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Full-Text Articles in Physics
Synchrotron Based Infrared Microspectroscopy Of Carbonaceous Chondrites., Mehmet Yesiltas
Synchrotron Based Infrared Microspectroscopy Of Carbonaceous Chondrites., Mehmet Yesiltas
Electronic Theses and Dissertations
Relationships between organic molecules and inorganic minerals are investigated in five carbonaceous chondrites, Northwest Africa 852 (CR2), Tagish Lake (C2-ungroupped), Orgueil (CI1), Sutter's Mill (CM), and Murchison (CM2), with micron spatial resolution using synchrotron-based imaging micro-FTIR spectroscopy. Correlations based on absorption strength for various constituents are determined using statistical correlation analysis. Silicate band is found to be positively correlated with stretching modes of aliphatic hydrocarbons in NWA 852 and Tagish Lake. The former is highly correlated with the hydration band in all meteorites. Negative correlation is observed between water+organics and carbonate bands in all meteorites. Two dimensional infrared maps for …
Characterization And Application Of Isolated Attosecond Pulses, Michael Chini
Characterization And Application Of Isolated Attosecond Pulses, Michael Chini
Electronic Theses and Dissertations
Tracking and controlling the dynamic evolution of matter under the influence of external fields is among the most fundamental goals of physics. In the microcosm, the motion of electrons follows the laws of quantum mechanics and evolves on the timescale set by the atomic unit of time, 24 attoseconds. While only a few time-dependent quantum mechanical systems can be solved theoretically, recent advances in the generation, characterization, and application of isolated attosecond pulses and few-cycle femtosecond lasers have given experimentalists the necessary tools for dynamic measurements on these systems. However, pioneering studies in attosecond science have so far been limited …
Random Transformations Of Optical Fields And Applications, Thomas Kohlgraf-Owens
Random Transformations Of Optical Fields And Applications, Thomas Kohlgraf-Owens
Electronic Theses and Dissertations
The interaction of optical waves with material systems often results in complex, seemingly random fields. Because the fluctuations of such fields are typically difficult to analyze, they are regarded as noise to be suppressed. Nevertheless, in many cases the fluctuations of the field result from a linear and deterministic, albeit complicated, interaction between the optical field and the scattering system. As a result, linear systems theory (LST) can be used to frame the scattering problem and highlight situations in which useful information can be extracted from the fluctuations of the scattered field. Three fundamental problems can be posed in LST …
Molecular Structure-Nonlinear Optical Property Relationships For A Series Of Polymethine And Squaraine Molecules, Jie Fu
Electronic Theses and Dissertations
This dissertation reports on the investigation of the relationships between molecular structure and two-photon absorption (2PA) properties for a series of polymethine and squaraine molecules. Current and emerging applications exploiting the quadratic dependence upon laser intensity, such as two-photon fluorescence imaging, three-dimensional microfabrication, optical data storage and optical limiting, have motivated researchers to find novel materials exhibiting strong 2PA. Organic materials are promising candidates because their linear and nonlinear optical properties can be optimized for applications by changing their structures through molecular engineering. Polymethine and squaraine dyes are particularly interesting because they are fluorescent and showing large 2PA. We used …