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Full-Text Articles in Physics

Heat Transport In Sb2àXvxte3 Single Crystals, Jeffrey Dyck, W. Chen, C. Uher, Č. DrašAr, P. LošŤÁK Sep 2002

Heat Transport In Sb2àXvxte3 Single Crystals, Jeffrey Dyck, W. Chen, C. Uher, Č. DrašAr, P. LošŤÁK

Jeffrey Dyck

Antimony telluride doped with small concentrations of vanadium was recently identified as a diluted magnetic semiconductor. We present a study of the heat transport in single crystals of [formula] with [formula] 0.01, 0.02, and 0.03. Thermopower and thermal conductivity were measured from 1.5 K to 300 K. The thermopower is positive for all samples investigated and has a modest dependence on vanadium content. At low temperatures, the lattice thermal conductivity has an approximate [formula] dependence and the data up to 100 K can be fitted well assuming that phonons scatter on boundaries, point defects, charge carriers, and other phonons. Theoretical …


Calorimetric Study Of Nematic Prewetting, Xuewu Liu, David W. Allender, D. Finotello Sep 2002

Calorimetric Study Of Nematic Prewetting, Xuewu Liu, David W. Allender, D. Finotello

David W Allender

We report specific-heat measurements for a series of liquid crystals imbedded in a porous cylindrical geometry. Above the nematic-to-isotropic transition and dependent on nematic width (or chain length), the specific heat shows a small peak. In analogy to known ellipsometry results, the peak is believed to be the signature of a nematic prewetting transition.


Maximization Of The Open Circuit Voltage For Hydrogenated Amorphous Silicon N–I–P Solar Cells By Incorporation Of Protocrystalline Silicon P-Type Layers, R. J. Koval, Chi Chen, G. M. Ferreira, A. S. Ferlauto, Joshua M. Pearce, P. I. Rovira, C. R. Wronski, R. W. Collins Aug 2002

Maximization Of The Open Circuit Voltage For Hydrogenated Amorphous Silicon N–I–P Solar Cells By Incorporation Of Protocrystalline Silicon P-Type Layers, R. J. Koval, Chi Chen, G. M. Ferreira, A. S. Ferlauto, Joshua M. Pearce, P. I. Rovira, C. R. Wronski, R. W. Collins

Joshua M. Pearce

In studies of hydrogenated amorphous silicon(a-Si:H) n–i–psolar cells fabricated by rf plasma-enhanced chemical vapor deposition (PECVD), we have found that the maximum open circuit voltage (Voc) is obtained by incorporating p-type doped Si:H layers that are protocrystalline in nature. Specifically, these optimum p layers are prepared by PECVD in the a-Si:H growth regime using the maximum hydrogen-to-silane flow ratio possible without crossing the thickness-dependent transition into the mixed-phase (amorphous+microcrystalline) growth regime for the ∼200 Å p-layer thickness. The strong dependence of the p-layer phase and solar cell Voc on the underlying i-layer phase also confirms the protocrystalline nature of the …


Highly Anisotropic Crystal Growth And Thermoelectric Properties Of K2bi8_Xsbxse13 Solid Solutions: Band Gap Anomaly At Low X, Jeffrey S. Dyck, Theodora Kyratsi, Wei Chan, Duck-Young Chung, Ctirad Uher, Konstantinos Paraskevopoulos, Mercouri Kanatzidis Jul 2002

Highly Anisotropic Crystal Growth And Thermoelectric Properties Of K2bi8_Xsbxse13 Solid Solutions: Band Gap Anomaly At Low X, Jeffrey S. Dyck, Theodora Kyratsi, Wei Chan, Duck-Young Chung, Ctirad Uher, Konstantinos Paraskevopoulos, Mercouri Kanatzidis

Jeffrey Dyck

The thermoelectric properties of solid solutions of the type B -K2Bi8_xSbxSe13 (0


Thermal-Lens Model Compared With The Sheik-Bahae Formalism In Interpreting Z-Scan Experiments On Lyotropic Liquid Crystals, Fabio Luiz Sant'anna Cuppo, Antonio Martins Figueiredo Neto, Sergio Leonardo Gomez, Peter Palffy-Muhoray May 2002

