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University of Denver

Theses/Dissertations

Perovskite

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Investigating New Methods To Develop Perovskite Solar Cells, Amani Hussain Alfaifi Jan 2020

Investigating New Methods To Develop Perovskite Solar Cells, Amani Hussain Alfaifi

Electronic Theses and Dissertations

Discovering the potential of organic-inorganic metal halide perovskites (MHP) as a harvesting material in solar cells has strongly affected the research direction in solar energy. The fascinating optical and electronic properties offered by MHP combined with tremendous effort from scientists around the world have improved the efficiency to about 25% in a decade.

In the first part of the dissertation, we studied the lamination process as a new fabrication method for producing self-encapsulated perovskite solar cells based on laminating half stacks,as opposed to the conventional layer-by-layer method. Our work focused on optimizing the lamination process of complex triple cations perovskite …


Multidimensional Spectroscopy Of Mixed-Cation Perovskite Thin Films, Geoffrey Michael Diederich Jan 2019

Multidimensional Spectroscopy Of Mixed-Cation Perovskite Thin Films, Geoffrey Michael Diederich

Electronic Theses and Dissertations

Metal halide perovskite (MHP) thin films are currently undergoing an intense re- search thrust due to the excellent performance of MHP based photovoltaic (PV) devices, which have the potential to revolutionize the worlds energy production via a unique combination of low-cost fabrication and high power conversion efficiency (PCE). However, the vast majority of research is currently aimed at incremental improvements in device PCE, resulting in a body of work without the foundational understanding of the charge-carrier dynamics of the system upon photoexcitation.

This thesis begins with the development of a phase-modulated multidimensional coherent spectroscopy (PM-MDCS) experiment. PM-MDCS is an ultrafast …