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Paul J. Simmonds

Selected Works

Quantum dots

Articles 1 - 7 of 7

Full-Text Articles in Physics

Tensile Gaas(111) Quantum Dashes With Tunable Luminescence Below The Bulk Bandgap, Paul J. Simmonds Aug 2014

Tensile Gaas(111) Quantum Dashes With Tunable Luminescence Below The Bulk Bandgap, Paul J. Simmonds

Paul J. Simmonds

Strain-based band engineering in quantum dots and dashes has been predominantly limited to compressively strained systems. However, tensile strain strongly reduces the bandgaps of nanostructures, enabling nanostructures to emit light at lower energies than they could under compressive strain. We demonstrate the self-assembled growth of dislocation-free GaAs quantum dashes on an InP(111)B substrate, using a 3.8% tensile lattice-mismatch. Due to the high tensile strain, the GaAs quantum dashes luminesce at 110–240 meV below the bandgap of bulk GaAs. The emission energy is readily tuned by adjusting the size of the quantum dashes via deposition thickness. Tensile self-assembly creates new opportunities …


Effects Of Gaas(Sb) Cladding Layers On Inas/Alassb Quantum Dots, Paul J. Simmonds Jan 2013

Effects Of Gaas(Sb) Cladding Layers On Inas/Alassb Quantum Dots, Paul J. Simmonds

Paul J. Simmonds

The structural and optical properties of InAs self-assembled quantum dots buried in AlAs0.56Sb0.44 barriers can be controlled using GaAs1−xSbx cladding layers. These cladding layers allow us to manage the amount of Sb immediately underneath and above the InAs quantum dots. The optimal cladding scheme has a GaAs layer beneath the InAs, and a GaAs0.95Sb0.05 layer above. This scheme results in improved dot morphology and significantly increased photoluminescence (PL) intensity. Both power-dependent and time-resolved photoluminescence confirm that the quantum dots have type-II band alignment. Enhanced carrier lifetimes in this quantum dot system …


Structural And Optical Properties Of Inas/Alassb Quantum Dots With Gaas(Sb) Cladding Layers, Paul J. Simmonds, Ramesh Babu Laghumavarapu, Meng Sun, Andrew Lin, Charles J. Reyner, Baolai Liang, Diana L. Huffaker Jun 2012

Structural And Optical Properties Of Inas/Alassb Quantum Dots With Gaas(Sb) Cladding Layers, Paul J. Simmonds, Ramesh Babu Laghumavarapu, Meng Sun, Andrew Lin, Charles J. Reyner, Baolai Liang, Diana L. Huffaker

Paul J. Simmonds

We investigate the effect of GaAs1−xSbxcladding layer composition on the growth and properties of InAsself-assembledquantum dots surrounded by AlAs0.56Sb0.44 barriers. Lowering Sb-content in the GaAs1−xSbx improves the morphology of the InAs quantum dots and reduces cladding layer alloy fluctuations. The result is a dramatic increase in photoluminescence intensity from the InAs quantum dots, with a peak at 0.87 eV. The emission energy exhibits a cube root dependence on excitation power, consistent with the type-II band alignment of the quantum dots. The characteristics of this quantum dot system show promise for …


Self-Assembled In0.5Ga0.5As Quantum Dots On Gap, Yuncheng Song, Paul J. Simmonds, Minjoo Larry Lee Nov 2010

Self-Assembled In0.5Ga0.5As Quantum Dots On Gap, Yuncheng Song, Paul J. Simmonds, Minjoo Larry Lee

Paul J. Simmonds

We demonstrate the growth and luminescence of coherently strained In0.5Ga0.5As self-assembled quantum dots on GaP. Cross-sectional and planar-view transmission electron microscopy confirmed the dislocation-free nature of the In0.5Ga0.5As quantum dots and GaP cap layers. Intense photoluminescence from the quantum dots was measured at 80 K and was visible to the unaided eye in ambient lighting. The photoluminescence results show that emission energy can be controlled by varying the In0.5Ga0.5As deposition thickness. In combination with recent advances in the growth of GaP on Si, the In0.5Ga0.5 …


Tensile Strained Iii-V Self-Assembled Nanostructures On A (110) Surface, Minjoo L. Lee, Paul J. Simmonds Aug 2010

Tensile Strained Iii-V Self-Assembled Nanostructures On A (110) Surface, Minjoo L. Lee, Paul J. Simmonds

Paul J. Simmonds

The vast majority of research on epitaxial quantum dots use compressive strain as the driving force for self-assembly on the (001) surface, with InAs/GaAs(001) and Ge/Si(001) being the best-known examples. In this talk, I will discuss our work on determining the feasibility of growing coherent, tensile-strained III-V nanostructures on a (110) surface. GaP on GaAs(110) was chosen as an initial test system. It is hoped that our efforts on self-assembled, tensile-strained dots on a (110) surface will lead the way to new devices exploiting the fundamental differences between the (110) and (001) surfaces. Furthermore it is anticipated that this work …


Quantum Dot Resonant Tunneling Diode For Telecommunication Wavelength Single Photon Detection, H. W. Li, B. E. Kardynał, P. See, A. J. Shields, P. Simmonds, H. E. Beere, D. A. Ritchie Aug 2007

Quantum Dot Resonant Tunneling Diode For Telecommunication Wavelength Single Photon Detection, H. W. Li, B. E. Kardynał, P. See, A. J. Shields, P. Simmonds, H. E. Beere, D. A. Ritchie

Paul J. Simmonds

The authors present a quantum dot (QD) based single photon detector operating at a fiber optic telecommunication wavelength. The detector is based on an AlAs/In0.53Ga0.47As/AlAs double-barrier resonant tunneling diode containing a layer of self-assembled InAs QDs grown on an InP substrate. The device shows an internal efficiency of about 6.3% with a dark count rate of 1.58 × 10−6 ns−1 for 1310 nm photons.


Growth By Molecular Beam Epitaxy Of Self-Assembled Inas Quantum Dots On Inalas And Ingaas Lattice-Matched To Inp, Paul J. Simmonds, H W. Li, H E. Beere, P See, A J. Shields, D A. Ritchie May 2007

Growth By Molecular Beam Epitaxy Of Self-Assembled Inas Quantum Dots On Inalas And Ingaas Lattice-Matched To Inp, Paul J. Simmonds, H W. Li, H E. Beere, P See, A J. Shields, D A. Ritchie

Paul J. Simmonds

The authors report the results of a detailed study of the effect of growth conditions, for molecular beam epitaxy, on the structural and optical properties of self-assembled InAs quantum dots (QDs) on In0.524Al0.476As. InAs QDs both buried in, and on top of, In0.524Al0.476As were analyzed using photoluminescence (PL) and atomic force microscopy. InAs QD morphology and peak PL emission wavelength both scale linearly with deposition thickness in monolayers (MLs). InAs deposition thickness can be used to tune QD PL wavelength by 170 nm/ML, over a range of almost 700 nm. Increasing growth …