Thermal-Lens Model Compared With The Sheik-Bahae Formalism In Interpreting Z-Scan Experiments On Lyotropic Liquid Crystals, Fabio Luiz Sant'anna Cuppo, Antonio Martins Figueiredo Neto, Sergio Leonardo Gomez, Peter Palffy-Muhoray

Peter Palffy-Muhoray

We carried out Z-scan measurements on lyotropic liquid crystals and on lyotropic liquid crystals doped with ferrofluid. In these experiments, the sample is translated through the focal region of a focused Gaussian laser beam. The dependence of the far-field intensity on sample position due to intensity-dependent optical nonlinearities has been analyzed on the basis of the thermal-lens model of Gordon et al. and the Gaussian decomposition analysis of Sheik-Bahae et al. The thermal-lens model is nonlocal in space and time, whereas the Gaussian decomposition is predicated on a strictly local response. We compare the goodness of fit of the predictions …


Transport Properties Of Polycrystalline Type-I Sn Clathrates, G. S. Nolas, J. L. Cohn, Jeffrey Dyck, C. Uher, J. Lang Apr 2002

Transport Properties Of Polycrystalline Type-I Sn Clathrates, G. S. Nolas, J. L. Cohn, Jeffrey Dyck, C. Uher, J. Lang

Jeffrey Dyck

Thermal conductivity, resistivity, Seebeck coefficient, and Hall measurements on polycrystalline Sn-clathrate compounds with the type-I hydrate crystal structure are reported. Interstitial alkali-metal atoms in these compounds reside inside polyhedral cavities formed by the tetrahedrally bonded Sn network atoms. Localized disorder associated with “rattling” motion of these interstitial atoms contributes to the low thermal conductivity of these semiconducting compounds. The Hall coefficient and resistivity for some compounds exhibit nonmonotonic temperature dependences consistent with a crossover with decreasing temperature from conduction-band to impurity-band conduction. The carrier mobility is found to be low even in the absence of interstitial atoms within the Sn …


Three-Dimensional Dye Distribution In Photo-Oriented Liquid-Crystal Alignment Layers, S. Bardon, D. Coleman, N. A. Clark, T. Kosa, H. Yuan, Peter Palffy-Muhoray Mar 2002

Three-Dimensional Dye Distribution In Photo-Oriented Liquid-Crystal Alignment Layers, S. Bardon, D. Coleman, N. A. Clark, T. Kosa, H. Yuan, Peter Palffy-Muhoray

Peter Palffy-Muhoray

The three-dimensional optical anisotropy of photo-buffed dye-doped polymer films and the resulting orientation imparted to a liquid crystal in contact are probed using total internal reflection. Although the linearly polarized writing light generates a uniaxial distribution of dye molecules, the polymer films are biaxial, a result of symmetry breaking by the film surface.


Thermoelectric Properties Of The N-Type Filled Skutterudite Ba0.3co4sb12 Doped With Ni, Jeffrey Dyck, Wei Chen, Ctirad Uher, Lidong Chen, Xinfeng Tang, Toshio Hirai Mar 2002

Thermoelectric Properties Of The N-Type Filled Skutterudite Ba0.3co4sb12 Doped With Ni, Jeffrey Dyck, Wei Chen, Ctirad Uher, Lidong Chen, Xinfeng Tang, Toshio Hirai

Jeffrey Dyck

Synthesis and electrical and thermal transport properties are reported for several filled skutterudite compounds doped with Ni: Ba0.3NixCo4_xSb12 with 0


Diluted Magnetic Semiconductors Based On Sb2àXvxte3 „0.01ïXï0.03., Jeffrey Dyck, Pavel Hájek, Petr LošŤÁK, Ctirad Uher Mar 2002

Diluted Magnetic Semiconductors Based On Sb2àXvxte3 „0.01ïXï0.03., Jeffrey Dyck, Pavel Hájek, Petr LošŤÁK, Ctirad Uher

Jeffrey Dyck

We report on a diluted magnetic semiconductor based on the [formula] tetradymite structure doped with very low concentrations of vanadium (1—3 at. %). The anomalous transport behavior and robust magnetic hysteresis loops observed in magnetotransport and magnetic measurements are experimental manifestations of the ferromagnetic state in these materials. The [formula] exchange between holes and vanadium [formula] spins is estimated from the behavior of the magnetoresistance. A Curie temperature of at least 22 K is observed for [formula] This discovery offers possibilities for exploring magnetic properties of other tetradymite structure semiconductors doped with a wide range of [formula] transition metals.


