Open Access. Powered by Scholars. Published by Universities.®
- Discipline
Articles 1 - 4 of 4
Full-Text Articles in Physics
Optimization Of The Nanolens Consisting Of Coupled Metal Nanoparticles: An Analytical Approach, Greg Sun, Jacob B. Khurgin
Optimization Of The Nanolens Consisting Of Coupled Metal Nanoparticles: An Analytical Approach, Greg Sun, Jacob B. Khurgin
Physics Faculty Publications
Using a simple and intuitive analytical approach, we perform optimization of a nanolens composed of coupled metal nanoparticles capable of subwavelength focusing of light inside the narrow gap separating the particles. Specifically, we optimize the structure of two nanospheres of different sizes to achieve maximum field enhancement at an off-center position in the gap. We demonstrate that the nanolens of two or more spheres acts simultaneously as an efficient antenna with large dipole and an efficient cavity with small effective volume.
Theory Of Optical Emission Enhancement By Coupled Metal Nanoparticles: An Analytical Approach, Greg Sun, Jacob B. Khurgin
Theory Of Optical Emission Enhancement By Coupled Metal Nanoparticles: An Analytical Approach, Greg Sun, Jacob B. Khurgin
Physics Faculty Publications
We present an analytical “coupled mode” model explaining enhancement of emission by an emitter placed within complexes of metal nanoparticles and apply it for an important case of an emitter placed inside the gap of two coupled Au nanospheres. This approach has dual advantages of exposing the underling physics of the enhancement and revealing a straightforward path toward optimization.
Analysis Of Interband, Intraband, And Plasmon Polariton Transitions In Silver Nanoparticle Films Via In Situ Real-Time Spectroscopic Ellipsometry, S. A. Little, R. W. Collins, S. Marsillac
Analysis Of Interband, Intraband, And Plasmon Polariton Transitions In Silver Nanoparticle Films Via In Situ Real-Time Spectroscopic Ellipsometry, S. A. Little, R. W. Collins, S. Marsillac
Electrical & Computer Engineering Faculty Publications
The dielectric function of Ag nanoparticle films, deduced from an analysis of in situ real-time spectroscopic ellipsometry (RTSE) measurements, is found to evolve with time during deposition in close consistency with the film structure, deduced in the same RTSE analysis. In the nucleation regime, the intraband dielectric function component is absent and plasmon polariton behavior dominates. Only at nuclei contact, does the intraband amplitude appear, increasing above zero. Both intraband and plasmon amplitudes coexist during surface smoothening associated with coalescence. The intraband relaxation time increases rapidly after surface smoothening is complete, also in consistency with the thin film structural evolution.
Localized Surface Plasmon Resonance Of Single Silver Nanoparticles Studied By Dark-Field Optical Microscopy And Spectroscopy, Wei Cao, Tao Huang, Xiao-Hong Nancy Xu, Hani E. Elsayed-Ali
Localized Surface Plasmon Resonance Of Single Silver Nanoparticles Studied By Dark-Field Optical Microscopy And Spectroscopy, Wei Cao, Tao Huang, Xiao-Hong Nancy Xu, Hani E. Elsayed-Ali
Electrical & Computer Engineering Faculty Publications
Localized surface plasmon resonance (LSPR) of Ag nanoparticles (NPs) with different shapes and disk-shaped Ag NP pairs with varying interparticle distance is studied using dark-field optical microscopy and spectroscopy (DFOMS). Disk-, square-, and triangular-shaped Ag NPs were fabricated on indium tin oxide-coated glass substrates by electron beam lithography. The LSPR spectra collected from single Ag NPs within 5×5 arrays using DFOMS exhibited pronounced redshifts as the NP shape changed from disk to square and to triangular. The shape-dependent experimental LSPR spectra are in good agreement with simulations using the discrete dipole approximation model, although there are small deviations in the …