useful to modeling and describing the quantum Hall system is the Haldane …

Alkane Adsorption On Mgo(100): Volumetric Isotherm, Inelastic Neutron Scattering, And Computational Studies, Andrew Spencer Hicks

Doctoral Dissertations

Volumetric adsorption isotherms and computational molecular dynamics (MD) simulations were performed for nonane and decane adfilms on MgO(100) nanocubes. From the isotherms, variety of thermodynamic quantities are calculated. These values, along with visual inspection of the isotherms, indicate a layer by layer trend from 2D to 3D behavior. This is attributed to the increasing importance of vertical adsorbate-adsorbate interactions as distance from the surface increases. Additionally, a 2D phase transition is observed for the first adsorbed layer as indicated by the evolution of the widths of the isotherm first derivative peaks. These experimental results are complemented by the MD calculations, …

Growth And Electric Field Control Of Phase Separated Manganites, Hangwen Guo

Doctoral Dissertations

Perovskite Manganites have received numerous attentions due to exotic behaviors such as colossal magnetoreistance (CMR) and electronic phase separation (EPS). The purpose of my research is to answer fundamental questions about the growth properties of manganites and electric field control of the EPS properties.

Experimental study was conducted on controlling the growth mode of La_0.7Sr_0.3MnO₃[Lanthanum Strontium Manganese Oxide] thin films using pulsed laser deposition. Different thin film morphology, crystallinity and stoichiometry have been observed depending on growth parameters. To understand the microscopic origin, the thermodynamic processes were theoretically analyzed and a growth diagram was …

Transport In Correlated And Uncorrelated Random Media, With Applications To Molecularly Doped Polymers, Nilanka Praveena Gurusinghe

Doctoral Dissertations

"The commonly observed Poole-Frenkel field dependence; of the mobility of photo-injected charges in molecularly-doped polymers has been shown to arise from the spatially-correlated, Gaussian energy distribution of transport sites encountered by charges moving through the material. Experimental current-time transients obtained for molecularly-doped polymers exhibit universality with respect to electric field and a metal-insulator-like transition from non-dispersive to dispersive transport, features usually identified with multiple trapping models that assume an uncorrelated exponential distribution of trap energies. For materials that exhibit both sets of features the possibility arises that both kinds of disorder coexist. We study here, analytically and numerically, transport in …

Characterization Of Nano-Scaled Metal-Hydrides Confined In Nano-Porous Carbon Frameworks, David Edward Peaslee

Doctoral Dissertations

"Metal hydrides are currently being studied to provide hydrogen for use in fuel cells and for transportation applications. Hydrogen can be stored in chemical compounds at higher density and lower volume than liquid H₂ or compressed gas. Thermodynamic properties of metal hydrides differ between bulk and nano-sized particles. Many metal hydrides with useful volumetric and gravimetric capacities have high decomposition temperatures, but when placed in nano-sized frameworks (or templates) desorption and adsorption temperatures can be fine-tuned to meet engineering requirements for real-world systems. Additionally, some metal hydrides have shown a change in the decomposition pathway when infiltrated into these frameworks, …

Quantum Phase Transitions In Disordered Magnets, David Nozadze

Doctoral Dissertations

"We study the effects of quenched weak disorder on quantum phase transitions in disordered magnets. The presence of disorder in the system can lead to a variety of exotic phenomena, e.g., the smearing of transitions or quantum Griffiths singularities. Phase transitions are smeared if individual spatial regions can order independently of the bulk system. In paper I, we study smeared quantum phase transitions in binary alloys A₁₋ₓBₓ that are tuned by changing the composition x. We show that in this case the ordered phase is extended over all compositions x < 1. We also study the composition dependence of observables. In paper II, we investigate the influence of spatial disorder correlations on smeared phase transitions. As an experimental example, we demonstrate in paper III, that the composition-driven ferromagnetic-toparamagnetic quantum phase transition in Sr₁₋ₓCaₓ RuO₃ is smeared. When individual spatial regions cannot order but fluctuate slowly, the phase transition is characterized by strong singularities in the quantum Griffiths phase. In paper IV, we develop a theory of the quantum Griffiths phases in disordered ferromagnetic metals. We show that the quantum Griffiths singularities are stronger than the usual power-law quantum Griffiths singularities in insulating magnets. In paper V, we present an efficient numerical method for studying quantum phase transitions in disordered systems with O(N) order parameter symmetry in the large-N limit. Our algorithm solves iteratively the large-N self-consistent equations for the renormalized distances from criticality. Paper VI is devoted to the study of transport properties in the quantum Griffiths phase associated with the antiferromagnetic quantum phase transition in a metal. We find unusual behavior of transport properties which is in contrast to the normal Fermi-liquid behavior"--Abstract, page v.

Structural And Magnetic Properties Of Ni And Cr Substituted La₀.₇Sr₀.₃Mno₃, Thomas Franklin Creel Jr.

Doctoral Dissertations

"The La₁₋ₓSrₓMn_1-yB_yO₃ perovskite systems where B represents a 3d transition metal such as Cr, Fe, Co, Ni, Cu, and Zn, are of significant interest due to their large magnetoresistance, and electronic transport properties that change significantly, depending on values of x and which transition metal used. Their applications in technology include cathodes for solid oxide fuel cells, resistance random access memory and catalysis. At certain doping concentrations on the B-site, metal-to-semiconductor or metal-to-insulator transitions coupled with colossal magnetoresistance occur, decreasing the resistivity (up to six orders of magnitude) upon the application of an external magnetic field. …