Effect Of Ni On The Transport And Magnetic Properties Of Co1àXnixsb3, Jeffrey Dyck, Wei Chen, Jihui Yang, Gregory P. Meisner, Ctirad Uher Mar 2002

Effect Of Ni On The Transport And Magnetic Properties Of Co1àXnixsb3, Jeffrey Dyck, Wei Chen, Jihui Yang, Gregory P. Meisner, Ctirad Uher

Jeffrey Dyck

The filled skutterudite compounds based on the binary skutterudite [formula] are currently being investigated for their potential applications as thermoelectric materials. One route to optimization of these compounds is by doping on the Co site. An obvious candidate for an n-type dopant is Ni, since it has one more electron in its valence shell than Co. Up to now, however, only high concentrations of Ni in [formula] have been studied; and the valence of Ni in this compound and its influence on the transport and magnetic properties has been an open question. We present electrical resistivity, thermopower, Hall effect, magnetoresistance, …


Influence Of Electron-Phonon Interaction On The Lattice Thermal Conductivity Of Co1àXnixsb3, J. Yang, D. T. Morelli, G. P. Meisner, W. Chen, Jeffrey Dyck, C. Uher Feb 2002

Influence Of Electron-Phonon Interaction On The Lattice Thermal Conductivity Of Co1àXnixsb3, J. Yang, D. T. Morelli, G. P. Meisner, W. Chen, Jeffrey Dyck, C. Uher

Jeffrey Dyck

We have investigated the effect of electron-phonon scattering in a series of n-type nickel-doped [formula] skutterudite materials. Samples were polycrystalline of the form [formula] with [formula] 0.001, 0.003, 0.005, 0.0075, and 0.01. The lattice thermal conductivity decreases dramatically with increasing Ni doping for [formula] For higher Ni concentration the reduction of the lattice thermal conductivity saturates. Our theoretical analysis indicates that this reduction of the lattice thermal conductivity cannot be explained solely by point-defect scattering of the phonons. Rather, we can fit the lattice thermal conductivity of Ni-doped [formula] by introducing an electron-phonon scattering mechanism, and this demonstrates that the …


Analysis And Classification Of Nonlinear Dispersive Evolution Equations In The Potential Representation, Andrei Ludu Dec 2001

Analysis And Classification Of Nonlinear Dispersive Evolution Equations In The Potential Representation, Andrei Ludu

Andrei Ludu

No abstract provided.


What Do We Learn From The Local Geometry Of Glass-Forming Liquids?, Francis W. Starr, S. Sastry, J. F. Douglas, S. C. Glotzer Dec 2001

What Do We Learn From The Local Geometry Of Glass-Forming Liquids?, Francis W. Starr, S. Sastry, J. F. Douglas, S. C. Glotzer

Francis Starr

No abstract provided.


The Single Particle Potential In Mean-Field Theory, Peter Palffy-Muhoray Dec 2001

The Single Particle Potential In Mean-Field Theory, Peter Palffy-Muhoray

Peter Palffy-Muhoray

The problem of determining the single particle energy in a mean-field description of interacting particles is considered. It is shown that the single particle energy must satisfy two consistency conditions, and a general procedure for obtaining the single particle energy from the pair energy is proposed. Interacting dipolar systems are examined, current approaches in the literature are discussed, and the usefulness of the proposed method is demonstrated.


Translational And Rotational Diffusion In Stretched Water, P. A. Netz, Francis Starr, M. C. Barbosa, H. E. Stanley Dec 2001

Translational And Rotational Diffusion In Stretched Water, P. A. Netz, Francis Starr, M. C. Barbosa, H. E. Stanley

Francis Starr

No abstract provided.